Recently, we predicted theoretically that in cavities that support several longitudinal modes, strong coupling can occur in very different manners, depending on the system parameters. Distinct longitudinal cavity modes are either entangled with each other via the material or independently coupled to the exciton mode. Here we experimentally demonstrate the transition between those two regimes as the cavity thickness is gradually increased while maintaining fixed coupling strength. We study the properties of the system using reflection and emission spectroscopy and show that even though the coupling strength is constant, different behavior in the spectral response is observed along the coupling-decoupling transition. In addition, we find that in such multimode cavities pronounced upper-polariton emission is observed, in contrast to the usual case of a single-mode cavity. Furthermore, we address the ultrafast dynamics of the multimode cavities by pump-probe spectroscopic measurements and observe that the transient spectra significantly change through the transition.
Coherent light-matter interaction at the single photon and electronic qubit level promises the remarkable potential for nonclassical information processing. Against the efforts of improving the figure of merit of the cavities, here we demonstrate strong anharmonicity in the polariton dressed states via dark state resonances in a highly dissipative cavity. It is shown that vacuum Rabi oscillation occurs for a single quantum emitter inside a cavity even with bosonic decay-to-interaction rate ratio exceeding $10^{2}$, when the photon field is coupled to an auxiliary high-$Q$ cavity. Moreover, pho…
Strong coupling of molecular vibrations to an infrared cavity mode affects their nature by creating dressed polariton states. We show how the single and double vibrational polariton manifolds may be controlled by varying the cavity coupling strength, and probed by a time domain 2DIR technique, Double Quantum Coherence (DQC). Applications are made to the amide-I ($CO$) and amide-II ($CN$) bond vibrations of $N-methylacetamide$ (NMA).
We perform a quantum-theoretical treatment of cavity linewidth narrowing with intracavity electromagnetically induced transparency (EIT). By means of intracavity EIT, the photons in the cavity are in the form of cavity polaritons: bright-state polariton and dark-state polariton. Strong coupling of the bright-state polariton to the excited state induces an effect known as vacuum Rabi splitting, whereas the dark-state polariton decoupled from the excited state induce a narrow cavity transmission window. Our analysis would provide a quantum theory of linewidth narrowing with a quantum field pulse…
Magnon-polaritons are hybrid light-matter quasiparticles originating from the strong coupling between magnons and photons. They have emerged as a potential candidate for implementing quantum transducers and memories. Owing to the dampings of both photons and magnons, the polaritons have limited lifetimes. However, stationary magnon-polariton states can be reached by a dynamical balance between pumping and losses, so the intrinsical nonequilibrium system may be described by a non-Hermitian Hamiltonian. Here we design a tunable cavity quantum electrodynamics system with a small ferromagnetic sph…
We have realised a semiconductor quantum structure that produces electroluminescence while operating in the light-matter strong coupling regime. The mid-infrared light emitting device is composed of a quantum cascade structure embedded in a planar microcavity, based on the GaAs/AlGaAs material system. At zero bias, the structure is characterised using reflectivity measurements which show, up to room temperature, a wide polariton anticrossing between an intersubband transition and the resonant cavity photon mode. Under electrical injection the spectral features of the emitted light change drast…
We present a microscopic theory describing the stimulated scattering of intersubband polariton excitations in a microcavity-embedded two-dimensional electron gas. In particular, we consider the polariton scattering induced by the spontaneous emission of optical phonons. Our theory demonstrates the possibility of final-state stimulation for the scattering of such composite excitations, accounting for the deviations from perfect bosonicity occurring at high excitation densities. By using realistic parameters for a GaAs semiconductor system, we predict how to achieve a quantum degenerate regime, …
By means of analytical and numerical methods we analyze the phase diagram of polaritons in one-dimensional coupled cavities. We locate the phase boundary, discuss the behavior of the polariton compressibility and visibility fringes across the critical point, and find a non-trivial scaling of the phase boundary as a function of the number of atoms inside each cavity. We also predict the emergence of a polaritonic glassy phase when the number of atoms fluctuates from cavity to cavity.
