We demonstrate that an optically driven spin of a carrier in a quantum dot undergoes indirect dephasing via conditional optically induced charge evolution even in the absence of any direct interaction between the spin and its environment. A generic model for the indirect dephasing with a three-component system with spin, charge, and reservoir is proposed. This indirect decoherence channel is studied for the optical spin manipulation in a quantum dot with a microscopic description of the charge-phonon interaction taking into account its non-Markovian nature.
We discuss the operational definition of decoherence in various solid state systems. In particular, we review, in the context of spin-based solid state quantum computation, the introduction of $T_1$ and $T_2$ to describe decoherence in a two level system. We provide a perspective on recent experiments involving the manipulation of spin coherence in semiconductors, and discuss specific decoherence and dephasing issues in electron spin-based quantum dot quantum computer architectures.
We present a remarkable finding that a recently discovered [G. S. Uhrig, Phys. Rev. Lett. 98, 100504 (2007)] series of pulse sequences, designed to optimally restore coherence to a qubit in the spin-boson model of decoherence, is in fact completely model-independent and generically valid for arbitrary dephasing Hamiltonians given sufficiently short delay times between pulses. The series maximizes qubit fidelity versus number of applied pulses for sufficiently short delay times because the series, with each additional pulse, cancels successive orders of a time expansion for the fidelity decay. …
We investigate pure dephasing decoherence (free induction decay and spin echo) of a spin qubit interacting with a nuclear spin bath. While for infinite magnetic field B the only decoherence mechanism is spectral diffusion due to dipolar flip-flops of nuclear spins, with decreasing B the hyperfine-mediated interactions between the nuclear spins become important. We give a theory of decoherence due to these interactions which takes advantage of their long-range nature. For a thermal uncorrelated bath we show that our theory is applicable down to B~10 mT, allowing for comparison with recent exper…
We consider qubits in a linear arrangement coupled to a bosonic field which acts as a quantum heat bath and causes decoherence. By taking the spatial separation of the qubits explicitly into account, the reduced qubit dynamics acquires an additional non-Markovian element. We investigate the time evolution of an entangled many-qubit W state, which for vanishing qubit separation remains robust under pure dephasing. For finite separation, by contrast, the dynamics is no longer decoherence-free. On the other hand, spatial noise correlations may prevent a complete dephasing. While a standard Bloch-…
We study electron-phonon interaction induced decoherence between two-electron singlet and triplet states in a semiconductor double quantum dot using a spin-boson model. We investigate the onset and time evolution of this dephasing, and study its dependence on quantum dot parameters such as dot size and double dot separations, as well as the host materials (GaAs and Si). At the short time limit, electron-phonon interaction only causes an incomplete initial Gaussian decay of the off-diagonal density matrix element in the singlet-triplet Hilbert space. A complete long-time exponential decay due t…
We model the decoherence and dephasing of nitrogen vacancy (NV) centers in diamond due to a noisy paramagnetic bath, with and without the presence of a rf field that couples levels of the ground electronic state manifold, using a simple quantum mechanical model that allows for analytical solutions. The model treats the NV three-level ground state system in the presence of fluctuating magnetic fields that arise from the environment, and that result in decoherence, dephasing and dissipation. We show that all 9 eigenmodes of the three-level system are coupled to each other due to interaction with…
We study the robustness and fragility of entanglement of open quantum systems in some exactly solvable models in which the decoherence is caused by a pure dephasing process. In particular, for the toy models presented in this paper, we identify two different time scales, one is responsible for local dephasing, while the other is for entanglement decay. For a class of fragile entangled states defined in this paper, we find that the entanglement of two qubits, as measured by concurrence, decays faster asymptotically than the quantum dephasing of an individual qubit.
