Highly Tunable Magnetic and Magnetotransport Properties of Exchange Coupled Ferromagnet/Antiferromagnet-based Heterostructures
Sri Sai Phani Kanth Arekapudi, Daniel Bülz, Fabian Ganss, Fabian Samad, Chen Luo, Dietrich R. T. Zahn, Kilian Lenz, Georgeta Salvan, Manfred Albrecht, Olav Hellwig
备注：
27 pages and 9 figures; 19 supplementary figures and 1 table
Antiferromagnets (AFMs) with zero net magnetization are proposed as active elements in future spintronic devices. Depending on the critical thickness of the AFM thin films and the measurement temperature, bimetallic Mn-based alloys and transition metal oxide-based AFMs can host various coexisting ordered, disordered, and frustrated AFM phases. Such coexisting phases in the exchange coupled ferromagnetic (FM)/AFM-based heterostructures can result in unusual magnetic and magnetotransport phenomena. Here, we integrate chemically disordered AFM IrMn3 thin films with coexisting AFM phases into complex exchange coupled MgO(001)/Ni3Fe/IrMn3/Ni3Fe/CoO heterostructures and study the structural, magnetic, and magnetotransport properties in various magnetic field cooling states. In particular, we unveil the impact of rotating the relative orientation of the disordered and reversible AFM moments with respect to the irreversible AFM moments on the magnetic and magnetoresistance properties of the exchange coupled heterostructures. We further found that the persistence of AFM grains with thermally disordered and reversible AFM order is crucial for achieving highly tunable magnetic properties and multi-level magnetoresistance states. We anticipate that the introduced approach and the heterostructure architecture can be utilized in future spintronic devices to manipulate the thermally disordered and reversible AFM order at the nanoscale.
We show that applying strain on half-doped manganites makes it possible to tune the system to the proximity of a metal-insulator transition and thereby generate a colossal magnetoresistance (CMR) response. This phase competition not only allows control of CMR in ferromagnetic metallic manganites but can be used to generate CMR response in otherwise robust insulators at half-doping. Further, from our realistic microscopic model of strain and magnetotransport calculations within the Kubo formalism, we demonstrate a striking result of strain engineering that, under tensile strain, a ferromagnetic…
Magnetoelastic Transport-Path Reconstruction and Giant Magnetotransport Responses in a Two-Dimensional Antiferromagnet
Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院固体物理研究所材料物理重点实验室）；University of Science and Technology of China（中国科学技术大学）；School of Physics, University of Electronic Science and Technology of China（电子科技大学物理学院）；Anhui Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院高磁场科学中心安徽省低能量子材料与器件重点实验室）；Collaborative Innovation Center of Microstructures, Nanjing University（南京大学微观结构协同创新中心）；Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska（内布拉斯加大学物理与天文学系及内布拉斯加材料与纳米科学中心）；State Key Laboratory of Semiconductor Physics and Chip Technologies, Institute of Semiconductors, Chinese Academy of Sciences（中国科学院半导体研究所半导体物理与芯片技术国家重点实验室）；Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences（中国科学院大学材料科学与光电工程学院）
We study the anomalous Hall-like effect (AHLE) and the effective anisotropic magnetoresistance (EAMR) in antiferromagnetic γ -IrMn3/Y3Fe5O12(YIG) and Pt/YIG heterostructures. For γ -IrMn3/YIG, the EAMR and the AHLE resistivity change sign with temperature due to the competition between the spin Hall magnetoresistance (SMR) and the magnetic proximity effect (MPE) induced by the interfacial antiferromagnetic uncompensated magnetic moment. In contrast, for Pt/YIG the AHLE resistivity changes sign with temperature whereas no sign change is observed in the EAMR. This is because the MPE and the SMR …
We probe the current-induced magnetic switching of insulating antiferromagnet/heavy metals systems, by electrical spin Hall magnetoresistance measurements and direct imaging, identifying a reversal occurring by domain wall (DW) motion. We observe switching of more than one third of the antiferromagnetic domains by the application of current pulses. Our data reveal two different magnetic switching mechanisms leading together to an efficient switching, namely the spin-current induced effective magnetic anisotropy variation and the action of the spin torque on the DWs.
