Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS typically takes microseconds to milliseconds, the applications of these spectrometers have generally been limited to systems and processes with time changes on the order of seconds or minutes due to the need to average many spectra to reach a high signal-to-noise ratio (SNR). Here, we demonstrate high-speed, continuous, fiber mode-locked laser DCS with down to 11 $μ$s time resolution. We achieve this by filtering the comb spectra using portable Fabry-Perot cavities to generate filtered combs with 1 GHz tooth spacing. The 1 GHz spacing increases the DCS acquisition speed and SNR for a given optical bandwidth while retaining a sufficient spacing to resolve absorption features over a wide range of conditions. We measure spectra of methane inside a rapid compression machine throughout the 16 ms compression cycle with 133 cm$^{-1}$ bandwidth (4000 comb teeth) and 1.4 ms time resolution by spectrally filtering one of the combs. By filtering both combs, we measured a single-shot, 25 cm$^{-1}$ (750 comb teeth) spectrum of CO around 6330 cm$^{-1}$ in 11 $μ$s. The technique enables simultaneously high-speed and high-resolution DCS measurements, and can be applied anywhere within the octave-spanning spectrum of robust and portable fiber mode-locked frequency combs.
We generate mode-locked picosecond pulses near 1110 nm by spectrally slicing and reamplifying an octave-spanning supercontinuum source pumped at 1550 nm. The 1110 nm pulses are near transform-limited, with 1.7 ps duration over their 1.2 nm bandwidth, and exhibit high interpulse coherence. Both the supercontinuum source and the pulse synthesis system are implemented completely in fiber. The versatile source construction suggests that pulse synthesis from sliced supercontinuum may be a useful technique across the 1000 - 2000 nm wavelength range.
We analyze the influence of spectrally modulated dispersion and loss on the stability of mode-locked oscillators. In the negative dispersion regime, a soliton oscillator can be stabilized in a close proximity to zero-dispersion wavelength, when spectral modulation of dispersion and loss are strong and weak, respectively. If the dispersion is close to zero but positive, we observe chaotic mode-locking or a stable coexistence of the pulse with the CW signal. The results are confirmed by experiments with a Cr:YAG oscillator.
The gain properties of an oscillator strongly affect its behavior. When the gain is homogeneous, different modes compete for gain resources in a `winner takes all' manner, whereas with inhomogeneous gain, modes can coexist if they utilize different gain resources. We demonstrate precise control over the mode competition in a mode locked Ti:sapphire oscillator by manipulation and spectral shaping of the gain properties, thus steering the competition towards a desired, otherwise inaccessible, oscillation. Specifically, by adding a small amount of spectrally shaped inhomogeneous gain to the stand…
Precision frequency and phase synchronization between distinct fiber interconnected nodes is critical for a wide range of applications, including atomic timekeeping, quantum networking, database synchronization, ultra-high-capacity coherent optical communications and hyper-scale data centers. Today, many of these applications utilize precision, tabletop laser systems, and would benefit from integration in terms of reduced size, power, cost, and reliability. In this paper we report a record low 3x10^-4 rad^2 residual phase error variance for synchronization based on independent, spectrally pure…
The linewidth enhancement factor (LEF) has recently moved into the spotlight of research on frequency comb generation in semiconductor lasers. Here we present a novel modulation experiment, which enables the direct measurement of the spectrally resolved LEF in a laser frequency comb. By utilizing a phase-sensitive technique, we are able to extract the LEF for each comb mode. We first investigate and verify this universally applicable technique using Maxwell-Bloch simulations and then present the experimental demonstration on a quantum cascade laser frequency comb.
