Zhi-Yong Wang, Cai-Dong Xiong, Ole Keller
In near-field optics and optical tunneling theory, photon wave mechanics, i.e., the first quantized theory of the photon, allows us to address the spatial field localization problem in a flexible manner which links smoothly to classical electromagnetics. In this letter, photon wave mechanics is developed in a rigorous and unified way, based on which field quantization is obtained in a new way.
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We demonstrate the coherent transfer of the orbital angular momentum of a photon to an atom in quantized units of hbar, using a 2-photon stimulated Raman process with Laguerre-Gaussian beams to generate an atomic vortex state in a Bose-Einstein condensate of sodium atoms. We show that the process is coherent by creating superpositions of different vortex states, where the relative phase between the states is determined by the relative phases of the optical fields. Furthermore, we create vortices of charge 2 by transferring to each atom the orbital angular momentum of two photons.
In this study we combine the classical models of the massive and massless spinning particles, derive the current-current interaction Lagrangian of the particles from the gauge transformations of the classical spinors, and discuss radiative processes in electrodynamics by using the solutions of the Dirac equation and the quantum wave equations of the photon. The longitudinal polarized photon states give a new idea about the vacuum concept in electrodynamics.
The interaction of a quantized field with three-level atoms in $Λ$ configuration inside a two-mode cavity is analyzed in the small noise approximation. The atoms are in a two-photon detuning with respect to the carriers of the field. We calculate the stationary quadrature noise spectrum of the field outside the cavity in the case where the input probe field is a squeezed state and the input pump field is a coherent state. The mean value of the field is unaltered in all the analysis: the atoms shows electromagnetically induced transparency (EIT). The effect of the atoms' base level decoherence …
Quantum emitters coupled to plasmonic resonators are known to allow enhanced broadband Purcell factors, and such systems have been recently suggested as possible candidates for on-demand single photon sources, with fast operation speeds. However, a true single photon source has strict requirements of high efficiency (brightness) and quantum indistinguishability of the emitted photons, which can be quantified through two-photon interference experiments. To help address this problem, we employ and extend a recently developed quantized quasinormal mode approach, which rigorously quantizes arbitra…
We report electromagnetically induced transparency using quantized fields in optomechanical systems. The weak probe field is a narrow band squeezed field. We present a homodyne detection of EIT in the output quantum field. We find that the EIT dip exists even though the photon number in the squeezed vacuum is at the single photon level. The EIT with quantized fields can be seen even at temperatures of the order of 100 mK paving the way for using optomechanical systems as memory elements.
Considering ultracold atoms traversing a high-Q Fabry-Perot cavity, we theoretically demonstrate a quantum nondemolition measurement of the photon number. This fully quantum mechanical approach may be understood utilizing concepts as effective mass and group velocity of the atom. The various photon numbers induce a splitting of the atomic wave packet, and a time-of-flight measurement of the atom thereby reveals the photon number. While repeated atomic measurements increase the efficiency of the protocol, it is shown that by considering long interaction times only a few atoms are needed to reso…
We study the absorption spectrum of a probe field by a Λ-type three-level system, which is coupled to a quantized control field through the two upper energy levels. The probe field is applied to the ground and the second excited states. When the quantized control field is in vacuum, we derive a threshold condition to discern vacuum induced transparency (VIT) and vacuum induced Autler- Townes splitting (ATS). We also find that the parameter change from VIT to vacuum induced ATS is very similar to that from broken PT symmetry to PT symmetry. Moreover, we find the photon number resolved spectrum …
We systematically study the interaction between two quantized optical fields and a cyclic atomic ensemble driven by a classic optical field. This so-called atomic cyclic ensemble consists of three-level atoms with Delta-type transitions due to the symmetry breaking, which can also be implemented in the superconducting quantum circuit by Yu-xi Liu et al. [Phys. Rev. Lett. 95, 087001 (2005)]. We explore the dynamic mechanisms to creating the quantum entanglements among photon states, and between photons and atomic collective excitations by the coherent manipulation of the atom-photon system. It …
Parametric model for high-order harmonic generation with quantized fields
本文提出一种高次谐波产生的量子光学模型，将激发场与谐波模式量子化，采用参量下转换哈密顿量描述光子交换，并给出时间演化的解析近似与数值验证。