The interaction of quantum light with matter like that inside a cavity is known to give rise to mixed light-matter states called polaritons. We discuss the impact of rotation of the cavity on the polaritons. It is shown that the number of polaritons increases due to this rotation. The structure of the original polaritons is modified and new ones are induced by the rotation that strongly depend on the angular velocity and the choice of axis of rotation. In molecules the rotation can change the number of light-induced conical intersections and their dimensionality and hence strongly impact their…
The strong coupling between an intersubband excitation in a quantum cascade structure and a photonic mode of a planar microcavity has been detected by angle-resolved photovoltaic measurements. A typical anticrossing behavior, with a vacuum-field Rabi splitting of 16 meV at 78K, has been measured, for an intersubband transition at 163 meV. These results show that the strong coupling regime between photons and intersubband excitations can be engineered in a quantum cascade opto-electronic device. They also demonstrate the possibility to perform angle-resolved mid-infrared photodetection and to d…
We theoretically demonstrate that chemical reaction rate constant can be significantly suppressed by coupling molecular vibrations with an optical cavity, exhibiting both the collective coupling effect and the cavity-frequency modification of the rate constant. When a reaction coordinate is strongly coupled to the solvent molecules, the reaction rate constant is reduced due to the dynamical caging effect. We demonstrate that collectively coupling the solvent to the cavity can further enhance this dynamical caging effect, leading to additional suppression of the chemical kinetics. This effect i…
We report the first observation of the magnon-polariton bistability in a cavity magnonics system consisting of cavity photons strongly interacting with the magnons in a small yttrium iron garnet (YIG) sphere. The bistable behaviors are emerged as sharp frequency switchings of the cavity magnon-polaritons (CMPs) and related to the transition between states with large and small number of polaritons. In our experiment, we align, respectively, the [100] and [110] crystallographic axes of the YIG sphere parallel to the static magnetic field and find very different bistable behaviors (e.g., clockwis…
Spoof surface modes on nanostructured metallic surfaces are known to have tailorable dispersion dependent on the geometric characteristics of the periodic pattern. Here we examine the spoof plasmon dispersion on an isolated grating and a grating-planar mirror cavity configuration. The spoof polariton dispersion in the cavity is obtained using the scattering matrix approach, and the related differential modal density of states is introduced to obtain the mode dispersion and classify the cavity polariton modes. The grating-mirror cavity geometry is an example of periodically nanostructured metal…
We demonstrate hybridization of optical cavity photons with atomic Rydberg excitations using electromagnetically induced transparency (EIT). The resulting dark state Rydberg polaritons exhibit a compressed frequency spectrum and enhanced lifetime indicating strong light-matter mixing. We study the coherence properties of cavity Rydberg polaritons and identify the generalized EIT linewidth for optical cavities. Strong collective coupling suppresses polariton losses due to inhomogeneous broadening, which we demonstrate by using different Rydberg levels with a range of polarizabilities. Our resul…
We analyse the effect of a strong perpendicular magnetic field on an intersubband transition in a disordered doped quantum well strongly coupled to an optical cavity. The magnetic field changes the lineshape of the intersubband optical transition due to the interface roughness of the quantum well from a Lorentzian to a Gaussian one. In this regime, a novel form of magnetic-field-induced cavity protection sets in, which strongly reduces the polariton linewidth to the cavity contribution only. Implications of our results for fundamental studies of nonlinear polariton dynamics and for technologic…
Strong coupling between cavity photons and various excitations in condensed matters boosts the field of light-matter interaction and generates several exciting sub-fields, such as cavity optomechanics and cavity magnon polariton. Axion quasiparticles, emerging in topological insulators, were predicted to strongly couple with the light and generate the so-called axion polariton. Here, we demonstrate that there arises a gapless level attraction in cavity axion polariton of antiferromagnetic topological insulators, which originates from a nonlinear interaction between axion and the odd-order reso…
The effect of disorder in the intensity of the driving laser on the dynamics of a disordered three-cavity system of four-level atoms is investigated. This system can be described by a Bose-Hubbard Hamiltonian for dark-state polaritons. We examine the evolution of the first- and second-order correlation functions, the photon and atomic excitation numbers and the basis state occupation probabilities. We use the full Hamiltonian and the approximate Bose-Hubbard Hamiltonian with uniform and speckle disorder, as well as with different dipole couplings. We find that the results for the two Hamiltoni…
We study the resonant electronic excitation dynamics for ultracold atoms trapped in a deep optical lattice prepared in a Mott insulator state. Excitons in these artificial crystals are similar to Frenkel excitons in Noble atom or molecular crystals. They appear when the atomic excited state line width is smaller than the exciton band width generated by dipole-dipole coupling. When the atoms are placed within a cavity the electronic excitations and the quantized cavity mode get coupled. In the collective strong coupling regime excitations form two branches of cavity polaritons with Rabi splitti…
Manipulation of Arbitrary-Order Cavity-Magnon Polariton Blockade
Fujian Key Laboratory of Quantum Information and Quantum Optics, College of Physics and Information Engineering, Fuzhou University（福建量子信息与光学重点实验室，福州大学物理与信息工程学院）
We demonstrate the strong coupling of both magnons and phonons to terahertz (THz) frequency electromagnetic (EM) waves confined to a photonic crystal (PhC) cavity. Our cavity consists of a two-dimensional array of air-holes cut into a hybrid slab of ferroelectric lithium niobate (LiNbO$_3$) and erbium orthoferrite (ErFeO$_3$), a canted antiferromagnetic crystal. The phonons in LiNbO$_3$ and the magnons in ErFeO$_3$ are strongly coupled to the electric and magnetic field components of the confined EM wave, respectively. This leads to the formation of new cavity magnon-phonon-polariton modes, wh…
We are interested in the emission characteristics of an atom interacting with the polaritonic excitations of a semiconductor or insulator embedded in a one-mode cavity. Since polaritons inside of the cavity exhibit intrinsic squeezing, we discuss how the squeezed polariton ground state modifies the atomic emission and how an indirect evidence of polariton squeezing outside of he cavity may be obtained.
