We demonstrate a new technique for characterizing two-photon quantum states based on joint temporal correlation measurements using time resolved single photon detection by femtosecond upconversion. We measure for the first time the joint temporal density of a two-photon entangled state, showing clearly the time anti-correlation of the coincident-frequency entangled photon pair generated by ultrafast spontaneous parametric down-conversion under extended phase-matching conditions. The new technique enables us to manipulate the frequency entanglement by varying the down-conversion pump bandwidth to produce a nearly unentangled two-photon state that is expected to yield a heralded single-photon state with a purity of 0.88. The time-domain correlation technique complements existing frequency-domain measurement methods for a more complete characterization of photonic entanglement in quantum information processing.
An experiment is performed to demonstrate the temporal distinguishability of a four-photon state and a six-photon state, both from parametric down-conversion. The experiment is based on a multi-photon interference scheme in a recent discovered NOON-state projection measurement. By measuring the visibility of the interference dip, we can distinguish the various scenarios in the temporal distribution of the pairs and thus quantitatively determine the degree of temporal (in)distinguishability of a multi-photon state.
The complementary principle of quantum mechanics relates qualitatively the visibility of quantum interference with path indistinguishability. Here we propose a scheme of constructive quantum interference involving superposition between an $N$-photon state and a single-photon state to characterize quantitatively the degree of temporal distinguishability of the $N$-photon state. This scheme is based on a generalized photon bunching effect. Such a scheme can be extended to other more general cases.
Single-photons with high spectro-temporal purity are an essential resource for quantum photonic technologies. The highest reported purity up until now from a conventional silicon photonic device is 92% without any spectral filtering. We have experimentally generated and observed single-photons with 98.0+-0.3 % spectro-temporal purity using a conventional micro racetrack resonator and an engineered dual pump pulse.
The measurement of joint signal-idler photon-number distribution of a field obtained from spontaneous parametric downconversion using an intensified CCD camera is presented. It is shown that a classicality criterion is violated directly by the measured data. Characteristic dimensions of the area of correlation are determined in the same experimental setup.
Some new temporal Bell inequalities are deduced under joint realism assumption, using some perfect correlation property. No locality condition is needed. When the measured system is a macroscopic system, joint realism assumption substitutes the non-invasive measurabilioty hypothesis advantegeously, provided that the system satisfies the perfect correlation property. The new inequalities are violated quantically. This violation can be more severe than the similar violation in the case of precedent temporal Bell inequalities. Some microscopic and mesoscopic situations in which these inequalities…
A number of recent interference experiments involving multiple photons are reviewed. These experiments include generalized photon bunching effects, generalized Hong-Ou-Mandel interference effects and multi-photon interferometry for demonstrations of multi-photon de Broglie wavelength. The multi-photon states used in these experiments are from two pairs of photons in parametric down-conversion. We find that the size of the interference effect in these experiments, characterized by the visibility of interference pattern, is governed by the degree of distinguishability among different pairs of ph…
We study the generation of single-photon pulses with the tailored temporal shape via nonlocal spectral filtering. A shaped photon is heralded from a time-energy entangled photon pair upon spectral filtering and time-resolved detection of its entangled counterpart. We show that the temporal shape of the heralded photon is defined by the time-inverted impulse response of the spectral filter and does not depend on the heralding instant. Thus one can avoid post-selection of particular heralding instants and achieve substantially higher heralding rate of shaped photons as compared to the generation…
We present experimental demonstrations of two-photon interference involving temporally separated photons within two types of interferometers: a Mach-Zehnder interferometer and a polarization-based Michelson interferometer. The two-photon states are probabilistically prepared in a symmetrically superposed state within the two interferometer arms by introducing a large time delay between two input photons; this state is composed of two temporally separated photons, which are in two different or the same spatial modes. We then observe two-photon interference fringes involving both the Hong-Ou-Man…
A method for reconstructing joint photon-number distributions of twin beams from the experimental photocount histograms is suggested and experimentally implemented. Contrary to the standard reconstruction methods, it incorporates spatial noise reduction based on spatial pairing of photons. Superior performance of the method above the usual one for the maximum-likelihood approach is demonstrated.
