We propose a wave packet basis for storing and processing several qubits of quantum information in a single multilevel atom. Using radially localized wave packet states in the Rydberg atom, we construct an orthogonal basis that is related to the usual energy level basis by a quantum Fourier transform. A transform-limited laser pulse that is short compared with the classical Kepler period of the system interacts mainly with the wave packet state localized near the atomic core, allowing selective control in this basis. We argue that wave packet control in this regime is useful for multilevel quantum information processing.
We discuss a simple example demonstrating that spontaneous emission from "space-time-superposed" atomic center-of-mass wave packets is nontrivially and time-dependent modified with respect to the standard dipole-pattern typical of "space-superposed" wave packets. Our approach provides an approximate description of a nonsimultaneous interaction of electromagnetic field with different parts of a wave packet.
The problems of cavity atom optics in the presence of an external strong coherent field are formulated as the problems of potential scattering of doubly-dressed atomic wave packets. Two types of potentials produced by various multiphoton Raman processes in a high-finesse cavity are examined. As an application the deflection of dressed atomic wave by a cavity mode is investigated. New momentum distribution of the atoms is derived that depends from the parameters of coherent field as well as photon states in the cavity.
We report on the realization of dynamical control of transport for ultra-cold Sr88 atoms loaded in an accelerated and amplitude-modulated 1D optical lattice. We tailor the energy dispersion of traveling wave packets and reversibly switch between Wannier-Stark localization and driven transport based on coherent tunneling. Within a Loschmidt-echo scheme where the atomic group velocities are reversed at once, we demonstrate a novel mirror for matter waves working independently of the momentum state and discuss possible applications to force measurements at micrometric scales.
A simple model allows us to study the nonclassical behavior of slowly moving atoms interacting with a quantized field. Atom and field become entangled and their joint state can be identified as a mesoscopic "Schroedinger-cat". By introducing appropriate observables for atom and field and by analyzing correlations between them based on a Bell-type inequality we can show the corresponding nonclassical behavior.
It is shown that the population Rabi-floppings in a lossless two-level atom, interacting with a monochromatic electromagnetic field, in general are convergent in time. The well-known continuous floppings take place because the restricted choosing of initial conditions, that is when the atom initially is chosen on ground or excited level before the interaction, simultaneously having a definite value of momentum there. The convergence of Rabi-floppings in atomic wave-packet-states is a direct consequence of Doppler effect on optical transition rates (Rabi-frequencies): it gradually leads to ''ir…
We study radial wave packets produced by short-pulsed laser fields acting on Rydberg atoms, using analytical tools from supersymmetry-based quantum-defect theory. We begin with a time-dependent perturbative calculation for alkali-metal atoms, incorporating the atomic-excitation process. This provides insight into the general wave packet behavior and demonstrates agreement with conventional theory. We then obtain an alternative analytical description of a radial wave packet as a member of a particular family of squeezed states, which we call radial squeezed states. By construction, these have c…
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
We analyze quantum entanglement of Stokes light and atomic electronic polarization excited during single-pass, linear-regime, stimulated Raman scattering in terms of optical wave-packet modes and atomic-ensemble spatial modes. The output of this process is confirmed to be decomposable into multiple discrete, bosonic mode pairs, each pair undergoing independent evolution into a two-mode squeezed state. For this we extend the Bloch-Messiah reduction theorem, previously known for discrete linear systems (S. L. Braunstein, Phys. Rev. A, vol. 71, 055801 (2005)). We present typical mode functions in…
We provide an intuitive interpretation of the optical Stern-Gerlach effect (OSGE) in the dressed-state point of view. We also analyze the effect of atomic damping in an experiment on the OSGE. We show that the atomic damping also causes the wave packet splitting, in a non-mechanical fashion, as opposed to the coherent process that is mechanical.
