We systematically study the interaction between two quantized optical fields and a cyclic atomic ensemble driven by a classic optical field. This so-called atomic cyclic ensemble consists of three-level atoms with Delta-type transitions due to the symmetry breaking, which can also be implemented in the superconducting quantum circuit by Yu-xi Liu et al. [Phys. Rev. Lett. 95, 087001 (2005)]. We explore the dynamic mechanisms to creating the quantum entanglements among photon states, and between photons and atomic collective excitations by the coherent manipulation of the atom-photon system. It is shown that the quantum information can be completely transferred from one quantized optical mode to another, and the quantum information carried by the two quantized optical fields can be stored in the collective modes of this atomic ensemble by adiabatically controlling the classic field Rabi frequencies.
We describe a theoretical scheme that allows for transfer of quantum states of atomic collective excitation between two macroscopic atomic ensembles localized in two spatially-separated domains. The conception is based on the occurrence of double-exciton dark states due to the collective destructive quantum interference of the emissions from the two atomic ensembles. With an adiabatically coherence manipulation for the atom-field couplings by stimulated Ramann scattering, the dark states will extrapolate from an exciton state of an ensemble to that of another. This realizes the transport of qu…
The symmetric collective states of an atomic spin ensemble (i.e., many-body states that are invariant under particle exchange) are not preserved by decoherence that acts identically but individually on members of the ensemble. We develop a class of collective states in an ensemble of N spin-1/2 particles that is invariant under symmetric local decoherence and find that the dimension of the Hilbert space spanned by these collective states scales only as N^2. We then investigate the open system dynamics of experimentally relevant non-classical collective atomic states, including Schroedinger cat…
When the dynamics of a spin ensemble are expressible solely in terms of symmetric processes and collective spin operators, the symmetric collective states of the ensemble are preserved. These many-body states, which are invariant under particle relabeling, can be efficiently simulated since they span a subspace whose dimension is linear in the number of spins. However, many open system dynamics break this symmetry, most notably when ensemble members undergo identical, but local, decoherence. In this paper, we extend the definition of symmetric collective states of an ensemble of spin-1/2 parti…
We study the collective radiation properties of cold, trapped ensembles of atoms. We consider the high density regime with the mean interatomic distance being comparable to, or smaller than, the wavelength of the resonant optical radiation emitted by the atoms. We find that the emission rate of a photon from an excited atomic ensemble is strongly enhanced for an elongated cloud. We analyze collective single-excitation eigenstates of the atomic ensemble and find that the absorption/emission spectrum is broadened and shifted to lower frequencies as compared to the non-interacting (low density) o…
We propose and analyze a simple method to squeeze dynamically and unconditionally the collective spin of a dilute atomic ensemble by interaction with a driven mode of an optical resonator, as recently demonstrated [I. D. L., M. H. S., and V. V., Phys. Rev. Lett. 104, 073602 (2010)]. We show that substantial squeezing can be achieved in the regime of strong collective ensemble-resonator coupling. The squeezing is ultimately limited either by photon emission into free space or by the curvature of the Bloch sphere. We derive both limits and show where each prevails.
