In this paper we investigate decoherence times of a double quantum dot (DQD) charge qubit due to it coupling with acoustic phonon baths. We individually consider the acoustic piezoelectric as well as deformation coupling phonon baths in the qubit environment. The decoherence times are calculated with two kinds of methods. One of them is based on the qusiadiabatic propagator path integral (QUAPI) and the other is based on Bloch equations, and two kinds of results are compared. It is shown that the theoretical decoherence times of the DQD charge qubit are shorter than the experimental reported results. It implies that the phonon couplings to the qubit play a subordinate role, resulting in the decoherence of the qubit.
We show that the influence of the shared phonon bath considered in H. Hossein-Nejad and G. D. Scholes, New J. Phys. 12, 065045 (2010) on the exciton transfer in a two-molecule system can be reproduced by that of an independent bath model.
A technique to measure the decoherence time of optical phonons in a solid is presented. Phonons are excited with a pair of time delayed 80 fs, near infrared pulses via spontaneous, transient Raman scattering. The fringe visibility of the resulting Stokes pulse pair, as a function of time delay, is used to measure the phonon dephasing time. The method avoids the need to use either narrow band or few femtosecond pulses and is useful for low phonon excitations. The dephasing time of phonons created in bulk diamond is measured to be tau = 6.8ps (1.56cm-1).
We apply modern techniques from quantum optics and quantum information science to Bose-Einstein Condensates (BECs) in order to study, for the first time, the quantum decoherence of phonons of isolated BECs. In the last few years, major advances in the manipulation and control of phonons have highlighted their potential as carriers of quantum information in quantum technologies, particularly in quantum processing and quantum communication. Although most of these studies have focused on trapped ion and crystalline systems, another promising system that has remained relatively unexplored is BECs.…
Recently, de Visser and Blaauboer [Phys. Rev. Lett. {\bf 96}, 246801 (2006)] proposed the most efficient deterministic teleportation protocol $\cal T$ for electron spins in a semiconductor nanostructure consisting of a single and a double quantum dot. However, it is as yet unknown if $\cal T$ can be completed before decoherence sets in. In this paper we analyze the detrimental effect of nuclear spin baths, the main source of decoherence, on $\cal T$. We show that nonclassical teleportation fidelity can be achieved with $\cal T$ provided certain conditions are met. Our study indicates that real…
We show how to improve the efficiency for preparing Bell states in coupled two quantum dots system. A measurement to the state of driven quantum laser field leads to wave function collapse. This results in highly efficiency preparation of Bell states. The effect of decoherence on the efficiency of generating Bell states is also discussed in this paper. The results show that the decoherence does not affect the relative weight of $|00>$ and $|11>$ in the output state, but the efficiency of finding Bell states.
We present an all-optical implementation of quantum computation using semiconductor quantum dots. Quantum memory is represented by the spin of an excess electron stored in each dot. Two-qubit gates are realized by switching on trion-trion interactions between different dots. State selectivity is achieved via conditional laser excitation exploiting Pauli exclusion principle. Read-out is performed via a quantum-jump technique. We analyze the effect on our scheme's performance of the main imperfections present in real quantum dots: exciton decay, hole mixing and phonon decoherence. We introduce a…
By using the Redfield form of the master equation, we investigate the decoherence times of a double quantum dot charge qubit (DQDCQ) in three different cases, namely when it is coupled to (I) the piezoelectric coupling phonon bath (PCPB), (II) the deformation coupling phonon bath (DCPB), and (III) the Ohmic bath. It is found that our results for case (I) and (II) are in the same magnitude with those obtained via the exact path integral methods, while for case (III), the decoherence time is in well agreement with the experimental value.
