A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric pressure and the simultaneous sensitive detection of multiple atoms or molecules are the key challenges. Here, an electro-optic microring-based dual-comb interferometer, fabricated on a low-loss lithium-niobate-on-insulator nanophotonic platform, demonstrates significant progress towards such an achievement. Spectra spanning 1.6 THz (53 cm-1) at a resolution of 10 GHz (0.33 cm-1) are obtained in a single measurement without requiring frequency scanning or moving parts. The frequency agility of the system enables spectrally-tailored multiplexed sensing, which allows for interrogation of non-adjacent spectral regions, here separated by 6.6 THz (220 cm-1), without compromising the signal-to-noise ratio.
Lithium niobate is an excellent photonic material with large $χ^2$ and $χ^3$ nonlinearities. Recent breakthroughs in nanofabrication technology have enabled ultralow-loss nanophotonic devices based on a lithium-niobate-on-insulator (LNOI) platform. Here we present an overview of recent developments in the LNOI platform for on-chip optical frequency comb generation. These devices could lead to new opportunities for integrated nonlinear photonic devices for classical and quantum photonic applications.
Optical frequency combs have become a very powerful tool in metrology and beyond thanks to their ability to link radio frequencies with optical frequencies via a process known as self-referencing. Typical self-referencing is accomplished in two steps: the generation of an octave-spanning supercontinuum spectrum and the frequency-doubling of one part of that spectrum. Traditionally, these two steps have been performed by two separate optical components. With the advent of photonic integrated circuits, the combination of these two steps has become possible in a single small and monolithic chip. …
We demonstrate efficient tuning of a monolithically integrated lithium niobate microdisk (LN) optical frequency microcomb. Utilizing the high optical quality (Q) factor (i.e., Q~7.1*10^6) of the microdisk, the microcomb spans over a spectral bandwidth of ~200 nm at a pump power as low as 20.4 mW. Combining the large eletro-optic coefficient of LN and optimum design of the geometry of microelectrodes, we demonstrate electro-optical tuning of the comb with a spectral range of 400 pm and a tuning efficiency of ~38 pm/100V.
We demonstrate fabrication of single-mode optical waveguides on lithium niobate on insulator (LNOI) by optical patterning combined with chemo-mechanical polishing. The fabricated LNOI waveguides have a nearly symmetric mode profile of a mode field size of ~2.5 micron (full-width at half maximum). We develop a high-precision measurement approach by which the single mode waveguides are characterized to have a propagation loss of ~0.042 dB/cm.
Quasi-phasematched interactions in waveguides with quadratic nonlinearities enable highly efficient nonlinear frequency conversion. In this article, we demonstrate the first generation of devices that combine the dispersion-engineering available in nanophotonic waveguides with quasi-phasematched nonlinear interactions available in periodically poled lithium niobate (PPLN). This combination enables quasi-static interactions of femtosecond pulses, reducing the pulse energy requirements by several orders of magnitude, from picojoules to femtojoules. We experimentally demonstrate two effects assoc…
We demonstrate ultra-high Q factor microring resonators close to the intrinsic material absorption limit on lithium niobate on insulator. The microrings are fabricated on pristine lithium niobate (LN) thin film wafer thinned from LN bulk via chemo-mechanical etching without ion slicing and ion etching. A record-high Q factor up to times ten to the power of 8th at the wavelength of 1550 nm is achieved because of the ultra-smooth interface of the microrings and the absence of ion induced lattice damage, indicating an ultra-low waveguide propagation loss of about 0.28 dB per meter. The ultra-high…
Electro-optic phase modulators are critical components in modern communication, microwave photonic, and quantum photonic systems. Important for these applications is to achieve modulators with low half-wave voltage at high frequencies. Here we demonstrate an integrated phase modulator, based on a thin-film lithium niobate platform, that simultaneously features small on-chip loss (~ 1 dB) and low half-wave voltage over a large spectral range (3.5 - 4.5 V at 5 - 40 GHz). By driving the modulator with a strong 30-GHz microwave signal corresponding to around four half-wave voltages, we generate an…
The linewidth enhancement factor (LEF) has recently moved into the spotlight of research on frequency comb generation in semiconductor lasers. Here we present a novel modulation experiment, which enables the direct measurement of the spectrally resolved LEF in a laser frequency comb. By utilizing a phase-sensitive technique, we are able to extract the LEF for each comb mode. We first investigate and verify this universally applicable technique using Maxwell-Bloch simulations and then present the experimental demonstration on a quantum cascade laser frequency comb.