We study the decoherence of Majorana modes of a fermion chain, where the fermions interact with their nearest neighbours. We investigate the effect of dissipation and dephasing on the Majorana modes of a fermionic chain. The dissipative and dephasing noises induce the non-parity- and parity-preserving transitions between the eigenstates of the system, respectively. Therefore, these two types of noises lead to the different decoherence mechanisms. In each type of noise, we discuss the low- and high-frequency regimes to describe the different environments. We numerically calculate the dissipatio…
We describe the mechanism of charge-spin transformation in a double quantum dot (DQD) with even occupation, where a time dependent gate voltage v(t) is applied to one of its two valleys, whereas the other one is coupled to the source and drain electrodes. The Kondo tunneling regime under strong Coulomb blockade may be realized when the spin spectrum of the DQD is formed by the ground state spin triplet and two singlet excitations. Charge fluctuations induced by v(t) result in transitions within the spin multiplet characterized by the SO(5) dynamical symmetry group. In a weakly non-adiabatic re…
The qubit (or a system of two quantum dots) has become a standard paradigm for studying quantum information processes. Our focus is Decoherence due to interaction of the qubit with its environment, leading to noise. We consider quantum noise generated by a dissipative quantum bath. A detailed comparative study with the results for a classical noise source such as generated by a telegraph process, enables us to set limits on the applicability of this process vis a vis its quantum counterpart, as well as lend handle on the parameters that can be tuned for analyzing decoherence. Both Ohmic and no…
In physical systems, decoherence can arise from both dissipative and dephasing processes. In mechanical resonators, the driven frequency response measures a combination of both, while time domain techniques such as ringdown measurements can separate the two. Here, we report the first observation of the mechanical ringdown of a carbon nanotube mechanical resonator. Comparing the mechanical quality factor obtained from frequency- and time-domain measurements, we find a spectral quality factor four times smaller than that measured in ringdown, demonstrating dephasing-induced decoherence of the na…
We examine the effect of multilevels on decoherence and dephasing properties of a quantum system consisting of a non-ideal two level subspace, identified as the qubit and a finite set of higher energy levels above this qubit subspace. The whole system is under interaction with an environmental bath through a Caldeira-Leggett type coupling. The model interaction we use can generate nonnegligible couplings between the qubit states and the higher levels upto $N\sim 10$. In contrast to the pure two-level system, in a multilevel system the quantum information may leak out of the qubit subspace thro…
Decoherence originates from the leakage of quantum information into external degrees of freedom. For a qubit the two main decoherence channels are relaxation and dephasing. Here, we report an experiment on a superconducting qubit where we retrieve part of the lost information in both of these channels. We demonstrate that raw averaging the corresponding measurement records provides a full quantum tomography of the qubit state where all three components of the effective spin-1/2 are simultaneously measured. From single realizations of the experiment, it is possible to infer the quantum trajecto…
Phonon-related decoherence effects in a quantum double-well two-level subsystem coupled to a solid are studied theoretically by the example of deformation phonons. Expressions for the reduced density matrix at T=0 are derived beyond the Markovian approximation by means of explicit solution of the non-stationary Schrodinger equation for the interacting electron-phonon system at the initial stage of its evolution. It is shown that as long as the difference between the energies of the electron in the left and the right well greatly exceeds the energy of the electron tunneling between the minima o…
We consider a particle coupled to a dissipative environment and derive a perturbative formula for the dephasing rate based on the purity of the reduced probability matrix. We apply this formula to the problem of a particle on a ring, that interacts with a dirty metal environment. At low but finite temperatures we find a dephasing rate $\propto T^{3/2}$, and identify dephasing lengths for large and for small rings. These findings shed light on recent Monte Carlo data regarding the effective mass of the particle. At zero temperature we find that spatial fluctuations suppress the possibility of h…
We propose and study a model of dephasing due to an environment of bistable fluctuators. We apply our analysis to decoherence of Josephson Qubits, induced by background charges present in the substrate, which are also responsible for the 1/f noise. The discrete nature of the environment leads to a number of new features which are mostly pronounced for slowly moving charges. Far away from degeneracy this model for the dephasing is solved exactly.