Subnatural-linewidth single-photon source is a potential candidate for exploring the time degree of freedom in photonic quantum information science. This type of single-photon source has been demonstrated to be generated and reshaped in atomic ensembles without any external cavity or filter, and is typically characterized through photon-counting technology. However, the full complex temporal mode function(TMF) of the photon source is not able to be revealed from direct photon counting measurement. Here, for the first time, we demonstrate the complete temporal mode of the subnatural-linewidth s…
Temporal-spectral modes of light provide a fundamental window into the nature of atomic and molecular systems and offer robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding quantum emitters and are a key requirement for quantum technologies that harness single-photon states. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the temporal-spectral state of single phot…
We propose a method to produce pure single photons with an arbitrary designed temporal shape in a heralded, lossless and scalable way. As the indispensable resource, the method uses pairs of time-energy entangled photons. To accomplish the shaping, one photon of a pair undergoes temporal modulation according to the desired shape. Subsequent frequency-resolving detection of the photon heralds its entangled counterpart in a pure quantum state with a temporal shape non-locally affected by the modulation. We found conditions for the shape of the heralded photon to reproduce the modulation function…
We demonstrate a way to prepare single photons with a temporal envelope that resembles the time reversal of photons from the spontaneous decay process. We use the photon pairs generated from a time-ordered atomic cascade decay: the detection of the first photon of the cascade is used as a herald for the ground-state transition resonant second photon. We show how the interaction of the heralding photon with an asymmetric Fabry-Perot cavity reverses the temporal shape of its twin photon from a decaying to a rising exponential envelope. This single photon is expected to be ideal for interacting w…
Real-time controls based on quantum measurements are powerful tools for various quantum protocols. However, their experimental realization have been limited by mode-mismatch between temporal mode of quadrature measurement and that heralded by photon detection. Here, we demonstrate real-time quadrature measurement of a single-photon wavepacket induced by a photon detection, by utilizing continuous temporal-mode-matching between homodyne detection and an exponentially rising temporal mode. Single photons in exponentially rising modes are also expected to be useful resources for interactions with…
We experimentally demonstrate a source of nearly pure single photons in arbitrary temporal shapes heralded from a parametric down-conversion (PDC) source at telecom wavelengths. The technology is enabled by the tailored dispersion of in-house fabricated waveguides with shaped pump pulses to directly generate the PDC photons in on-demand temporal shapes. We generate PDC photons in Hermite-Gauss and frequency-binned modes and confirm a minimum purity of 0.81, even for complex temporal shapes.
Heralded single photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal and signal-signal-idler coincidences of photons generated by continuous wave pumped cavity-enhanced spontaneous pa…
We demonstrate a method to reconstruct the joint photon statistics of two or more modes of radiation using on/off photodetection performed at different quantum efficiencies. The two-mode case is discussed in details and experimental results are presented for the bipartite states obtained after a beam-splitter fed by a single photon state or a thermal state.
We present a multi-mode model to describe an arbitrary N-photon state with a wide spectral range and some arbitrary temporal distribution. In general, some of the $N$ photons are spread out in time while other may overlap and become indistinguishable. From this model, we find that the temporal (in)distinguishability of photons is related to the exchange symmetry of the multi-photon wave function. We find that simple multi-photon detection scheme gives rise to a more general photon bunching effect with the famous two-photon effect as a special case. We then send this N-photon state into a recen…
Joint probability distributions of photon polarization correlations are computed, as well as those corresponding to the cases when only one of the photon's polarization is measured in $e^{+}e^{-}$ annihilation, in flight, in QED. This provides a dynamical, rather than a kinematical, description of photon polarization correlations as stemming from the ever precise and realistic QED theory. Such computations may be relevant to recent and future experiments involved in testing Bell-like inequalities as described.
Semiconductor quantum dots, as promising solid-state platform, have exhibited deterministic photon pair generation with high polarization entanglement f\textcompwordmark idelity for quantum information applications. However, due to temporal correlation from inherently cascaded emission, photon indistinguishability is limited, which restricts their potential scalability to multi-photon experiments. Here, by utilizing quantum interferences to decouple polarization entanglement from temporal correlation, we improve multi-photon entanglement f\textcompwordmark idelity from $(58.7\pm 2.2)\%$ to $(7…
The observation of the so-called dispersion cancelation (Opt. Express 17, 19244, 2009) and temporal phase modulation (Phys. Rev. Lett. 103, 163601, 2009) of paired photons is generally attributed to the presence of frequency entanglement between two frequency anticorrelated photons. In this paper, it is shown that by introducing the appropriate amount of chromatic dispersion or phase modulation between non-entangled photons, it is also possible to observe these effects. Indeed, it is found that the relevant characteristic for the observation of dispersion cancelation or the cancelation of temp…
Joint signal-idler photoelectron distributions of twin beams containing several tens of photons per mode have been measured recently. Exploiting a microscopic quantum theory for joint quasi-distributions in parametric down-conversion developed earlier we characterize properties of twin beams in terms of quasi-distributions using experimental data. Negative values as well as oscillating behaviour in quantum region are characteristic for the subsequently determined joint signal-idler quasi-distributions of integrated intensities. Also the conditional and difference photon-number distributions ar…
In spontaneous parametric down-conversion photons are known to be created coherently and with equal probability over the entire length of the crystal. Then, there is no particular position in the crystal where a photon pair is created. We make the seemingly contradictory observation that we can control the time delay with the crystal position along the propagation direction. We resolve this contradiction by showing that the spatio-temporal correlations critically affect the temporal properties of the pair of photons, when using a finite detector size. We expect this to have important implicati…
We implemented a joint weak measurement of the trajectories of two photons in a photonic version of Hardy's experiment. The joint weak measurement has been performed via an entangled meter state in polarization degrees of freedom of the two photons. Unlike Hardy's original argument in which the contradiction is inferred by retrodiction, our experiment reveals its paradoxical nature as preposterous values actually read out from the meter. Such a direct observation of a paradox will give us a new insight into the spooky action of quantum mechanics.
