A photon-magnon hybrid system can be realised by coupling the electron spin resonance of a magnetic material to a microwave cavity mode. The quasiparticles associated with the system dynamics are the cavity magnon polaritons, which arise from the mixing of strongly coupled magnons and photons. We illustrate how these particles can be used to probe the magnetisation of a sample with a remarkable sensitivity, devising suitable spin-magnetometers which ultimately can be used to directly assess oscillating magnetic fields. Specifically, the capability of cavity magnon polaritons of converting magnetic excitations to electromagnetic ones, allows for translating to magnetism the quantum-limited sensitivity reached by state-of-the-art electronics. Here we employ hybrid systems composed of microwave cavities and ferrimagnetic spheres, to experimentally implement two types of novel spin-magnetometers.
Manipulation of Arbitrary-Order Cavity-Magnon Polariton Blockade
Fujian Key Laboratory of Quantum Information and Quantum Optics, College of Physics and Information Engineering, Fuzhou University（福建量子信息与光学重点实验室，福州大学物理与信息工程学院）
Magnon-polaritons are hybrid light-matter quasiparticles originating from the strong coupling between magnons and photons. They have emerged as a potential candidate for implementing quantum transducers and memories. Owing to the dampings of both photons and magnons, the polaritons have limited lifetimes. However, stationary magnon-polariton states can be reached by a dynamical balance between pumping and losses, so the intrinsical nonequilibrium system may be described by a non-Hermitian Hamiltonian. Here we design a tunable cavity quantum electrodynamics system with a small ferromagnetic sph…
The dynamics of arbitrary-order quantum correlations in a cavity magnon-polariton system are investigated based on the quantum master equation in the coherent state representation. The phenomena of Rabi-like oscillation and level repulsion of the average cavity-photon number agree remarkably well with existing experimental observations. The competing nature of coherent and incoherent components in these two cases is further revealed by the second-order quantum coherence of the cavity photons and magnons, which can be systematically tuned by the driving microwave and thermal bath. Our results d…
Due to the small photon momentum, optical spectroscopy commonly probes magnetic excitations only at the center of the Brillouin zone; however, there are ways to override this restriction. In the case of the distorted kagome quantum magnet Y-kapellasite, Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$, under scrutiny here, the magnon density of states can be accessed over the entire Brillouin zone through three-center magnon excitations. This mechanism is aided by the three different magnetic sublattices and strong short-range correlations in the distorted kagome lattice. The results of THz time-domain experiment…
We report the first observation of the magnon-polariton bistability in a cavity magnonics system consisting of cavity photons strongly interacting with the magnons in a small yttrium iron garnet (YIG) sphere. The bistable behaviors are emerged as sharp frequency switchings of the cavity magnon-polaritons (CMPs) and related to the transition between states with large and small number of polaritons. In our experiment, we align, respectively, the [100] and [110] crystallographic axes of the YIG sphere parallel to the static magnetic field and find very different bistable behaviors (e.g., clockwis…
Strong coupling between light and matter occurs when the two interact strongly enough to form new hybrid modes called polaritons. Here we report on the strong coupling of both the electric and magnetic degrees of freedom to an ultrafast terahertz (THz) frequency electromagnetic wave. In our system, optical phonons in a slab of ferroelectric lithium niobate (LiNbO$_3$) are strongly coupled to a THz electric field to form phonon-polaritons, which are simultaneously strongly coupled to magnons in an adjacent slab of canted antiferromagnetic erbium orthoferrite (ErFeO$_3$) via the THz magnetic fie…
Single crystal Lithium Ferrite (LiFe) spheres of sub-mm dimension are examined at mK temperatures, microwave frequencies and variable DC magnetic field, for use in hybrid quantum systems and condensed matter and fundamental physics experiments. Strong coupling regimes of the photon-magnon interaction (cavity magnon polariton quasi-particles) were observed with coupling strength of up to 250 MHz at 9.5 GHz (2.6\%) with magnon linewidths of order 4 MHz (with potential improvement to sub-MHz values). We show that the photon-magnon coupling can be significantly improved and exceed that of the wide…
