Abstract We investigate the spectral shift in collective forward scattering for a cold dense atomic cloud. The shift, sometimes called collective Lamb shift, results from resonant dipole-dipole interaction mediated by real and virtual photon exchange, forming many-body states displaying various super- and subradiant spectral behavior. The scattering spectrum reflects the overall radiative behavior from these states. However, it also averages out the radiative details associated with a single collective state, causing ambiguity in explaining the origin of the spectral shift and raising controversy on its scaling property. We employ a Monte-Carlo simulation to study how the collective states are occupied and contribute to emission. We thus distinguish two kinds of collective shift that follow different scaling laws. One results from dominant occupation of the near-resonant collective states. This shift is usually small and insensitive to the density or the number of participating atoms. The other comes from large spatial correlation of dipoles, associated with the states of higher degree of emission. This corresponds to larger collective shift that is approximately linearly dependent on the optical depth. Our analysis provides not only a novel perspective for the spectral features in collective scattering, but also a possible resolution to the controversy on the scaling property that has been reported elsewhere because of different origins.
Resonant dipole-dipole interaction (RDDI) is ubiquitous in light-matter interacting systems and is responsible for many fascinating properties of collective radiations. Here we theoretically investigate the role of RDDI in electromagnetically induced transparency (EIT). The resonant dipole-dipole interactions manifest in the cooperative spontaneous emission of the probe light transition, which give rise a broadened linewidth and associated collective frequency shift. This cooperative linewidth originates from the nonlocal and long-range RDDI, which can be determined by the atomic density, opti…
On the basis of a quantum microscopic approach we study the cooperative effects induced by the dipole-dipole interaction in an ensemble of point-like impurity centers located near a charged perfectly conducting surface. We analyze the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the transition spectrum of an excited atom inside an ensemble and on the radiation trapping. We show that the electric field modifies the cooperative Lamb shift, as well as the character of sub- and superradiant decay. We also demonstrate …
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions between Rydberg pairs onto the optical field. We characterize the non-linearity as a function of electric field and density, and demonstrate the enhancement of the optical non-linearity due to cooperativity.
Multiparticle entangled states generated via interaction between narrow-band light and an ensemble of identical two-level atoms are considered. Depending on the initial photon statistics, correlation between atoms and photons can give rise to entangled states of these systems. It is found that the state of any pair of atoms interacting with weak single-mode squeezed light is inseparable and robust against decay. Optical schemes for preparing entangled states of atomic ensembles by projective measurement are described.
On the basis of the general quantum microscopic theory we study the process of spontaneous decay of an excited atom in a dense and disordered ensemble of point-like impurity atoms embedded into transparent dielectric and located near a charged perfectly conducting surface. We have analyzed the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the character of interatomic dipoledipole interaction. This leads to the modification of the transition spectrum of an excited atom inside an ensemble and the spontaneous decay dy…
By coupling a probe transition to a Rydberg state using electro-magnetically induced transparency (EIT) we map the strong dipole-dipole interactions onto an optical field. We characterize the resulting cooperative optical non-linearity as a function of probe strength and density. We show that the effect of dipole blockade cannot be described using a mean-field but requires an $N$-atom cooperative model. Good quantitative agreement is obtained for three atoms per blockade with the $n=60$ Rydberg state. We place an upper-limit on the dephasing rate of the blockade spheres of $<110$ kHz.
The influence of evanescent waves on the nature of optical cooperative effects in atomic ensembles in a waveguide
Peter the Great St. Petersburg Polytechnic University（圣彼得堡彼得大帝理工大学）；Institute for Analytical Instrumentation of RAS（俄罗斯科学院分析仪器研究所）；Ioffe Institute（约费研究所）
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of the Stokes fields from the two cells, after they interfere on a beam splitter. The entanglement of the collective atomic fields can be transferred to the anti-Stokes fields in a readout process. By measuring the operator moments of the anti-Stokes fields, we can verify the presence of entanglement. We model the effects of practical factors such as Stokes fiel…
The one-dimensional homonuclear periodic array of nuclear spins I = 1/2, owing to hyperfine interaction of nuclear spins with electronic magnetic moments in antiferromagnetic structure, is considered. The neighbor nuclear spins in such array are opposite oriented and have resonant frequencies determined by hyperfine interaction constant, applied magnetic field value and interaction with the left and right nuclear neighbor spins. The resonant frequencies difference of nuclear spins, when the neighbor spins have different and the same states, is used to control the spin dynamics by means of sele…
We propose a scheme that employs dissipation to deterministically generate entanglement in an ensemble of strongly interacting Rydberg atoms. With a combination of microwave driving between different Rydberg levels and a resonant laser coupling to a short lived atomic state, the ensemble can be driven towards a dark steady state that entangles all atoms. The long-range resonant dipole-dipole interaction between different Rydberg states extends the entanglement beyond the van der Walls interaction range with perspectives for entangling large and distant ensembles.