Atomic wave packets in optical lattices which are both spatially finite and time-dependent exhibit many striking similarities with light pulses in photonic crystals. We analytically characterize the transmission properties of such a potential geometry for an ideal gas in terms of a position-dependent band structure. In particular, we find that at specific energies, wave packets at the center of the finite lattice may be enclosed by pairs of band gaps. These act as mirrors between which the atomic wave packet is reflected, thereby effectively yielding a matter wave cavity. We show that long tra…
We show that a conspicuous wave packet of ultracold noninteracting Bosonic atoms emerges in a 1-dimensional parabolic optical lattice as in the setup of the Aarhus experiment [P. L. Pedersen ${\it et}$ ${\it al.}$, Phys. Rev. A ${\bf 88}$, 023620 (2013)], given the lattice height is harmonically modulated with a particular amplitude at a resonant frequency. We show that this wave packet, coined "${\it 4bandPWP}$" here, executes stable time-wise periodic motion for infinitely long time. We apply the Floquet theory to analyze the parameter dependence of ${\it 4bandPWP}$ in detail. Our analysis s…
We propose a simple scheme capable of adiabatically splitting an atomic wave packet using two independent translating traps. Implemented with optical dipole traps, our scheme allows a high degree of flexibility for atom interferometry arrangements and highlights its potential as an efficient and high fidelity atom optical beam splitter.
The paper first discusses theoretically the off-resonance selective excitation method that is dependent on the atomic internal states and used to generate approximately a standard coherent state of harmonic oscillator. The coherent average method then is proposed to construct the state-selective trigger pulse. A state-selective trigger pulse can keep Gaussian shape unchanged but change in an internal-state-dependent form the center-of-mass position and/or momentum of an atomic Gaussian wave-packet motional state. A Gaussian wave-packet state is one of the simplest wave-packet states that can b…
We analyse the experiment by Hultgren et al. [Phys. Rev. A {\bf 87}, 031404 (2013)] on orbital alignment and quantum beats in coherently excited atomic fine-structure manifolds produced by short-pulse laser photodetachment of C$^-$, Si$^-$ and Ge$^-$ negative ions, and derive a formula that describes the beats. Analysis of the experimental data enables us to extract the non-coherent background contribution for each species, and indicates the need for a full density matrix treatment of the problem.
Coherent manipulation of single-photon wave packets is essentially important for optical quantum communication and quantum information processing. In this paper, we realize controllable splitting and modulation of single-photon-level pulses by using a tripod-type atomic medium. The adoption of two control beams enable us to store one signal pulse into superposition of two distinct atomic collective excitations. By controlling the time delay between the two control pulses, we observe splitting of a stored wave packet into two temporally-distinct modes. By controlling the frequency detuning of t…
Controls of waveforms (pulse durations) of single photons are important tasks for effectively interconnecting disparate atomic memories in hybrid quantum networks. So far, the waveform control of single photon that is entangled with an atomic memory remains unexplored. Here, we demonstrated control of waveform length of the photon that is entangled with an atomic spin-wave memory by varying light-atom interaction time in cold atoms. The Bell parameter S as a function of the duration of photon pulse is measured, which shows that violations of Bell equality can be achieved for the photon pulse i…
We propose an implementation of the quantum fast Fourier transform algorithm in an entangled system of multilevel atoms. The Fourier transform occurs naturally in the unitary time evolution of energy eigenstates and is used to define an alternate wave-packet basis for quantum information in the atom. A change of basis from energy levels to wave packets amounts to a discrete quantum Fourier transform within each atom. The algorithm then reduces to a series of conditional phase transforms between two entangled atoms in mixed energy and wave-packet bases. We show how to implement such transforms …
We present a universal physical picture for describing storage and retrieval of photon wave packets in a Lambda-type atomic medium. This physical picture encompasses a variety of different approaches to pulse storage ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo based techniques. Furthermore, we derive an optimal control strategy for storage and retrieval of a photon wave packet of any given shape. All these approaches, when optimized, yield identical maximum efficiencies, which only depend on the optica…
We study the output coupling of atoms from a magnetic trap into a linear potential slope of gravity using a weak radio-frequency field. We present a one-dimensional wave-packet model based on a continuous loading of a continuous spectrum of generalised eigenstates to describe the scenario. Analyzing the model, we show how the interference of the classical coupling fields maps to the interference of the resulting atomic streams.