We introduce an exactly solvable model to study decoherence of a central spin interacting with a spin bath where the coupling is mediated by phonons which we assume to be in a coherent state or thermal distribution. For the coherent state case, we find that the decoherence factor decays in a Gaussian fashion and it becomes independent of the phonon frequencies at short times. If the phonon energies are much larger than spin-phonon coupling or bath spins are fully polarized, decoherence time becomes independent of the initial phonon state. For the thermal state case, phonons play more important…
The dynamics of coherent electron-phonon (el-ph) states is investigated for a suspended nanostructure. Exact quantum dynamics calculations reveal that electron and phonons (comprising a thermal bath) couple quantum mechanically to perform coherent oscillations with periods in the range of tens of nanoseconds, despite the finite temperature of the phonon bath. Mechanical energy dissipation due to clamping loss is taken into account in the calculations. Although the lifetime of the coupled el-ph states decreases with the temperature, well defined Rabi oscillations are obtained for temperatures u…
We analyze decoherence of an electron in a double-dot due to the interaction with acoustic phonons. For large tunneling rates between the quantum dots, the main contribution to decoherence comes from the phonon emission relaxation processes, while for small tunneling rates, the virtual-phonon, dephasing processes dominate. Our results show that in common semiconductors, such as Si and GaAs, the latter mechanism determines the upper limit for the double-dot charge qubit performance measure.
We review results on evaluation of loss of information in quantum registers due to their interactions with the environment. It is demonstrated that an optimal measure of the level of quantum noise effects can be introduced via the maximal absolute eigenvalue norm of deviation of the density matrix of a quantum register from that of ideal, noiseless dynamics. For a semiconductor quantum dot charge qubits interacting with acoustic phonons, explicit expressions for this measure are derived. For a broad class of environmental modes, this measure is shown to have the property that for small levels …
We predict dominating cooperative two-photon emission from two quantum dots coupled with a single mode photonic crystal cavity. The cooperative two photon emission occurs when excitons in two off-resonantly coupled quantum dots decay simultaneously. The interaction with common cavity field leads to cavity induced two-photon emission which is strongly inhibited by electron phonon coupling. The interaction with common phonon bath produces phonon induced two-photon emission which increases on increasing temperature. For identical quantum dots cavity induced two-photon emission is negligible but p…
We discuss decoherence in charge qubits formed by multiple lateral quantum dots in the framework of the spin-boson model and the Born-Markov approximation. We consider the intrinsic decoherence caused by the coupling to bulk phonon modes. Two distinct quantum dot configurations are studied: (i) Three quantum dots in a ring geometry with one excess electron in total and (ii) arrays of quantum dots where the computational basis states form multipole charge configurations. For the three-dot qubit, we demonstrate the possibility of performing one- and two-qubit operations by solely tuning gate vol…
Many quantum dot qubits operate in regimes where the energy splittings between qubit states are large and phonons can be the dominant source of decoherence. The recently proposed charge quadrupole qubit, based on one electron in a triple quantum dot, employs a highly symmetric charge distribution to suppress the influence of charge noise. To study the effects of phonons on the charge quadrupole qubit, we consider Larmor and Ramsey pulse sequences to identify favorable operating parameters. We show that it is possible to implement typical gates with $>99.99\%$ fidelity in the presence of phonon…
We study the effect of decoherence on a weak value measurement in a paradigm system consisting of a double quantum dot continuously measured by a quantum point contact. Fluctuations of the parameters controlling the dot state induce decoherence. We find that, for measurements longer than the decoherence time, weak values are always reduced within the range of the eigenvalues of the measured observable. For measurements at shorter time scales, the measured weak value strongly depends on the interplay between the decoherence dynamics of the system and the detector backaction. In particular, depe…
Recent experiments by Hayashi et al. [Phys. Rev. Lett. 91, 226804 (2003)] demonstrate coherent oscillations of a charge quantum bit (qubit) in laterally defined quantum dots. We study the intrinsic electron-phonon decoherence and gate performance for the next step: a system of two coupled charge qubits. The effective decoherence model contains properties of local as well as collective decoherence. Decoherence channels can be classified by their multipole moments, which leads to different low-energy spectra. It is shown that due to the super-Ohmic spectrum, the gate quality is limited by the si…