Decoherence is an essential mechanism that defines the boundary between classical and quantum behaviours, while imposing technological bounds for quantum devices. Little is known about quantum coherence of mechanical systems, as opposed to electromagnetic degrees of freedom. But decoherence can also be thought of in a purely classical context, as the loss of phase coherence in the classical phase space. Indeed the bridge between quantum and classical physics is under intense investigation, using in particular classical nanomechanical analogues of quantum phenomena. In the present work, by sepa…
Exchange coupled {\it spin} qubits in semiconductor nanostructures are shown to be vulnerable to dephasing caused by {\it charge noise} invariably present in the semiconductor environment. This decoherence of exchange gate by environmental charge fluctuations arises from the fundamental Coulombic nature of the Heisenberg coupling, and presents a serious challenge to the scalability of the widely studied exchange gate solid state spin quantum computer architectures. We estimate dephasing times for coupled spin qubits in a wide range (from 1 ns up to $> 1 μ$s) depending on the exchange coupling …
We solve the long-standing central spin problem for a general set of inhomogeneous bath couplings and a large class of initial bath states. We compute the time evolution of the coherence of a central spin coupled to a spin bath by resumming all orders of the time-convolutionless master equation, thus avoiding the need to assume weak coupling to the bath. The fully quantum, non-Markovian solution is obtained in the large-bath limit and is valid up to a timescale set by the largest coupling constant. Our result captures the full decoherence of an electron spin qubit coupled to a nuclear spin bat…
Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted emission. Here, we study theoretically and experimentally the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity as a function of temperature. We show that a large coupling to a high quality factor cavity can simultaneously reduce the effect of both phonon-induced sources of decoherence. It first limits the effect of pure dephasi…
A general semiclassical approach to quantum systems with system-bath interactions is developed. We study system decoherence in detail using a coherent state semiclassical wavepacket method which avoids singularity issues arising in the usual Green's function approach. We discuss the general conditions under which it is approximately correct to discuss quantum decoherence in terms of a ``dephasing'' picture and we derive semiclassical expressions for the phase and phase distribution. Remarkably, an effective system wavefunction emerges whose norm measures the decoherence and is equivalent to a …
We demonstrate through exact solutions that a spin bath leads to stronger (faster) dephasing of a qubit than a bosonic bath with identical bath-coupling spectrum. This difference is due to the spin-bath "dressing" by the coupling. Consequently, the quantum statistics of the bath strongly affects the pulse sequences required to dynamically decouple the qubit from its bath.
We analyze decoherence of an electron in a double-dot due to the interaction with acoustic phonons. For large tunneling rates between the quantum dots, the main contribution to decoherence comes from the phonon emission relaxation processes, while for small tunneling rates, the virtual-phonon, dephasing processes dominate. Our results show that in common semiconductors, such as Si and GaAs, the latter mechanism determines the upper limit for the double-dot charge qubit performance measure.
We investigate decoherence due to pure dephasing of a localized spin qubit interacting with a nuclear spin bath. Although in the limit of a very large magnetic field the only decoherence mechanism is spectral diffusion due to dipolar flip-flops of nuclear spins, with decreasing field the hyperfine-mediated interactions between the nuclear spins become important. We take advantage of their long-range nature, and resum the leading terms in an 1/N expansion of the decoherence time-evolution function (N, being the number of nuclear spins interacting appreciably with the electron spin, is large). F…
We discuss decoherence due to electromagnetic fluctuations in charge qubits formed by two lateral quantum dots. We use an effective circuit model to evaluate correlations of voltage fluctuations in the qubit setup. These correlations allows us to estimate energy (T1) and phase (T2) relaxation times of the the qubit system. Our theoretical estimate of the quality factor due to dephasing by electromagnetic fluctuations yields values much higher than those found in recent experiments, indicating that other sources of decoherence play a dominant role.
We study the phonon-induced dephasing of the exciton state in a quantum dot excited by a sequence of ultra-short pulses. We show that the multiple-pulse control leads to a considerable improvement of the coherence of the optically excited state. For a fixed control time window, the optimized pulsed control often leads to a higher degree of coherence than the control by a smooth single Gaussian pulse. The reduction of dephasing is considerable already for 2-3 pulses.