The elementary optical excitations of a two-dimensional electron system strongly coupled to a microcavity are trion-polaritons. Using a variational approach, we demonstrate that the competition between Coulomb interaction and light-matter coupling plays a crucial role in determining the lowest-energy orbital and spin properties of trion-polaritons. When the light-matter interaction exceeds the bare trion binding, singlet and triplet trion states are mixed due to a cavity-mediated spin-orbit effect, which in turn results in a strong increase of the outer electron Bohr radius. In this strong cav…
This paper investigates a novel hybrid cavity QED-optomechanics situation. We solve the Hamiltonian problem of a cavity coupled both to a two-level atom via a Jaynes-Cummings coupling and to a mechanical motion via radiation pressure coupling. The atom-cavity polariton number operator commutes with the total Hamiltonian leading to an exact analytical solution involving tripartite atom-cavity-mechanics polarons. Under optical pumping of polaronic transitions the system displays unusual atom-assisted cooling and amplification of mechanical motion. We demonstrate the possibility to obtain enhance…
Through a non-perturbative quantum theory, we investigate how the quasi-electron excitations of a two-dimensional electron gas are modified by strong coupling to the vacuum field of a microcavity. We show that the electronic dressed states originate from a Fano-like coupling between the bare electron states and the continuum of intersubband cavity polariton excitations. In particular, we calculate the electron spectral function modified by light-matter interactions and its impact on the electronic injection of intersubband cavity polaritons. The domain of validity of the present theoretical re…
We study the scattering problem of photon and polariton in a one-dimensional coupled-cavity system. Analytical approximate analysis and numerical simulation show that a photon can stimulate the photon emission from a polariton through polariton-photon collisions. This observation opens the possibility of photon-stimulated transition from insulating to radiative phase in a coupled-cavity QED system. Inversely, we also find that a polariton can be generated by a two-photon Raman scattering process. This paves the way towards single photon storage by the aid of atom-cavity interaction.