Electro-optic modulators with low voltage and large bandwidth are crucial for both analog and digital communications. Recently, thin-film lithium niobate modulators have enable dramatic performance improvements by reducing the required modulation voltage while maintaining high bandwidths. However, the reduced electrode gaps in such modulators leads to significantly higher microwave losses, which limit electro-optic performance at high frequencies. Here we overcome this limitation and achieve a record combination of low RF half-wave voltage of 1.3 V while maintaining electro-optic response with…
Lithium niobate on insulator (LNOI), regarded as an important candidate platform for optical integration due to its excellent nonlinear, electro-optic and other physical properties, has become a research hotspot. Light source, as an essential component for integrated optical system, is urgently needed. In this paper, we reported the realization of 1550-nm band on-chip LNOI microlasers based on erbium-doped LNOI ring cavities with loaded quality factors higher than one million, which were fabricated by using electron beam lithography and inductively coupled plasma reactive ion etching processes…
Electrically driven acousto-optic devices that provide beam deflection and optical frequency shifting have broad applications from pulse synthesis to heterodyne detection. Commercially available acousto-optic modulators are based on bulk materials and consume Watts of radio frequency power. Here, we demonstrate an integrated 3-GHz acousto-optic frequency shifter on thin-film lithium niobate, featuring a carrier suppression over 30 dB. Further, we demonstrate a gigahertz-spaced optical frequency comb featuring more than 200 lines over a 0.6-THz optical bandwidth by recirculating the light in an…
Atomic frequency combs memories that coherently store optical signals are a key building block for optical quantum computers and quantum networks. Integrating such memories into compact and chip-scale devices is essential for scalable quantum technology, but to date most demonstrations have been in bulk materials or waveguides with large cross-sections, or using fabrication techniques not easily adaptable to wafer scale processing. We demonstrate compact chip-integrated atomic frequency comb storage in rare earth doped thin-film lithium niobate. Our optical memory exhibits a broad storage band…
Recent advances in the processing of thin-film LNOI have enabled low-loss photonic integrated circuits, modulators with improved half-wave voltage, electro-optic frequency combs and novel on-chip electro-optic devices, with applications ranging from 5G telecommunication and microwave photonics to microwave-to-optical quantum interfaces. Lithium niobate integrated photonic circuits could equally be the basis of integrated narrow-linewidth frequency-agile lasers. Pioneering work on polished lithium niobate crystal resonators has led to the development of electrically tunable narrow-linewidth las…
Lithium Niobate on insulator (LNOI) photonics promises to combine the excellent nonlinear properties of Lithium Niobate with the high complexity achievable by high contrast waveguides. However, to date, fabrication challenges have resulted in high-loss and sidewall-angled waveguides, limiting its applicability. We report LNOI single mode waveguides with ultra low propagation loss of 0.4 dB/cm and sidewall angle of 75°. Our results open the route to a highly efficient photonic platform with applications ranging from high-speed telecommunication to quantum technology.
