We fabricated two dimensional photonic crystal structures in zinc oxide films with focused ion beam etching. Lasing is realized in the near ultraviolet frequency at room temperature under optical pumping. From the measurement of lasing frequency and spatial profile of the lasing modes, as well as the photonic band structure calculation, we conclude that lasing occurs in the strongly localized defect modes near the edges of photonic band gap. These defect modes originate from the structure disorder unintentionally introduced during the fabrication process.
Great potential of photonic band-gap (PBG) structures for the development of continuous wave ultraviolet all-solid-state laser, including UV femtosecond pulse source, as well as for increase of output laser power at short-wave optical range is shown. The basic idea is a decrease of the laser threshold via suppression of the spontaneous emission in the active medium by means of embedding it into 2D or 3D PBG structure having the midgap frequency close to the frequency of the laser transition. Different schemes of 2D and 3D photonic crystal laser for ultraviolet range are proposed.
We studied numerically and experimentally the effects of structural disorder on the performance of ultraviolet photonic crystal slab lasers. Optical gain selectively amplifies the high-quality modes of the passive system. For these modes, the in-plane and out-of-plane leakage rates may be automatically balanced in the presence of disorder. The spontaneous optimization of in-plane and out-of-plane confinement of light in a photonic crystal slab may lead to a reduction of the lasing threshold.
Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies and laser power. Here we report efficient generation of deep and vacuum UV light using hydrogen-filled hollow-core photonic crystal fiber (HC-PCF). Pumping above the stimulated Raman threshold at 532 nm, coherent molecular vibrations are excited in the gas, permitting highly efficient thresholdless wavelength conversion in the UV. The system is uniquely press…
We report the generation of a purely vibrational Raman comb, extending from the vacuum ultraviolet (184 nm) to the visible (478 nm), in hydrogen-filled kagomé-style photonic crystal fiber pumped at 266 nm. Stimulated Raman scattering and molecular modulation processes are enhanced by higher Raman gain in the ultraviolet. Owing to the pressure-tunable normal dispersion landscape of the fiber-gas system in the ultraviolet, higher-order anti-Stokes bands are generated preferentially in higher-order fiber modes. The results pave the way towards tunable fiber-based sources of deep- and vacuum ultra…
We report on the generation of a three-octave-wide supercontinuum extending from the vacuum ultraviolet (VUV) to the near-infrared, spanning at least 113 to 1000 nm (i.e., 11 to 1.2 eV), in He-filled hollow-core kagome-style photonic crystal fiber. Numerical simulations confirm that the main mechanism is a novel and previously undiscovered interaction between dispersive-wave emission and plasma-induced blueshifted soliton recompression around the fiber zero dispersion frequency. The VUV part of the supercontinuum, which modeling shows to be coherent and possess a simple phase structure, has su…
A solid-state organic thin-film laser with intracavity frequency doubling is reported. Tunable ultraviolet emission from 309 to 322 nm is achieved from a vertical external cavity surface-emitting organic laser, with 2 % efficiency (1 $μ$J at 315 nm). The laser comprises a polymethyl(methacrylate) layer doped with Rhodamine 640, spun-cast onto a plane mirror, a remote concave mirror, a nonlinear crystal and a dichroic separator. The output is spectrally narrow (<0.5 nm FWHM) and tunable through phase-matching selection of the fundamental radiation lasing modes. These results highlight a low-cos…
Photonic crystal lasers operating at room temperature based on high Q/V nanobeam cavities have been demonstrated. We reported a large spontaneous emission factor (~0.97) by fitting the L-L curve with the rate equations.
