It is shown that under the definite regime of interaction of the acoustic waves with low-temperature, partially ionized plasma it is possible to change the intensity of some spectral lines of atomic argon. It is shown also, that the dependence of the intensities of these spectral lines on the intensity of the acoustic wave has a hysteresis behavior.
This study is designed to explore the two dimensional temperature maps of the atmospheric argon discharge consisting of pin-to-plane electrodes supplied by a high voltage DC source. After checking the stability of the micro discharge, the two dimensional image plane focused by a quartz lens was scanned by the fiber probe driven by a 3D Mobile Platform. The rotational and vibrational temperatures are calculated using nitrogen emissions collected by the high resolution spectrometer and high sensitive intensified charge coupled device (ICCD). The rotational temperature varies from 1558.15 K to 26…
A novel kind of electron beam sustained discharge is presented in which a 12keV electron beam is combined with a 2.45GHz microwave power to excite argon gas at atmospheric pressure in a continuous mode of operation. Optical emission spectroscopy is performed over a wide wavelength range from the vacuum ultraviolet (VUV) to the near infrared (NIR). Several effects which modify the emission spectra compared to sole electron beam excitation are observed and interpreted by the changing plasma parameters such as electron density, electron temperature and gas temperature.
An argon-xenon (Ar/Xe) plasma is used as a model system for complex plasmas. Based on this system, symmetric low-pressure capacitively coupled radio-frequency discharges are examined utilizing Particle-In-Cell/Monte Carlo Collisions (PIC/MCC) simulations. In addition to the simulation, an analytical energy balance model fed with the simulation data is applied to analyze the findings further. This work focuses on investigating the ion dynamics in a plasma with two ion species and a gas mixture as background. By varying the gas composition and driving voltage of the single-frequency discharge, f…
The reactivity of water vapor introduced in the flowing post-discharge of an RF atmospheric plasma torch is investigated through electrical characterization, optical emission spectroscopy and mass spectrometry measurements. Due to the technical features of the plasma torch, the post-discharge can be considered as divided into two regions: an inner region (inside the plasma torch device) where the water vapor is injected and an outer region which directly interacts with the ambient air. The main reactions induced by the injection of water vapor are identified as well as those indicative of the …
Space and time resolved concentrations of Ar ($^{3}P_2$) metastable atoms at the exit of an atmospheric pressure radio-frequency micro-plasma jet were measured using tunable diode laser absorption spectroscopy. The discharge features a coaxial geometry with a hollow capillary as an inner electrode and a ceramic tube with metal ring as outer electrode. Absorption profiles of metastable atoms as well as optical emission measurements reveal the dynamics and the filamentary structure of the discharge. The average spatial distribution of Ar metastables is characterized with and without a target in …
A self-consistent hybrid model of standing and moving striations was developed for low-current DC discharges in noble gases. We introduced the concept of surface diffusion in phase space described by a tensor diffusion in the nonlocal Fokker-Planck kinetic equation for electrons in the collisional plasma. Electrons diffuse along surfaces of constant total energy between energy jumps in inelastic collisions with atoms. Numerical solutions of the 1d1u kinetic equation for electrons were obtained by two methods and coupled to ion transport and Poisson solver. We studied the dynamics of striation …
Using Monte Carlo Collisions (MCC) method, we have performed simulations of ion velocity distribution functions (IVDF) taking into account both elastic collisions and charge exchange collisions of ions with atoms in uniform electric fields for argon and helium background gases. The simulation results are verified by comparison with the experiment data of the ion drift velocities and the ion transverse diffusion coefficients in argon and helium. The recently published experimental data for the first seven coefficients of the Legendre polynomial expansion of the ion energy and angular distributi…
The electron kinetics in moving and standing striations in direct current and radio-frequency discharges is studied. The discharge current is such that the thermalizing electron-electron collisions are negligible and the hydrodynamic description of electron component of plasma is not valid. Therefore, the one-dimensional hybrid model is used which models the electron component by particle method, while the ions are described using the drift-diffusion approximation. It is obtained that the electron transport is non-local in space. The electron energy distribution in both discharges is of non-eq…