Coherent single electron spin oscillation in a double quantum dot system driven by a magnetic electron spin resonance field is studied theoretically using a Bloch-type rate equation approach. The oscillation frequency and relaxation time obtained using typical model parameters are consistent with experiment findings. The dominant decoherence mechanism is identified to be a leakage current through a Coulomb blockade barrier at a quantum dot during the spin manipulation. Nuclear field fluctuations which induce a long relaxation time are found to contribute only negligibly to the decoherence desp…
We discuss the coherent splitting and recombining of a nanoparticle in a mesoscopic "closed-loop" Stern-Gerlach interferometer in which the observable is the spin of a single impurity embedded in the particle. This spin, when interacting with a pulsed magnetic gradient, generates the force on the particle. We calculate the internal decoherence which arises as the displaced impurity excites internal degrees of freedom (phonons) that may provide Welcher Weg information and preclude interference. We estimate the constraints this decoherence channel puts on future interference experiments with mas…
Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted emission. Here, we study theoretically and experimentally the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity as a function of temperature. We show that a large coupling to a high quality factor cavity can simultaneously reduce the effect of both phonon-induced sources of decoherence. It first limits the effect of pure dephasi…
Paramagnetic defects in diamond and hexagonal boron nitride possess a unique combination of spin and optical properties that make them prototypical solid-state qubits. Despite the coherence of these spin qubits being critically limited by spin-phonon relaxation, a full understanding of this process is not yet available. Here we apply ab initio spin dynamics simulations to this problem and quantitatively reproduce the experimental temperature dependence of spin relaxation time and spin coherence time. We demonstrate that low-frequency two-phonon modulations of the zero-field splitting are respo…
We theoretically study the nuclear spin induced decoherence of a quantum dot in Si that is confined at a SiGe interface. We calculate decoherence time dependence on $^{73}$Ge in the barrier layer to evaluate the importance of Ge as well as Si enrichment for long decoherence times. We use atomistic tight-binding modeling for an accurate account of the electron wavefunction which is particularly important for determining the contact hyperfine interactions with the Ge nuclear spins. We find decoherence times due to Ge spins at natural concentrations to be milliseconds. This suggests SiGe/Si quant…
We discuss decoherence due to electromagnetic fluctuations in charge qubits formed by two lateral quantum dots. We use an effective circuit model to evaluate correlations of voltage fluctuations in the qubit setup. These correlations allows us to estimate energy (T1) and phase (T2) relaxation times of the the qubit system. Our theoretical estimate of the quality factor due to dephasing by electromagnetic fluctuations yields values much higher than those found in recent experiments, indicating that other sources of decoherence play a dominant role.
We propose a method based on optically detected magnetic resonance (ODMR) to measure the decoherence time $T_{2}$ of a single electron spin in a semiconductor quantum dot. The electron spin resonance (ESR) of a single excess electron on a quantum dot is probed by circularly polarized laser excitation. Due to Pauli blocking, optical excitation is only possible for one of the electron-spin states. The photoluminescence is modulated due to the ESR which enables the measurement of electron spin decoherence. We study different possible schemes for such an ODMR setup.
We uncover two microscopic physical settings with significant pure spin decoherence. First, for quantum dots (QD) electrostatically confined in two-dimensional hole gas, decoherence comes from qubit spin-orbit (SO) coupling to phonons, whose decay due to free charge carriers in contacts is described by Ohmic weighted phonon spectral function. We derive significant SO interactions affecting holes with origin and symmetry distinct from that of conventionally considered Dresselhaus and Rashba terms. In the second setting of electron or hole QDs coupled to a linear chain of atoms, decoherence is d…
We demonstrate that an optically driven spin of a carrier in a quantum dot undergoes indirect dephasing via conditional optically induced charge evolution even in the absence of any direct interaction between the spin and its environment. A generic model for the indirect dephasing with a three-component system with spin, charge, and reservoir is proposed. This indirect decoherence channel is studied for the optical spin manipulation in a quantum dot with a microscopic description of the charge-phonon interaction taking into account its non-Markovian nature.
