Transport properties of arrays of metallic quantum dots are governed by the distance-dependent exchange coupling between the dots. It is shown that the effective value of the exchange coupling, as measured by the charging energy per dot, depends monotonically on the size of the array. The effect saturates for hexagonal arrays of over 7^5 unit cells. The discussion uses a multi-stage block renormalization group approach applied to the Hubbard Hamiltonian. A first order phase transition occurs upon compression of the lattice and the size dependence is qualitatively different for the two phases.
The universal quantum computation is obtained when there exists asymmetric anisotropic exchange between electron spins in coupled semiconductor quantum dots. The asymmetric Heisenberg model can be transformed into the isotropic model through the control of two local unitary rotations for the realization of essential quantum gates. The rotations on each qubit are symmetrical and depend on the strength and orientation of asymmetric exchange. The implementation of the axially symmetric local magnetic fields can assist the construction of quantum logic gates in anisotropic coupled quantum dots. Th…
We present a finite-size scaling analysis of the entanglement in a two-dimensional arrays of quantum dots modeled by the Hubbard Hamiltonian on a triangular lattice. Using multistage block renormalization group approach, we have found that there is an abrupt jump of the entanglement when a first-order quantum phase transition occurs. At the critical point, the entanglement is constant, independent of the block size.
In this work, the exchange energy J for a system of two laterally-coupled quantum dots, each one with an electron, is calculated analytically and in a detailed form, considering them as hydrogen-like atoms, under the Heitler-London approach. The atomic orbitals, associated to each quantum dot, are obtained from translation relations, as functions of the Fock-Darwin states. Our results agree with the reported ones by Burkard, Loss and DiVincenzo in their model of quantum gates based on quantum dots, as well as with some recent experimental reports.
We present Monte Carlo wavefunction simulations for quantum computations employing an exchange-coupled array of quantum dots. Employing a combination of experimentally and theoretically available parameters, we find that gate fidelities greater than 98 % may be obtained with current experimental and technological capabilities. Application to an encoded 3 qubit (nine physical qubits) Deutsch-Josza computation indicates that the algorithmic fidelity is more a question of the total time to implement the gates than of the physical complexity of those gates.
We study optically driven Rabi rotations of a quantum dot exciton transition between 5 and 50 K, and for pulse-areas of up to $14π$. In a high driving field regime, the decay of the Rabi rotations is nonmonotonic, and the period decreases with pulse-area and increases with temperature. By comparing the experiments to a weak-coupling model of the exciton-phonon interaction, we demonstrate that the observed renormalization of the Rabi frequency is induced by fluctuations in the bath of longitudinal acoustic phonons, an effect that is a phonon analogy of the Lamb-shift.
Coupling nanocrystals (quantum dots) to a high-$Q$ whispering gallery mode (WGM) of a silica microsphere, can produce a strong coherent interaction between the WGM and the electronic states of the dots. Shifting the resonance frequencies of the dots, for instance by placing the entire system in an electric potential, then allows this interaction to be controlled, permitting entangling interactions between different dots. Thus, this system could potentially be used to implement a quantum computer.
We investigate how decoherence affects the entanglement established between two quantum dots in micro cavities, and propose a tomographic scheme able to measure the entangled state. The scheme we consider establishes the entanglement via the exchange and measurement of a photon. Making the realistic assumption of noise dominated by pure-dephasing processes, we find that the photon must be exchanged and measured on timescales shorter than the quantum dots' characteristic dephasing time for appreciable levels of entanglement to be achieved. The tomographic scheme is able to reconstruct the full …
We propose a version of functional renormalization-group (fRG) approach, which is, due to including Litim-type cutoff and switching off (or reducing) the magnetic field during fRG flow, capable describing singular Fermi liquid (SFL) phase, formed due to presence of local moments in quantum dot structures. The proposed scheme allows to describe the first-order quantum phase transition from "singular" to the "regular" paramagnetic phase with applied gate voltage to parallel quantum dots, symmetrically coupled to leads, and shows sizable spin splitting of electronic states in the SFL phase in the…
Achieving low-error, exchange-interaction operations in quantum dots for quantum computing imposes simultaneous requirements on the exchange energy's dependence on applied voltages. A double quantum dot (DQD) qubit, approximated with a quadratic potential, is solved using a full configuration interaction method. This method is more accurate than Heitler-London and Hund-Mulliken approaches and captures new and significant qualitative behavior. We show that multiple regimes can be found in which the exchange energy's dependence on the bias voltage between the dots is compatible with current quan…
A spin qubit in semiconductor quantum dots holds promise for quantum information processing for scalability and long coherence time. An important semiconductor qubit system is a double quantum dot trapping two electrons or holes, whose spin states encode either a singlet-triplet qubit or two single-spin qubits coupled by exchange interaction. In this article, we report progress on spin dephasing of two exchange-coupled spins in a double quantum dot. We first discuss the schemes of two-qubit gates and qubit encodings in gate-defined quantum dots or donor atoms based on the exchange interaction.…
Recent experiments on semiconductor quantum dots have demonstrated the ability to utilize a large quantum dot to mediate superexchange interactions and generate entanglement between distant spins. This opens up a possible mechanism for selectively coupling pairs of remote spins in a larger network of quantum dots. Taking advantage of this opportunity requires a deeper understanding of how to control superexchange interactions in these systems. Here, we consider a triple-dot system arranged in linear and triangular geometries. We use configuration interaction calculations to investigate the int…
The exchange coupling between quantum dot spin qubits is isotropic, which restricts the types of quantum gates that can be formed. Here, we propose a method for controlling anisotropic interactions between spins arranged in a bus geometry. The symmetry is broken by an external magnetic field, resulting in XXZ-type interactions that can efficiently generate Greenberger-Horne-Zeilinger (GHZ) states or universal gate sets for exchange-only quantum computing. Analysis of the bus ground state provides a link between quantum critical phenomena and the communication capacity.