We study the excitation dynamics of an inhomogeneously broadened spin ensemble coupled to a single cavity mode. The collective excitations of the spin ensemble can be described in terms of generalized spin waves and, in the absence of the cavity, the free evolution of the spin ensemble can be described as a drift in the wave number without dispersion. In this article we show that the dynamics in the presence of coupling to the cavity mode can be described solely by a modified time evolution of the wave numbers. In particular, we show that collective excitations with a well- defined wave number…
We analyse the possibility to create two-mode spin squeezed states of two separate spin ensembles by inverting the spins in one ensemble and allowing spin exchange between the ensembles via a near resonant cavity field. We investigate the dynamics of the system using a combination of numerical and analytic calculations, and we obtain squeezing for a wide range of parameters. We also investigate the transfer of the squeezing properties to the cavity field and to an output mode from the cavity. Finally, we investigate how the squeezing is affected by effects of inhomogeneities which would be pre…
We demonstrate deterministic generation of two distinct collective excitations in one atomic ensemble, and we realize the Hong-Ou-Mandel interference between them. Using Rydberg blockade we create single collective excitations in two different Zeeman levels, and we use stimulated Raman transitions to perform a beam-splitter operation between the excited atomic modes. By converting the atomic excitations into photons, the two-excitation interference is measured by photon coincidence detection with a visibility of 0.89(6). The Hong-Ou-Mandel interference witnesses an entangled NOON state of the …
We propose a new physical approach for encoding and processing of quantum information in ensembles of multi-level quantum systems, where the different bits are not carried by individual particles but associated with the collective population of different internal levels. One- and two-bit gates are implemented by collective internal state transitions taking place in the presence of an excitation blockade mechanism which restricts the population of each internal state to the values zero and unity. 10-20 bit quantum computers can be built via this scheme in single trapped clouds of ground state a…
We analyze the magnetic dipole coupling of an ensemble of spins to a superconducting microwave stripline structure, incorporating a Josephson junction based transmon qubit. We show that this system is described by an embedded Jaynes-Cummings model: in the strong coupling regime, collective spin-wave excitations of the ensemble of electrons pick up the nonlinearity of the cavity mode, such that the two lowest eigenstates of the coupled spin-wave + microwave-cavity + Josephson-junction system define a hybrid two-level system. The proposal described here enables the use of spin ensembles as qubit…
We consider the optical generation and verification of entanglement in atomic ensembles under non-uniform interaction between the ensemble and an optical mode. We show that for a wide range of parameters a system of non-uniformly coupled atomic spins can be described as an ensemble of uniformly coupled spins with a reduced effective atom-light coupling and a reduced effective atom number, with a reduction factor of order unity given by the ensemble-mode geometry. This description is valid even for complex entangled states with arbitrary phase-space distribution functions as long as the detecti…
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
We investigate the quantum dynamics of an atomic mixture composed of two multi-atom ensembles. Each ensemble is driven separately by a coherent laser field, respectively, and dampens via the interactions with the environmental vacuum electromagnetic field reservoir. We find that, due to the photon exchange among the two components, long-time excitation oscillations appear, which may be significantly longer than the inverse lifetime of a single emitter. Furthermore, few-atom "jumps" to the excited state occur as a function of the parameter characterizing the inter-component interactions around …
Superradiance, the enhanced collective emission of energy from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study theoretically the enhanced emission of energy from coherent ensembles of harmonic oscillators. We show that it should be possible to observe harmonic oscillator superradiance for the first time in waveguide arrays in integrated photonics. Furthermore, we describe how pairwise correlations within the ensemble can be measured with this architecture. These pairwise correlations are an integral part of the phenomenon of superra…
We study the quantum statistical properties of the collective excitations of an atomic ensemble inside a high-finesse cavity. In the large-detuning regime, it is found that the virtual photon exchange can induce a long-range interaction between atoms, which results in correlated excitations. In particular, the atomic blockade phenomenon occurs when the induced long-range interaction effectively suppresses the double atomic excitation, when the average photon number takes certain values, which makes the two nearest energy levels degenerate. We also show that quantum phase transitions occur in t…
We study the dynamics of a single excitation coherently shared amongst an ensemble of atoms and coupled to a one-dimensional wave guide. The coupling between the matter and the light field gives rise to collective phenomena such as superradiant states with an enhanced initial decay rate, but also to the coherent exchange of the excitation between the atoms. We find that the competition between the two phenomena provides a characteristic dynamics for the decay of the excitations, and remarkably exhibits an algebraic behavior, instead of the expected standard exponential one, for a large number …
We present an analysis of transfer of quantum information between the collective spin degrees of freedom of a large ensemble of two-level systems and a single central qubit. The coupling between the central qubit and the individual ensemble members may be varied and thus provides access to more than a single storage mode. Means to store and manipulate several independent qubits are derived for the case where the variation in coupling strengths does not allow addressing of orthogonal modes of the ensemble. While our procedures and analysis may apply to a number of different physical systems, fo…
The setting of Moessbauer nuclei embedded in thin-film cavities has facilitated an aspiring platform for x-ray quantum optics as shown in several recent experiments. Here, we generalize the theoretical model of this platform that we developed earlier [Phys. Rev. A 88, 043828 (2013)]. The theory description is extended to cover multiple nuclear ensembles and multiple modes in the cavity. While the extensions separately do not lead to qualitatively new features, their combination gives rise to cooperative effects between the different nuclear ensembles and distinct spectral signatures in the obs…
We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting ``dipole blockade'' can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. An example involving a cold Rydberg gas is analyzed.