We study the spectrum of a one-dimensional Kitaev chain placed in a microwave cavity. In the off-resonant regime, the frequency shift of the cavity can be used to identify the topological phase transition of the coupled system. In the resonant regime, the topology of the system can be controlled via the microwave cavity occupation and, moreover, for a large number of photons (classical limit), the physics becomes similar to that of periodically-driven systems (Floquet insulators). We also analyze numerically a finite chain and show the existence of a degenerate subspace in the presence of the …
We present a complete analytical solution for a single four-level atom strongly coupled to a cavity field mode and driven by external coherent laser fields. The four-level atomic system consists of a three-level subsystem in an EIT configuration, plus an additional atomic level; this system has been predicted to exhibit a photon blockade effect. The solution is presented in terms of polaritons. An effective Hamiltonian obtained by this procedure is analyzed from the viewpoint of an effective two-level system, and the dynamic Stark splitting of dressed states is discussed. The fluorescence spec…
The dynamics of arbitrary-order quantum correlations in a cavity magnon-polariton system are investigated based on the quantum master equation in the coherent state representation. The phenomena of Rabi-like oscillation and level repulsion of the average cavity-photon number agree remarkably well with existing experimental observations. The competing nature of coherent and incoherent components in these two cases is further revealed by the second-order quantum coherence of the cavity photons and magnons, which can be systematically tuned by the driving microwave and thermal bath. Our results d…
We consider a new approach to the problem of Bose-Einstein condensation (BEC) of polaritons for atom-field interaction under the strong coupling regime in the cavity. We investigate the dynamics of two macroscopically populated polariton modes corresponding to the upper and lower branch energy states coupled via Kerr-like nonlinearity of atomic medium. We found out the dispersion relations for new type of collective excitations in the system under consideration. Various temporal regimes like linear (nonlinear) Josephson transition and/or Rabi oscillations, macroscopic quantum self-trapping (MQ…
We present a full analysis of the mode spectrum in a cavity formed by two parallel plates, one of which is a magneto-dielectric, e.g. a metamaterial, while the other one is metallic, and obtain dispersion relations in closed form. The optical properties of the cavity walls are described in terms of realistic models for the effective permittivity and the permeability. Surface polaritons, i.e. electromagnetic modes that have at least partly an evanescent character, are shown to dominate the Casimir interaction at small separations. We analyze in detail the s-polarized polaritons, which are a cha…
Plasmonic dimer cavities can induce extreme electric-field hot spots that allow one to access ultrastrong coupling regimes using Raman-type spectroscopy on single vibrating molecules. Using a generalized master equation, we study resonant Raman scattering in the strong coupling regime of cavity-QED, when also in the vibrational ultrastrong coupling regime, leading to "phonon-dressed polaritons". The master equation rigorously includes spectral baths for the cavity and vibrational degrees of freedom, as well as a pure dephasing bath for the resonant two-level system, which play a significant ro…
A photon-magnon hybrid system can be realised by coupling the electron spin resonance of a magnetic material to a microwave cavity mode. The quasiparticles associated with the system dynamics are the cavity magnon polaritons, which arise from the mixing of strongly coupled magnons and photons. We illustrate how these particles can be used to probe the magnetisation of a sample with a remarkable sensitivity, devising suitable spin-magnetometers which ultimately can be used to directly assess oscillating magnetic fields. Specifically, the capability of cavity magnon polaritons of converting magn…
We describe a design to implement a two-qubit geometric phase gate, by which a pair of electrons confined in adjacent quantum dots are entangled. The entanglement is a result of the Coulomb exchange interaction between the optically excited exciton-polaritons and the localized spins. This optical coupling, resembling the electron-electron Ruderman-Kittel-Kasuya-Yosida (RKKY) inter- actions, offers high speed, high fidelity two-qubit gate operation with moderate cavity quality factor Q. The errors due to the finite lifetime of the polaritons can be minimized by optimizing the optical pulse para…
In a circuit quantum eletrodynamic system, a chain of N qubits inhomogeneously coupled to a cavity field forms a mesoscopic quasi-lattice, which is characterized by its degree of deformation from a normal lattice. This deformation is a function of the relative spacing, that is the ratio of the qubit spacing to the cavity wavelength. A polariton mode arise in the quasi-lattice as the dressed mode of the lattice excitation by the cavity photon. We show that the transition probability of the polariton mode is either enhanced or decreased compared to that of a single qubit by the deformation, givi…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
We demonstrate Resonant Tunneling Diodes, embedded in double metal cavities, strongly coupled to the cavity field, while maintaining their electronic properties. We measure the polariton dispersion and find a relative vacuum Rabi splitting of 16%, which explicitly qualifies for the strong-coupling regime. Additionally we show that electronic transport has a significant influence on the polaritons by modulating the coupling strength. The merge between electronic transport and polaritonic physics in our devices opens up a new aspect of cavity quantum electro-dynamics and integrated photonics.