We consider a fully quantized model of spontaneous emission, scattering, and absorption, and study propagation of a single photon from an emitting atom to a detector atom both with and without an intervening scatterer. We find an exact quantum analog to the classical complex analytic signal of an electromagnetic wave scattered by a medium of charged oscillators. This quantum signal exhibits classical phase delays. We define a time of detection which, in the appropriate limits, exactly matches the predictions of a classically defined delay for light propagating through a medium of charged oscil…
We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical properties of high-order harmonic modes. To this end, we use a simplified model describing an elementary quantum emitter: the model of a two-level atom. While the material system is extremely simplified in this description, the conclusions and the methods may be generalized for more complex cases. Our primary interest is an effective model of HHG in which the exciti…
Ultrafast non-adiabatic molecular energy conversion into photons induced by quantized electromagnetic fields
本文提出基于Holstein-量子-Rabi哈密顿量的分子模型，研究量子化腔中双原子分子的超快光动力学，发现非绝热耦合与反向旋转耦合在将振动-电子能量转化为光子中起关键作用，为强光-物质相互作用驱动的多光子产生铺平道路。
We recently introduced a quantized fluctuational electrodynamics (QFED) formalism that provides a physically insightful definition of an effective position-dependent photon-number operator and the associated ladder operators. However, this far the formalism has been applicable only for the normal incidence of the electromagnetic field in planar structures. In this work, we overcome the main limitation of the one-dimensional QFED formalism by extending the model to three dimensions, allowing us to use the QFED method to study, e.g., plasmonic structures. To demonstrate the benefits of the devel…
Covariant photon current
基于光子连续性方程的物理解释，对标准拉格朗日量进行二次量子化，提出了一种Lorentz和规范不变的单光子理论，并通过分离物质源电流推广了连续性方程。
Non-classical excitation of a solid-state quantum emitter
本研究利用量子化输入光对固态量子发射体进行共振激发，观察到单光子干涉、光子数依赖的非线性及双光子受激发射，并证明单光子可改变发射体状态，为量子网络和光子量子计算奠定基础。
Implications of field quantization on Ramsey interferometry are discussed and general conditions for the occurrence of interference are obtained. Interferences do not occur if the fields in two Ramsey zones have precise number of photons. However in this case we show how two atom (like two photon) interferometry can be used to discern a variety of interference effects as the two independent Ramsey zones get entangled by the passage of first atom. Generation of various entangled states like |0,2>+|2,0> are discussed and in far off resonance case generation of entangled state of two coherent sta…
We introduce a simple model for electromagnetically induced transparency in which all fields are treated quantum mechanically. We study a system of three separated atoms at fixed positions in a one-dimensional multimode optical cavity. The first atom serves as the source for a single spontaneously emitted photon; the photon scatters from a three-level Lambda-configuration atom which interacts with a single-mode field coupling two of the atomic levels; the third atom serves as a detector of the total transmitted field. We find an analytical solution for the quantum dynamics. From the quantum am…
The interaction of two quantized fields and three-level quantum system in a lambda-type configuration is investigated in the presence of cross-Kerr nonlinearity. We consider three models of coupling for the atom-photon interaction. First, we study the dynamical behavior of the atom-photon entanglement and show that increasing the cross-Kerr nonlinearity results in different behaviors in three considered models. Moreover, it is demonstrated that the two quantized modes can be entangled, on the other hand, by applying a classical driving field to the lower levels. Increasing the classical drivin…
The simplest cosmology --- the Friedmann-Robertson-Walker-Lemaître (FRW) model --- describes a spatially homogeneous and isotropic universe where the scale factor is the only dynamical parameter. Here we consider how quantized electromagnetic fields become entangled with the scale factor in a toy version of the FRW model. A system consisting of a photon, source, and detector is described in such a universe, and we find that the detection of a redshifted photon by the detector system constrains possible scale factor superpositions. Thus, measuring the redshift of the photon is equivalent to a w…
Microscopic approach to the quantized light-matter interaction in semiconductor nanostructures: Complex coupled dynamics of excitons, biexcitons, and photons
本文提出一个微观量子模型，研究半导体纳米结构中光-物质相互作用，揭示双激子连续态对动力学的显著影响。
We investigate the quantum fluctuations of a single atom in a weakly driven cavity, where the center of mass motion of the atom is quantized in one dimension. We present analytic results for the second order intensity correlation function $g^{(2)}(τ)$ and the intensity-field correlation function $h_θ(τ)$, for both transmitted and fluorescent light for weak driving fields. We find that the coupling of the center of mass motion to the intracavity field mode can be deleterious to nonclassical effects in photon statistics; less so for the intensity-field correlations.
