The introduction of nonlinear nanophotonic devices to the field of optical frequency comb metrology has enabled new opportunities for low-power and chip-integrated clocks, high-precision frequency synthesis, and broad bandwidth spectroscopy. However, most of these advances remain constrained to the near-infrared region of the spectrum, which has restricted the integration of frequency combs with numerous quantum and atomic systems in the ultraviolet and visible. Here, we overcome this shortcoming with the introduction of multi-segment nanophotonic thin-film lithium niobate (LN) waveguides that combine engineered dispersion and chirped quasi-phase matching for efficient supercontinuum generation via the combination of $χ^{(2)}$ and $χ^{(3)}$ nonlinearities. With only 90 pJ of pulse energy at 1550 nm, we achieve gap-free frequency comb coverage spanning 330 to 2400 nm. The conversion efficiency from the near-infrared pump to the UV-Visible region of 350-550 nm is nearly 20%. Harmonic generation via the $χ^{(2)}$ nonlinearity in the same waveguide directly yields the carrier-envelope offset frequency and a means to verify the comb coherence at wavelengths as short as 350 nm. Our results provide an integrated photonics approach to create visible and UV frequency combs that will impact precision spectroscopy, quantum information processing, and optical clock applications in this important spectral window.
Modern communication networks require high performance and scalable electro-optic modulators that convert electrical signals to optical signals at high speed. Existing lithium niobate modulators have excellent performance but are bulky and prohibitively expensive to scale up. Here we demonstrate scalable and high-performance nanophotonic electro-optic modulators made of single-crystalline lithium niobate microring resonators and micro-Mach-Zehnder interferometers. We show a half-wave electro-optic modulation efficiency of 1.8V$\cdot$cm and data rates up to 40 Gbps.
In this paper, we have investigated the interplay between the second and third-order nonlinearities in lithium-niobate waveguides with strong waveguide dispersion using uniform and linearly-chirped poling patterns at input powers in the pico-joule range. We have implemented the accurate unidirectional pulse propagation model to take into account all the possible nonlinear interactions inside these structures. In particular, the poling period has been designed to quasi-phase-match single and multiple sum- and difference-frequency generation processes. We have shown how the poling period can be …
Strong amplification in integrated photonics is one of the most desired optical functionalities for computing, communications, sensing, and quantum information processing. Semiconductor gain and cubic nonlinearities, such as four-wave mixing and stimulated Raman and Brillouin scattering, have been among the most studied amplification mechanisms on chip. Alternatively, material platforms with strong quadratic nonlinearities promise numerous advantages with respect to gain and bandwidth, among which nanophotonic lithium niobate is one of the most promising candidates. Here, we combine quasi-phas…
Highly-tunable coherent light generation is crucial for many important photonic applications. Second-harmonic generation (SHG) is a dominant approach for this purpose, which, however, exhibits a trade-off between the conversion efficiency and the wavelength tunability in a conventional nonlinear platform. Recent development of the integrated lithium niobate (LN) technology makes it possible to achieve a large wavelength tuning while maintaining a high conversion efficiency. Here we report on-chip SHG that simultaneously achieves a large tunability and a high conversion efficiency inside a sing…
Squeezed light is a key quantum resource that enables quantum advantages for sensing, networking, and computing applications. The scalable generation and manipulation of squeezed light with integrated platforms are highly desired for the development of quantum technology with continuous variables. In this letter, we demonstrate squeezed light generation with thin-film lithium niobate integrated photonics. Para-metric down-conversion is realized with quasi-phase matching using ferroelectric domain engineering. With sub-wavelength mode confinement, efficient nonlinear processes can be observed w…
Quasi-phasematched interactions in waveguides with quadratic nonlinearities enable highly efficient nonlinear frequency conversion. In this article, we demonstrate the first generation of devices that combine the dispersion-engineering available in nanophotonic waveguides with quasi-phasematched nonlinear interactions available in periodically poled lithium niobate (PPLN). This combination enables quasi-static interactions of femtosecond pulses, reducing the pulse energy requirements by several orders of magnitude, from picojoules to femtojoules. We experimentally demonstrate two effects assoc…
Chip-integrated nonlinear photonics holds the key for advanced optical information processing with superior performance and novel functionalities. Here, we present an optimally mode-matched, periodically poled lithium niobate nanowaveguide for efficient parametric frequency conversions on chip. Using a 4-mm nanowaveguide with subwavelength mode confinement, we demonstrate second harmonic generation with efficiency over $2200\%~W^{-1}cm^{-2}$, and broadband difference frequency generation with similar efficiency over a 4.5-THz spectral span. These allow us to generate correlated photon pairs ov…
