arXivDaily arXiv每日学术速递 周一至周五更新
arXiv周末暂无论文更新,休息一下吧,周末愉快~~
arXiv 2603.25317cond-mat.str-elcond-mat.mtrl-sci
收藏

平带驱动的交替磁体CrSb中的竞争电荷和自旋不稳定性

Flat band driven competing charge and spin instabilities in the altermagnet CrSb

Donostia International Physics Center (DIPC)(多诺斯蒂亚国际物理中心);Centro de Física de Materiales (CFM-MPC), CSIC-UPV/EHU(材料物理中心,西班牙国家研究委员会/巴斯克国立大学);Fisika Aplikatua Saila, Gipuzkoako Ingeniaritza Eskola, University of the Basque Country (UPV/EHU)(应用物理系,吉普斯夸工程学院,巴斯克国立大学);Department of Applied Physics, KTH Royal Institute of Technology(皇家理工学院应用物理系);Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(凝聚态物理北京实验室,中国科学院物理研究所);Swiss-Norwegian BeamLines at European Synchrotron Radiation Facility(欧洲同步辐射装置瑞士-挪威光束线);European Synchrotron Radiation Facility (ESRF)(欧洲同步辐射装置);Département de Physique et Institut Quantique, Université de Sherbrooke(物理系与量子研究所,舍布鲁克大学)

A. Korshunov, M. Alkorta, C. -Y. Lim, F. Ballester, Cong Li, Zhilin Li, D. Chernyshov, A. Bosak, M. G. Vergniory, Ion Errea, S. Blanco-Canosa

AI总结:

研究揭示CrSb中在布里渊区M点的短程电荷有序波动在Neel温度以上存在,但进入磁序相后消失,表明电荷与自旋有序之间的竞争,通过平带物理驱动声子异常及重构。

摘要:

电子波函数在动量空间中的限制可以产生平带,其中动能的淬灭增强态密度并放大相互作用效应。此类条件是新兴量子相的肥沃土壤,因为自旋、电荷和晶格自由度变得高度纠缠。在这些状态下,细微的交织序参量竞争往往决定宏观基态,产生复杂且有时出人意料的集体行为。本文展示交替磁体CrSb实现了这一场景,并揭示了在布里渊区M点的短程电荷有序波动,其在Neel温度(TN)以上持续存在。值得注意的是,这些波动在进入磁序相时消失,揭示了电荷和自旋有序之间的直接且稳健的竞争。在TN时,q*点的声子色散发展出显著的Kohn类异常,表明磁相变附近存在强电子-声子耦合。在TN以下,交换斯特里克松显著地将相关软声子模式重正化约6 meV,这是迄今为止报告的最大自旋-声子耦合。第一性原理计算将这种行为归因于近无色散电子态与一个在谐波水平上仅当不考虑磁序时才显得不稳定的声子分支之间的强耦合,揭示了晶格对磁对称破缺的高敏感性。电荷和自旋序参量之间的竞争,通过平带物理放大,驱动了观察到的声子异常及其在TN时的突然重构。凭借其化学简单结构和受对称性保护的交替磁性态,CrSb成为研究平带电子态如何介导巨量自旋-声子耦合和竞争破缺对称性的模型平台。

英文摘要:

The confinement of electronic wavefunctions in momentum space can give rise to flat electronic bands, where the quenching of kinetic energy enhances the density of states and amplifies interaction effects. Such conditions are fertile ground for emergent quantum phases, as spin, charge and lattice degrees of freedom become strongly entangled. In these regimes, subtle competitions between intertwined order parameters often dictate the macroscopic ground state, producing complex and sometimes unexpected collective behavior. Here we show that the altermagnet CrSb provides a realization of this scenario, and uncover short-range charge-order fluctuations at the M point of the Brillouin zone, q*=(1/2 0), persisting above the Neel temperature (TN). Remarkably, these fluctuations collapse upon entering the magnetically ordered phase, revealing a direct and robust competition between charge and spin order. At TN, the phonon dispersion at q* develops a pronounced Kohn-like anomaly, signaling strong electron-phonon coupling in the vicinity of the magnetic transition. Below TN, exchange striction dramatically renormalizes the associated soft phonon mode by approximately ~6 meV, the largest spin-phonon coupling ever reported. First-principles calculations attribute this behavior to a strong coupling between nearly dispersionless electronic states and a phonon branch that appears unstable at the harmonic level only when no magnetic order is considered, revealing the large sensitivity of the lattice to magnetic symmetry breaking. The competition between charge and spin order parameters, amplified by flat-band physics, drives the observed phonon anomaly and its abrupt reconstruction at TN. With its chemically simple structure and symmetry-protected altermagnetic state, CrSb emerges as a model platform to explore how flat electronic bands mediate giant spin-phonon coupling and competing broken symmetries.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