We introduce the negative binomial states with negative binomial distribution as their photon number distribution. They reduce to the ordinary coherent states and Susskind-Glogower phase states in different limits. The ladder and displacement operator formalisms are found and they are essentially the Perelomov's su(1,1) coherent states via its Holstein-Primakoff realisation. These states exhibit strong squeezing effect and they obey the super-Poissonian statistics. A method to generate these states is proposed.
Is the EPR paradox really a paradox?
本文通过分析含双光子单态源与双探测器的量子化场系统，指出探测器工作条件可唯一确定另一探测器的偏振与方向选择，认为EPR佯谬符合量子场激发的运动与守恒定律，并非真正的佯谬。
We consider the interaction between a Bose-Einstein condensate and a single-mode quantized light field in the presence of a strong far off-resonant pump laser. The dynamics is characterized by an exponential instability, hence the system acts as an atom-photon parametric amplifier. Triggered by a small injected probe field, or simply by quantum noise, entangled atom-photon pairs are created which exhibit non-classical correlations similar to those seen between photons in the optical parametric amplifier. In addition, the quantum statistics of the matter and light fields depend strongly on the …
Ultrafast quantum gates with fully quantized free-electron quantum optics
针对自由电子量子光学的量子操控需求，提出基于光栅的完全量子化架构，通过布洛赫-弗洛奎分析映射光子-电子相互作用至经典量子模型，设计出无腔飞行电子的超快量子门，为通用量子计算及多领域量子技术发展提供平台。
Photons may have homogeneous polarization and may carry quantized orbital angular momentum (OAM). Photon entanglement has been realized in various degrees of freedom such as polarization and OAM. Using a pair of orthogonally polarized states carrying opposite-handedness quantized OAMs could create "quantized" vector polarization states with space-variant polarization structures. It is thus possible to extend the polarization degree of freedom from two dimensional space to indefinite dimensional discrete Hilbert space. We present a class of vector-polarization entangled Bell states, which use t…
Whether the total angular momentum of the photon can be separated into spin and orbital parts has been a long-standing problem due to the constraint of transversality condition on its vector wavefunction. A careful analysis shows that the situation arises from a misuse of the constraint in quantum mechanics. To use the constraint properly, we convert the vector representation into a two-component representation in which the wavefunction is not constrained by any conditions. Upon doing so, we not only separate the spin conceptually from the orbital angular momentum but also identify the Berry g…
We investigate the effect of the cumulative phase on the photon statistics of the three-mode state whose evolution is described by the trilinear Hamiltonian $\hat{H}_{I}=i\hbarκ\big(\hat{a}\hat{b}\hat{c}^{\dagger}-\hat{a}^{\dagger}\hat{b}^{\dagger}c\big)$, wherein the pump is taken to be quantized (and prepared in a coherent state) and the signal and idler modes are initially seeded with coherent states. We provide a brief review of the two-mode squeezed coherent states generated by non-degenerate coherently-stimulated parametric down-conversion, whereby the nonlinear crystal is driven by a st…
Nonlinear Compton scattering in a quantized pump field
本研究建立了单模量子场驱动的非线性康普顿散射全量子理论，分析了有限福克态泵浦的光谱特性，给出弱损耗区域的近似形式，并揭示压缩相干光的压缩角对高能发射的调控作用。