One-dimensional particle-in-cell simulation is used to simulate the capacitively coupled argon plasma for a range of driving frequency from 13.56 MHz to 100 MHz. The argon chemistry set can, selectively, include two metastable levels enabling multi-step ionization and metastable pooling. The results show that the plasma density decreases when metastable atoms are included with higher discrepancy at higher excitation frequency. The contribution of multistep ionization to overall density increases with excitation frequency. The electron temperature increases with the inclusion of metastable atom…
Optical emission spectroscopy applied to non-equilibrium plasmas in molecular gases can give important information on basic plasma parameters, including the rotational, vibrational temperatures and densities of the investigated radiative states. In order to precisely understand the non-equilibrium of rotational-vibrational state distribution from investigated spectra without limiting presumptions, a state-by- state temperature-independent fitting procedure is the ideal approach. In this paper we present a novel software tool developed for this purpose, freely available for scientific community…
The plasma parameters such as electron distribution function and electron density of three atmospheric-pressure transient discharges namely filamentary and homogeneous dielectric barrier discharges in air, and the spark discharge of argon plasma coagulation (APC) system are determined. A combination of numerical simulation as well as diagnostic methods including current measurement and optical emission spectroscopy (OES) based on nitrogen emissions is used. The applied methods supplement each other and resolve problems, which arise when these methods are used individually. Nitrogen is used as …
Substantial developments in pattern recognition and machine learning offer unique advancements to study the deeper structures of plasma physics. We have employed the Kernel principal component analysis(KPCA) of Argon glow discharge plasmas over time-resolved UV-Vis spectra for different pressure scans. 3D vector fields obtained by KPCA reveal the chaotic structure, strange attractors. The presence of the cross magnetic field (B=100G) and the addition of pressure increase the degree of chaos. Lower scale vector fields show that phonon sinks and traps and cool the plasma electron temperatures. T…
Disruptions in tokamak plasmas may lead to the generation of runaway electrons that have the potential to damage plasma-facing components. Improved understanding of the runaway generation process requires interpretative modelling of experiments. In this work we simulate eight discharges in the ASDEX Upgrade and JET tokamaks, where argon gas was injected to trigger the disruption. We use a fluid modelling framework with the capability to model the generation of runaway electrons through the hot-tail, Dreicer and avalanche mechanisms, as well as runaway electron losses. Using experimentally base…
The electron sheath formation in a DC magnetised plasma of modified hollow cathode source is studied. The discharge consists of two plane parallel cathodes and a small cubical anode placed off axis at the center. The argon plasma is produced and the properties of the plasma in response to the sheath formation near the anode are studied using electrical and optical diagnostics. In particular, the effect of pressure, magnetic field on discharge parameters such as discharge current, plasma potential, plasma density and electron temperature is studied. The discharge showed an onset of anode glow a…
This brief communication reports a new method for generation of cold atmospheric pressure plasma jet at the downstream end of a flexible plastic tube. The device consists of a small chamber where dielectric barrier discharge (DBD) is ignited in Argon. The discharge is driven by a conventional low frequency AC power supply. The exit of DBD reactor is connected to a commercial flexible plastic tube (up to 4 meters long) with a thin floating Cu wire inside. Under certain conditions an Ar plasma jet can be extracted from the downstream tube end and there is no discharge inside the plastic tube. Th…
A new combined PIC-MCC approach is developed for accurate and fast simulation of a radio frequency discharge at low gas pressure and high density of plasma. Test calculations of transition between different modes of electron heating in a ccrf discharge in helium and argon show a good agreement with experimental data. We demonstrate high efficiency of the combined PIC-MCC algorithm, especially for the collisionless regime of electron heating.