By using an asymmetric beam splitter, we observe the generalized Hong-Ou-Mandel effects for three and four photons, respectively. Furthermore, we can use this generalized Hong-Ou-Mandel interferometer to characterize temporal distinguishability.
Photonic qubits constitute a leading platform to disruptive quantum technologies due to their unique low-noise properties. The cost of the photonic approach is the non-deterministic nature of many of the processes, including single-photon generation, which arises from parametric sources and negligible interaction between photons. Active temporal multiplexing - repeating a generation process in time and rerouting to single modes using an optical switching network - is a promising approach to overcome this challenge and will likely be essential for large-scale applications with greatly reduced r…
Quantum state preparation is important for quantum information processing. In particular, in optical quantum computing with continuous variables, non-Gaussian states are needed for universal operation and error correction. Optical non-Gaussian states are usually generated by heralding schemes using photon detectors. In previous experiments, the temporal resolution of the photon detectors was sufficiently high relative to the time width of the quantum state, so that the conventional theory of non-Gaussian state preparation treated the detector's temporal resolution as negligible. However, when …
We report on the implementation of a new interferometric scheme that allows the generation of photon pairs entangled in the time-energy degree of freedom. This scheme does not require any kind of temporal post-selection on the generated pairs and can be used even with lasers with short coherence time.
Quintino et. al. (Phys. Rev. Lett. 113, 160402 (2014)) and Uola et. al. (Phys. Rev. Lett. 113, 160403 (2014)) have recently established an intrinsic relation between non-joint measurability and Einstein-Podolsky- Rosen steering. They showed that a set of measurements is incompatible (i.e., not jointly measurable) if and only if it can be used for the demonstration of steering. In this paper, we prove the temporal analog of this result viz., a set of measurements are incompatible if and only if it exhibits temporal steering.
Two-photon time-frequency entanglement is a valuable resource in quantum information. Resolving the wavepacket of ultrashort pulsed single-photons, however, is a challenge. Here, we demonstrate remote spectral shaping of single photon states and probe the coherence properties of two-photon quantum correlations in the time-frequency domain, using engineered parametric down-conversion (PDC) and a quantum pulse gate (QPG) in nonlinear waveguides. Through tailoring the joint spectral amplitude function of our PDC source we control the temporal mode structure between the generated photon pairs and …
Current proposals for scalable photonic quantum technologies require on-demand sources of indistinguishable single photons with very high efficiency (having unheralded loss below $1\%$). Even with recent progress in the field there is still a significant gap between the requirements and state of the art performance. Here, we propose an on-chip source of multiplexed, heralded photons. Using quantum feedback control on a photon storage cavity with an optimized driving protocol, we estimate an on-demand efficiency of $99\%$ and unheralded loss of order $1\%$, assuming high efficiency detectors an…
We demonstrate how to efficiently implement extremely high-dimensional compressive imaging of a bi-photon probability distribution. Our method uses fast-Hadamard-transform Kronecker-based compressive sensing to acquire the joint space distribution. We list, in detail, the operations necessary to enable fast-transform-based matrix-vector operations in the joint space to reconstruct a 16.8 million-dimensional image in less than 10 minutes. Within a subspace of that image exists a 3.2 million-dimensional bi-photon probability distribution. In addition, we demonstrate how the marginal distribution…
We present a multiplexed single photon source that re-synchronises heralded single photons generated by four-wave mixing in photonic crystal fibre using a fibre delay loop controlled by a single switch. By combining the probabilities of generating heralded single photons on four consecutive pump pulses we obtain an enhancement of the per-bin single-photon delivery probability. Our source demonstrates a way in which single-photon source multiplexing may be carried out with minimised resource overhead while retaining the benefits of a robust and alignment-free platform.