We report a mode-locked Ti:sapphire femtosecond laser with 5GHz repetition rate. Spectral broadening of the 24 fs pulses in a microstructured fiber yields an octave-spanning spectrum and permits self-referencing and active stabilization of the emitted femtosecond laser frequency comb (FLFC). The individual modes of the 5GHz FLFC are resolved with a high-resolution spectrometer based on a virtually imaged phased array (VIPA) spectral disperser. Isolation of single comb elements at a microwatt average power level is demonstrated. The combination of the high-power, frequency-stabilized 5GHz laser…
Amplified spontaneous emission (ASE) causes fluctuations of pulse energy, of the optical phase and of the timing of the pulse intensity envelope in a mode-locked laser or frequency comb. Starting from the assumption of one ASE photon per longitudinal laser mode and roundtrip, we rederive analytic equations for the three fundamental types of quantum noise in a laser. To this end, we analyze the interference of the coherent intracavity field and a spectrally localized ASE photon as a function of wavelength and phase of the latter. Performing an integration over all wavelengths and phases and tak…
A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric pressure and the simultaneous sensitive detection of multiple atoms or molecules are the key challenges. Here, an electro-optic microring-based dual-comb interferometer, fabricated on a low-loss lithium-niobate-on-insulator nanophotonic platform, demonstrates significant progress towards such an achievement. Spectra spanning 1.6 THz (53 cm-1) at a resolution of…
We report on the observation of a novel mode locked optical comb generated at the Raman offset (Raman comb) in an optically pumped crystalline whispering gallery mode resonator. Mode locking is confirmed via measurement of the radio-frequency beat note produced by the optical comb on a fast photodiode. Neither the conventional Kerr comb nor hyper-parametric oscillation is observed when the Raman comb is present.
Microresonator-based optical frequency combs have been a topic of extensive research during the last few years. Several theoretical models for the comb generation have been proposed; however, they do not comprehensively address experimental results that show a variety of independent comb generation mechanisms. Here, we present frequency-domain experiments that illuminate the transition of microcombs into phase-locked states, which show characteristics of injection locking between ensembles of comb modes. In addition, we demonstrate the existence of equidistant optical frequency combs that are …
We report on an optical frequency comb with 14nm (~1.8 THz) spectral bandwidth at -3 dB level that is generated using a passively mode-locked quantum-well (QW) laser in photonic integrated circuits (PICs) fabricated through an InP generic photonic integration technology platform. This 21.5-GHz colliding-pulse mode-locked laser cavity is defined by on-chip reflectors incorporating intracavity phase modulators followed by an extra-cavity SOA as booster amplifier. A 1.8-THz-wide optical comb spectrum is presented with ultrafast pulse that is 0.35-ps-wide. The radio frequency beat note has a 3-dB …
We generate multiple optical carriers with ultra-low phase noise, over a useable bandwidth of 160 GHz, from an externally injected gain-switched comb source with exceptional low linewidth below 10 Hz. We show successful transmission of 17 demultiplexed channels using 64-quadrature amplitude modulation signals at 5 GBaud.
We calculate the quantum-limited shape of the comb lines from a mode-locked Ti:sapphire laser using experimentally-derived parameters for the linear response of the laser to perturbations. The free-running width of the comb lines is found across the laser spectrum. By modeling the effect of a simple feedback loop, we calculate the spectrum of the residual phase noise in terms of the quantum noise and the feedback parameters. Finally, we calculate the frequency uncertainty in an optical frequency measurement if the limiting factor is quantum noise in the detection of the optical heterodyne beat…
Microresonator frequency combs harness the nonlinear Kerr effect in an integrated optical cavity to generate a multitude of phase-locked frequency lines. The line spacing can reach values in the order of 100 GHz, making it an attractive multi-wavelength light source for applications in fiber-optic communications. Depending on the dispersion of the microresonator, different physical dynamics have been observed. A recently discovered comb state corresponds to the formation of mode-locked dark pulses in a normal-dispersion microcavity. Such dark-pulse combs are particularly compelling for advance…