Currently, direct-write waveguide fabrication is probably the most widely studied application of femtosecond laser micromachining in transparent dielectrics. Devices such as buried waveguides, power splitters, couplers, gratings and optical amplifiers have all been demonstrated. Waveguide properties depend critically on the sample material properties and writing laser characteristics. In this paper we discuss the challenges facing researchers using the femtosecond laser direct-write technique with specific emphasis being placed on the suitability of fused silica and phosphate glass as device h…
We proposed and realized a two-dimensional (2D) photonic bandedge laser surrounded by the photonic bandgap. The heterogeneous photonic crystal structure consists of two triangular lattices of the same lattice constant with different air hole radii. The photonic crystal laser was realized by room-temperature optical pumping of air-bridge slabs of InGaAsP quantum wells emitting at 1.55 micrometer. The lasing mode was identified from its spectral positions and polarization directions. A low threshold incident pump power of 0.24mW was achieved. The measured characteristics of the photonic crystal …
We present a simple method for narrowing the intrinsic Lorentzian linewidth of a commercial ultraviolet grating extended-cavity diode laser (TOPTICA DL Pro) using weak optical feedback from a long external cavity. We achieve a suppression in frequency noise spectral density of 20 dB measured at frequencies around 1 MHz, corresponding to the narrowing of the intrinsic Lorentzian linewidth from 200 kHz to 2 kHz. The system is suitable for experiments requiring a tunable ultraviolet laser with narrow linewidth and low high-frequency noise, such as precision spectroscopy, optical clocks, and quant…
We report the results on theoretical investigation about possible simultaneous laser generation in all, closely spaced modes of chirped photonic crystals layer in all visible region of the spectrum. With the possible ability to control the chirping contrast, it allows to obtain a white laser with a simple system on a chip, which can find wide application.
Ultrafast broadband ultraviolet radiation is of importance in spectroscopy and photochemistry, since high photon energies enable single-photon excitations and ultrashort pulses allow time-resolved studies. Here we report the use of gas-filled hollow-core photonic crystal fibers (HC-PCFs) for efficient ultrafast nonlinear optics in the ultraviolet. Soliton self-compression of 400 nm pulses of (unprecedentedly low) ~500 nJ energies down to sub-6-fs durations is achieved, as well as resonant emission of tunable dispersive waves from these solitons. In addition, we discuss the generation of a flat…
We show the designs of one- and two-dimensional photonic negative index metamaterials around telecom wavelengths. Designed bulk structures are inherently connected, which render their fabrication feasible by direct laser writing and chemical vapor deposition.
Surface nanoscale axial photonics (SNAP) structures are fabricated with a femtosecond laser for the first time. The inscriptions introduced by the laser pressurize the fiber and cause its nanoscale effective radius variation. We demonstrate the subangstrom precise fabrication of individual and coupled SNAP microresonators having the effective radius variation of several nanometers. Our results pave the way to a novel ultraprecise SNAP fabrication technology based on the femtosecond laser inscription.
A coupled-wave model is developed for photonic-crystal quantum cascade lasers. The analytical model provides an efficient analysis of full three-dimensional large-area device structure, and the validity is confirmed via simulations and previous experimental results.
Broad aperture semiconductor lasers usually suffer from low spatial quality of the emitted beams. Due to the highly compact character of such lasers the use of a conventional intra-cavity spatial filters is problematic. We demonstrate that extremely compact Photonic Crystal spatial filters, incorporated into the laser resonator, can improve the beam spatial quality, and correspondingly, increase the brightness of the emitted radiation. We report the decrease of the M2 from 47 down to 28 due to Photonic Crystal spatial intra-cavity filtering, and the increase of the brightness by a factor of 1.…
We demonstrate a high-power narrow-linewidth ultraviolet (UV) laser system at 318.6 nm for direct 6S1/2-nP (n = 70 to 100) Rydberg excitation of cesium atoms. Based on commercial fiber lasers and efficient nonlinear frequency conversion technology, 2.26 W of tunable UV laser power is obtained from cavity-enhanced second harmonic generation following sum-frequency generation of two infrared lasers at 1560.5 nm and 1076.9 nm to 637.2 nm. The maximum doubling efficiency is 57.3%. The typical UV laser power root-mean-square fluctuation is less than 0.87% over 30 minutes, and the continuously tunab…
Deep ultraviolet (DUV) laser pulses with tuneable wavelength and very short duration are a key enabling technology for next-generation technology and ultrafast science. Their generation has been the subject of extensive experimental effort, but no technique demonstrated thus far has been able to meet all requirements in one light source. Here we demonstrate a bright, efficient, and compact source of tuneable deep ultraviolet ultrafast laser pulses based on resonant dispersive wave emission in hollow capillary fibre. In a total footprint of only 120 x 75 cm, including the ytterbium-based drive …
We demonstrate experimentally the full tunability of a coherent femtosecond source in the whole ultraviolet spectral region. The experiment relies on the technique of high-order harmonic generation driven by a near-infrared parametric laser source in krypton gas. By tuning the drive wavelength in the range between 1100 to 1900 nm, we generated intense harmonics from near to extreme ultraviolet. A number of photons per shot of the order of 10^7 has been measured for the first harmonic orders. Many novel scientific prospects are expected to benefit from the use of such a table-top tunable source…
We report a photonic crystal surface emitting laser using monolayer tungsten disulfide as the gain medium. The cavity design utilizes a heterostructure in the photonic crystal lattice to provide lateral confinement for a high quality factor with a compact active region. Room temperature continuous wave lasing is realized after integrating monolayer tungsten disulfide flakes onto the silicon nitride photonic crystal on quartz substrate. Highly directional, near surface normal emission has also been experimentally demonstrated.