The hybridization of distinct quantum systems is now seen as an effective way to engineer the properties of an entire system leading to applications in quantum metamaterials, quantum simulation, and quantum metrology. One well known example is superconducting circuits coupled to ensembles of microscopic natural atoms. In such cases, the properties of the individual atom are intrinsic, and so are unchangeable. However, current technology allows us to fabricate large ensembles of macroscopic artificial atoms such as superconducting flux qubits, where we can really tailor and control the properti…
We describe a general technique that allows for an ideal transfer of quantum correlations between light fields and metastable states of matter. The technique is based on trapping quantum states of photons in coherently driven atomic media, in which the group velocity is adiabatically reduced to zero. We discuss possible applications such as quantum state memories, generation of squeezed atomic states, preparation of entangled atomic ensembles and quantum information processing.
Collective effects in the interaction of light with ensembles of identical scatterers play an important role in many fields of physics. However, often the term ``identical'' is not accurate due to the presence of hyperfine fields which induce inhomogeneous transition shifts and splittings. Here we develop a formalism based on the Green function method to model the linear response of such inhomogeneous ensembles in one-dimensional waveguides. We obtain a compact formula for the collective spectrum, which exhibits deviations from the uniform frequency shift and broadening expected of two level s…
The effective Hamiltonian describing resonant interaction of an ensemble of identical quantum particles with a photon-free vacuum electromagnetic field has been obtained with allowance for the second-order terms over the coupling constant (the Stark interaction) by means of the perturbation theory on the basis of the unitary transformation of the system quantum state. It has been shown that in the Markov approximation the effective Hamiltonian terms of the first-order coupling constant are represented as the quantum Wiener process, whereas the second-order terms are expressed by the quantum Po…
The ignition of two-quantum collective emission of inverted sub-ensemble of radiators due to mutual interaction of this sub-ensemble with other two dipole active atomic subsystems in process of two-photon exchanges between the atoms through the vacuum field is proposed. The three particle resonances between two-photon and single quantum transitions of inverted radiators from the ensemble are proposed for acceleration of collective decay rate of bi-photons, obtained relatively dipole-forbidden transitions of excited atomic sub-ensemble. This mutual interaction between three super-fluorescent pr…
We study the three-dimensional nature of the quantum interface between an ensemble of cold, trapped atomic spins and a paraxial laser beam, coupled through a dispersive interaction. To achieve strong entanglement between the collective atomic spin and the photons, one must match the spatial mode of the collective radiation of the ensemble with the mode of the laser beam while minimizing the effects of decoherence due to optical pumping. For ensembles coupling to a probe field that varies over the extent of the cloud, the set of atoms that indistinguishably radiates into a desired mode of the f…
We show that errors are not generated correlatedly provided that quantum bits do not directly interact with (or couple to) each other. Generally, this no-qubits-interaction condition is assumed except for the case where two-qubit gate operation is being performed. In particular, the no-qubits-interaction condition is satisfied in the collective decoherence models. Thus, errors are not correlated in the collective decoherence. Consequently, we can say that current quantum error correcting codes which correct single-qubit-errors will work in most cases including the collective decoherence.
We show that atomic motion leads not only to noticeable quantitative, but in some cases also to qualitative modification of collective effects in dense and cold atomic ensembles even in the case when the characteristic Doppler shifts are tens of times smaller than the natural linewidth. The observed influence is explained as a result of the suppression of the impact of sub-radiant collective states caused by the displacement of the atoms.
We propose a simple heralded amplification scheme for small rotations of the collective spin of an ensemble of particles. Our protocol makes use of two basic primitives for quantum memories, namely partial mapping of light onto an ensemble, and conversion of a collective spin excitation into light. The proposed scheme should be realizable with current technology, with potential applications to atomic clocks and magnetometry.
We propose to use a collective excitation blockade mechanism to identify errors that occur due to disturbances of single atoms in ensemble quantum registers where qubits are stored in the collective population of different internal atomic states. A simple error correction procedure and a simple decoherence-free encoding of ensemble qubits in the hyperfine states of alkali atoms are presented.
