arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2204.04593cond-mat.str-elcond-mat.supr-con
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Na3Co2SbO6中的巨磁面内各向异性和竞争不稳定性

Giant magnetic in-plane anisotropy and competing instabilities in Na3Co2SbO6

Xintong Li, Yuchen Gu, Yue Chen, V. Ovidiu Garlea, Kazuki Iida, Kazuya Kamazawa, Yangmu Li, Guochu Deng, Qian Xiao, Xiquan Zheng, Zirong Ye, Yingying Peng, I. A… 展开作者

Xintong Li, Yuchen Gu, Yue Chen, V. Ovidiu Garlea, Kazuki Iida, Kazuya Kamazawa, Yangmu Li, Guochu Deng, Qian Xiao, Xiquan Zheng, Zirong Ye, Yingying Peng, I. A. Zaliznyak, J. M. Tranquada, Yuan Li

摘要:

我们报告获得的无孪晶单晶Na3Co2SbO6,这被认为是一种候选材料,用于实现量子自旋液体的Kitaev蜂窝模型的磁学数据。与人们普遍认为这种材料可以用理想蜂窝晶格的对称性来建模相反,我们的数据显示出明显的双重对称性和超过200%的面内各向异性,尽管蜂窝层的微小正交畸变小于0.2%。我们进一步使用磁中子衍射来阐明丰富多样的磁场中观察到的磁场诱导相。这些阶段表现在顺磁状态的扩散散射信号与竞争的铁和反铁磁不稳定性,符合理论,也预测附近的量子自旋液体相。我们的研究结果要求所观察到的面内各向异性的理论理解,并呈现Na3Co2SbO6一个有希望的理由,通过有针对性的外部调谐找到异国情调的量子相。

英文摘要:

We report magnetometry data obtained on twin-free single crystals of Na3Co2SbO6, which is considered a candidate material for realizing the Kitaev honeycomb model for quantum spin liquids. Contrary to a common belief that such materials can be modeled with the symmetries of an ideal honeycomb lattice, our data reveal a pronounced two-fold symmetry and in-plane anisotropy of over 200%, despite the honeycomb layer's tiny orthorhombic distortion of less than 0.2%. We further use magnetic neutron diffraction to elucidate a rich variety of field-induced phases observed in the magnetometry. These phases manifest themselves in the paramagnetic state as diffuse scattering signals associated with competing ferro- and antiferromagnetic instabilities, consistent with a theory that also predicts a quantum spin liquid phase nearby. Our results call for theoretical understanding of the observed in-plane anisotropy, and render Na3Co2SbO6 a promising ground for finding exotic quantum phases by targeted external tuning.

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