Motivated by recent experiments with Josephson-junction circuits we reconsider decoherence effects in quantum two-level systems (TLS). On one hand, the experiments demonstrate the importance of 1/f noise, on the other hand, by operating at symmetry points one can suppress noise effects in linear order. We, therefore, analyze noise sources with a variety of power spectra, with linear or quadratic coupling, which are longitudinal or transverse relative to the eigenbasis of the unperturbed Hamiltonian. To evaluate the dephasing time for transverse 1/f noise second-order contributions have to be t…
We investigate theoretically acoustic phonon induced decoherence in quantum dots. We calculate the dephasing of fundamental (interband or intraband) optical transitions due to real and virtual transitions with higher energy levels. Up to two acoustic phonon processes (absorption and/or emission) are taken into account simultaneously in a non-perturbative manner. An analytic expression of acoustic phonon induced broadening is given as a function of the electron-phonon matrix elements and is physically interpreted. The theory is applied to the dephasing of intersublevel transitions in self-assem…
We provide insight into the qubit measurement process involving a switching type of detector. We study the switching-induced decoherence during escape events. We present a simple method to obtain analytical results for the qubit dephasing and bit-flip errors, which can be easily adapted to various systems. Within this frame we investigate potential of switching detectors for a fast but only weakly invasive type of detection. We show that the mechanism that leads to strong dephasing, and thus fast measurement, inverts potential bit flip errors due to an intrinsic approximate time reversal symme…
We investigate the effects of dephasing on the current statistics of mesoscopic conductors with a recently developed statistical model, focusing in particular on mesoscopic cavities and Aharonov-Bohm rings. For such devices, we analyze the influence of an arbitrary degree of decoherence on the cumulants of the current. We recover known results for the limiting cases of fully coherent and totally incoherent transport and are able to obtain detailed information on the intermediate regime of partial coherence for a varying number of open channels. We show that dephasing affects the average curren…
We review our recent contributions to two topics that have become of interest in the field of open, dissipative quantum systems: non-Gaussian noise and decoherence in fermionic systems. Decoherence by non-Gaussian noise, i.e. by an environment that cannot be approximated as a bath of harmonic oscillators, is important in nanostructures (e.g. qubits) where there might be strong coupling to a small number of fluctuators. We first revisit the pedagogical example of dephasing by classical telegraph noise. Then we address two models where the quantum nature of the noise becomes essential: "quantum …
We investigate the effect of dephasing/decoherence on quantum transport through open chaotic ballistic conductors in the semiclassical limit of small Fermi wavelength to system size ratio, $λ_F/L << 1$. We use the trajectory-based semiclassical theory to study a two-terminal chaotic dot with decoherence originating from: (i) an external closed quantum chaotic environment, (ii) a classical source of noise, (iii) a voltage probe, i.e. an additional current-conserving terminal. We focus on the pure dephasing regime, where the coupling to the external source of dephasing is so weak that it does no…
1/f noise, the major source of dephasing in Josephson qubits, may be produced by an ensemble of two-level systems. Depending on the statistical properties of their distribution, the noise distribution can be Gaussian or non-Gaussian. The latter situation is realized, for instance, when the distribution of coupling strengths has a slowly decaying power-law tail. In this regime questions of self-averaging and sample-to-sample fluctuations become crucial. We study the dephasing process for a class of distribution functions and analyze the self-averaging properties of the results.
