A new interferometric technique is demonstrated for measuring Coherent Anti-Stokes Raman Scattering (CARS) signals. Two forward-directed CARS signals are generated, one in each arm of an interferometer. The deterministic nature of the CARS process allows for these two signals, when spatially and temporally overlapped, to interfere with one another. Heterodyne detection can therefore be employed to increase the sensitivity in CARS signal detection. In addition, nonlinear CARS interferometry will facilitate the use of this spectroscopic technique for molecular contrast in Optical Coherence Tomography (OCT).
The efficiency of the frequency conversion process at the heart of Raman heterodyne spectroscopy was improved by nearly four orders of magnitude by resonant enhancement of both the pump and signal optical fields. Our results using an erbium doped Y$_2$SiO$_5$ crystal at temperatures near 4K suggest that such an approach is promising for the quantum conversion of microwave to optical photons.
We present the first demonstration of real-time closed-loop control and deterministic tuning of an independently suspended Fabry-Perot optical cavity using digitally-enhanced heterodyne interferometry, realising a peak sensitivity of $\sim$10 pm$/\sqrt{\mathrm{Hz}}$ over the 10-1000 Hz frequency band. The methods presented are readily extensible to multiple coupled cavities. As such, we anticipate that refinements of this technique may find application in future interferometric gravitational-wave detectors.
We present a digital algorithm for measuring the phase difference between two sinusoidal signals that combines the modified fringe-counting method with two-sample zero crossing to enable sequential signal processing. This technique can be applied to a phase meter for measuring dynamic phase differences with high resolution, particularly for heterodyne interferometry. The floor noise obtained from a demonstration with an electrical apparatus is $5\times10^{-8} \mathrm{rad/\sqrt{Hz}}$ at frequencies above approximately 0.1 Hz. In addition, by applying this method to a commercial heterodyne inter…
Searching systematically for coupling of laser and phase-modulation noise in heterodyne interferometry
University of Maryland, Baltimore County（马里兰大学巴尔的摩县分校）；NASA Goddard Space Flight Center（美国国家航空航天局戈达德太空飞行中心）；Center for Research and Exploration in Space Science and Technology, NASA/GSFC（NASA/GSFC空间科学与技术研究探索中心）；Max-Planck-Institut für Gravitationsphysik (Albert-Einstein-Institut)（马克斯·普朗克引力物理学研究所（爱因斯坦研究所））；Leibniz Universität Hannover（汉诺威莱布尼茨大学）
Coherent Raman scattering (CRS) spectroscopy techniques have been widely developed and optimized for different applications in biomedicine and fundamental science. The most utilized CRS technique has been coherent anti-Stokes Raman scattering (CARS), and more recently, stimulated Raman scattering (SRS). Coherent Stokes Raman scattering (CSRS) has been largely ignored mainly because it is often strongly affected by fluorescence, particularly for resonance enhanced measurements. However, in the cases of resonant excitation the information contained in the CSRS signal can be different and complem…
Low-phase-noise and pure-spectrum Raman light is vital for high-precision atom interferometry by two-photon Raman transition. A preferred and prevalent solution for Raman light generation is electro-optic phase modulation. However, phase modulation inherently brings in double sidebands, resulting in residual sideband effects of multiple laser pairs beside Raman light in atom interferometry. Based on a well-designed rectangular fiber Bragg grating and an electro-optic modulator, optical single-sideband modulation has been realized at 1560 nm with a stable suppression ratio better than -25 dB de…
Clock Noise Cancellation in Heterodyne Links between Optical Cavities for Space-Borne Gravitational-Wave Telescopes
Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency（宇宙科学研究所，日本宇宙航空研究开发机构）；Department of Physics, The University of Tokyo（东京大学物理学系）
Displacement measuring interferometry is a crucial component in metrology applications. In this paper, we propose a fiber-based two-wavelength heterodyne interferometer as a compact and highly sensitive displacement sensor that can be used in inertial sensing applications. In the proposed design, two individual heterodyne interferometers are constructed using two different wavelengths, 1064 nm and 1055 nm; one of which measures the target displacement and the other monitors the common-mode noise in the fiber system. A narrow-bandwidth spectral filter separates the beam paths of the two interfe…
The Laser Interferometer Space Antenna is a foreseen gravitational wave detector, which aims to detect $10^{-20}$ strains in the frequency range from 0.1 mHz to 1 Hz. It is a triangular constellation, with equal sides of $2,5 \times 10^9$ m, of three spacecraft, where heterodyne interferometry measures the spacecraft distances. The stray light from the powerful transmitted beam can overlap with the received one and interfere with the heterodyne signal. We investigated the contribution of random phase variations of the stray photons to the noise of the heterodyne signal. A balanced detection sc…
Laser heterodyne interferometry plays a key role in the proof mass's monitor and control by measuring its multiple degrees of freedom motions in the Space Gravitational Wave Detection. Laboratory development of polarization-multiplexing heterodyne interferometer (PMHI) using quadrant photodetectors (QPD) is presented in this paper, intended for measuring the translation and tilt of a proof mass. The system is of symmetric design, which can expand to five degrees of freedom measurements based on polarization-multiplexing and differential wavefront sensing (DWS). The ground-simulated experimenta…
We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines are generated by successive passes of the CW laser through an acousto-optic frequency shifter. We report the generation of frequency combs with more than 1500 mutually coherent lines, without resorting to non-linear broadening phenomena or external electronic modulation. The comb line spacing is easily reconfigurable from tens of MHz down to the kHz region. W…