Bound states in the continuum (BICs) have been extensively studied in various systems since its first proposal in quantum mechanics. Photonic BICs can enable optical mode confinement and provide field enhancement for nonlinear optics, but they have rarely been explored in nonlinear integrated photonic waveguides. Applying BICs in photonic integrated circuits enables low-loss light guidance and routing in low-refractive-index waveguides on high-refractive-index substrates, which is suitable for integrated photonics with nonlinear materials. Here, we report experimental demonstration of second-h…
Optical nonlinear functions are crucial for various applications in integrated photonics, such as all-optical information processing, photonic neural networks and on-chip ultrafast light sources. Due to the weak nonlinearities in most integrated photonic platforms, realizing optical nonlinear functions typically requires large driving energies in the picojoules level or beyond, thus imposing a barrier for most applications. Here, we tackle this challenge and demonstrate an integrated nonlinear splitter device in lithium niobate nano-waveguides by simultaneous engineering of the dispersion and …
Lithium-Niobate-On-Insulator (LNOI) is emerging as a promising platform for integrated quantum photonic technologies because of its high second-order nonlinearity and compact waveguide footprint. Importantly, LNOI allows for creating electro-optically reconfigurable circuits, which can be efficiently operated at cryogenic temperature. Their integration with superconducting nanowire single-photon detectors (SNSPDs) paves the way for realizing scalable photonic devices for active manipulation and detection of quantum states of light. Here we report the first demonstration of these two key compon…
Lithium niobate-on-insulator (LNOI) is an emerging photonic platform that exhibits favorable material properties (such as low optical loss, strong nonlinearities, and stability) and enables large-scale integration with stronger optical confinement, showing promise for future optical networks, quantum processors, and nonlinear optical systems. However, while photonics engineering has entered the era of automated "inverse design" via optimization in recent years, the design of LNOI integrated photonic devices still mostly relies on intuitive models and inefficient parameter sweeps, limiting the …
Wavelength transduction of single-photon signals is indispensable to networked quantum applications, particularly those incorporating quantum memories. Lithium niobate nanophotonic devices have demonstrated favorable linear, nonlinear, and electro-optical properties to deliver this crucial function while offering superiror efficiency, integrability, and scalability. Yet, their quantum noise level--an crucial metric for any single-photon based application--has yet to be understood. In this work, we report the first study with the focus on telecom to near-visible conversion driven by a telecom p…
Lithium niobate is an excellent photonic material with large $χ^2$ and $χ^3$ nonlinearities. Recent breakthroughs in nanofabrication technology have enabled ultralow-loss nanophotonic devices based on a lithium-niobate-on-insulator (LNOI) platform. Here we present an overview of recent developments in the LNOI platform for on-chip optical frequency comb generation. These devices could lead to new opportunities for integrated nonlinear photonic devices for classical and quantum photonic applications.
Lithium niobate (LN) exhibits unique material characteristics that have found many important applications. Scaling LN devices down to a nanoscopic scale can dramatically enhance light-matter interaction that would enable nonlinear and quantum photonic functionalities beyond the reach of conventional means. However, developing LN-based nanophotonic devices turns out to be nontrivial. Although significant efforts have been devoted in recent years, LN photonic crystal structures developed to date exhibit fairly low quality. Here we demonstrate LN photonic crystal nanobeam resonators with optical …
Optical frequency comb is an enabling technology for a multitude of applications from metrology to ranging and communications. The tremendous progress in sources of optical frequency combs has mostly been centered around the near-infrared spectral region while many applications demand sources in the visible and mid-infrared, which have so far been challenging to achieve, especially in nanophotonics. Here, we report frequency combs tunable from visible to mid-infrared on a single chip based on ultra-widely tunable optical parametric oscillators in lithium niobate nanophotonics. Using picosecond…
In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the Continuum and the excellent nonlinear optical crystal of lithium niobate. The enhancement factor is defined as the ratio of the second harmonic signal generated by the structure (lithium niobate membrane with Si grating) divided by the signal generated by lithium niobate membrane alone. Furthermore, a minimum interaction time of 350 ps is achieved despite the etch…
High complexity, dense integrated nanophotonic circuits possessing strong nonlinearities are desirable for a breadth of applications in classical and quantum optics. In this work, we study natural phase matching via modal engineering in lithium niobate (LN) waveguides and microring resonators on chip for second harmonic generation (SHG). By carefully engineering the geometry dispersion, we observe a $26\%~W^{-1}cm^{-2}$ normalized efficiency for SHG in a waveguide with submicron transverse mode confinement. With similar cross-sectional dimensions, we demonstrate phase matched SHG in a microrin…