We present the results of the experimental study of the influence of dusty structures on plasma. We have studied glow discharges in neon and argon with $\text{Al}_2 \text{O}_3$ polydisperse particles and melamine-formaldehyde monodisperse particles with the diameter of $\text{4.83} \; μm$. We used optical emission spectroscopy and laser-induced fluorescence methods to measure shift of excited atoms populations, which led to similar results. In most cases, the population change was negligible as compared to the inaccuracy. $\text{Al}_2 \text{O}_3$ particles in argon formed large structures whic…
Cold atmospheric plasma (CAP) has been emerged as a novel technology for cancer treatment. CAP can directly treat cells and tissue but such direct application is limited to skin or can be invoked as a supplement during open surgery. In this study we report indirect plasma treatment using CAP discharged in DI water using three gases as carriers (argon, helium and nitrogen). Plasma stimulated water was applied to human breast cancer cell line (MDA-MB-231). MTT assay tests showed that using argon plasma had the strongest effect on inducing apoptosis in cultured human breast cancer cells. This res…
A coaxial microwave plasma setup was designed for investigation by optical and laser diagnostics. The plasma is sustained by two microwave power sources located at both ends of a coaxial line. This allows generating an axially homogeneous glow discharge at low pressure. For increasing pressures, this glow-like mode is found to be unstable and various self-organized patterns are observed including finger-like structures which can be sustained after the visible end of the plasma column.
A volume-averaged global model is developed to investigate surface-wave discharges inside either cylindrical or coaxial structures. The neutral and ion wall flux is self-consistently estimated based on a simplified analytical description both for electropositive and electronegative plasmas. The simulation results are compared with experimental data from various discharge setups of either argon or oxygen, measured or obtained from literature, for a continuous and a pulse-modulated power input. A good agreement is observed between the simulations and the measurements. The calculations show that …
Using dust grains as probes in gas discharge plasma is a very promising, but at the same time very challenging method, as the individual external control of dust grains has to be solved. We propose and demonstrate the applicability of the RotoDust experiment, where the well controlled centrifugal force is balanced by the horizontal confinement field in plane electrode argon radio frequency gas discharges. We have reached a resolution of 0.1 V/cm for the electric field. This technique is used to verify numerical simulations and to map symmetry properties of the confinement in dusty plasma exper…
The experimental observation of the self$-$excited dust acoustic waves (DAWs) and its propagation characteristics in the absence and presence of a floating cylindrical object are investigated. The experiments are carried out in a direct current (DC) glow discharge dusty plasma in the background of argon gas. Dust particles are found levitated at the interface of plasma and cathode sheath region. The DAWs are spontaneously excited in the dust medium and found to propagate in the direction of ion drift (along the gravity) above a threshold discharge current at lower pressure. The excitation of s…
The kinetic theory for the cylindrical plasma, produced by the cylindrically symmetric (azimuthal mode number m=0) helicon wave, is developed with accounting for the cylindrical geometry and the radial inhomogeneity of the helicon wave and plasma. This theory reveals macroscale effect of the azimuthal steady rotation of electrons with a radially inhomogeneous angular velocity, caused by radial inhomogeneity of the helicon electric field. It is found that this sheared rotation as well as the electron density and temperature inhomogeneity are responsible for the development of the high frequency…
A microwave discharge of atmospheric pressure, maintained by focused CW radiation of a 24-GHz gyrotron in an argon flow in an external air atmosphere, was investigated. The electron temperature was determined by the current-voltage curve of a dual Langmuir probe placed in a plasma torch. The electron temperature was also estimated from plasma emission spectra within the framework of a coronal plasma model. The obtained values of the electron temperature coincide within the measurement accuracy. Also, the electron temperature is many times higher than the gas temperature. This fact allows us to…