Atom interferometry with quantized light pulses
本文研究原子干涉仪中量子化光脉冲的影响，证明强相干态光脉冲下干涉信号趋近经典极限，而低光子数时因路径信息编码导致可见度下降。
Achieving quantized transport in Floquet topological insulators via energy filters
针对周期驱动 Floquet 拓扑绝缘体中光子辅助过程破坏边缘输运量子化的问题，本文提出窄带能量滤波器并推导 Floquet–Landauer 描述，证明其可抑制边带输运、恢复量子化电导及平衡型分布。
The quantum behaviour of the electromagnetic field in mesoscopic elements is intimately linked to the quantization of the charge. In order to probe nonclassical aspects of the field in those elements, it is essential that thermal noise be reduced to the quantum level, i.e. to scales where kT < hν. This is easily achieved in dilution refrigerators for frequencies of a few GHz, i.e. in the microwave domain. Several recent experiments have highlighted the link between discrete charge transport and discrete photon emission in simple mesoscopic elements such as a tunnel junction. Photocount statist…
It is shown a complex function $Φ$ defined to be the product of a real Gaussian function and a complex Dirac delta function satisfies the Cauchy-Riemann equations. It is also shown these harmonic $Φ$-functions can be included in the solution of the classical electromagnetic field equations to generate the quantum field as a many-particle solution such that the $Φ$-functions represent the particle states. Creation and destruction operators are defined as usual to add or subtract photons from the particle states. The orbital angular momentum of the $Φ$-states is interpreted as spin since it emer…
Exact solution of the master equation for interacting quantized fields at finite temperature decay
本文利用超算符和非幺正变换将有限温度衰减下双量子化场相互作用的Lindblad主方程转化为对角化的有效非厄米哈密顿量形式，求得了精确解，可计算任意初始态演化，并给出了腔内两不可区分光子的符合率。
We show that the standard method of introducing the quantum description of the electromagnetic field -- by canonical field quantization -- is not the only one. We have chosen here the relativistic quantum mechanics of the photon as the starting point. The treatment of photons as elementary particles merges smoothly with the description in terms of the quantized electromagnetic field but it also reveals some essential differences. The most striking result is the appearance of various measures of fidelity for quantum states of photons. These measures are used to characterize the localization of …
James Clerk Maxwell unknowingly discovered a correct relativistic, quantum theory for the light quantum, forty-three years before Einstein postulated the photon's existence. In this theory, the usual Maxwell field is the quantum wave function for a single photon. When the non-operator Maxwell field of a single photon is second quantized, the standard Dirac theory of quantum optics is obtained. Recently, quantum-state tomography has been applied to experimentally determine photon wave functions.
We prove an adiabatic theorem for the ground state of the Dicke model in a slowly rotating magnetic field and show that for weak electron-photon coupling, the adiabatic time scale is close to the time scale of the corresponding two level system--without the quantized radiation field. There is a correction to this time scale which is the Lamb shift of the model. The photon field affect the rate of approach to the adiabatic limit through a logarithmic correction originating from an infrared singularity characteristic of QED.