Quantum cascade lasers (QCL) have revolutionized the generation of mid-infrared light. Yet, the ultrafast carrier transport in mid-infrared QCLs has so far constituted a seemingly insurmountable obstacle for the formation of ultrashort light pulses. Here, we demonstrate that careful quantum design of the gain medium and control over the intermode beat synchronization enable transform-limited picosecond pulses from QCL frequency combs. Both an interferometric radio-frequency technique and second-order autocorrelation shed light on the pulse dynamics and confirm that mode-locked operation is ach…
The two-frequency problem of synchronization of the pulse train of a passively mode locked soliton laser to an externally injected pulse train is solved in the weak injection regime. The source and target frequency combs are distinguished by the spacing and offset frequency mismatches. Locking diagrams map the domain in the mismatch parameter space where stable locking of the combs is possible. We analyze the dependence of the locking behavior on the relative frequency and chirp of the source and target pulses, and the conditions where the relative offset frequency has to be actively stabilize…
The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter enables using interferogram self-correction to fully retrieve the coherence of a dual-comb beat note between two independent fiber lasers. This approach allows to forego the $f - 2f$ self-referencing of both combs, which is a significant simplification. Broadband near-infrared methane spectroscopy has been conducted as a demonstration of the simplified system'…
Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers (QCLs) are suitable candidates for frequency comb and dual-comb operation. For a single laser frequency comb, the repetition rate can be locked using a microwave injection locking and the carrier frequency can be locked to a highly stable source. However, for the locking of two laser combs, four frequencies (two repetition rates and two carrier offset frequenci…
We propose a simple approach to implement a tunable, high power and narrow linewidth laser source based on a series of highly coherent tones from an electro-optic frequency comb and a set of 3 DFB slave lasers. We experimentally demonstrate approximately 1.25 THz (10 nm) of tuning within the C-Band centered at 192.9 THz (1555 nm). The output power is approximately 100 mW (20 dBm), with a side band suppression ratio greater than 55 dB, and a linewidth below 400 Hz across the full range of tunability. This approach is scalable and may be extended to cover a significantly broader optical spectral…
We have specifically investigated the free-space mode locking dynamics of erbium-doped fiber (EDF) mode-locked ultrafast lasers via nonlinear polarization rotation (NPR) in the normal dispersion regime. To do so, we built a passively mode-locked fiber laser based on NPR with a repetition rate of 89 MHz producing an octave-spanning spectrum due to supercontinuum (SC) generation in highly nonlinear fiber (HNLF). Most significantly, we have achieved highly stable self-starting NPR mode-locked femtosecond fiber laser based frequency comb which has been running mode locked for the past one year wit…
We report the first experimental demonstration of frequency-locking of an extended-cavity quantum-cascade-laser (EC-QCL) to a near-infrared frequency comb. The locking scheme is applied to carry out absolute spectroscopy of N2O lines near 7.87 μm with an accuracy of ~60 kHz. Thanks to a single mode operation over more than 100 cm^{-1}, the comb-locked EC-QCL shows great potential for the accurate retrieval of line center frequencies in a spectral region that is currently outside the reach of broadly tunable cw sources, either based on difference frequency generation or optical parametric oscil…
To date, MXene has been discovered for its viability as alternatives to conventional saturable absorber such as carbon nanotube and graphene. The characteristics of high nonlinear saturable absorption, astounding modulation depth, flexible bandgap tunability, and high electron density near Fermi level are the fundamentals of the MXene as an excellent saturable absorber candidate. In particular, the research effort contributed to MXene in nonlinear ul-trafast optics are extensively growing because MXene comprises one of the largest families in 2D nanomaterials that provides huge combination pos…
A bidirectional mode-locked fiber laser producing two correlated frequency combs of the same repetition rate is demonstrated. The intensity dependence of pulse and phase velocities are measured simultaneously. As expected, the phase delay is determined by the linear and nonlinear indices of refraction. The nonlinear Kerr effect contribution to the pulse velocity is dwarfed by a contribution from saturable gain dynamics.