In recent years, the computational demands of deep learning applications have necessitated the introduction of energy-efficient hardware accelerators. Optical neural networks are a promising option; however, thus far they have been largely limited by the lack of energy-efficient nonlinear optical functions. Here, we experimentally demonstrate an all-optical Rectified Linear Unit (ReLU), which is the most widely used nonlinear activation function for deep learning, using a periodically-poled thin-film lithium niobate nanophotonic waveguide and achieve ultra-low energies in the regime of femtojo…
Periodically poled thin-film lithium niobate (TFLN) waveguides have emerged as a leading platform for highly efficient frequency conversion in the near-infrared. However, the commonly used silica bottom-cladding results in high absorption loss at wavelengths beyond 2.5 $μ$m. In this work, we demonstrate efficient frequency conversion in a TFLN-on-sapphire platform, which features high transparency up to 4.5 $μ$m. In particular, we report generating mid-infrared light up to 3.66 $μ$m via difference-frequency generation of a fixed 1-$μ$m source and a tunable telecom source, with normalized effic…
Lithium niobate (LN), an outstanding and versatile material, has influenced our daily life for decades: from enabling high-speed optical communications that form the backbone of the Internet to realizing radio-frequency filtering used in our cell phones. This half-century-old material is currently embracing a revolution in thin-film LN integrated photonics. The success of manufacturing wafer-scale, high-quality, thin films of LN on insulator (LNOI), accompanied with breakthroughs in nanofabrication techniques, have made high-performance integrated nanophotonic components possible. With rapid d…
A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric pressure and the simultaneous sensitive detection of multiple atoms or molecules are the key challenges. Here, an electro-optic microring-based dual-comb interferometer, fabricated on a low-loss lithium-niobate-on-insulator nanophotonic platform, demonstrates significant progress towards such an achievement. Spectra spanning 1.6 THz (53 cm-1) at a resolution of…
Scalable photonic quantum computing architectures pose stringent requirements on photonic processing devices. The need for low-loss high-speed reconfigurable circuits and near-deterministic resource state generators are some of the most challenging requirements. Here we develop an integrated photonic platform based on thin-film lithium niobate and interface it with deterministic solid-state single-photon sources based on quantum dots in nanophotonic waveguides. The generated photons are processed with low-loss circuits programmable at speeds of several GHz. We realize a variety of key photonic…
Polarization is a fundamental degree of freedom for light and is widely leveraged in free space and fiber optics. Non-reciprocal polarization rotation, enabled via the magneto-optic Faraday effect, has been essentially unbeatable for broadband isolators and circulators. For integrated photonics foundries, however, there is still no good path to producing low-loss magneto-optic components, which has prompted a search for alternatives that do not use polarization rotation. Moreover, magneto-optic materials tend to be highly lossy, and while large (10-100 rad/cm) polarization rotation can be achi…
We demonstrate conversion of up to 4.5 GHz-frequency microwaves to 1500 nm-wavelength light using optomechanical interactions on suspended thin-film lithium niobate. Our method utilizes an interdigital transducer that drives a free-standing 100 $μ$m-long thin-film acoustic resonator to modulate light travelling in a Mach-Zehnder interferometer or racetrack cavity. Owing to the strong microwave-to-acoustic coupling offered by the transducer in conjunction with the strong photoelastic, piezoelectric, and electro-optic effects of lithium niobate, we achieve a half-wave voltage of $V_π$ = 4.6 V an…
Periodically poled lithium niobate (PPLN) waveguide is a powerful platform for efficient wavelength conversion. Conventional PPLN converters however typically require long device lengths and high pump powers due to the limited nonlinear interaction strength. Here we use a nanostructured PPLN waveguides to demonstrate an ultrahigh normalized efficiency of 2600%/W-cm$^2$ for second-harmonic generation of 1.5-$μ$m radiation, more than 20 times higher than that in state-of-the-art diffused waveguides. This is achieved by a combination of sub-wavelength optical confinement and high-fidelity periodi…
Several applications in modern photonics require compact on-chip optical filters with a tailored spectral response. However, achieving sub-nanometric bandwidths and high extinction ratios is particularly challenging, especially in low-footprint device formats. Phase shifted Bragg gratings implemented by sidewall modulation of photonic nanowire waveguides are a good solution for on-chip narrowband operation with reasonable requirements in fabrication and scalability. In this work we report on their implementation and optimization in thin film lithium niobate, a photonic platform that affords re…
The integration of complex oxides on silicon presents opportunities to extend and enhance silicon technology with novel electronic, magnetic, and photonic properties. Among these materials, barium titanate (BaTiO3) is a particularly strong ferroelectric perovskite oxide with attractive dielectric and electro-optic properties. Here we demonstrate nanophotonic circuits incorporating ferroelectric BaTiO3 thin films on the ubiquitous silicon-on-insulator (SOI) platform. We grow epitaxial, single-crystalline BaTiO3 directly on SOI and engineer integrated waveguide structures that simultaneously con…