We demonstrate that photonic crystals can be used to generate powerful and highly coherent laser radiation when injecting a beam of free electrons. Using theoretical investigations we present the startup dynamics and coherence properties of such laser, in which gain is provided by matching the optical phase velocity in the photonic crystal to the velocity of the electron beam.
A photonic crystal (PhC) nanocavity formed in an optically very thick slab can support reasonably high-Q modes for lasing. Experimentally, we demonstrate room-temperature pulsed lasing operation from the PhC dipole mode emitting at 1324 nm, which is fabricated in an InGaAsP slab with thickness (T) of 606 nm. Numerical simulation reveals that, when T > 800 nm, over 90% of the laser output power couples to the PhC slab modes, suggesting a new route towards an efficient in-plane laser for photonic integrated circuits.
Topological photonics has recently been proved a robust framework for manipulating light. Active topological photonic systems, in particular, enable richer fundamental physics by employing nonlinear light-matter interactions, thereby opening a new landscape for applications such as topological lasing. Here we report an all-dielectric topological insulator laser scheme based on semiconductor cavities formed by topologically distinct Kagome photonic crystals. The proposed planar semiconductor Kagome lattice allows broadband edge states below the light line due to photonic valley hall effect in t…
We measure the lasing dynamics of single and coupled photonic crystal nanocavity array lasers fabricated in the indium gallium arsenide phosphide material system. Under short optical excitation, single cavity lasers produce pulses as fast as 11 ps (FWHM), while coupled cavity lasers show significantly longer lasing duration which is not explained by a simple rate equations model. A Finite Difference Time Domain simulation including carrier gain and diffusion suggests that asynchronous lasing across the nanocavity array extends the laser's pulse duration.
We present the use of linearly down-tapered gas-filled hollow-core photonic crystal fiber in a single-stage, pumped with pulses from a compact infrared laser source, to generate a supercontinuum carrying significant spectral power in the deep ultraviolet (200 - 300 nm). The generated supercontinuum extends from the near infrared down to around 213 nm with up to 0.83 mW/nm in the deep ultraviolet.
A general coupled-wave model is presented for square-lattice photonic crystal (PC) lasers with transverse-electric polarization. This model incorporates the high-order coupling effects that are important for two-dimensional PC laser cavities and gives a general and rigorous coupled-wave formulation for the full three-dimensional structures of typical laser devices. Numerical examples based on our model are presented for PC structures with different air-hole shapes. The accuracy of the results obtained is verified using three-dimensional finite-difference time-domain simulations.