We describe an efficient numerical method for simulating the dynamics of interacting spin ensembles in the presence of dephasing and decay. The method builds on the discrete truncated Wigner approximation for isolated systems, which combines the mean-field dynamics of a spin ensemble with a Monte Carlo sampling of discrete initial spin values to account for quantum correlations. Here we show how this approach can be generalized for dissipative spin systems by replacing the deterministic mean-field evolution by a stochastic process, which describes the decay of coherences and populations while …
Photoionization of an atom via interatomic correlations to N neighboring atoms may be strongly enhanced due to constructive interference of quantum pathways. The ionization proceeds via resonant photoexcitation of a neighbor atom and subsequent interatomic Coulombic decay. The enhancement can scale with N^2, leading to "super-enhanced photoionization".
In a closely packed ensemble of quantum emitters, cooperative effects are typically suppressed due to the dephasing induced by the dipole-dipole interactions. Here, we show that by adding sufficiently strong collective dephasing cooperative effects can be restored. In particular, we show that the dipole force on a closely packed ensemble of strongly driven two-level quantum emitters, which collectively dephase, is enhanced in comparison to the dipole force on an independent non-interacting ensemble. Our results are relevant to solid state systems with embedded quantum emitters such as colour c…
An ensemble of multilevel atoms is a good candidate for a quantum information storage device. The information is encrypted in the collective ground state atomic coherence, which, in the absence of external excitation, is decoupled from the vacuum and therefore decoherence free. However, in the process of manipulation of atoms with light pulses (writing, reading), one inadvertently introduces a coupling to the environment, i.e. a source of decoherence. The dissipation process is often treated as an independent process for each atom in the ensemble, an approach which fails at large atomic optica…
We show that two groups of slow two-level atoms in a weak resonant laser field, are entangled. The considered groups can be separated by a macroscopic distance, and be parts of a larger atomic ensemble. In a dilute regime, for two very distant groups of atoms, in a plane wave laser beam, we determine the maximum attainable entanglement negativity, and a laser intensity below which they are certainly entangled. They both decrease with increasing distance between the two groups, but increase with enlarging groups sizes. As a consequence, for given laser intensity, far separated groups of atoms a…
Quantum theoretical treatment of coherent forward scattering of light in a polarized atomic ensemble with an arbitrary angular momentum is developed. We consider coherent forward scattering of a weak radiation field interacting with a realistic multi-level atomic transition. Based on the concept of an effective Hamiltonian and on the Heisenberg formalism, we discuss the coupled dynamics of the quantum fluctuations of the polarization Stokes components of propagating light and of the collective spin fluctuations of the scattering atoms. We show that in the process of coherent forward scattering…
We study photon emission by an ensemble of two-level systems, with strong inhomogeneous broadening and coupled to a cavity mode whose frequency has linear time-dependence. The analysis shows that, regardless the distribution of energy level splittings, a sharp phase transition occurs between the weak and strong cooperative emission phases near a critical photonic frequency sweeping rate. The associated scaling exponent is determined. We suggest that this phase transition can be observed in an ensemble of negatively charged NV centers in diamond interacting with a microwave half-wavelength cavi…
We discuss the generation of two-atom entanglement inside a resonant microcavity under stimulated emission (STE) interaction. The amount of entanglement is shown based on different atomic initial state. For each kind of intial state, we obtain the entanglement period and the entanglement critical point, which are found to deeply depend on driving field density. In case of atomic state $| ee >$, the entanglement can be induced due to STE. In case of atomic state $| eg >$, there is a competition between driving field indued entanglement and STE induced entanglement. When two atoms are initially …
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
We report on the direct observation of resonant electric dipole-dipole interactions in a cubic array of atoms in the many-excitation limit. The interactions, mediated by single-atom couplings to the shared electromagnetic vacuum, are shown to produce spatially-dependent cooperative Lamb shifts when spectroscopically interrogating the mHz-wide optical clock transition in strontium-87. We show that the ensemble-averaged shifts can be suppressed below the level of evaluated systematic uncertainties for state-of-the-art optical atomic clocks. Additionally, we demonstrate that excitation of the ato…
We study theoretically the scattering of light by an ensemble of $N$ resonant atoms in a sub-wavelength volume. We consider the low intensity regime so that each atom responds linearly to the field. While $N$ non-interacting atoms would scatter $N^2$ more than a single atom, we find that $N$ interacting atoms scatter less than a single atom near resonance. In addition, the scattered power presents strong fluctuations, either from one realization to another or when varying the excitation frequency. We analyze this counter-intuitive behavior in terms of collective modes resulting from the light-…
We propose a scheme for realizing quantum repeaters with Rydberg-blockade coupled atomic ensembles, based on a recently proposed collective encoding strategy. Rydberg-blockade mediated two-qubit gates and efficient cooperative photon emission are employed to create ensemble-photon entanglement. Thanks to deterministic entanglement swapping operations via Rydberg-based two-qubit gates, and to the suppression of multi-excitation errors by the blockade effect, the entanglement distribution rate of the present scheme is higher by orders of magnitude than the rates achieved by other ensemble-based …
We present here a microscopic analysis of the cooperative light scattering on an atomic system consisting of Λ-type configured atoms with the spin-degenerate ground state. The results are compared with a similar system consisting of standard "two-level" atoms of the Dicke model. We discuss advantages of the considered system in context of its possible implications for light storage in a macroscopic ensemble of dense and ultracold atoms.