We present a generalized model for the evolution of atomic wave-packets in matter-wave interferometers. This method provides an efficient tool for analyzing the performance of atomic interferometers using atom clouds prepared in a trap as a Bose-Einstein condensate (BEC) or as a thermal ensemble. Predictions of the model for dynamic properties such as wave-packet size and phase are in excellent agreement with explicit numerical solutions of the non-linear Gross-Pitaevskii equations and enable fast calculations of interferometric performance in regimes where full numerical solutions become impr…
We present a Maxwell-Bloch description of the dynamics of a light pulse propagating through a spatially inhomogeneous system consisting of alternating layers of EIT media and vacuum. We study the effect of a dynamical modulation of the EIT control field on the shape of the wave packet: interesting effects due to the presence of interfaces with group velocity mismatch are found. An effective description based on a continuity equation is developed. Modulation schemes that can be realized in ultracold atomic samples with standard experimental techniques are proposed and discussed.
We investigate orbital alignment dynamics within the valence shell of atoms in coherently excited $j=3/2,1/2$ fine-structure manifolds generated by short-pulse photodetachment of F$^-$, Cl$^-$ and Br$^-$ anions. Using Keldysh-type theory, we calculate the density matrix of the residual atoms generated by few-cycle pulses, whose elements determine the populations and coherence among the electronic states. Our calculations demonstrate that the degree of atomic coherence can be represented by a near universal function of the ratio between the pulse duration $\tildeτ_p$ and the beat period $τ_{j'j…
We find analytical solutions to the evolution of interacting two-level atoms when the master equation is symmetric under the permutation of atomic labels. The master equation includes atomic independent dissipation. The method to obtain the solutions is: First, we use the system symmetries to describe the evolution in an operator space whose dimension grows polynomially with the number of atoms. Second, we expand the solutions in a basis composed of eigenvectors of the dissipative part of the master equation that models the independent dissipation of the atoms. This atomic damping basis is an …
Localized quantum wave packets can be produced in a variety of physical systems and are the subject of much current research in atomic, molecular, chemical, and condensed-matter physics. They are particularly well suited for studying the classical limit of a quantum-mechanical system. The motion of a localized quantum wave packet initially follows the corresponding classical motion. However, in most cases the quantum wave packet spreads and undergoes a series of collapses and revivals. We present a generic treatment of wave-packet evolution, and we provide conditions under which various types …
We propose and experimentally demonstrate a method to prepare a nonspreading atomic wave packet. Our technique relies on a spatially modulated absorption constantly chiseling away from an initially broad de Broglie wave. The resulting contraction is balanced by dispersion due to Heisenberg's uncertainty principle. This quantum evolution results in the formation of a nonspreading wave packet of Gaussian form with a spatially quadratic phase. Experimentally, we confirm these predictions by observing the evolution of the momentum distribution. Moreover, by employing interferometric techniques, we…
A new quantum mechanical description of the dynamics of wave packet under continuous measurement is formulated via Bohmian mechanics. The solution to this equation is found through a wave packet approach which establishes a direct correlation between a classical variable with a quantum variable describing the dynamics of the center of mass and the width of the wave packet. The approach presented in this paper gives a comparatively clearer picture than approaches using restrited path integrals and master equation approaches. This work shows how the extremely irregular character of classical cha…
Time evolution of wave packets built from the eigenstates of the Dirac equation for a hydrogenic system is considered. We investigate the space and spin motion of wave packets which, in the non-relativistic limit, are stationary states with a probability density distributed uniformly along the classical, elliptical orbit (elliptic WP). We show that the precession of such a WP, due to relativistic corrections to the energy eigenvalues, is strongly correlated with the spin motion. We show also that the motion is universal for all hydrogenic systems with an arbitrary value of the atomic number Z.