We recently reported on the first realization of ultraviolet photonic crystal laser based on zinc oxide [Appl. Phys. Lett. {\bf 85}, 3657 (2004)]. Here we present the details of structural design and its optimization. We develop a computational super-cell technique, that allows a straightforward calculation of the photonic band structure of ZnO photonic crystal slab on sapphire substrate. We find that despite of small index contrast between the substrate and the photonic layer, the low order eigenmodes have predominantly transverse-electric (TE) or transverse-magnetic (TM) polarization. Becaus…
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do not simultaneously fulfill those two requirements, and few if any are truly compact, cost-effective and easy to use by non-specialists. Here we introduce a novel approach that goes a long way to meeting this challenge. It is based on hydrogen-filled hollow-core photonic crystal fiber pumped simultaneously by two spectrally distant pulses. Stimulated Raman sca…
We examine the cavity resonance tuning of high-Q silicon photonic crystal heterostructures by localized laser-assisted thermal oxidation using a 532 nm continuous wave laser focused to a 2.5 mm radius spot-size. The total shift is consistent with the parabolic rate law. A tuning range of up to 8.7 nm is achieved with ~ 30 mW laser powers. Over this tuning range, the cavity Q decreases from 3.2\times10^5 to 1.2\times10^5. Numerical simulations model the temperature distributions in the silicon photonic crystal membrane and the cavity resonance shift from oxidation.
Current quantum cascade lasers based upon conduction band electron transitions are predominantly TM (electrical field normal to the epitaxial direction) polarized. Here we present a study of localized defect modes, with the requisite TM polarization, in connected square and hexagonal lattice two-dimensional (2D) photonic crystals for application as quantum cascade laser resonators. A simple group-theory based analysis is used to produce an approximate description of the resonant modes supported by defects situated at different high symmetry points within the host photonic lattice. The results …
High power single mode quantum cascade lasers with a narrow far field are important for several applications including surgery or military countermeasure. Existing technologies suffer from drawbacks such as operation temperature and scalability. In this paper we introduce a fabrication approach that potentially solves simultaneously these remaining limitations. We demonstrate and characterize deep etched, buried photonic crystal quantum cascade lasers emitting around a wavelength of 8.5 μm. The active region was dry etched before being regrown with semi-insulating Fe:InP. This fabrication stra…
We propose an equivalent circuit model for photonic spike processing laser neurons with an embedded saturable absorber---a simulation model for photonic excitable lasers (SIMPEL). We show that by mapping the laser neuron rate equations into a circuit model, SPICE analysis can be used as an efficient and accurate engine for numerical calculations, capable of generalization to a variety of different laser neuron types found in literature. The development of this model parallels the Hodgkin--Huxley model of neuron biophysics, a circuit framework which brought efficiency, modularity, and generaliz…
The threshold properties of photonic crystal quantum dot lasers operating in the slow-light regime are investigated experimentally and theoretically. Measurements show that, in contrast to conventional lasers, the threshold gain attains a minimum value for a specific cavity length. The experimental results are explained by an analytical theory for the laser threshold that takes into account the effects of slow-light and random disorder due to unavoidable fabrication imperfections. Longer lasers are found to operate deeper into the slow-light region, leading to a trade-off between slow-light in…
We report on femtosecond laser writing of single mode optical waveguides in chalcogenide Gallium Lanthanum Sulphide (GLS) glass. A multiscan fabrication process was employed to create waveguides with symmetric single mode guidance and low insertion losses at 800 nm wavelength, compatible with Ti:Sapphire ultrafast lasers. μRaman and X-Ray microanalysis were used to elucidate the origin of the laser-induced refractive index change in GLS. Nonlinear refractive index measurements of the waveguides were performed by finding the optical switching parameters of a directional coupler, demonstrating t…
The use of an optically thick slab may provide versatile solutions for the realization of a current injection type laser using photonic crystals. Here, we show that a transversely higher-order defect mode can be designed to be confined by a photonic band gap in such a thick slab. Using simulations, we show that a high-Q of 10^5 is possible from a finely tuned second-order hexapole mode. Experimentally, we achieve optically pumped pulsed lasing at 1347 nm from the second-order hexapole mode with a peak threshold pump power of 88 uW.