We study theoretically the phonon-induced relaxation and decoherence of spin states of two electrons in a lateral double quantum dot in a SiGe/Si/SiGe heterostructure. We consider two types of singlet-triplet spin qubits and calculate their relaxation and decoherence times, in particular as a function of level hybridization, temperature, magnetic field, spin orbit interaction, and detuning between the quantum dots, using Bloch-Redfield theory. We show that the magnetic field gradient, which is usually applied to operate the spin qubit, may reduce the relaxation time by more than an order of ma…
We study decoherence in an interacting qubit system described by infinite range Heisenberg model (IRHM) in a situation where the system is coupled to a bath of local optical phonons. Using perturbation theory in polaron frame of reference, we derive an effective Hamiltonian that is valid in the regime of strong spin-phonon coupling under non-adiabatic conditions. It is shown that the effective Hamiltonian commutes with the IRHM upto leading orders of perturbation and thus has the same eigenstates as the IRHM. Using a quantum master equation with Markovian approximation of dynamical evolution, …
We study two anisotropically interacting spins coupled to optical phonons; we restrict our analysis to the regime of strong coupling to the environment, to the antiadiabatic region, and to the subspace with zero value for $S^z_T$ (the z-component of the total spin). In the case where each spin is coupled to a different phonon bath, we assume that the system and the environment are initially uncorrelated (and form a simply separable state) in the polaronic frame of reference. By analyzing the {polaron} dynamics through non-Markovian quantum master equation, we find that the system manifests a s…
We present a theoretical model for the dynamics of an electron that gets trapped by means of decoherence and quantum interference in the central quantum dot (QD) of a semiconductor nanoring (NR) made of five QDs, between 100 K and 300 K. The electron's dynamics is described by a master equation with a Hamiltonian based on the tight-binding model, taking into account electron-LO phonon interaction (ELOPI). Based on this configuration, the probability to trap an electron with no decoherence is almost 27%. In contrast, the probability to trap an electron with decoherence is 70% at 100 K, 63% at 2…
We theoretically investigate the spin dynamics of a heavy hole confined to an unstrained III-V semiconductor quantum dot and interacting with a narrowed nuclear-spin bath. We show that band hybridization leads to an exponential decay of hole-spin superpositions due to hyperfine-mediated nuclear pair flips, and that the accordant single-hole-spin decoherence time T2 can be tuned over many orders of magnitude by changing external parameters. In particular, we show that, under experimentally accessible conditions, it is possible to suppress hyperfine-mediated nuclear-pair-flip processes so strong…
Understanding coherent dynamics of excitons, spins, or hard-core bosons (HCBs) has tremendous scientific and technological implications for light harvesting and quantum computation. Here, we study decay of excited-state population and decoherence in two models for HCBs, namely: an infinite-range HCB model governed by Markovian dynamics and a two-site HCB model with site-dependent strong potentials and subject to non-Markovian dynamics. Both models are investigated in the regimes of antiadiabaticity and strong HCB-phonon coupling with each site providing a different local optical phonon environ…
We develop a general microscopic theory describing the phonon decoherence of quantum dots and indistinguishability of the emitted photons in photonic structures. The coherence is found to depend fundamentally on the dimensionality of the structure resulting in vastly different performance for quantum dots embedded in a nano-cavity (0D), waveguide (1D), slab (2D), or bulk medium (3D). In bulk, we find a striking temperature dependence of the dephasing rate scaling as $T^{11}$ implying that phonons are effectively 'frozen out' for $T \lesssim 4 \mathrm{K}$. The phonon density of states is strong…
We report on exciton-acoustic-phonon coupling effects on the generation of exciton maximally entangled states in N=2 and 3 quantum dot systems. In particular, we address the question of the combined effect of laser pulses, appropriate for generating Bell and Greenberger-Horne-Zeilinger entangled states, together with decoherence mechanisms as provided by a phonon reservoir. By solving numerically the master equation for the optically driven exciton-phonon kinetics, we show that the generation of maximally entangled exciton states is preserved over a reasonable parameter window.