We propose an all-optical implementation of quantum-information processing in semiconductor quantum dots, where electron-hole excitations (excitons) serve as the computational degrees of freedom (qubits). We show that the strong dot confinement leads to an overall enhancement of Coulomb correlations and to a strong renormalization of the excitonic states, which can be exploited for performing conditional and unconditional qubit operations.
We present a theory for understanding the exchange interaction between electron spins in neighboring quantum dots, either by changing the detuning of the two quantum dots or independently tuning the tunneling barrier between quantum dots. The Hubbard model and a more realistic confining-potential model are used to investigate how the tilting and barrier control affect the effective exchange coupling and thus the gate fidelity in both the detuning and symmetric regimes. We show that the exchange coupling is less sensitive to the charge noise through tunnel barrier control (while allowing for ex…
We analyze the effects of hyperfine interactions on coherent control experiments in triple quantum dots. By exploiting Hamiltonian symmetries and the SU(3) structure of the triple-dot system under pseudo-exchange and longitudinal hyperfine couplings, we provide analytic formulae for the hyperfine decay of triple-dot Rabi and dephasing experiments.
We present a modulated microwave approach for quantum computing with qubits comprising three spins in a triple quantum dot. This approach includes single- and two-qubit gates that are protected against low-frequency electrical noise, due to an operating point with a narrowband response to high frequency electric fields. Furthermore, existing double quantum dot advances, including robust preparation and measurement via spin-to-charge conversion, are immediately applicable to the new qubit. Finally, the electric dipole terms implicit in the high frequency coupling enable strong coupling with sup…
Exchange interaction in gate-defined quantum dots beyond the Hubbard model
RWTH Aachen University（亚琛工业大学）；Forschungszentrum Jülich GmbH（于利希研究中心有限公司）；IMEC（比利时imec研究院）；Department of Physics, University of Wisconsin-Madison（威斯康星大学麦迪逊分校物理系）；School of Electrical Engineering and Telecommunication, UNSW Sydney（新南威尔士大学悉尼电气与电信工程学院）；Center for Quantum Devices, Niels Bohr Institute, University of Copenhagen（哥本哈根大学尼尔斯玻尔研究所量子设备中心）；Lehrstuhl für Angewandte Festkörperphysik, Ruhr-Universität Bochum（鲁尔大学波鸿分校应用固体物理学讲座）
The presence of valley states is a significant obstacle to realizing quantum information technologies in Silicon quantum dots, as leakage into alternate valley states can introduce errors into the computation. We use a perturbative analytical approach to study the dynamics of exchange-coupled quantum dots with valley degrees of freedom. We show that if the valley splitting is large and electrons are not properly initialized to valley eigenstates, then time evolution of the system will lead to spin-valley entanglement. Spin-valley entanglement will also occur if the valley splitting is small an…
Addressability of spin qubits in a silicon double quantum dot setup in the (1,1) charge configuration relies on having a large difference between the Zeeman splittings of the electrons. When the difference is not sufficiently large, the rotating wave approximation becomes inaccurate. We consider a device working in this regime, with always-on exchange coupling, and describe how a CZ gate and arbitrary one-qubit gates which are robust against charge noise can be implemented by smoothly pulsing the microwave source, while eliminating the crosstalk. We find that the most significant deviations fr…
We study the effect of the spin-orbit interaction on quantum gate operations based on the spin exchange coupling where the qubit is represented by the electron spin in a quantum dot or a similar nanostructure. Our main result is the exact cancellation of the spin-orbit effects in the sequence producing the quantum XOR gate for the ideal case where the pulse shapes of the exchange and spin-orbit interactions are identical. For the non-ideal case, the two pulse shapes can be made almost identical and the gate error is strongly suppressed by two small parameters, the spin-orbit constant and the d…
The study of charge and spin transport through semiconductor quantum dots is experiencing a renaissance due to recent advances in nano-fabrication and the realization of quantum dots as candidates for quantum computing. In this work, we combine atomistic electronic structure calculations with quantum master equation methods to study the transport of electrons and holes through strongly confined quantum dots coupled to two leads with a voltage bias. We find that a competition between the energy spacing between the two lowest quasiparticle energy levels and the strength of the exchange interacti…
We present a scheme for correcting for crosstalk- and noise-induced errors in exchange-coupled singlet-triplet semiconductor double quantum dot qubits. While exchange coupling allows the coupling strength to be controlled independently of the intraqubit exchange couplings, there is also the problem of leakage, which must be addressed. We show that, if a large magnetic field difference is present between the two qubits, leakage is suppressed. We then develop pulse sequences that correct for crosstalk- and noise-induced errors and present parameters describing them for the 24 Clifford gates. We …