A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum system's dipole response. We develop an analytic description of the comb spectral structure, depending on both the atomic and the phase-control properties. We further suggest an experimental implementation of our scheme: Generating a frequency comb in the soft-x-ray spectral region, which can be realized with currently available techniques and radiation sources. The universality of this mechanism allows the generalization of…
Laser frequency combs are coherent light sources that simultaneously provide pristine frequency spacings for precision metrology and the fundamental basis for ultrafast and attosecond sciences. Recently, nonlinear parametric conversion in high-Q microresonators has been suggested as an alternative platform for optical frequency combs, though almost all in 100 GHz frequencies or more. Here we report a low-phase-noise on-chip Kerr frequency comb with mode spacing compatible with high-speed silicon optoelectronics. The waveguide cross-section of the silicon nitride spiral resonator is designed to…
Femtosecond frequency combs have boosted progress in various fields of precision metrology. Nevertheless, demanding applications such as front-end frequency and time standards, ultrastable microwave generation or high-resolution spectroscopy still necessitate improved stability. The spectral bandwidth and absolute position of individual comb lines are crucial in this context. Typically, both parameters are controlled on short and long time scales by tight locking to external optical and microwave references which represent costly and cumbersome additions to the entire setup. Here, we demonstra…
In this paper, we present an experimental study of the metrological stabilization of a solid-state frequency comb for embedded metrology applications. The comb is a passively mode-locked laser diode based on InGaAs/InP Quantum-dash structure emitting optical lines into a 9 nm bandwidth centered at 1.55 $μ$m with a repetition rate of 10.09 GHz. The frequency stabilization is achieved by optical injection locking of the comb with an external cavity laser diode referenced onto a metrological frequency standard. One observes the transfer of the spectral purity from the injection laser to the neigh…
We propose and theoretically investigate a dispersion-engineered Si3N4 microring resonator, based on a cross-section containing a partially-etched trench, that supports phase-locked, two-color soliton microcomb states. These soliton states consist of a single circulating intracavity pulse with a modulated envelope that sits on a continuous wave background. Such temporal waveforms produce a frequency comb whose spectrum is spread over two widely-spaced spectral windows, each exhibiting a squared hyperbolic secant envelope, with the two windows phase-locked to each other via Cherenkov radiation.…
Dual-comb lasers from which asynchronous ultrashort pulses can be simultaneously generated have recently become an interesting research subject. They could be an intriguing alternative to the current dual-laser optical-frequency-comb source with highly sophisticated electronic control systems. If generated through a common light path traveled by all pulses, the common-mode noises between the spectral lines of different pulse trains could be significantly reduced. Therefore, coherent dual-comb generation from a completely common-path, unidirectional lasing cavity would be an interesting territo…
Quantum-dash (QD) mode-locked laser diodes (MLLD) lend themselves as chip-scale frequency comb generators for highly scalable wavelength-division multiplexing (WDM) links in future data-center, campus-area, or metropolitan networks. Driven by a simple DC current, the devices generate flat broadband frequency combs, containing tens of equidistant optical tones with line spacings of tens of GHz. Here we show that QD-MLLDs can not only be used as multi-wavelength light sources at a WDM transmitter, but also as multi-wavelength local oscillators (LO) for parallel coherent reception. In our experim…
Chip-scale frequency comb generators have the potential to become key building blocks of compact wavelength-division multiplexing (WDM) transceivers in future metropolitan or campus-area networks. Among the various comb generator concepts, quantum-dash (QD) mode-locked laser diodes (MLLD) stand out as a particularly promising option, combining small footprint with simple operation by a DC current and offering flat broadband comb spectra. However, the data transmission performance achieved with QD-MLLD was so far limited by strong phase noise of the individual comb tones, restricting experiment…
Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad suspended-silicon waveguides for infrared frequency comb generation with optical bandwidth limited only by the silicon transparency. The achieved spectra are lithographically tailored to span 2.1 octaves in the mid-infrared (2.0-8.5 um or 1170--5000 cm-1) when pumped at 3.10 um with 100 pJ pulses. Novel fork-shaped couplers provide efficient input coupling with onl…
We combine a graphene mode-locked oscillator with an external compressor and achieve~29fs pulses with~52mW average power. This is a simple, low-cost, and robust setup, entirely fiber based, with no free-space optics, for applications requiring high temporal resolution.
We study the effect of noise on the dynamics of passively mode-locked semiconductor lasers both experimentally and theoretically. A method combining analytical and numerical approaches for estimation of pulse timing jitter is proposed. We investigate how the presence of dynamical features such as wavelength bistability affects timing jitter.