The dynamics of a spin-1/2 particle coupled to a nuclear spin bath through an isotropic Heisenberg interaction is studied, as a model for the spin decoherence in quantum dots. The time-dependent polarization of the central spin is calculated as a function of the bath-spin distribution and the polarizations of the initial bath state. For short times, the polarization of the central spin shows a gaussian decay, and at later times it revives displaying nonmonotonic time dependence. The decoherence time scale dep ends on moments of the bath-spin distribuition, and also on the polarization strength…
We develop a "chain-boson model" master equation, within the Born-Markov approximation, for a few superconducting quantum interference devices (SQUIDs) coupled into a chain and exchanging their angular momenta with a low temperature phonon bath. Our master equation has four generators; we concentrate on the damping and diffusion and use them to study the relaxation and decoherence of a Heisenberg SQUID chain whose spectrum exhibits critical point energy-level crossings, entangled states, and pairs of resonant transitions. We note that at an energy-level crossing the relevant bath wavelengths a…
We study theoretically the phonon-induced relaxation and decoherence processes in the hybrid qubit in silicon. Hybrid qubit behaves as a charge qubit when the detuning is close to zero and as spin qubit for large detuning values. It is realized starting from an electrostatically defined double quantum dot where three electrons are confined and manipulated through only electrical tuning. By employing a three-level effective model for the qubit and describing the environment bath as a series of harmonic oscillators in the thermal equilibrium states, we extract the relaxation and decoherence time…
Long-range quantum communication for spin qubits is an important open problem. Here we study decoherence of an electron spin qubit that is being transported in a moving quantum dot. We focus on spin decoherence due to spin-orbit interaction and a random electric potential. We find that at the lowest order, the motion induces longitudinal spin relaxation, with a rate linear in the dot velocity. Our calculated spin relaxation time ranges from sub $μ$s in GaAs to above ms in Si, making this relaxation a significant decoherence channel. Our results also give clear indications on how to reduce the …
Strain-induced gradients of local electric fields in semiconductor quantum dots can couple to the quadrupole moments of nuclear spins. We develop a theory describing the influence of this quadrupolar coupling (QC) on the spin correlators of electron and hole "central" spins localized in such dots. We show that when the QC strength is comparable to or larger than the hyperfine coupling strength between nuclei and the central spin, the relaxation rate of the central spin is strongly enhanced and can be exponential. We demonstrate a good agreement with recent experiments on spin relaxation in hol…
We study decoherence in an infinite range Heisenberg model (IRHM) in the two situations where the system is coupled to a bath of either local optical phonons or global optical phonons. Using a non-perturbative treatment, we derive an effective Hamiltonian that is valid in the regime of strong spin-phonon coupling under non-adiabatic conditions. It is shown that the effective Hamiltonian commutes with the IRHM and thus has the same eigenstates as the IRHM. By analyzing the dynamics of the system using a quantum master equation approach, we show that the quantum states of the IRHM system do not …
A theoretical model for the phonon-mediated off-resonant coupling between a quantum dot and a cavity, under resonant excitation of the quantum dot, is presented. We show that the coupling is caused by electron-phonon interaction in the quantum dot and is enhanced by the cavity. We analyze recently observed resonant quantum dot spectroscopic data by our theoretical model.
Quantum computation in solid state quantum dots faces two significant challenges: Decoherence from interactions with the environment and the difficulty of generating local magnetic fields for the single qubit rotations. This paper presents a design of composite qubits to overcome both challenges. Each qubit is encoded in the degenerate ground-state of four (or six) electrons in a system of five quantum dots arranged in a two-dimensional pattern. This decoherence-free subspace is immune to both collective and local decoherence, and resists other forms of decoherence, which must raise the energy…
We study the influence of the environment on an optically induced rotation of a single electron spin in a charged semiconductor quantum dot. We analyze the decoherence mechanisms resulting from the dynamical lattice response to the charge evolution induced in a trion-based optical spin control scheme. Moreover, we study the effect of the finite trion lifetime and of the imperfections of the unitary evolution such as off-resonant excitations and the nonadiabaticity of the driving. We calculate the total error of the operation on a spin-based qubit in an InAs/GaAs quantum dot system and discuss …
We propose a model for spectral diffusion of localized spins in semiconductors due to the dipolar fluctuations of lattice nuclear spins. Each nuclear spin flip-flop is assumed to be independent, the rate for this process being calculated by a method of moments. Our calculated spin decoherence time $T_{M}=0.64$ ms for donor electron spins in Si:P is a factor of two longer than spin echo decay measurements. For $^{31}$P nuclear spins we show that spectral diffusion is well into the motional narrowing regime. The calculation for GaAs quantum dots gives $T_{M}=10-50$ $μ$s depending on the quantum …
We study the robustness and fragility of entanglement of open quantum systems in some exactly solvable models in which the decoherence is caused by a pure dephasing process. In particular, for the toy models presented in this paper, we identify two different time scales, one is responsible for local dephasing, while the other is for entanglement decay. For a class of fragile entangled states defined in this paper, we find that the entanglement of two qubits, as measured by concurrence, decays faster asymptotically than the quantum dephasing of an individual qubit.