We have observed the diffraction of a Bose-Einstein condensate of rubidium atoms on a vibrating mirror potential. The matter wave packet bounces back at normal incidence on a blue-detuned evanescent light field after a 3.6 mm free fall. The mirror vibrates at a frequency of 500 kHz with an amplitude of 3.0 nm. The atomic carrier and sidebands are directly imaged during their ballistic expansion. The locations and the relative weights of the diffracted atomic wave packets are in very good agreement with the theoretical prediction of Carsten Henkel et al. [1].
An ultracold wave packet of bosonic atoms loaded into a travelling laser wave may form a many-atom soliton.This is disturbed by a homogeneous force field, for example by the inevitable gravitation. The wave packet is accelerated and therefore the laser frequency appears to be chirped in the rest frame of the atoms. We derive the effective nonlinear Schrödinger equation. It shows a time dependent nonlinearity coefficient which amounts to a damping or antidamping, respectively. The accelerated packet solution remains a soliton which changes its shape adiabatically. Similarly, an active shaping c…
We demonstrate an atomic interferometer in which the atom passes through a single-zone optical beam, consisting of a pair of bichromatic counter-propagating fields. During the passage, the atomic wave packets in two distinct internal states trace out split trajectories, guided by the optical beams, with the amplitude and spread of each wave-packet varying continuously, producing fringes that can reach a visibility close to unity. We show that the rotation sensitivity of this continuous interferometer (CI) can be comparable to that of the Borde-Chu Interferometer (BCI). The relative simplicity …
We report the experimental demonstration of a controlled-NOT (CNOT) quantum logic gate between motional and internal state qubits of a single ion where, as opposed to previously demonstrated gates, the conditional dynamics depends on the extent of the ion's wave-packet. Advantages of this CNOT gate over one demonstrated previously are its immunity from Stark shifts due to off-resonant couplings and the fact that an auxiliary internal level is not required. We characterize the gate logic through measurements of the post-gate ion state populations for both logic basis and superposition input sta…
Cavity-assisted storage and retrieval of single-photon wave packets in optically thin spatially extended resonant materials are analyzed. It is shown that the use of cavity tuning allows one to store and recall time-symmetric double-sided exponential pulses with near unit efficiency. The optimal regime of the cavity tuning is determined and the effect of time jitter on the storage efficiency is analyzed.
The conditions for optimal reflection-free complex-absorbing potentials (CAPs) are discussed. It is shown that the CAPs as derived from the smooth-exterior-scaling transformation of the Hamiltonian,[J. Phys. B. 31, 1431 (1998)], serve as optimal reflection-free CAPs (RF-CAPs) in wave-packet propagation calculations of open systems. The initial wave packet, can be located in the interaction region (as in half collision experiments) where the CAPs have vanished or in the asymptote where the absorbing potential non zero. As we show the optimal CAPs can be introduced also in the region where the p…
Ultra-cold atoms which are subject to ultra-relativistic dynamics are investigated. By using optically induced gauge potentials we show that the dynamics of the atoms is governed by a Dirac type equation. To illustrate this we study the trembling motion of the centre of mass for an effective two level system, historically called Zitterbewegung. Its origin is described in detail, where in particular the role of the finite width of the atomic wave packets is seen to induce a damping of both the centre of mass dynamics and the dynamics of the populations of the two levels.
Quantum time dilation occurs when a clock moves in a superposition of relativistic momentum wave packets. We utilize the lifetime of an excited hydrogen-like atom as a clock to demonstrate how quantum time dilation manifests in a spontaneous emission process. The resulting emission rate differs when compared to the emission rate of an atom prepared in a mixture of momentum wave packets at order $v^2/c^2$. This effect is accompanied by a quantum correction to the Doppler shift due to the coherence between momentum wave packets. This quantum Doppler shift affects the spectral line shape at order…
We study the generation of atom vortex beams in the case where an atomic wave-packet, moving in free space, is diffracted from a properly tailored light mask with a spiral transverse profile. We show how such a diffraction scheme could lead to the production of an atomic Ferris wheel beam.