We propose a multidimensional quantum information encoding approach based on temporal modulation of single photons, where the Hilbert space can be spanned by an in-principle infinite set of orthonormal temporal profiles. We analyze two specific realizations of such modulation schemes, and show that error rate per symbol can be smaller than 1% for practical implementations. Temporal modulation may enable multidimensional quantum communication over the existing fiber optical infrastructure, as well as provide an avenue for probing high-dimensional entanglement approaching the continuous limit.
It is a fundamental challenge in quantum optics to deterministically generate indistinguishable single photons through non-deterministic nonlinear optical processes, due to the intrinsic coupling of single- and multi-photon generation probabilities in these processes. Actively multiplexing photons generated in many temporal modes can decouple these probabilities, but key issues are to minimize resource requirements to allow scalability, and to ensure indistinguishability of the generated photons. We demonstrate the multiplexing of photons from four temporal modes solely using fiber-integrated …
We experimentally demonstrate a bright pulsed source of correlated photon pairs at 1550 nm telecom band by pumping 300 m dispersion shifted fiber with a 4 ps pulse train. We investigate the coherence property of the source by measuring the second order intensity correlation function $g^{(2)}$ of individual signal (idler) photons. A preliminary Hong-Ou-Mandel type two-photon interference experiment with two such sources confirms the high temporal and spatial coherence of the source. The source is suitable for multi-photon quantum interference of independent sources, required in quantum informat…
Single-photon coherent optics represents a fundamental importance for the investigation of quantum light-matter interactions. While most work has considered the interaction in the steady-state regime, here we demonstrate that a single-photon pulse shorter than any relaxation time in a medium propagates without energy loss and is consistently transformed into a zero-area pulse. A general analytical solution is found for photon passage through a cold ensemble of $Λ$-type atoms confined inside a hollow core of a single-mode photonic-crystal fiber. We use the robust far off-resonant Raman scheme t…
The development of new quantum light sources requires robust and convenient methods of characterizing their joint spectral properties. Measuring the joint spectral intensity between a photon pair ignores any correlations in spectral phase which may be responsible for degrading the quality of quantum interference. A fully phase-sensitive characterization tends to require significantly more experimental complexity. Here, we investigate the sensitivity of the frequency-resolved double-pair emission to spectral phase correlations, in particular to the presence of a simple form of correlated phase …
We study the entanglement creation between two flux qubits interacting with electromagnetic field modes. No direct interaction between the qubits exists. Entanglement is reached using entanglement swapping method by an interference measurement performed on photons. We discuss the influence of off-resonance and multi-photon initial states on the qubit-qubit entanglement. The presented scheme is able to drive an initially separable state of two qubits into an highly entangled state suitable for quantum information processing.
It has been proposed that the ability to perform joint weak measurements on post-selected systems would allow us to study quantum paradoxes. These measurements can investigate the history of those particles that contribute to the paradoxical outcome. Here, we experimentally perform weak measurements of joint (i.e. nonlocal) observables. In an implementation of Hardy's Paradox, we weakly measure the locations of two photons, the subject of the conflicting statements behind the Paradox. Remarkably, the resulting weak probabilities verify all these statements but, at the same time, resolve the Pa…
We present an experimental realization of a 16 element, temporal-array, photon-number-resolving (PNR) detector, which is a multiplexed single-photon detector that splits an input signal over multiple time-bins, and the time-bins are detected using two superconducting nanowire single-photon detectors (SNSPD). A theoretical investigation of the PNR capabilities of the detector is performed and it is concluded that compared to a single-photon detector, our array detector can resolve one order of magnitude higher mean photon numbers, given the same number of input pulses to measure. This claim is …
We prepare heralded single photons from a photon pair source based on non-degenerate four-wave mixing in a cold atomic ensemble via a cascade decay scheme. Their statistics shows strong antibunching with g(2)(0) < 0.03, indicating a near single photon character. In an optical homodyne experiment, we directly measure the temporal envelope of these photons and find, depending on the heralding scheme, an exponentially decaying or rising profile. The rising envelope will be useful for efficient interaction between single photons and microscopic systems like single atoms and molecules. At the same …
Precise information about the temporal mode of optical states is crucial for optimizing their interaction efficiency between themselves and/or with matter in various quantum communication devices. Here we propose and experimentally demonstrate a method of determining both the real and imaginary components of a single photon's temporal density matrix by measuring the autocorrelation function of the photocurrent from a balanced homodyne detector at multiple local oscillator frequencies. We test our method on single photons heralded from biphotons generated via four-wave mixing in an atomic vapor…