We demonstrate cavity sideband cooling of a single collective motional mode of an atomic ensemble down to a mean phonon occupation number of 2.0(-0.3/+0.9). Both this minimum occupation number and the observed cooling rate are in good agreement with an optomechanical model. The cooling rate constant is proportional to the total photon scattering rate by the ensemble, demonstrating the cooperative character of the light-emission-induced cooling process. We deduce fundamental limits to cavity-cooling either the collective mode or, sympathetically, the single-atom degrees of freedom.
We analyze the creation of spin squeezed atomic ensembles by simultaneous dispersive interactions with several optical frequencies. A judicious choice of optical parameters enables optimization of an interferometric detection scheme that suppresses inhomogeneous light shifts and keeps the interferometer operating in a balanced mode that minimizes technical noise. We show that when the atoms interact with two-frequency light tuned to cycling transitions the degree of spin squeezing $ξ^2$ scales as $ξ^2\sim 1/d$ where $d$ is the resonant optical depth of the ensemble. In real alkali atoms there …
We show that a cooperative atom response in an optical lattice to resonant incident light can be employed for precise control and manipulation of light on a subwavelength scale. Specific collective excitation modes of the system that result from strong light-mediated dipole-dipole interactions can be addressed by tailoring the spatial phase-profile of the incident light. We demonstrate how the collective response can be used to produce optical excitations at well-isolated sites on the lattice.
A new scheme of photon echo based quantum memory in the optimal optical QED cavity with off-resonant Raman atomic transition is proposed. The scheme employs the atomic ensembles characterized by an optically thin resonant transition and natural inhomogeneous broadening of the resonant line composed of the arbitrary narrow homogeneous spectral components. The scheme provides robust and quite simple coherent control of the light-atoms dynamics that can be implemented by using an existing optical technique and opens a practical way for realization of the efficient long-lived multi-mode optical qu…
Spins bound to point defects are increasingly viewed as an important resource for solid-state implementations of quantum information technologies. In particular, there is a growing interest in the identification of new classes of defect spin that can be controlled optically. Here we demonstrate ensemble optical spin polarization and optically detected magnetic resonance (ODMR) of the S = 1 electronic ground state of chromium (Cr4+) impurities in silicon carbide (SiC) and gallium nitride (GaN). Spin polarization is made possible by the narrow optical linewidths of these ensembles (< 8.5 GHz), w…
Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical emission were observed. Under relatively weak pumping and high medium density, when the condition of strong coupling between field and resonant matter is fulfilled, the probe amplification spectrum has a form of spectral doublet. Stronger pumping leads to the appearance of a single peak of the probe beam amplification at the transition frequency. The greater…
Long-range quantum communication requires the development of in-out light-matter interfaces to achieve a quantum advantage in entanglement distribution. Ideally, these quantum interconnections should be as fast as possible to achieve high-rate entangled qubits distribution. Here, we demonstrate the coherent quanta exchange between single photons generated on-demand from a GaAs quantum dot and atomic ensemble in a $^{87}$Rb vapor quantum memory. Through an open quantum system analysis, we demonstrate the mapping between the quantized electric field of photons and the coherence of the atomic ens…
The spontaneous creation and persistence of ground-state coherence in an ensemble of intracavity Rb atoms has been observed as a quantum beat. Our system realizes a quantum eraser, where the detection of a first photon prepares a superposition of ground-state Zeeman sublevels, while detection of a second erases the stored information. Beats appear in the time-delayed photon-photon coincidence rate (intensity correlation function). We study the beats theoretically and experimentally as a function of system parameters, and find them remarkably robust against perturbations such as spontaneous emi…
We analyse the possibility to create two-mode spin squeezed states of two separate spin ensembles by inverting the spins in one ensemble and allowing spin exchange between the ensembles via a near resonant cavity field. We investigate the dynamics of the system using a combination of numerical and analytic calculations, and we obtain squeezing for a wide range of parameters. We also investigate the transfer of the squeezing properties to the cavity field and to an output mode from the cavity. Finally, we investigate how the squeezing is affected by effects of inhomogeneities which would be pre…
The setting of Moessbauer nuclei embedded in thin-film cavities has facilitated an aspiring platform for x-ray quantum optics as shown in several recent experiments. Here, we generalize the theoretical model of this platform that we developed earlier [Phys. Rev. A 88, 043828 (2013)]. The theory description is extended to cover multiple nuclear ensembles and multiple modes in the cavity. While the extensions separately do not lead to qualitatively new features, their combination gives rise to cooperative effects between the different nuclear ensembles and distinct spectral signatures in the obs…
In this paper we show that three cavity fields can be entangled when they are tuned on resonance with an ensemble of dressed three-level atoms. The master equation for the three cavity modes is derived by using atomic dressed states and the inseparability of the three output cavity modes is described by using a sufficient criterion proposed by van Loock and Furusawa. The physical cause is the atomic coherence effects, by which the quantum correlations are created in the field dynamics.