General expressions for the longitudinal and transverse resistivities of single-crystalline cubic and tetragonal ferromagnets are derived from a series expansion of the resistivity tensor with respect to the magnetization orientation. They are applied to strained (Ga,Mn)As films, grown on (001)- and (113)A-oriented GaAs substrates, where the resistivities are theoretically and experimentally studied for magnetic fields rotated within various planes parallel and perpendicular to the sample surface. We are able to model the measured angular dependences of the resistivities within the framework o…
Anomalous magnetotransport in a non-collinear correlated kagome ferromagnet MgMn6Sn6
S. N. Bose National Centre for Basic Sciences（S.N. 玻色基础科学国家中心）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；ISIS Neutron and Muon Source, Science and Technology Facilities Council, Rutherford Appleton Laboratory（ISIS中子与μ子源，科学与技术设施委员会，拉瑟福德阿普尔顿实验室）；School of Physical Sciences, Indian Institute of Technology Goa（印度果阿理工学院物理科学学院）
The antiferromagnet Mn$_5$Si$_3$ has recently attracted attention because a noncollinear spin arrangement has been shown to produce a topological anomalous Hall effect and an inverse magnetocaloric effect. Here we synthesize single crystals of Mn$_5$Si$_3$ using flux growth. We determine the phase diagram through magnetization and measure the magnetoresistance and the Hall effect. We find the collinear and noncollinear antiferromagnetic phases at low temperatures and, in addition, a third magnetic phase, in between the two antiferromagnetic phases which has ferromagnetic character. The latter …
Topological insulators have emerged as an important material class for efficient spin-charge interconversion. Most topological insulators considered to date are binary or ternary compounds, with the exception of $α$-Sn. Here we report a comprehensive characterization of the growth, magnetotransport properties, and current-induced spin-orbit torques of $α$-Sn and $β$-Sn-based ferromagnetic heterostructures. We show that $α$-Sn grown with a Bi surfactant on CdTe(001) promotes large spin-orbit torques in a ferromagnetic FeCo layer at room temperature, comparable to Pt, whereas $α$-Sn grown withou…
Artificial superlattices designed with ferromagnetic Pr0.85Ca0.15MnO3 insulating layer and ferroelectric Ba0.6Sr0.4TiO3 layer were grown on (100) SrTiO3 substrates. The magnetotransport properties were measured with the current perpendicular to the plane geometry. An increase in magnetoresistance (MR), with no significant low field effect, was observed as the number of ferroelectric Ba0.6Sr0.4TiO3 layer thickness increases even up to 9 unit cells. For example, the superlattice [(Pr0.85Ca0.15MnO3)10(Ba0.6Sr0.4TiO3)9]25 shows 35 % MR at 100 K, though the Pr0.85Ca0.15MnO3 film was a robust insula…
The magnetotransport behaviour is investigated in detail across the first order magnetic phase transition from ferromagnetic to antiferromagnetic state in polycrystalline Ce(Fe$_{0.96}$Al$_{0.04}$)$_2$ sample. The study clearly brings out various generic features associated with a first order transition, viz., hysteresis, phase coexistence, supercooling and superheating, presence and limits of the metastable regimes. These results of magnetotransport study exhibit and support all the interesting thermomagnetic history effects that were observed in our earlier dc-magnetisation study on the same…
The discovery of fascinating ways to control and manipulate antiferromagnetic materials have garnered considerable attention as an attractive platform to explore novel spintronic phenomena and functionalities. Layered antiferromagnets (AFMs) exhibiting interesting magnetic structures, can serve as an attractive starting point to establish novel functionalities down to the two-dimensional limit. In this work, we explore the magnetoresistive properties of the spin-ladder AFM TaFe$_{1.25}$Te$_3$. Magnetization studies reveal an anisotropic magnetic behavior resulting in the stabilization of a spi…