We present a theoretical analysis of the intensity autocorrelation for the spontaneous emission from a planar ensemble of self-assembled quantum dots. Using the quantum jump approach, we numerically simulate the evolution of the system and construct photon-photon delay time statistics that approximates the second order correlation function of the field. The form of this correlation function in the case of collective emission from a highly homogeneous ensemble qualitatively differs form that characterizing an ensemble of independent emitters (inhomogeneous ensemble of uncoupled dots). The signa…
The creation of single collective excitations in atomic ensembles via spontaneous Raman emission plays a key role in several quantum communication protocols, starting with the seminal DLCZ protocol [L.-M.Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature {\bf 414}, 413 (2001).] This process is usually analyzed theoretically under the assumptions that the write laser pulse inducing the Raman transition is far off-resonance, and that the atomic ensemble is only homogeneously broadened. Here we study the impact of near-resonance excitation for inhomogeneously broadened ensembles on the collectiv…
In an ensemble of laser-driven atoms involving strongly interacting Rydberg states, the excitation probability is usually strongly suppressed. In contrast, here we identify a regime in which the steady-state Rydberg excited fraction is enhanced by the interaction. This effect is associated with the build-up of many-body coherences, induced by coherent multi-photon excitations between collective states. The excitation enhancement should be observable under currently-existing experimental conditions, and may serve as a direct probe for the presence of coherent multi-photon dynamics involving col…
Abstract We investigate the spectral shift in collective forward scattering for a cold dense atomic cloud. The shift, sometimes called collective Lamb shift, results from resonant dipole-dipole interaction mediated by real and virtual photon exchange, forming many-body states displaying various super- and subradiant spectral behavior. The scattering spectrum reflects the overall radiative behavior from these states. However, it also averages out the radiative details associated with a single collective state, causing ambiguity in explaining the origin of the spectral shift and raising controve…
We report a prolonged coherence time of the collective spin wave of a thermal 87Rb atomic ensemble in a paraffin coated cell. The spin wave is prepared through a stimulated Raman Process. The long coherence time time is achieved by prolonging the lifetime of the spins with paraffin coating and minimize dephasing with optimal experimental configuration. The observation of the long time delayed-stimulated Stokes signal in the writing process suggests the prolonged lifetime of the prepared spins; a direct measurement of the decay of anti-Stokes signal in the reading process shows the coherence ti…
For mesoscopic ensembles containing 100 or more atoms we measure the total atom number and the number of atoms in a specific hyperfine state with single-atom resolution. The measurement detects the atom-induced shift of the resonance frequency of an optical cavity containing the ensemble. This work extends the range of cavity-based detection with single-atom resolution by more than an order of magnitude in atom number, and provides the readout capability necessary for Heisenberg-limited interferometry with atomic ensembles.
Hybrid quantum systems consisting of an ensemble of two--level systems interacting with a single--mode electromagnetic field are important for the development of quantum information processors and other quantum devices. These systems are characterized by the set of energy level hybridizations, split by collective Lamb shifts, that occur when the ensemble and field mode interact coherently with high cooperativity. Computing the full set of Lamb shifts is generally intractable given the high dimensionality of many devices. In this work, we present a set of techniques that allow a compact descrip…
In large ensembles of identical atoms or spins, the interaction with a mode of the electromagnetic radiation field concentrates in a single superradiant degree of freedom with a collectively enhanced coupling. Given a controllable inhomogeneous broadening, such ensembles may be used for multi-mode storage of quantum states of the radiation field with applications in quantum communication networks and quantum computers. In this paper we analyze how the width and shape of the inhomogeneous broadening influence the collective enhancement and the dynamics of the cavity-ensemble system with focus o…
We investigate the collective scattering of coherent light from a thermal alkali-metal vapor with temperatures ranging from 350 to 450 K, corresponding to average atomic spacings between $0.7 λ$ and $0.1 λ$. We develop a theoretical model treating the atomic ensemble as coherent, interacting, radiating dipoles. We show that the two-time second-order correlation function of a thermal ensemble can be described by an average of randomly positioned atomic pairs. Our model illustrates good agreement with the experimental results. Furthermore, we show how fine-tuning of the experimental parameters m…
Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters that are strongly coupled to a photonic mode. However, in these approaches, unavoidable dissipation, like photon loss, blurs nonlinear quantum effects. Here, we generate strongly correlated photon states using only weak coupling and taking advantage of dissipation. We launch light through an ensemble of non-interacting waveguide-coupled atoms, which induce c…
We present a theoretical treatment of light scattering by an ensemble of N dipoles, taking into account recurrent multiple scattering. We study the intrinsic optical properties of collective dipolar systems without specifying a particular illumination condition. We apply this formalism to study the collective absorption modes for an ensemble of small nanoparticles and then to derive collective radiative corrections due to mutual interactions in dipolar ensembles, a topic of major importance in the development of collective nanophotonic systems or atomic networks used as optical clocks.