The effects of the discharge voltage on the formation and nature of electric field transients in a symmetric, collisionless, very high frequency, capacitively coupled plasma are studied using a self-consistent particle-in-cell (PIC) simulation code. At a driving frequency of 60 MHz and 5 mTorr of argon gas pressure, the discharge voltage is varied from 10V to 150 V for a fixed discharge gap. It is observed that an increase in the discharge voltage causes filamentation in the electric field transients and to create multiple higher harmonics in the bulk plasma. Correspondingly, higher harmonics,…
The available diagnostics for atmospheric micro-plasmas remain limited and relatively complex to implement; so we present a radio-frequency technique for diagnosing a key parameter here. The technique allows one to estimate the dependencies of the electron density by measuring the RF-impedance of the micro-plasma and analyzing it with an appropriate equivalent circuit. This technique is inexpensive, can be used in real time and gives reasonable results for argon and helium DC micro-plasmas in holes over a wide pressure range. The electron density increases linearly with current in the expected…
Dusty plasma crystals have traditionally been observed and studied in radio frequency (RF) discharge plasmas and their formation in a DC glow discharge plasma remains experimentally challenging. We report the first ever observation of a stable dusty plasma Coulomb crystal in the cathode sheath region of a DC glow discharge plasma. The observations are made in the DPEx device where crystals of mono-disperse Melamine Formaldehyde grains are produced in the background of an Argon plasma. The crystalline nature of the structure is confirmed through a host of measurements that includes the radial p…
We apply particle based kinetic simulations to explore the characteristics of a low-pressure gas discharge driven by high-voltage ( $\sim$ kV) pulses with alternating polarity, with a duty cycle of $\approx$ 1% and a repetition rate of 5 kHz. The computations allow tracing the spatio-temporal development of several discharge characteristics, the potential and electric field distributions, charged particle densities and fluxes, the mean ion energy at the electrode surfaces, etc. As such discharges have important surface processing applications, e.g. in the treatment of artificial bones, we anal…
In this article, the stability of a complex plasma monolayer levitating in the sheath of the poweredelectrode of an asymmetric capacitively coupled radio-frequency argon discharge is studied. Com-pared to earlier studies, a better integration of the experimental results and theory is achieved byoperating with actual experimental control parameters such as the gas pressure and the dischargepower. It is shown that for a given microparticle monolayer at a fixed discharge power there existtwo threshold pressures: (i) above a specific pressure p cryst , the monolayer always crystallises; (ii)below …
Microplasmas operated at atmospheric pressure show a number of peculiar dynamic phenomena. One of these phenomena is self-pulsing, which is characterized by intrinsic pulsing behavior of a DC driven plasma discharge. This work focuses on the numerical simulation of self-pulsing in a micro thin cathode discharge operated in atmospheric pressure argon. By means of a hybrid plasma model we show self-pulsing of the discharge in the expected MHz frequency range and described its actual origin.
The sputtering of inside wall components of tokamaks can lead to the injection of supersaturated vapour in the plasma edge. The resulting condensation favours the formation of clusters which can give rise to solid particulates by further accretion. Sputtering discharges are proposed to have highlight on the formation of carbonaceous dust observed in the tokamaks with graphite based wall components. The flux of the sputtered carbon atoms is evaluated in the conditions of our laboratory discharges as well as the evolution of their energy distribution. It is shown that a cooling mechanism occurs …
This paper presents the principles and application of a super-resolution (SR) technique, based on a L1-Norm minimization procedure. In particular, the technique is applied to improve low-resolution resolution spectra as obtained from the optogalvanic effect in Neon and Argon discharges over the 413-423 nm wavelength range. By applying the super-resolution algorithm to the experimental data, a surprising 70-fold reduction of the linewidth is achieved allowing to resolve prior indistinguishable peaks. It is found that further improvements on the resolution are limited by the signal to noise rati…
The paper considers an effect of intensive ultrasound on the suspension of soot microparticles and nanoparticles in the inert gas, resulting in the coagulation of relatively large soot particles and leading to the improvement of the efficiency of production of nanoparticles, as has been observed in experiments. The effect of the particles charge on the possibility of coagulation is analyzed.