The exact analytic solutions of the energy eigenvalue equation of the system consisting of a free electron and one mode of the quantized radiation field are used for studying the physical meaning of a class of number-phase minimum uncertainty states. The states of the mode which minimize the uncertainty product of the photon number and the Susskind and Glogower (1964) cosine operator have been obtained by Jackiw (1968). However, these states have so far been remained mere mathematical constructions without any physical significance. It is proved that the most fundamental interaction in quantum…
The purpose of this article is to show that the standard method of introducing the quantum description of the electromagnetic field -- by canonical field quantization -- is not the only one. We have chosen instead as the starting point the relativistic quantum mechanics of photons. Our present understanding of the nature of photons significantly differs from what has been known years ago when the concept of a photon has only been emerging. We show how the description of photons treated as elementary particles merges smoothly with the classical description of the electromagnetic field and leads…
First and second quantized digital quantum simulations of bosonic systems
研究比较玻色子系统一次和二次量子化映射的资源需求，涉及\(k\)体约化密度矩阵等。发现一次量子化映射对\(k\)-RDM非对角项资源需求少，虽二进制一次量子化映射门数随\(M\)增加快，但综合更优，是量子相位估计的有效选择。
We investigate the effects of dynamical Casimir effect in superradiant light scattering by Bose-Einstein condensate in an optomechanical cavity. The system is studied using both classical and quantized mirror motions. The cavity frequency is harmonically modulated in time for both the cases. The main quantity of interest is the number of intracavity scattered photons. The system has been investigated under the weak and strong modulation. It has been observed that the amplitude of the scattered photons is more for the classical mirror motion than the quantized mirror motion. Also, initially, th…
Second-quantized numerical simulations of tunable entanglement in quantum high harmonic generation
本文通过二次量子化方法精确求解HHG中的纠缠问题，展示纠缠随激光功率振荡并可调，揭示长程电子行为对纠缠的影响，为多光子态工程提供新思路。
In a previous work [Phys. Rev. Lett. 123, 047202 (2019)] a translationally invariant framework called quantum-electrodynamical Bloch (QED-Bloch) theory was introduced for the description of periodic materials in homogeneous magnetic fields and strongly coupled to the quantized photon field in the optical limit. For such systems, we show that QED-Bloch theory predicts the existence of fractal polaritonic spectra as a function of the cavity coupling strength. In addition, for the energy spectrum as a function of the relative magnetic flux we find that a terahertz cavity can modify the standard H…
We consider multiphoton dynamics of a quantum system composed of a three-state atom (a qutrit) and a single-mode photonic field in the ultrastrong and deep strong coupling regimes, when the coupling strength is comparable to or larger than the oscillator energy scale. We assume a qutrit to be in a polar-$Λ$ configuration in which two lower levels have mean dipole moments. Direct multiphoton resonant transitions revealing generalized Rabi oscillations, collapse, and revivals in atomic excitation probabilities for the ultrastrong couplings are studied. In the deep strong coupling regime particul…
The quantization of optical fields in vacuum has been known for decades, but extending the field quantization to lossy and dispersive media in nonequilibrium conditions has proven to be complicated due to the position-dependent electric and magnetic responses of the media. In fact, consistent position-dependent quantum models for the photon number in resonant structures have only been formulated very recently and only for dielectric media. Here we present a general position-dependent quantized fluctuational electrodynamics (QFED) formalism that extends the consistent field quantization to desc…
We study quantum dynamics of many-qubit systems strongly coupled to a quantized electromagnetic cavity mode, in the presence of decoherence and dissipation for both fermions and cavity photons. The analytic solutions are derived for a broad class of open quantum systems in Lindblad approximation. They include identical qubits, an ensemble of qubits with a broad distribution of transition frequencies, and multi-level electron systems. Compact analytic solutions for time-dependent quantum state amplitudes and observables become possible with the use of the stochastic equation of evolution for th…
The notion of intrinsic system of coordinates is introduced for the photon from the constraint of transversality condition. The degree of freedom to specify the intrinsic system is extracted from the same constraint, which turns out to be responsible for the spin Hall effect of light. It is shown that the fundamental quantization conditions that break down in the laboratory system of coordinates restore in the intrinsic system, which make it realizable to canonically quantize the radiation field. It is also shown that the dependence of the intrinsic system on the momentum underlies the noncomm…