We present a multichannel photoelectron interferometry technique based on trichromatic pulse shaping for unambiguous determination of quantum phases in multiphoton ionization (MPI) of potassium atoms. The colors of the laser field are chosen to produce three energetically separated photoelectron interferograms in the continuum. While the red pulse is two-photon resonant with the $3d$-state resulting in a (2+1) resonance-enhanced MPI (REMPI), a (1+2) REMPI occurs via the non-resonant intermediate $4p$-state with an initial green or blue pulse. We show that ionization via a non-resonant intermed…
The evolution of the quantum wave packet describing an atom trapped in the surface-tip junction of the scanning tunneling microscope is investigated by using the time-dependent Schroedinger equation, and by a quasi-classical Hamiltonian approach. The estimates concern a Xe atom in a biased double-well junction potential. The exact treatment shows that quantum coherence oscillations of the metastable ground state may occur at particular resonant values of the bias voltage. The effect of decoherence by partial localization is studied within the quasi-classical frame.
We propose to shape biphoton wave packets with an electromagnetically induced grating in a four-level double-$Λ$ cold atomic system. We show that the induced hybrid grating plays an essential role in directing the new fields into different angular positions, especially to the zeroth-order diffraction. A number of interesting features appear in the shaped two-photon waveforms. For example, broadening or narrowing the spectrum would be possible in the proposed scheme even without the use of a cavity.
Transport and scattering phenomena in open quantum-systems with a continuous energy spectrum are conveniently solved using the time-dependent Schrodinger equation. In the time-dependent picture, the evolution of an initially localized wave-packet reveals the eigenstates and eigenvalues of the system under consideration. We discuss applications of the wave-packet method in atomic, molecular, and mesoscopic systems and point out specific advantages of the time-dependent approach. In connection with the familiar initial value formulation of classical mechanics, an intuitive interpretation of tran…
Considering ultracold atoms traversing a high-Q Fabry-Perot cavity, we theoretically demonstrate a quantum nondemolition measurement of the photon number. This fully quantum mechanical approach may be understood utilizing concepts as effective mass and group velocity of the atom. The various photon numbers induce a splitting of the atomic wave packet, and a time-of-flight measurement of the atom thereby reveals the photon number. While repeated atomic measurements increase the efficiency of the protocol, it is shown that by considering long interaction times only a few atoms are needed to reso…
We present a time dependent quantum calculation of the scattering of a few-photon pulse on a single atom. The photon wave packet is assumed to propagate in a transversely strongly confined geometry, which ensures strong atom-light coupling and allows a quasi 1D treatment. The amplitude and phase of the transmitted, reflected and transversely scattered part of the wave packet strongly depend on the pulse length (bandwidth) and energy. For a transverse mode size of the order of $λ^2$, we find nonlinear behavior for a few photons already, or even for a single photon. In a second step we study the…
We propose the suppression of dispersive spreading of wave packets governed by the free-space Schrödinger equation with a periodically pulsed nonlinear term. Using asymptotic analysis, we construct stroboscopically-dispersionless quantum states that are physically reminiscent of, but mathematically different from, the well-known one-soliton solutions of the nonlinear Schrödinger equation with a constant (time-independent) nonlinearity. Our analytics are strongly supported by full numerical simulations. The predicted dispersionless wave packets can move with arbitrary velocity and can be realiz…
We propose a novel platform for the investigation of quantum wave packet dynamics, offering a complementary approach to existing theoretical models and experimental systems. It relies on laser-cooled neutral atoms which orbit around an optical nanofiber in an optical potential produced by a red-detuned guided light field. We show that the atomic center-of-mass motion exhibits genuine quantum effects like collapse and revival of the atomic wave packet. As distinctive advantages, our approach features a tunable dispersion relation as well as straightforward readout for the wave packet dynamics a…