Thermophoresis is a tool often applied in complex plasma experiments. One of the usual stated benefits over other experimental tools is that changes induced by thermophoresis neither directly depend on, nor directly influence, the plasma parameters. From electronic data, plasma emission profiles in the sheath, and Langmuir probe data in the plasma bulk, we conclude that this assumption does not hold. An important effect on the levitation of dust particles in argon plasma is observed as well. The reason behind the changes in plasma parameters seems to be the change in neutral atom density accom…
This paper reports experiments on self$-$excited dust acoustic waves (DAWs) and its propagation characteristics in a magnetized rf discharge plasma. The DAWs are spontaneously excited in dusty plasma after adding more particles in the confining potential well and found to propagate in the direction of streaming ions. The spontaneous excitation of such low-frequency modes is possible due to the instabilities associated with streaming ions through the dust grain medium. The background E-field and neutral pressure determine the stability of excited DAWs. The characteristics of DAWs strongly depen…
Plasma kinetics of molecular hydrogen in the electrical discharge in Ar/CH3OH/H2O mixture is theoretically investigated for the first time. It is researched the dependence of [H2] on the breakdown field, the discharge power, solution compound and the argon pumping rate through the interelectrode gap. The highest hydrogen concentration is reached with the 20% methanol fraction in the solution. It is shown that [H2] grows as the linear function of the discharge power and decreases with the gas volume velocity increase.
Using a relaxation oscillator circuit, breakdown ($V_{\mathrm{BD}}$) and quench ($V_{\mathrm{Q}}$) voltages of a DC discharge microplasma between two needle probes are measured. High resolution modified Paschen curves are obtained for argon microplasmas including a quench voltage curve representing the voltage at which the plasma turns off. It is shown that, for a point to point microgap (e.g. the microgap between two needle probes) which describes many realistic microdevices, neither Paschen's law applies nor field emission is noticeable. Although normally $V_{\mathrm{BD}}>V_{\mathrm{Q}}$, it…
Particle-in-cell with Monte Carlo collisions (PIC/MCC) is a fully kinetic, particle based numerical simulation method with increasing popularity in the field of low temperature gas discharge physics. Already in its simplest form (electrostatic, one-dimensional geometry, and explicit time integration), it can properly describe a wide variety of complex, non-local, non-linear phenomena in electrical gas discharges at the microscopic level with high accuracy. However, being a numerical model working with discretized temporal and (partially) spatial coordinates, its stable and accurate operation l…
The results of a detailed kinetic study of the main plasma chemical processes in non-equilibrium ethanol/argon plasma are presented. It is shown that at the beginning of the discharge the molecular hydrogen is mainly generated in the reaction of ethanol H-abstraction. Later hydrogen is formed from active H, CH2OH and CH3CHOH and formaldehyde. Comparison with experimental data has shown that the used kinetic mechanism predicts well the concentrations of main species at the reactor outlet.
An experimental investigation on the periodic and chaotic oscillations in a reflex plasma source in presence of magnetic field is presented. The experiment is conducted in a reflex plasma source, consisting of two cathodes and a ring anode. A penning type DC glow discharge in an uniform axial magnetic field is initiated in the background of argon gas. The current-voltage characteristics near the breakdown voltage show a hysteresis with two distinct discharge current regimes. The effect of magnetic field on the discharge current and floating potential oscillations is studied when the discharge …
The in-depth oxygen diffusion into a low density polyethylene film is performed in the post-discharge of an atmospheric plasma torch, supplied in argon as carrier gas and with or without oxygen as reactive gas. The chemical and structural properties of the polymer surface and bulk are studied in terms of plasma parameters (treatment time, power, and reactive gas flow rate). A good correlation between XPS and Fourier transform infrared spectroscopy analyses is demonstrated. The penetration depth of oxygen into the bulk of the polymer is investigated by angle resolved-XPS and time-of-flight SIMS…
Discharge characteristics and parameter diagnosis of dielectric barrier discharge patterns in double-gap configuration
College of Physics Science and Technology, Hebei University(河北大学物理科学与技术学院);Engineering Research Center of Zero-carbon Energy Buildings and Measurement Techniques, Ministry of Education(教育部零碳能源建筑及测量技术工程研究中心)