Flatband photonic lattices, i.e. arrays of waveguides or resonators displaying a flat Bloch band, offer new routes for light trapping and distortion-free imaging. Here it is shown that flatland lattices can show stable and cooperative laser emission when optical gain is supplied to the system, despite the large degree of degeneracy of flatland supermodes. By considering a quasi one-dimensional rhombic lattice of coupled semiconductor microrings, selective pumping of the outer sublattices can induce cooperative lasing in a supermode of the flat band
An influence of plasma channel created by a filament of focused UV or IR femtosecond laser pulse (λ=248 nm or 740 nm) on characteristics of other plasma channel formed by a femtosecond pulse at the same wavelength following the first one with varied nanosecond time delay was experimentally studied. A dependence of optical transparency of the first channel and plasma density of the second channel on the time delay was demonstrated to be quite different for such a double UV and IR femtosecond pulses.
Random lasers have been recently approached as a photonic platform for disordered complex systems, such as spin glasses. In this work, using a Nd$^{3+}$:YBO$_3$ random laser system operating in the nonresonant (diffusive) feedback regime, we measured the distinct statistics of intensity fluctuations and show the physical origin of the complex interplay between the Lévy regime and the replica-symmetry-breaking transition to the photonic spin-glass phase. A novel result is reported: the unsaturated spin-glass behavior for high excitation pulse energies, not observed for systems with coherent fee…
We present the design of mid-infrared and THz quantum cascade laser cavities formed from planar photonic crystals with a complete in-plane photonic bandgap. The design is based on a honeycomb lattice, and achieves a full in-plane photonic gap for transverse-magnetic polarized light while preserving a connected pattern for efficient electrical injection. Candidate defects modes for lasing are identified. This lattice is then used as a model system to demonstrate a novel effect: under certain conditions - that are typically satisfied in the THz range - a complete photonic gap can be obtained by …
We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few $μ$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle puls…
A long existing issue for microdisk lasers is the small spontaneous emission coupling rate (β) in microdisk,. We found that it is due to the coupling of emitter spontaneous emission into competing Fabry-Perot (FP) modes in the microdisk cavity. Based on this analysis, we propose a new type of photonic crystal microdisk (PCM) laser to drastically suppress the photonic density of states in the vertical FP modes. As a result, we obtained a three fold increase of β than previously reported highest β of 0.15 at room temperature. The spontaneous emission control in truncated photonic crystals become…
Semiconductor lasers in use today rely on mirrors based on the reflection at a cleaved facet or Bragg reflection from a periodic stack of layers. Here, we demonstrate an ultra-small laser with a mirror based on the Fano resonance between a continuum of waveguide modes and the discrete resonance of a nanocavity. The Fano resonance leads to unique laser characteristics. Since the Fano mirror is very narrow-band compared to conventional lasers, the laser is single-mode and in particular, it can be modulated via the mirror. We show, experimentally and theoretically, that nonlinearities in the mirr…
By design access to laser wavelength, especially with integrated photonics, is critical to advance quantum sensors like optical clocks and quantum-information systems, and open opportunities in optical communication. Semiconductor-laser gain provides exemplary efficiency and integration but merely in developed wavelength bands. Alternatively, nonlinear optics requires control of phase matching, but the principle of nonlinear conversion of a pump laser to a designed wavelength is extensible. We report on laser-wavelength access by versatile customization of optical-parametric oscillation (OPO) …
We demonstrate that the shift of the stop band position with increasing oblique angle in periodic structures results in a wide transverse exponential field distribution corresponding to strong angular confinement of the radiation. The beam expansion follows an effective diffusive equation depending only upon the spectral mode width. In the presence of gain, the beam cross section is limited only by the size of the gain area. As an example of an active periodic photonic medium, we calculate and measure laser emission from a dye-doped cholesteric liquid crystal film.
Kramers-Kronig causality in integrated photonics: The spectral tension between ultraviolet transition and mid-infrared absorption
Southern University of Science and Technology（南方科技大学）；International Quantum Academy（国际量子科学院）；Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering（深圳福田南科大量子技术与工程研究院）；College of Physics and Optoelectronic Engineering, Shenzhen University（深圳大学物理与光电工程学院）；Institute of Advanced Photonics Technology, School of Information Engineering, Guangdong University of Technology（广东工业大学信息工程学院先进光子技术研究所）
Stimulated globular scattering (SGS) characteristics (frequency shifts, threshold, conversion efficiency) have been studied in photonic crystals (synthetic opal matrices and opal nanocomposites) at different temperatures. Results have been compared with stimulated Raman scattering investigations in calcite single crystals. In both cases temperature lowering from +20 C to -196 C resulted in the stimulated scattering energy increase and its redistribution to the higher order components.