We demonstrate the strong coupling of both magnons and phonons to terahertz (THz) frequency electromagnetic (EM) waves confined to a photonic crystal (PhC) cavity. Our cavity consists of a two-dimensional array of air-holes cut into a hybrid slab of ferroelectric lithium niobate (LiNbO$_3$) and erbium orthoferrite (ErFeO$_3$), a canted antiferromagnetic crystal. The phonons in LiNbO$_3$ and the magnons in ErFeO$_3$ are strongly coupled to the electric and magnetic field components of the confined EM wave, respectively. This leads to the formation of new cavity magnon-phonon-polariton modes, wh…
Cavity-magnon polaritons (CMPs) are the associated quasiparticles of the hybridization between cavity photons and magnons in a magnetic sample placed in a microwave resonator. In the strong coupling regime, where the macroscopic coupling strength exceeds the individual dissipation, there is a coherent exchange of information. This renders CMPs as promising candidates for future applications such as in information processing. Recent advances on the study of the CMP now allow not only for creation of CMPs on demand, but also for tuning of the coupling strength - this can be thought of as enhanci…
Cavity control of quantum matter may offer new ways to study and manipulate many-body systems. A particularly appealing idea is to use cavities to enhance superconductivity, especially in unconventional or high-$T_c$ systems. Motivated by this, we propose a scheme for coupling Terahertz resonators to the antiferromagnetic fluctuations in a cuprate parent compound, which are believed to provide the glue for Cooper pairs in the superconducting phase. First, we derive the interaction between magnon excitations of the Neél-order and polar phonons associated with the planar oxygens. This mode also …
We study the phase controlled transmission properties in a compound system consisting of a 3D copper cavity and an yttrium iron garnet (YIG) sphere. By tuning the relative phase of the magnon pumping and cavity probe tones, constructive and destructive interferences occur periodically, which strongly modify both the cavity field transmission spectra and the group delay of light. Moreover, the tunable amplitude ratio between pump-probe tones allows us to further improve the signal absorption or amplification, accompanied by either significantly enhanced optical advance or delay. Both the phase …
We present that two spin defects (SDs) can be entangled through a magnon polariton mode, within the strong coupling regime. The magnonic modes are provided by an antiferromagnetic (AF) MnF$_{2}$ layer and their dispersion is characterized by the layer's thickness. The macroscopic quantum electrodynamics theory is used to describe the light-matter interactions, where the Green's functions are its core element. The individual SD relaxes by exciting the magnon polariton modes, exhibiting high enhancement values of the Purcell factor. When two SDs are considered, an oscillatory population exchange…
A scheme of an ultra-sensitive magnetometer in the cavity quantum electromagnonics where the intracavity microwave mode coupled to a magnonic mode via magnetic dipole interaction is proposed. It is shown that by driving both magnonic and microwave modes with external classical fields and controlling the system parameters, one can reduce the added noise of magnetic field measurement below the standard quantum limit (SQL). Surprisingly, we show that beyond the rotating wave approximation (RWA), not only the added noise can be suppressed, but also the output cavity response to the input signal ca…
We characterize some of the distinctive hallmarks of magnon-magnon interaction mediated by the intracavity field of a microwave cavity, along with their testable ramifications. In general, we foreground two widely dissimilar parameter domains that bring forth the contrasting possibilities of level splitting and level crossing. The former is observed in the regime of strong magnon-photon couplings, particularly when the three modes bear comparable relaxation rates. This character is marked by the appearance of three distinguishable and non-converging polariton branches in the spectral response …
In this work, the ultra-strong photon-to-magnon coupling is demonstrated for on-chip multilayered superconductor/ferromagnet/insulator hybrid thin film structures reaching the coupling strength above 6 GHz, the coupling ratio about 0.6, the single-spin coupling strength about 350 Hz, and cooperativity about 10^4. High characteristics of coupling are achieved owing to a radical suppression of the photon phase velocity in electromagnetic resonator. With achieved coupling the spectrum reveals inapplicability of the Dicke model, and evidences contribution of the diamagnetic A^2 interaction term in…