We report coherent interactions within an ensemble of silicon-vacancy color centers in diamond. The interactions are ascribed to resonant dipole-dipole coupling. Further, we demonstrate control over resonant center pairs by using a driving optical pulse to induce collective, interaction-enabled Rabi-oscillations in the ensemble. Non-resonant center pairs do not undergo collective oscillations.
We theoretically analyze the experimental observations of a spectral line collapse in a metamaterial array of asymmetric split ring resonators [Fedotov et al., Phys. Rev. Lett. 104, 223901 (2010)]. We show that the ensemble of closely-spaced resonators exhibits cooperative response, explaining the observed system-size dependent narrowing of the transmission resonance linewidth. We further show that this cooperative narrowing depends sensitively on the lattice spacing and that significantly stronger narrowing could be achieved in media with suppressed ohmic losses.
We study the contributions of off-resonant transitions to the dynamics of a system of N multilevel atoms sharing one excitation and interacting with the quantized vector electromagnetic field. The Rotating Wave Approximation significantly simplifies the derivation of the equations of motion describing the collective atomic dynamics, but it leads to an incorrect expression for the dispersive part of the atom-atom interaction terms. For the case of two-level atoms and a scalar electromagnetic field, it turns out that the atom-atom interaction can be recovered correctly if integrals over the phot…
Optical depth dictates universal bounds on many-body decay in atomic ensembles
Instituto de Física Fundamental - Consejo Superior de Investigaciones Científica (CSIC)（基础物理研究所 - 西班牙国家研究委员会）；Department of Physics, Columbia University（哥伦比亚大学物理系）；Institute for Quantum Information and Matter, California Institute of Technology（加州理工学院量子信息与物质研究所）；Department of Physics, Harvard University（哈佛大学物理系）；Physikalisches Institut, University of Bonn（波恩大学物理研究所）
We report enhanced transmission in measurements of the spectral dependence of forward light scattering by a high-density and cold ensemble of 87Rb atoms. This phenomenon, which is a result of dipole-dipole interaction induced cooperative light scattering in the atomic sample, implies a significant departure from the traditional density dependence of the transmitted light as embodied in the Beer-Lambert Law. Absolute values of the density-dependent forward light scattering cross-section are extracted from the measurements.
On the basis of general theoretical results developed previously in [JETP 112, 246 (2011)], we analyze the reflection of quasiresonant light from a plane surface of dense and disordered ensemble of motionless point scatters. Angle distribution of the scattered light is calculated both for s and p polarizations of the probe radiation. The ratio between coherent and incoherent (diffuse) components of scattered light is calculated. We analyze the contributions of scatters located at different distances from the surface and determine on this background the thickness of surface layer responsible fo…
Cavity-assisted storage and retrieval of single-photon wave packets in optically thin spatially extended resonant materials are analyzed. It is shown that the use of cavity tuning allows one to store and recall time-symmetric double-sided exponential pulses with near unit efficiency. The optimal regime of the cavity tuning is determined and the effect of time jitter on the storage efficiency is analyzed.
We investigate the cooperative behavior of regular monolayers of driven two-level dipoles, using classical electrodynamics simulations. The dipolar response results from the interference of many cooperative eigenmodes, each frequency-shifted from the single resonant dipole case, and with a modified lifetime, due to the interactions between dipoles. Of particular interest is the kagome lattice, where the semiregular geometry permits simultaneous excitation of two dominant modes, one strongly subradiant, leading to an electromagnetically-induced-transparency-like interference in a two-level syst…
We examine the possibility of coherent, reversible information transfer between solid-state superconducting qubits and ensembles of ultra-cold atoms. Strong coupling between these systems is mediated by a microwave transmission line resonator that interacts near-resonantly with the atoms via their optically excited Rydberg states. The solid-state qubits can then be used to implement rapid quantum logic gates, while collective metastable states of the atoms can be employed for long-term storage and optical read-out of quantum information.