We propose a method to track signals from quadrant photodiodes (QPD) in heterodyne laser interferometers that employ digital phase-locked loops for phase readout. Instead of separately tracking the four segments from the QPD and then combining the results into length and Differential Wavefront Sensing (DWS) signals, this method employs a set of coupled tracking loops that operate directly on the combined length and angular signals. Benefits are increased signal-to-noise ratio in the loops and the possibility to adapt the loop bandwidths to the different dynamical behavior of the signals being …
We present here a new type of cold atom interferometry gravimeter based on Bragg diffraction, which is able to increase the gravity measurement sensitivity and stability of common Raman atom gravimeters significantly. By comparing with Raman transition, the principles and advantages of Bragg diffraction-based atom gravimeters have been introduced. The theoretical model for a time-domain Bragg atom gravimeter with atomic incident direction parallels to the wave vector of Bragg lasers has been constructed. Some key technical requirements for an nth-order Bragg diffraction-based atom gravimeter h…
Unveiling and controlling the coherent evolution of low energy states is a key to attain light driven new functionalities of materials. Here we investigate the coherent evolution of non-equilibrium photon-phonon Raman interactions in the low photon number regime via femtosecond time-resolved multimode heterodyne detection. The time dependence of the weak probe spectral components is revealed by interferential amplification with shaped phase-locked reference fields that allow for a frequency selective amplification. We report measurements on $α$-quartz that show that both amplitude and phase of…
The influence of an external test mass on the phase of the signal of an atom interferometer is studied theoretically. Using traditional techniques in atom optics based on the density matrix equations in the Wigner representation, we are able to extract the various contributions to the phase of the signal associated with the classical motion of the atoms, the quantum correction to this motion resulting from atomic recoil that is produced when the atoms interact with Raman field pulses, and quantum corrections to the atomic motion that occur in the time between the Raman field pulses. By increas…
Atom interferometry has become one of the most powerful technologies for precision measurements. To develop simple, precise, and versatile atom interferometers for inertial sensing, we demonstrate an atom interferometer measuring acceleration, rotation, and inclination by pointing Raman beams toward individual faces of a pyramidal mirror. Only a single diode laser is used for all functions, including atom trapping, interferometry, and detection. Efficient Doppler-sensitive Raman transitions are achieved without the velocity selecting the atom sample, and with zero differential AC Stark shift b…
Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual coherence, high acquisition speed and flexible repetition-rate operation. A challenge with the operation of this kind of frequency comb in dual-comb interferometry is its limited optical bandwidth. Here, we use coherent spectral broadening and demonstrate electro-optic dual-comb interferometry over the entire telecommunications C band (200 lines covering ~ 40 n…
High-Speed Coherent Raman Fingerprint Imaging of Biological Tissues
我们开发了一种使用宽带相干反斯托克斯拉曼散射（BCARS）的相干拉曼成像平台，该平台提供了前所未有的速度，灵敏度和光谱宽度的组合。该系统利用独特的激光源配置，探测3,000 cm $^{-1}$上的拉曼光谱，并通过外差放大具有大非共振背景（NRB）的反斯托克斯光子，同时保持$<$ 13 cm $^{-1}$的高光谱分辨率，在通常较弱的拉曼“指纹”区域产生特别强的响应。对于组织学和病理学，该系统显示出以非破坏性、无标记的方式突出显示主要组织成分的前景。我们展示了高速化学成像的二维和三维视图的健康小鼠肝脏和胰腺组织之间的异种移植脑肿瘤和周围的健康脑物质的接口。
We demonstrate a Raman laser system based on phase modulation technology and phase feedback control. The two laser beams with frequency difference of 6.835 GHz are modulated using electro-optic and acousto-optic modulators, respectively. Parasitic frequency components produced by the electro-optic modulator are filtered using a Fabry-Perot Etalon. A straightforward phase feedback system restrains the phase noise induced by environmental perturbations. The phase noise of the laser system stays below -125 rad2/Hz at frequency offset higher than 500 kHz. Overall phase noise of the laser system is…
We explore the application of heterodyne interferometry for a weak-field coherent detection scheme. The methods detailed here will be used in ALPS II, an experiment designed to search for weakly-interacting, sub-eV particles. For ALPS II to reach its design sensitivity this detection system must be capable of accurately measuring fields with equivalent amplitudes on the order of 10$^{-5}$ photons per second or greater. We present initial results of an equivalent dark count rate on the order of $10^{-5}$ photons per second as well as successful generation and detection of a signal with a field …
Ultrafast atomic vibrations mediate heat transport, serve as fingerprints for chemical bonds and drive phase transitions in condensed matter systems. Light pulses shorter than the atomic oscillation period can not only probe, but even stimulate and control collective excitations. In general, such interactions are performed with free-propagating pulses. Here, we demonstrate intra-cavity excitation and time-domain sampling of coherent optical phonons inside an active laser oscillator. Employing real-time spectral interferometry, we reveal that Terahertz beats of Raman-active optical phonons can …
Bright-state source cancellation in dissipative shortcut Raman atom optics
Qatar Center for Quantum Computing, College of Science and Engineering, Hamad Bin Khalifa University（卡塔尔量子计算中心，科学与工程学院，哈马德·本·哈利法大学）；School of Particles and Accelerators, Institute for Research in Fundamental Sciences (IPM)（粒子与加速器学院，基础科学研究所）