The conduction electrons' dephasing rate, $τ_ϕ^{-1}$, is expected to vanish with the temperature. A very intriguing apparent saturation of this dephasing rate in several systems was recently reported at very low temperatures. The suggestion that this represents dephasing by zero-point fluctuations has generated both theoretical and experimental controversies. We start by proving that the dephasing rate must vanish at the $T\to 0$ limit, unless a large ground state degeneracy exists. This thermodynamic proof includes most systems of relevance and it is valid for any determination of $τ_ϕ$ from …
We study three-electron-spin decoherence in a semiconductor triple quantum dot with a linear geometry. The three electron spins are coupled by exchange interactions J_{12} and J_{23}, and we clarify inhomogeneous and homogeneous dephasing dynamics for a logical qubit encoded in the (S=1/2,S_{z} =1/2) subspace. We first justify that qubit leakage via the fluctuating Overhauser field can be effectively suppressed by sufficiently large Zeeman and exchange splittings. For J_{12}=J_{23} and the case of J_{12} and J_{23} being different, we construct an effective pure dephasing Hamiltonian with the …
We study the neutral exciton energy spectrum fine structure and its spin dephasing in transition metal dichalcogenides such as MoS$_2$. The interaction of the mechanical exciton with its macroscopic longitudinal electric field is taken into account. The splitting between the longitudinal and transverse excitons is calculated by means of the both electrodynamical approach and $\mathbf k \cdot \mathbf p$ perturbation theory. This long-range exciton exchange interaction can induce valley polarization decay. The estimated exciton spin dephasing time is in the picosecond range, in agreement with av…
We examine the logical qubit system of a pair of electron spins in double quantum dots. Each electron experiences a different hyperfine interaction with the local nuclei of the lattice, leading to a relative phase difference, and thus decoherence. Methods such as nuclei polarization, state narrowing, and spin-echo pulses have been proposed to delay decoherence. Instead we propose to suppress hyperfine dephasing by adiabatic rotation of the dots in real space, leading to the same average hyperfine interaction. We show that the additional effects due to the motion in the presence of spin-orbit c…
We present an experimental realization of the transmon qubit, an improved superconducting charge qubit derived from the Cooper pair box. We experimentally verify the predicted exponential suppression of sensitivity to 1/f charge noise [J. Koch et al., Phys. Rev. A 76, 042319 (2007)]. This removes the leading source of dephasing in charge qubits, resulting in homogenously broadened transitions with relaxation and dephasing times in the microsecond range. Our systematic characterization of the qubit spectrum, anharmonicity, and charge dispersion shows excellent agreement with theory, rendering t…
We consider pure dephasing of Bell states of electron spin qubits interacting with a sparse bath of nuclear spins. Using the newly developed two-qubit generalization of cluster correlation expansion method, we calculate the spin echo decay of $|Ψ\rangle$ and $|Φ\rangle$ states for various interqubit distances. Comparing the results with calculations in which dephasing of each qubit is treated independently, we identify signatures of influence of common part of the bath on the two qubits. At large interqubit distances, this common part consists of many nuclei weakly coupled to both qubits, so t…
We demonstrate that electron-electron interactions fundamentally restrict the penetration length of superconducting correlations into a diffusive normal metal (N) attached to a superconductor (S). We evaluate the subgap magnetoconductance $G$ of SN hybrids in the presence of electron-electron interactions and demonstrate that the effect of the magnetic field on $G$ is twofold: It includes ($i$) additional temperature independent dephasing of Cooper pairs and ($ii$) Zeeman splitting between the states with opposite spins. The dephasing length of Cooper pairs can be directly extracted from measu…
We analyze dephasing in single and double quantum dot systems. The decoherence is introduced by the Büttiker model with current conserving fictitious voltage leads connected to the dots. By using the non-equilibrium Green function method, we investigate the dephasing effect on the tunneling current. It is shown that a finite dephasing rate leads to observable effects. The result can be used to measure dephasing rates in quantum dots.