We investigate the phonon-induced decoherence and dissipation in a donor-based charge quantum bit realized by the orbital states of an electron shared by two dopant ions which are implanted in a silicon host crystal. The dopant ions are taken from the group-V elements Bi, As, P, Sb. The excess electron is coupled to deformation potential acoustic phonons which dominate in the Si host. The particular geometry tailors a non-monotonous frequency distribution of the phonon modes. We determine the exact qubit dynamics under the influence of the phonons by employing the numerically exact quasi-adiab…
We study electron-phonon interaction induced decoherence between two-electron singlet and triplet states in a semiconductor double quantum dot using a spin-boson model. We investigate the onset and time evolution of this dephasing, and study its dependence on quantum dot parameters such as dot size and double dot separations, as well as the host materials (GaAs and Si). At the short time limit, electron-phonon interaction only causes an incomplete initial Gaussian decay of the off-diagonal density matrix element in the singlet-triplet Hilbert space. A complete long-time exponential decay due t…
The time evolution of spin states of two electrons interacting with a nuclear spin bath in a quantum dot system is studied. The hyperfine interaction between the electrons and the nuclear spins is modeled by an isotropic Heisenberg interaction, and the interaction between the electron spins by Heisenberg exchange. Depending on the extent of the overlap between the spatial wave functions of the electrons, there are two physically different cases, namely the two qubits either interact with the same set of nuclear spins or they see different nuclear spin environment. In the two cases, the decoher…
We present experimental results showing phonon-mediated coupling between two quantum dots embedded inside a photonic crystal microcavity. With only one of the dots being spectrally close to the cavity, we observe both frequency up-conversion and down-conversion of the pump light via a $\sim1.2$ THz phonon. We demonstrate this process for both weak and strong regimes of dot-cavity coupling, and provide a simple theoretical model explaining our observations.
We study the effect of phonons on a proposed scheme for the direct measurement of two-electron spin states in a double quantum dot by monitoring the the noise of the current flowing through a quantum point contact coupled to one of the dots. We show that although the effect of phonons is damaging to the procedure at extremely low temperatures characteristic of spin-in-quantum-dots experiments, and may even be fatal, increasing the temperature leads to a revival of the schemes usefulness. Furthermore, at higher, but still reasonably low temperatures phonon effects become advantageous to the mea…
We report on the feedback stabilization of the zero-phonon emission frequency of a single InAs quantum dot. The spectral separation of the phonon-assisted component of the resonance fluorescence provides a probe of the detuning between the zero-phonon transition and the resonant driving laser. Using this probe in combination with active feedback, we stabilize the zero-phonon transition frequency against environmental fluctuations. This protocol reduces the zero-phonon fluorescence intensity noise by a factor of 22 by correcting for environmental noise with a bandwidth of 191 Hz, limited by the…
Experimental observation of the decoherence of macroscopic objects is of fundamental importance to the study of quantum collapse models and the quantum to classical transition. Optomechanics is a promising field for the study of such models because of its fine control and readout of mechanical motion. Nevertheless, it is challenging to monitor a mechanical superposition state for long enough to investigate this transition. We present a scheme for entangling two mechanical resonators in spatial superposition states such that all quantum information is stored in the mechanical resonators. The sc…
We find an interference effect for electron-phonon interactions in coupled semiconductor quantum dots that can dominate the nonlinear transport properties even for temperatures close to zero. The intradot electron tunnel process leads to a `shake up' of the phonon system and is dominated by a double-slit-like interference effect of spontaneously emitted phonons. The effect is closely related to subradiance of photons (Dicke effect) in a laser-trapped two-ion system and explains the oscillations in the nonlinear current-voltage characteristics of coupled dots observed recently.