By altering the lattice geometry of the photonic crystal surface-emitting lasers (PCSELs), we tune the regular lasing band edges of quadratic dispersions to form a single accidental Dirac point of linear dispersion at the Brillouin zone center. This not only increases the mode spacing by orders of magnitude, but also eliminates the distributed in-plane feedback to enable single-mode PCSELs of substantially larger area thus substantially higher output power. The advantages of using accidental Dirac cones are systematically evaluated through two-dimensional in-plane calculations and confirmed by…
We show that the threshold of a photonic crystal surface-emitting laser can be calculated from first-principles by the method of rigorous coupled wave analysis (RCWA), which has been widely used to simulate the response spectra of passive periodic structures. Here, the scattering matrix (S-matrix) of a surface-emitting laser structure with added gain is calculated on the complex frequency plane using RCWA, and the lasing threshold is determined by the value of gain for which the pole of the S-matrix reaches the real axis. This approach can be used for surface emitting laser struc tures in gene…
We demonstrate the first buried optical waveguides in diamond using focused femtosecond laser pulses. The properties of nitrogen vacancy centers are preserved in the waveguides, making them promising for diamond-based magnetometers or quantum information systems.
Tunable lasers emitting at a 2-3 $μ$m wavelength range and compatible with photonic integration platforms are of great interest for sensing applications. To this end, combining GaSb-based semiconductor gain chips with Si$_3$N$_4$ photonic integrated circuits offers an attractive platform. Herein, we exploit the low-loss features of Si$_3$N$_4$ waveguides and demonstrate a hybrid laser comprising a GaSb gain chip with an integrated tunable Si$_3$N$_4$ Vernier mirror. At room temperature, the laser exhibited a maximum output power of 15 mW and a tuning range of 80 nm (1937-2017 nm). The low-loss…
We demonstrated sub-wavelength (~111 nm diameter) single nanowire (NW) continuous wave (CW) lasers on silicon photonic crystal in the telecom-band with direct modulation at 10 Gb/s by optical pumping at cryogenic temperatures. To estimate the small signal response and pseudo-random bit sequence (PRBS) modulation of our CW lasers, we employed a new signal detection technique that employs a superconducting single photon detector and a time-correlated single photon counting module. The results showed that our NW laser was unambiguously modulated at above 10 Gb/s and an open eye pattern was obtain…
We report an approach to achieve this goal via build a plasmonic-dielectric photonic hybrid system. We induce a defect mode based photonic crystal (PC) cavity to work as a intermedium storage as well as a near-field light source to excite a plasmonic nanoantenna (NA). In this way, a plasmonic-photonic nano-laser source is created in present experiment. The coupling condition between the two elements is investigated in far-field and near-field level. We found that the NA reduces the Q-factor of the PC-cavity. Meanwhile, the NA concentrates and enhances the laser emission of the PC-cavity. This …
Photonic systems and technologies traditionally relegated to table-top experiments are poised to make the leap from the laboratory to real-world applications through integration. Stimulated Brillouin scattering (SBS) lasers, through their unique linewidth narrowing properties, are an ideal candidate to create highly-coherent waveguide integrated sources. In particular, cascaded-order Brillouin lasers show promise for multi-line emission, low-noise microwave generation and other optical comb applications. Photonic integration of these lasers can dramatically improve their stability to environme…
Trapped ions are one of the most promising approaches for the realization of a universal quantum computer. Faster quantum logic gates could dramatically improve the performance of trapped-ion quantum computers, and require the development of suitable high repetition rate pulsed lasers. Here we report on a robust frequency upconverted fiber laser based source, able to deliver 2.5 ps ultraviolet (UV) pulses at a stabilized repetition rate of 300.00000 MHz with an average power of 190 mW. The laser wavelength is resonant with the strong transition in Ytterbium (Yb+) at 369.53 nm and its repetitio…