Due to the potential application in quantum information process, geometric phase of interacting system arouse many interests. Some physicists concentrate on the system in pure classical envi- ronment, while others study the system in pure quantized environment. So a natural question is asked: how about an interacting system in composite environments made up of both classical and quantized field. In this letter, we analyze a quantum system composed of two interacting spins, of which one is in classical magnetic field and the other is in quantized field. First, classical magnetic field driven Be…
We consider an approach in which the usual wave function in the quadrature representation of mode j of the electromagnetic field is further quantized to produce a field operator. Since the electromagnetic field is already second quantized, this corresponds to an additional or third quantization. The third-quantization approach can be used to perform certain quantum optics calculations in the Heisenberg picture that could only be performed in the Schrodinger picture when using the conventional second-quantized theory. This approach also allows an interesting generalization of quantum optics and…
We consider a model for describing a QED system consisting of a photon beam interacting with quantized charged spinless particles. We restrict ourselves by a photon beam that consists of photons with two different momenta moving in the same direction. Photons with each moment may have two possible linear polarizations. The exact solutions correspond to two independent subsystems, one of which corresponds to the electron medium and another one is described by vectors in the photon Hilbert subspace and is representing a set of some quasi-photons that do not interact with each other. In addition,…
Hybrid sub- and superradiant states in emitter arrays with quantized motion
研究在具有量化运动的发射器阵列中亚辐射和超辐射态的形成及其特性，探讨电子和振动激发的混合态。
We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tri-state entanglement are realized near the parametric resonances in a coupled system. The model includes decoherence effects due to coupl…
Dynamics and Resonance Fluorescence from a Superconducting Artificial Atom Doubly Driven by Quantized and Classical Fields
本文实验研究了超导transmon量子比特在量子化场与经典场双重驱动下的共振荧光，通过调控腔内光子数实现驱动场从量子到经典的过渡，观察到边带反交叉和发射谱不对称性，并分析了动力学演化与退相干特性。
Open Quantum Systems Driven by Chirped Pulses: Quantized versus Semiclassical Fields and the Validity of the Rotating-Wave Approximation
研究啁啾快速绝热通道中的布居转移，使用开放量子与半经典模型，检验半经典场描述和旋转波近似的准确性，发现鲁棒的布居转移对参数不敏感。
The polarization analysis of quantized probe light transmitted through an atomic ensemble has been used to prepare entangled collective atomic states. In a "balanced" detection configuration, where the difference signal from two detection ports is analyzed, the continuous monitoring of a component of the Stokes field vector provides a means for conditional projective measurements on the atomic system. Here, we make use of classical driving fields, in the pulsed regime, and of an "unbalanced" detection setup (single detector) where the effective photon number of scattered photons is the detecte…
The dynamics of an atomic few-level system can depend on the phase of driving fields coupled to the atom if certain conditions are satisfied. This is of particular interest to control interference effects, which can alter the system properties considerably. In this article, we discuss the mechanisms of such phase control and interference effects in an atomic three-level system in $Λ$ configuration, where the upper state spontaneously decays into the two lower states. The lower states are coupled by a driving field, which we treat as quantized. This allows for an interpretation on the single ph…
Based on the quantized electromagnetic field described by the Riemann-Silberstein complex vector $F$, we construct the eigenvector set of $% F$, which makes up an orthonormal and complete representation. In terms of $% F $ we then introduce a new operator which can describe the relative ratio of the left-handed and right-handed polarization states of a polarized photon .In $F^{\prime}s$ eigenvector basis the operator manifestly exhibits a behaviour which is similar to a phase difference between two orientations of polarization of a light beam in classical optics.
The quantum oscillator model of electromagnetic excitations revisited
本文重新考察电磁场的量子振子模型，阐明实Maxwell场二次量子化所得Hermitian算符描述局域耦合于费米子物质的光子-反光子对，并指出单光子场应解释为概率幅。
Stability and instability of quantum evolution are studied in the interaction between a two-level atom with photon recoil and a quantized field mode in an ideal cavity, the basic model of cavity quantum electrodynamics (QED). It is shown that the Jaynes-Cummings dynamics can be unstable in the regime of chaotic walking of the atomic center-of-mass in the quantized field of a standing wave in the absence of any kind of interaction with environment. This kind of quantum instability manifests itself in strong variations of reduced quantum purity and entropy, correlating with the respective classi…
Floquet physics from quantized light-matter interaction: geometric phases, gauge consistency, and entanglement
本文通过大光子数相位基表示腔场，证明经典驱动系统的薛定谔方程直接从量子化问题涌现，建立准能量与量子能量的一一对应，并揭示光-物质纠缠编码于Floquet模式关联中。
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