Decoherence of the hole angular momentum in bulk crystals is described within the framework of non-Markovian stochastic theory. We present the analytical result for the rate of this process. The derivation is based on the new formulation of the multiband Luttinger-Kohn Hamiltonian that reflects the dynamic symmetry of the system.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and …
We develop a general microscopic theory describing the phonon decoherence of quantum dots and indistinguishability of the emitted photons in photonic structures. The coherence is found to depend fundamentally on the dimensionality of the structure resulting in vastly different performance for quantum dots embedded in a nano-cavity (0D), waveguide (1D), slab (2D), or bulk medium (3D). In bulk, we find a striking temperature dependence of the dephasing rate scaling as $T^{11}$ implying that phonons are effectively 'frozen out' for $T \lesssim 4 \mathrm{K}$. The phonon density of states is strong…
In a recent paper, Phys. Rev. Lett. 81, 1074 (1998), Golubev and Zaikin (GZ) found that ``zero-point fluctuations of electrons'' contribute to the dephasing rate extracted from the magnetoresistance. As a result, the dephasing rate remains finite at zero temperature. GZ claimed that their results ``agree well with the experimental data''. We point out that the GZ results are incompatible with (i) conventional perturbation theory of the effects of interaction on weak localization (WL), and (ii) with the available experimental data. More detailed criticism of GZ findings can be found in cond-mat…
Electron spin qubit in a quantum dot has been studied extensively for scalable quantum information processing over the past two decades. Recently, high-fidelity and fast single-spin control and strong spin-photon coupling have been demonstrated using a synthetic spin-orbit coupling created by a micromagnet. Such strong electrical driving suggests a strongly coupled spin-photon system. Here we study the relaxation, pure dephasing, and electrical manipulation of a dressed-spin qubit based on a driven single electron in a quantum dot. We find that the pure dephasing of a dressed qubit due to char…
Decoherence of Josephson qubits can be substantially reduced by tuning their parameters to optimal operation points, with only quadratic coupling to fluctuations. We analyze dephasing due to 1/f noise for a two-level system, detuned from an optimal point, i.e., the crossover to the linear-coupling regime, both for free induction decay and for spin-echo experiments. Influence of several noise sources is also discussed.
Decoherence of a localized electron spin in a solid state material (the ``central spin'' problem) at low temperature is believed to be dominated by interactions with nuclear spins in the lattice. This decoherence is partially suppressed through the application of a large magnetic field that splits the energy levels of the electron spin and prevents depolarization. However, dephasing decoherence resulting from a dynamical nuclear spin bath cannot be removed in this way. Fluctuations of the nuclear field lead to uncertainty of the electron's precessional frequency in a process known as spectral …
Quasiparticle excitations adversely affect the performance of superconducting devices in a wide range of applications. They limit the sensitivity of photon detectors in astronomy, the accuracy of current sources in metrology, the cooling power of micro-refrigerators, and could break the topological protection of Majorana qubits. In superconducting circuits for quantum information processing, tunneling of quasiparticles across Josephson junctions constitutes a decoherence mechanism. As relaxation and pure dephasing times of transmon-type charge qubits now reach 100 microseconds, understanding w…
We benchmark the decoherence of superconducting qubits to examine the temporal stability of energy-relaxation and dephasing. By collecting statistics during measurements spanning multiple days, we find the mean parameters $\overline{T_{1}}$ = 49 $μ$s and $\overline{T_{2}^{*}}$ = 95 $μ$s, however, both of these quantities fluctuate explaining the need for frequent re-calibration in qubit setups. Our main finding is that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems (TLS). Through statistical analysis, we determine swit…
The control of discrete quantum states in solids and their use for quantum information processing is complicated by the lack of a detailed understanding of the mechanisms responsible for qubit decoherences. For spin qubits in semiconductor quantum dots, phenomenological models of decoherence currently recognize two Basic stages; fast ensemble dephasing due to the coherent precession of spin qubits around nearly static but randomly distributed hyperfine fields and a much slower process of irreversible relaxation of spin qubit polarization due to dynamics of the nuclear spin bath induced by comp…
Current induced forces are not only related with the discrete nature of electrons but also with its quantum character. It is natural then to wonder about the effect of decoherence. Here, we develop the theory of current induced forces including dephasing processes and we apply it to study adiabatic quantum motors (AQMs). The theory is based on Büttiker's fictitious probe model which here is reformulated for this particular case. We prove that it accomplishes fluctuation-dissipation theorem. We also show that, in spite of decoherence, the total work performed by the current induced forces remai…
We present a nonperturbative approach which allows to evaluate the weak localization correction to the conductivity of disordered conductors in the presence of interactions. The effect of the electron-electron interaction on the magnetoconductance is described by the function A(t)\exp (-f(t)). The dephasing time is determined only by f(t), and this time remains finite down to T=0 due to the electron-electron interactions. In order to establish the relation between our nonperturbative analysis and the perturbative results the effect of interaction on the pre-exponent A(t) should be taken into a…