The article reports the excitation of a helical argon atmospheric pressure plasma jet using a pulse modulated 13.56 MHz radiofrequency (RF) power source. This helical structure is observed in open ambient air which is far different from the conventional conical shape. This helical structure originates due to the periodic pressure variation in the discharge region caused by pulse modulated RF (2 kHz modulation frequency (fp)) and propagates downstream into the ambient air. The geometrical characteristics of the observed structure are explored using optical imaging. Moreover, the influence of va…
This paper studies a continuous atmospheric-pressure discharge maintained by focused subterahertz radiation of a 263 GHz gyrotron. A plasma torch propagating towards microwave radiation was sustained on an argon flow exiting a metal gas tube in the surrounding atmosphere of air. Using a high-speed camera, the spatial structure of the torch was studied and the temporal dynamics on timescales of the order of 20 ns was examined. The emission spectra of the optical wavelength range were used to estimate the excitation temperature of argon atoms and electron density. It was shown that a discharge o…
We conducted experimental studies and computer simulations of standing striations in capacitive coupled plasma in Argon gas. Standing striations were observed at frequencies 3.6, 8.4 and 19.0 MHz, in a pressure range 0.05-10 Torr, tube radius R=1.1 cm, for a certain range of discharge currents (plasma densities). Numerical simulations revealed similar nature of standing striations in CCP and moving striations in DC discharges under similar discharge conditions. Comparison of computer simulations with experimental observations helped clarify the nature of these striations. The non-linear depend…
Using particle-in-cell simulation technique, we investigate the plasma and ionization asymmetry, electron and ion energy distribution function in capacitive discharges excited by tailored waveforms. At a base frequency of 13.56 MHz, three different waveforms namely, sinusoidal, saw-tooth, and square are applied for a constant current density of 50 A/m2 and 5 mTorr argon gas pressure. The simulation results show that the square waveform produces the highest plasma density in the discharge, whereas maximum asymmetry is observed for plasma excited by sawtooth like waveform. Both square and sawtoo…
The formation of self-consistent dust crystal and its melting is a well known phenomenon in rf generated plasma but remains challenging in DC glow discharge plasma. Here, we report the melting of a two dimensional dusty plasma crystal, suspended in the cathode sheath of a DC glow discharge plasma. The experiments are carried out in a $Π-$shaped Dusty Plasma Experimental (DPEx) device where a stationary crystal of melamine formaldehyde particles is formed between the confining strips in a background of Argon plasma. The stable structure breaks and leads to a fluid state on reducing the neutral …
Through a systematically developed theory, we demonstrate that the motion of instanton identified in [Y. Z. Zhang, Z. Y. Liu, T. Xie, S. M. Mahajan, and J. Liu, Physics of Plasmas 24, 122304 (2017)] is highly correlated to the intermittent excitation and propagation of geodesic acoustic mode (GAM) that are observed in tokamaks. While many numerical simulations have observed the phenomena, it is the first theory that reveals the physical mechanism behind GAM intermittent excitation and propagation. The preceding work is based on the micro-turbulence associated with toroidal ion temperature grad…
There are two distinct phases in the evolution of drift wave envelope in the presence of zonal flow. A long-lived standing wave phase, which we call the Caviton, and a short-lived traveling wave phase (in radial direction) we call the Instanton. For drift wave turbulence driven by ion temperature gradient mode (ITG), these two stages of dynamics were displayed in [Zhang Y Z, Liu Z Y, Xie T, Mahajan S M and Liu J 2017 Physics of Plasmas 24 122304]. In this paper we show that the dynamical attributes of ITG turbulence are readily replicated when the turbulence rotates in the electron direction; …
We report on experimental evidence of visco-elastic effects in a strongly coupled dusty plasma through investigations of the propagation characteristics of low frequency dust acoustic waves and by excitations of transverse shear waves in a DC discharge Argon plasma.
This research focuses on interaction of ionization waves (IW) generated in long discharge tubes (1 m length and 1.5 cm in diameter) filled with neon or argon under pressure about 1 Torr and, in particular, on simplest case of such interference which is collision of the opposite directed IW of positive polarity. The waves were triggered from two electrodes of the tube by simultaneous application of the same high voltage pulse and propagated toward the tube center until their collision. Space and time stability of the collisions was achieved via decreasing time delay of the initial breakdowns wh…
Experimental investigation of an electronegative cylindrical capacitively coupled geometrically asymmetric plasma discharge with an axisymmetric magnetic field