As the counterpart of PT symmetry, abundant phenomena and potential applications of anti-PT symmetry have been predicted or demonstrated theoretically. However, experimental realization of the coupling required in the anti-PT symmetry is difficult. Here, by coupling two YIG spheres to a microwave cavity, the large cavity dissipation rate makes the magnons coupled dissipatively with each other, thereby obeying a two-dimensional anti-PT Hamiltonian. In terms of the magnon-readout method, a new method adopted here, we demonstrate the validity of our method in constructing an anti-PT system and pr…
We investigate a hybrid quantum system where an ensemble of nitrogen-vacancy (NV) centers in diamond is interfaced with a piezomagnetic superlattice that supports surface phonon polaritons (SPhPs). We show that the strong magnetic coupling between the collective spin waves in the NV spin ensemble and the quantized SPhPs can be realized, thanks to the subwavelength nature of the SPhPs and relatively long spin coherence times. The magnon-polariton coupling allows different modes of the SPhPs to be mapped and orthogonally stored in different spatial modes of excitation in the solid medium. Becaus…
Strong coupling between cavity photons and various excitations in condensed matters boosts the field of light-matter interaction and generates several exciting sub-fields, such as cavity optomechanics and cavity magnon polariton. Axion quasiparticles, emerging in topological insulators, were predicted to strongly couple with the light and generate the so-called axion polariton. Here, we demonstrate that there arises a gapless level attraction in cavity axion polariton of antiferromagnetic topological insulators, which originates from a nonlinear interaction between axion and the odd-order reso…
We experimentally investigate magnon-polaritons, arising in ferrimagnetic resonance experiments in a microwave cavity with a tuneable quality factor. To his end, we simultaneously measure the electrically detected spin pumping signal and microwave reflection (the ferrimagnetic resonance signal) of a yttrium iron garnet (YIG) / platinum (Pt) bilayer in the microwave cavity. The coupling strength of the fundamental magnetic resonance mode and the cavity is determined from the microwave reflection data. All features of the magnetic resonance spectra predicted by first principle calculations and a…
Anticrossing behavior between magnons in a non-collinear chiral magnet Cu$_2$OSeO$_3$ and a two-mode X-band microwave resonator was studied in the temperature range 5-100K. In the field-induced ferrimagnetic phase, we observed a strong coupling regime between magnons and two microwave cavity modes with a cooperativity reaching 3600. In the conical phase, cavity modes are dispersively coupled to a fundamental helimagnon mode, and we demonstrate that the magnetic phase diagram of Cu$_2$OSeO$_3$ can be reconstructed from the measurements of the cavity resonance frequency. In the helical phase, a …
Several experimental implementations of cavity-magnon systems are presented. First an Yttrium Iron Garnet (YIG) block is placed inside a re-entrant cavity where the resulting hybrid mode is measured to be in the ultra strong coupling regime. When fully hybridised the ratio between the coupling rate and uncoupled mode frequencies is determined to be $g/ω=0.46$. Next a thin YIG cylinder is placed inside a loop gap cavity. The bright mode of this cavity couples to the YIG sample and is similarly measured to be in the ultra strong coupling regime with ratio of coupling rate to uncoupled mode frequ…
Nitrogen vacancy (NV) centers, optically active atomic defects in diamond, have been widely applied to emerging quantum sensing, imaging, and network efforts, showing unprecedented field sensitivity and nanoscale spatial resolution. Many of these advantages derive from their excellent quantum-coherence, controllable entanglement, and high fidelity of operations, enabling opportunities to outperform the classical counterpart. Exploiting this cutting-edge quantum metrology, we report noninvasive measurement of intrinsic spin fluctuations of magnetic insulator thin films with a spontaneous out-of…
The spin resonance of electrons can be coupled to a microwave cavity mode to obtain a photon-magnon hybrid system. These quantum systems are widely studied for both fundamental physics and technological quantum applications. In this article, the behavior of a large number of ferrimagnetic spheres coupled to a single cavity is put under test. We use second-quantization modeling of harmonic oscillators to theoretically describe our experimental setup and understand the influence of several parameters. The magnon-polariton dispersion relation is used to characterize the system, with a particular …