We introduce and experimentally demonstrate a new class of electrically driven thermal emitter based on globally aligned carbon nanotube metamaterials patterned as nanoscale ribbons. The metamaterial ribbons exhibit electronic and photonic properties with extreme anisotropy, which enable low loss, wavelength-compressed hyperbolic photonic modes along one axis and high electrical resistivity and efficient Joule heating along the other axis. Devices batch-fabricated on a single chip emit linearly polarized thermal radiation with peak wavelengths dictated by their hyperbolic resonances, and their…
We present a method of phase-locking any number of continuous-wave lasers to an optical frequency comb (OFC) that enables independent frequency positioning and control of each laser while still maintaining lock to the OFC. The scheme employs an acousto-optic modulator (AOM) in a double pass configuration added to each laser before its light is compared by optical heterodyne with the comb. The only requirement is that the tuning bandwidth of the double pass AOM setup be larger than half the OFC repetition rate. We demonstrate this scheme and achieve an arbitrary frequency tuning precision, a tu…
Microresonator-based Kerr frequency comb (microcomb) generation can potentially revolutionize a variety of applications ranging from telecommunications to optical frequency synthesis. However, phase-locked microcombs have generally had low conversion efficiency limited to a few percent. Here we report experimental results that achieve ~30% conversion efficiency (~200 mW on-chip comb power excluding the pump) in the fiber telecommunication band with broadband mode-locked dark-pulse combs. We present a general analysis on the efficiency which is applicable to any phase-locked microcomb state. Th…
We report on a new design for a femtosecond Ti:sapphire oscillator in which dispersion compensation is realized exclusively using mirrors, including special mirrors with third order dispersion. This makes the oscillator dynamically tunable over a spectral range of 45 nm using an intracavity wedge-pair; and it delivers 40 fs pulses at 80 MHz repetition rate. Due to the all-mirror design, the oscillator represents an attractive base for a tunable frequency comb for high precision spectroscopy applications.
We demonstrate a convenient and fast method to measure the spectrally resolved far-fields of multimode terahertz quantum cascade lasers by combining a microbolometer focal plane array with an FTIR spectrometer. Far-fields of fundamental TM0 and higher lateral order TM1 modes of multimode Fabry-Pérot type lasers have been distinguished, which very well fit to the results obtained by a 3D finite-element simulation. Furthermore, multimode random laser cavities have been investigated, analyzing the contribution of each single laser mode to the total far-field. The presented method is thus an impor…
We demonstrate two fully and tightly phase locked 750 MHz ytterbium (Yb) fiber frequency combs that are independently stabilized to a continuous wave (CW) laser with <1 rad RMS phase error. A bulk EOM and a single stack PZT are separately utilized as the fast actuators for cavity length stabilization. The carrier envelop frequencies are phase locked by single loop feedback to laser diode current, showing 1.6 MHz servo bumps. The in-loop fractional frequency instabilities are ~1.5e-18 at 1s for both combs. To the best of our knowledge, this is the highest repetition rate in fiber based low phas…
By identifying the similarities between the coupled-wave equations and the parametrically driven nonlinear Schrödinger equation, we unveil the existence condition of the quadratic soliton mode-locked degenerate optical parametric oscillator in the previously unexplored parameter space of near-zero group velocity mismatch. We study the nature of the quadratic solitons and divide their dynamics into two distinctive branches depending on the system parameters. We find the nonlinear interaction between the resonant pump and signal results in phenomena that resemble the dispersive two-photon absorp…
Dual comb spectroscopy (DCS) is a broadband technique offering high resolution and fast data acquisition. We describe a hybrid dual comb spectrometer comprising a broadband commercial fiber laser system offering a wide range of sample interrogation, and an actively mode locked semiconductor laser (MLL) having a widely tunable, relatively narrow spectrum. The mutual coherence over 100 seconds has been realized between the two combs. We employed the DCS system to characterize the absorption spectrum of rubidium atoms at 313 K with a high signal to noise ratio. The broadband laser is directly loc…
Quantum cascade laser (QCL) frequency combs are a promising candidate for chemical sensing and biomedical diagnostics, requiring only milliseconds of acquisition time to record absorption spectra without any moving parts. They are electrically pumped and have a small footprint, making them an ideal platform for on-chip integration. Until now, optical feedback is fatal for frequency comb generation in QCLs and destroys intermodal coherence. This property imposes strict limits on the possible degree of integration. Here, we demonstrate coherent injection locking of the repetition frequency to a …
Recent progress in the application of color centers to nanoscale spin sensing makes the combined use of noise spectroscopy and scanning probe imaging an attractive route for the characterization of arbitrary material systems. Unfortunately, the traditional approach to characterizing the environmental magnetic field fluctuations from the measured probe signal typically requires the experimenter's input, thus complicating the implementation of automated imaging protocols based on spectrally resolved noise. Here, we probe the response of color centers in diamond in the presence of externally engi…