We propose an all optical quantum computation scheme, with trapped electron spin qubits, using their Coulomb exchange interaction with optically excited microcavity exciton-polaritons. This paper describes a single qubit rotation, which together with two-qubit controlled-z gate presented in PRB 85, 241403(R) (2012), form a set of universal logic gates. The errors due to finite cavity lifetime and incorrect orientation of the rotation axis are minimized by optimizing pump pulse parameters. With projective homodyne phase measurement and initialization, our scheme is a promising candidate for the…
Nonadiabatic phenomena are investigated in the rovibrational motion of molecules confined in an infrared cavity. Conical intersections (CIs) between vibrational polaritons, similar to CIs between electronic polaritonic surfaces, are found. The spectral, topological, and dynamic properties of the vibrational polaritons show clear fingerprints of nonadiabatic couplings between molecular vibration, rotation and the cavity photonic mode. Furthermore, it is found that for the investigated system, composed of two rovibrating HCl molecules and the cavity mode, breaking the molecular permutational sym…
Cavity quantum electrodynamics has been studied as a potential approach to modify free charge carrier generation in donor-acceptor heterojunctions because of the delocalization and controllable energy level properties of hybridized light-matter states known as polaritons. However, in many experimental systems, cavity coupling decreases charge separation. Here, we theoretically study the quantum dynamics of a coherent and dissipative donor-acceptor cavity system, to investigate the dynamical mechanism and further discover the conditions under which polaritons may enhance free charge carrier gen…
We apply a microscopic theory of exciton-polaritons in cavity-confined monolayer transition-metal dichalcogenides including both optical polarizations in the monolayer plane, allowing to describe how chiral cavity photons interact with the valley degrees of freedom of the active material. Upon polariton formation, the degenerate excitons inhabiting the two inequivalent valleys are shown to assume bonding and antibonding superpositions as a result of cavity-mediated intravalley interactions combined with intervalley Coulomb interactions. This is representative of a polariton-induced coherent mi…
We propose a scheme which can realize an extended two-component Bose-Hubbard model using polaritons confined in an array of optical cavities. In addition to the density-dependent interactions, this model also contains nonlinear coupling terms between the two components of the polariton. Using a mean-field calculation, we obtain the phase diagram which shows how these terms affect the transition between the Mott insulator and the superfluid phase. In addition, we employ both a perturbation approach and an exact diagonalization method to gain more insights into the phase diagram.
Considering two-level media in the array of weakly coupled nano-cavities, we reveal a variety of dynamical regimes, such as diffusion, self-trapping, soliton, and breathers for the wave-packets in the presence of photon tunneling processes between the next-nearest cavities. We focus our attention on the low branch (LB) bright polariton soliton formation, due to the two-body polariton-polariton scattering processes. When detuning frequency is manipulated adiabatically, the low-branch lattice polariton localized states, i.e., that are solitons and breathers evolving between photon-like and matte…
Electric dipole transitions between different cavity polariton branches or between dressed atomic states with the same excitation number are strictly forbidden in centro-symmetric systems. For doped quantum wells in semiconductor microcavities, the strong coupling between an intersubband transition in the conduction band and a cavity mode produces two branches of intersubband cavity polaritons, whose normal-mode energy splitting is tunable and can be in the terahertz region. Here, we show that, by using asymmetric quantum wells, it is possible to have allowed dipolar transitions between differ…
We investigated coherence delocalization on a coupled-cavity molecular polariton platform in time, frequency, and spatial domains, enabled by ultrafast two-dimensional infrared hyperspectral imaging. Unidirectional coherence delocalization (coherence prepared in one cavity transfer to another cavity) was observed in frequency and real spaces. This directionality was enabled by dissipation of delocalized photon from high-energy to low-energy modes, described by Lindblad dynamics. Further experiments showed that when coherences were directly prepared across cavities (superpositions between polar…
Semiconductor microresonators embedding quantum wells can host tightly confined and mutually interacting excitonic, optical and mechanical modes at once. We theoretically investigate the case where the system operates in the strong exciton-photon coupling regime, while the optical and excitonic resonances are parametrically modulated by the interaction with a mechanical mode. Owing to the large exciton-phonon coupling at play in semiconductors, we predict an enhancement of polariton-phonon interactions by two orders of magnitude with respect to mere optomechanical coupling: a near-unity single…
We present a microscopic semi-analytical theory for the description of organic molecules interacting strongly with a cavity mode. Exciton-vibration coupling within the molecule and exciton-cavity interaction are treated on an equal footing by employing a temperature-dependent variational approach. The interplay between strong exciton-vibration coupling and strong exciton-cavity coupling gives rise to a hybrid ground state, which we refer to as the lower polaron polariton. Explicit expressions for the ground-state wave function, the zero-temperature quasiparticle weight of the lower polaron pol…
We propose a cavity QED approach to describe light-matter interaction between an individual anharmonic molecular vibration and an infrared cavity field. Starting from a generic Morse oscillator with quantized nuclear motion, we derive a multi-level quantum Rabi model to study vibrational polaritons beyond the rotating-wave approximation. We analyze the spectrum of vibrational polaritons in detail and compare with available experiments. For high excitation energies, the spectrum exhibits a dense manifold of true and avoided level crossings as the light-matter coupling strength and cavity freque…