Many technologies in quantum photonics require cryogenic conditions to operate. However, the underlying platform behind active components such as switches, modulators and phase shifters must be compatible with these operating conditions. To address this, we demonstrate an electro-optic polarisation converter for 1550nm light at 0.8K in titanium in-diffused lithium niobate waveguides. To do so, we exploit the electro-optic properties of lithium niobate to convert between orthogonal polarisation modes with a fiber-to-fiber transmission >43%. We achieve a modulation depth of 23.6 +/-3.3dB and a c…
Acousto-optic interactions involving propagating phonons can break the time-reversal and frequency-modulation symmetry of light. However, conventional acousto-optic modulators based on bulk materials have frequency bandwidth limited to hundreds of megahertz due to their large structural sizes. Here, we experimentally demonstrate gigahertz single-sideband acousto-optic modulation on an etchless lithium niobate integrated platform by using photonic bound states in the continuum. The upper- or lower-sideband modulation of light can be obtained conveniently by choosing specific combinations of inp…
Integrated lithium niobate (LN) photonic circuits have recently emerged as a promising candidate for advanced photonic functions such as high-speed modulation, nonlinear frequency conversion and frequency comb generation. For practical applications, optical interfaces that feature low fiber-to-chip coupling losses are essential. So far, the fiber-to-chip loss (commonly > 10 dB) dominates the total insertion losses of typical LN photonic integrated circuits, where on-chip propagation losses can be as low as 0.03 - 0.1 dB/cm. Here we experimentally demonstrate a low-loss mode size converter for …
Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS typically takes microseconds to milliseconds, the applications of these spectrometers have generally been limited to systems and processes with time changes on the order of seconds or minutes due to the need to average many spectra to reach a high signal-to-noise ratio (SNR). Here, we demonstrate high-speed, continuous, fiber mode-locked laser DCS with down to 11 $…
Push-Pull acousto-optic modulator based on non-suspended thin-film lithium niobate on silicon substrate
Elmore Family School of Electrical and Computer Engineering, Purdue University（普渡大学埃尔莫电气与计算机工程学院）；Department of Electrical and Computer Engineering, University of Michigan（密歇根大学电气与计算机工程系）
Thin-film lithium niobate on insulator (LNOI) is a promising platform for optical communications, microwave photonics, and quantum technologies. While many high-performance devices like electro-optic modulators and frequency comb sources have been achieved on LNOI platform, it remains challenging to realize photodetectors (PDs) on LNOI platform using simple and low-cost fabrication techniques. Two-dimensional (2D) materials are excellent candidates to achieve photodetection since they feature strong light-matter interaction, excellent mechanical flexibility, and potential large-scale complemen…
The measurement and stabilization of the carrier-envelope offset frequency $f_{\textrm{CEO}}$ via self-referencing is paramount for optical frequency comb generation which has revolutionized precision frequency metrology, spectroscopy, and optical clocks. Over the past decade, the development of chip-scale platforms has enabled compact integrated waveguides for supercontinuum generation. However, there is a critical need for an on-chip self-referencing system that is adaptive to different pump wavelengths, requires low pulse energy, and does not require complicated processing. Here, we demonst…
Lithium niobate (LN), an outstanding and versatile material, has influenced our daily life for decades: from enabling high-speed optical communications that form the backbone of the Internet to realizing radio-frequency filtering used in our cell phones. This half-century-old material is currently embracing a revolution in thin-film LN integrated photonics. The success of manufacturing wafer-scale, high-quality, thin films of LN on insulator (LNOI), accompanied with breakthroughs in nanofabrication techniques, have made high-performance integrated nanophotonic components possible. With rapid d…
We demonstrate up-conversion single-photon detectors based on integrated periodically poled lithium niobate waveguides, which incorporate two mode filters and a directional coupler. The two mode filters are optimized for the fiber-waveguide coupling efficiencies for 1550 nm and 1950 nm respectively while the directional coupler plays the role of wavelength combiner, making the overall system portable and low-cost. The two wavelengths pump each other in our detection system. We achieve detection efficiencies of 28% for 1550 nm and 27% for 1950 nm, respectively. This scheme provides an efficient…
Optical modulators are at the heart of optical communication links. Ideally, they should feature low insertion loss, low drive voltage, large modulation bandwidth, high linearity, compact footprint and low manufacturing cost. Unfortunately, these criteria have only been achieved on separate occasions.Based on a Silicon and Lithium Niobate hybrid integration platform, we demonstrate Mach-Zehnder modulators that simultaneously fulfill these criteria. The presented device exhibits an insertion loss of 2.5 dB, voltage-length product of 2.2 Vcm, high linearity, electro-optic bandwidth of at least 7…
Optical frequency comb is an enabling technology for a multitude of applications from metrology to ranging and communications. The tremendous progress in sources of optical frequency combs has mostly been centered around the near-infrared spectral region while many applications demand sources in the visible and mid-infrared, which have so far been challenging to achieve, especially in nanophotonics. Here, we report frequency combs tunable from visible to mid-infrared on a single chip based on ultra-widely tunable optical parametric oscillators in lithium niobate nanophotonics. Using picosecond…
Low-loss phononic integrated circuits based on a silicon nitride-lithium niobate platform
Bradley Department of Electric and Computer Engineering, Virginia Tech（弗吉尼亚理工大学电气与计算机工程布拉德利系）；Department of Electrical and Computer Engineering, University of Virginia（弗吉尼亚大学电气与计算机工程系）；Department of Physics and Center for Quantum Information Science and Engineering (VTQ), Virginia Tech（弗吉尼亚理工大学物理系及量子信息科学与工程中心）