The quantum state of the photon pair generated from type-II spontaneous parametric down-conversion pumped by a ultrafast laser pulse exhibits strong decoherence in its polarization entanglement, an effect which can be attributed to the clock effect of the pump pulse or, equivalently, to distinguishing spectral information in the two-photon state. Here, we propose novel temporal and spectral engineering techniques to eliminate these detrimental decoherence effects. The temporal engineering of the two-photon wavefunction results in a universal Bell-state synthesizer that is independent of the ch…
We present a scheme for generating polarization-entangled photons pairs with arbitrary joint spectrum. Specifically, we describe a technique for spontaneous parametric down-conversion in which both the center frequencies and the bandwidths of the down-converted photons may be controlled by appropriate manipulation of the pump pulse. The spectral control offered by this technique permits one to choose the operating wavelengths for each photon of a pair based on optimizations of other system parameters (loss in optical fiber, photon counter performance, etc.). The combination of spectral control…
We report on a fast, bandwidth-tunable single-photon source based on an epitaxial GaAs quantum dot. Exploiting spontaneous spin-flip Raman transitions, single photons at $780\,$nm are generated on-demand with tailored temporal profiles of durations exceeding the intrinsic quantum dot lifetime by up to three orders of magnitude. Second-order correlation measurements show a low multi-photon emission probability ($g^{2}(0)\sim\,0.10-0.15$) at a generation rate up to $10\,$MHz. We observe Raman photons with linewidths as low as $200\,$MHz, narrow compared to the $1.1\,$GHz linewidth measured in re…
Multi-photon interference is at the heart of the recently proposed linear optical quantum computing scheme and plays an essential role in many protocols in quantum information. Indistinguishability is what leads to the effect of quantum interference. Optical interferometers such as Michaelson interferometer provide a measure for second-order coherence at one-photon level and Hong-Ou-Mandel interferometer was widely employed to describe two-photon entanglement and indistinguishability. However, there is not an effective way for a system of more than two photons. Recently, a new interferometric …
Time-bin entangled single-photons are highly demanded for long distance quantum communication. We propose a heralded source of tunable narrowband single photons entangled in well-separated multiple temporal modes (time bins) with controllable amplitudes. The detection of a single Stokes photon generated in a cold atomic ensemble via Raman scattering of a weak write pulse heralds the preparation of one spin excitation stored within the atomic medium. A train of read laser pulses deterministically converts the atomic excitation into a single anti-Stokes photon delocalized in multi-time-bins. The…
Field-orthogonal temporal modes of photonic quantum states provide a new framework for quantum information science (QIS). They intrinsically span a high-dimensional Hilbert space and lend themselves to integration into existing single-mode fiber communication networks. We show that the three main requirements to construct a valid framework for QIS -- the controlled generation of resource states, the targeted and highly efficient manipulation of temporal modes and their efficient detection -- can be fulfilled with current technology. We suggest implementations of diverse QIS applications based …
As four-wave-mixing-based photon-pair sources mature, accurate modelling of the photon-pair properties becomes important. Unlike spontaneous parametric down-conversion, four-wave mixing is accompanied by a number of parasitic effects such as nonlinear phase modulation. Currently, most modelling of photon-pair states are analytic in nature, which limits the number and type of effects that can be taken into account. In this work, we derive a complete, dual-pump evolution equation for the joint amplitude of photon pairs, wherein any desired effects can be included. We describe how to efficiently …
Quantum interfaces (QIs) that generate entanglement between a multimode atomic memory and a photon forms a multiplexed repeater node and hold promise to greatly improve quantum repeater rates. Recently, the temporal multimode spin-wave memory that is entangled with a photon has been demonstrated with cold atoms. However, due to additional noise generated in multimode operation, the fidelity of spin-wave-photon entanglement significantly decreases with the mode number. So far, the improvement on temporal-multimode entanglement fidelity via suppressing the additional noise remains unexplored. He…
The ability to determine the joint spectral properties of photon pairs produced by the processes of spontaneous parametric downconversion (SPDC) and spontaneous four wave mixing (SFWM) is crucial for guaranteeing the usability of heralded single photons and polarization-entangled pairs for multi-photon protocols. In this paper, we compare six different techniques that yield either a characterization of the joint spectral intensity or of the closely-related purity of heralded single photons. These six techniques include: i) scanning monochromator measurements, ii) a variant of Fourier transform…