Current proposals focusing on neutral atoms for quantum computing are mostly based on using single atoms as quantum bits (qubits), while using cavity induced coupling or dipole-dipole interaction for two-qubit operations. An alternative approach is to use atomic ensembles as qubits. However, when an atomic ensemble is excited, by a laser beam matched to a two-level transition (or a Raman transition) for example, it leads to a cascade of many states as more and more photons are absorbed^1. In order to make use of an ensemble as a qubit, it is necessary to disrupt this cascade, and restrict the …
Ramsey interferometry is routinely used in quantum metrology for the most sensitive measurements of optical clock frequencies. Spontaneous decay to the electromagnetic vacuum ultimately limits the interrogation time and thus sets a lower bound to the optimal frequency sensitivity. In dense ensembles of two-level systems the presence of collective effects such as superradiance and dipole-dipole interaction tends to decrease the sensitivity even further. We show that by a redesign of the Ramsey-pulse sequence to include different rotations of individual spins that effectively fold the collective…
We explore how to cool atomic collective excitations in an optically-driven three-level atomic ensemble, which may be described by a model of coupled two harmonic oscillators (HOs) with a time-dependent coupling. Moreover, the coupled two-HO model is further generalized to address other cooling issues, where the lower-frequency HO can be cooled whenever the cooling process dominates over the heating one during the sideband transitions. Unusually, due to the absence of the heating process, the optimal cooling of our first cooling protocol for collective excitations in an atomic ensemble could b…
The dipole blockade of multiple Rydberg excitations in mesoscopic atomic ensembles allows the implementation of various quantum information tasks using collective states of cold, trapped atoms. Precise coherent manipulations of the collective ground and single Rydberg excitation states of an atomic ensemble requires the knowledge of the number of atoms with small uncertainty. We present an efficient method to acquire such information by interrogating the atomic ensemble with resonant pulses while monitoring the resulting Rydberg excitations. We show that after several such steps accompanied by…
We study the spectra of collective low excitations of two atomic ensembles coupled indirectly through a single-mode cavity field. When the left ensemble is driven with an external optical field, its corresponding response spectrum to the incident optical light shows an electromagnetically induced transparency- (EIT-) like phenomenon when the layers are arranged in the sequence of node-antinode but not in the sequence of antinode-node. In the case of antinode-antinode sequence, the response spectrum shows an EIT-like phenomenon with two transparent windows. We also investigate the fluctuation s…
We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build-up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic life…
We study collective effects in an inhomogeneously broadened ensemble of two-level emitters coupled to an optical cavity with narrow linewidth. Using second order mean field theory we find that the emitters within a few times the cavity linewidth exhibit synchronous behaviour and undergo collective Rabi oscillations. Under proper conditions, the synchronized oscillations give rise to a modulated intracavity field which can excite emitters detuned by many linewidths from the cavity resonance. To study the synchronization in further detail, we simplify the model and consider two ensembles and stu…
We report on the observation of quantum interference of a collective single spin excitation with a spin ensemble of $N_{\text{atom}} =10^5$ atoms. Detection of a single photon scattered from the atoms creates the single spin excitation, a Fock state embedded in the collective spin of the ensemble. The state of the atomic ensemble is then detected by tomography via a quantum non-demolition measurement of the collective spin. A macroscopic difference of the order of $\sqrt{N_{\text{atom}}}$ in the marginal distribution of the collective spin state arises from the interference between the single …
We theoretically investigate an ensemble of three-level room-temperature atoms in a two-mode optical cavity, focusing on the case of counterpropagating light fields. We find that in the limit of large detunings the problem admits relatively simple and intuitive solutions. When a classical field drives one of the transitions, the system becomes equivalent to an ensemble of two-level atoms with suppressed Doppler broadening. In contrast, when the same transition is driven with a single photon, the system collectively behaves like a single two-level atom. This latter result is particularly releva…
Rayleigh scattering is usually considered to be the elastic scattering of photons from sub-wavelength physical objects, such as small particles or molecules. Here, we present the spectroscopic study of the scattering properties of molecules embedded in an optical cavity under strong coupling conditions, where the collective interaction between the molecules and the cavity gives rise to composite light-matter excitations known as cavity polaritons. We show that the polaritonic states exhibit strong resonant Rayleigh scattering, reaching 25% efficiency. Since the polaritonic wavefunctions in suc…