Several prominent proposals have suggested that spins of localized electrons could serve as quantum computer qubits. The exchange interaction has been invoked as a means of implementing two qubit gates. In this paper, we analyze the strength and form of the exchange interaction under relevant conditions. We find that, when several spins are engaged in mutual interactions, the quantitative strengths or even qualitative forms of the interactions can change. It is shown that the changes can be dramatic within a Heitler-London model. Hund-Mulliken calculations are also presented, and support the q…
The Heisenberg exchange interaction between neighboring quantum dots allows precise voltage control over spin dynamics, due to the ability to precisely control the overlap of orbital wavefunctions by gate electrodes. This allows the study of fundamental electronic phenomena and finds applications in quantum information processing. Although spin-based quantum circuits based on short-range exchange interactions are possible, the development of scalable, longer-range coupling schemes constitutes a critical challenge within the spin-qubit community. Approaches based on capacitative coupling and ca…
Quantum gates between spin qubits can be implemented leveraging the natural Heisenberg exchange interaction between two electrons in contact with each other. This interaction is controllable by electrically tailoring the overlap between electronic wavefunctions in quantum dot systems, as long as they occupy neighbouring dots. An alternative route is the exploration of superexchange - the coupling between remote spins mediated by a third idle electron that bridges the distance between quantum dots. We experimentally demonstrate direct exchange coupling and provide evidence for second neighbour …
Electron spins in silicon quantum dots are promising qubits due to their long coherence times, scalable fabrication, and potential for all-electrical control. However, charge noise in the host semiconductor presents a major obstacle to achieving high-fidelity single- and two-qubit gates in these devices. In this work, we measure the charge-noise spectrum of a Si/SiGe singlet-triplet qubit over nearly 12 decades in frequency using a combination of methods, including dynamically-decoupled exchange oscillations with up to 512 π pulses during the qubit evolution. The charge noise is colored across…
Orbital modeling of two electron spins confined in a double quantum dot is revisited. We develop an extended Hund Mulliken approach that includes excited orbitals, allowing for a triplet configuration with both electrons residing in a single dot. This model improves the reliability and applicability of the standard Hund Mulliken approximation, while remaining largely analytical, thus it enables us to identify the mechanisms behind the exchange coupling dynamics that we find. In particular, our calculations are in close agreement with exchange values that were recently measured at a high interd…
The effective coupling of two distant quantum dots through virtual photon exchange in a semiconductor microcavity is studied. The experimental conditions for strong coupling and its manifestation in the spectra of emission are analyzed.
The spin-orbit interaction lies at the heart of quantum computation with spin qubits, research on topologically non-trivial states, and various applications in spintronics. Hole spins in Ge/Si core/shell nanowires experience a spin-orbit interaction that has been predicted to be both strong and electrically tunable, making them a particularly promising platform for research in these fields. We experimentally determine the strength of spin-orbit interaction of hole spins confined to a double quantum dot in a Ge/Si nanowire by measuring spin-mixing transitions inside a regime of spin-blockaded t…
We review progress on the spintronics proposal for quantum computing where the quantum bits (qubits) are implemented with electron spins. We calculate the exchange interaction of coupled quantum dots and present experiments, where the exchange coupling is measured via transport. Then, experiments on single spins on dots are described, where long spin relaxation times, on the order of a millisecond, are observed. We consider spin-orbit interaction as sources of spin decoherence and find theoretically that also long decoherence times are expected. Further, we describe the concept of spin filteri…
Two electron spins in quantum dots coupled through coherent tunneling are generally acknowledged to approximately obey Heisenberg isotropic exchange. This has not been established for two holes. Here we measure the spectra of two holes and of two electrons in two vertically stacked self-assembled InAs quantum dots using optical spectroscopy as a function of electric and magnetic fields. We find that the exchange is approximately isotropic for both systems, but that significant asymmetric contributions, arising from spin-orbit and Zeeman interactions combined with spatial asymmetries, are requi…
Quantum dots are artificial atoms used for a multitude of purposes. Charge defects are commonly present and can significantly perturb the designed energy spectrum and purpose of the dots. Voltage controlled exchange energy in silicon double quantum dots (DQD) represents a system that is very sensitive to charge position and is of interest for quantum computing. We calculate the energy spectrum of the silicon double quantum dot system using a full configuration interaction that uses tight binding single particle wavefunctions. This approach allows us to analyze atomic scale charge perturbations…