In this tutorial we provide a short review of attosecond pulse characterization techniques and a pedagogical account of a recently proposed method called Pulse Analysis by Delayed Absorption (PANDA) [Pabst and Dahlström, Phys. Rev. A, 94, 13411 (2016)]. We discuss possible implementations of PANDA in alkali atoms using either principal quantum number wave packets or spin-orbit wave packets. The main merit of the PANDA method is that it can be used as a pulse characterization method that is free from atomic latency effects, such as scattering phase shifts and long-lived atomic resonances. Final…
Continuous change of the propagation direction of a classical control field in the process of its off-resonant Raman interaction with a weak signal field in a three-level atomic medium is suggested for quantum storage of a single-photon wave packet. It is shown that due to phase matching condition such an angular control allows one to reversibly map the single-photon wave packet to the Raman spatial coherence grating. Thus, quantum storage and retrieval can be realized without using inhomogeneous broadening of the atomic transitions or manipulating the amplitude of the control field. Under som…
Laser photons carrying non-zero orbital angular momentum are known and exploited during the last twenty years. Recently it has been demonstrated experimentally that such (twisted) electrons can be produced and even focused to a subnanometer scale. Thus, twisted electrons emerge as a new tool in atomic physics. The state of a twisted electron can be considered as a specific wave packet of plane waves. In the present paper-I we consider elastic scattering of the wave packets of fast non-relativistic particles on a potential field. We obtain simple and convenient formulae for a number of events i…
A pulse of matter waves may dramatically change its shape when traversing an absorbing barrier with time-dependent transparency. Here we show that this effect can be utilized for controlled manipulation of spatially-localized quantum states. In particular, in the context of atom-optics experiments, we explicitly demonstrate how the proposed approach can be used to generate spatially shifted, split, squeezed and cooled atomic wave packets. We expect our work to be useful in devising new interference experiments with atoms and molecules and, more generally, to enable new ways of coherent control…
We present here an all--optical scheme for the experimental realization of a quantum phase gate. It is based on the polarization degree of freedom of two travelling single photon wave-packets and exploits giant Kerr nonlinearities that can be attained in coherently driven ultracold atomic media.
The problem of photoionization of atomic hydrogen in a white-dwarf-strength magnetic field is revisited to understand the existing discrepancies in the positive-energy spectra obtained by a variety of theoretical approaches reported in the literature. Oscillator strengths for photoionization are calculated with the adiabatic-basis-expansion method developed by Mota-Furtado and O'Mahony [Phys. Rev. A {\bf 76}, 053405 (2007)]. A comparative study is performed between the adiabatic-basis-expansion method and our previously developed coupled-channel theory [Phys. Rev. A {\bf 94}, 033422 (2016)]. A…
We propose a novel class of atomic clocks based on highly charged ions. We consider highly-forbidden laser-accessible transitions within the $4f^{12}$ ground-state configurations of highly charged ions. Our evaluation of systematic effects demonstrates that these transitions may be used for building exceptionally accurate atomic clocks which may compete in accuracy with recently proposed nuclear clock.
The charged wave packets with non-Gaussian spatial profiles are shown to possess intrinsic multipole moments. The magnetic dipole moment and the electric quadrupole moment are found for a wide class of the packets, including the vortex electrons with orbital angular momentum $\ell$, the Airy beams, the so-called Schrödinger's cat states, and their generalizations. For the packets with no phase vortices, the electric quadrupole moment is shown to grow quadratically with the packet's width, $|Q_{αβ}| \sim e\cdot σ_{\perp}^2$, while it is also $|\ell|$ times enhanced for the vortex beams. For ava…
We consider the effect of relativistic boosts on single particle Gaussian wave packets. The coherence of the wave function as measured by the boosted observer is studied as a function of the momentum and the boost parameter. Using various formulations of coherence it is shown that in general the coherence decays with the increase of the momentum of the state, as well as the boost applied to it. Employing a basis-independent formulation, we show however, that coherence may be preserved even for large boosts applied on narrow uncertainty wave packets. Our result is exemplified quantitatively for…