Antiferromagnetic spintronics allows us to explore storing and processing information in magnetic crystals with vanishing magnetization. In this manuscript, we investigate magnetoresistance effects in antiferromagnetic CuMnAs upon switching into high-resistive states using electrical pulses. By employing magnetic field sweeps up to 14 T and magnetic field pulses up to $\sim$ 60 T, we reveal hysteretic phenomena and changes in the magnetoresistance, as well as the resilience of the switching signal in CuMnAs to the high magnetic field. These properties of the switched state are discussed in the…
The synthesis and structural study of the stoichiometric perovskite La0.5Ba0.5CoO3 have allowed three forms to be isolated. Besides the disordered La0.5Ba0.5CoO3 and the perfectly ordered layered LaBaCo2O6, a third form called nanoscale-ordered LaBaCo2O6, is obtained. As evidenced by transmission electron microscopy investigations, the latter consists of 112-type 90 degree oriented domains fitted into each other at a nanometer scale which induce large strains and consequently local atomic scale lattice distortions. These three ferromagnetic perovskites exhibit practically the same Tc (174-179 …
We perform classical Monte Carlo and stochastic Landau-Lifshitz-Gilbert simulations to study temperature dependent magnetism of Kagome antiferromagnet (AFM) Weyl metal $\text{Mn}_3\text{Ge}$ and find that a long range chiral order sets in at a transition temperature well below the N{é}el temperature ($T_N$). Based on the crystalline symmetries, imposed by the chiral magnetic order, we argue for the presence of multiple iso-energetic Weyl nodes (nodes that are at same energy and with congruent Fermi surface around them) near chemical potential. Using the semi-classical Boltzmann equations, we s…
We report on the evolution of the average and depth-dependent magnetic order in thin film samples of biaxially stressed and electron-doped EuTiO$_3$ for samples across a doping range $<$0.1 to 7.8 $\times 10^{20}$ cm$^{-3}$. Under an applied in-plane magnetic field, the G-type antiferromagnetic ground state undergoes a continuous spin-flop phase transition into in-plane, field-polarized ferromagnetism. The critical field for ferromagnetism slightly decreases with an increasing number of free carriers, yet the field evolution of the spin-flop transition is qualitatively similar across the dopin…
We have studied the magneto-optical and magnetotrasnport properties of GaMnAs thin films with high Mn concentrations (x= 12.2 - 21.3%) grown by molecular-beam epitaxy. These heavily Mn-doped GaMnAs films were formed by decreasing the growth temperature to as low as 150-190 degree C and by reducing the film thickness to 10 nm in order to prevent precipitation of hexagonal MnAs clusters. Magnetic circular dichroism (MCD) and anomalous Hall effect measurements indicate that these GaMnAs films have the nature of intrinsic ferromagnetic semiconductors with high ferromagnetic transition temperature …
Complex electronic topography and magnetotransport in an in-plane ferromagnetic kagome metal
University of Central Florida（中佛罗里达大学）；Hiroshima University（广岛大学）；The University of Tennessee（田纳西大学）；Northeastern University（东北大学）；S. N. Bose National Centre for Basic Sciences（S.N.玻色基础科学国家中心）
We report the magnetotransport properties of HoSb, a semimetal with antiferromagnetic ground state. HoSb shows extremely large magnetoresistance (XMR) and Shubnikov-de Haas (SdH) oscillation at low temperature and high magnetic field. Different from previous reports in other rare earth monopnictides, kinks in $ρ(B)$ and $ρ_{xy}(B)$ curves and the field dependent resistivity plateau are observed in HoSb, which result from the magnetic phase transitions. The fast Fourier transform analysis of the SdH oscillation reveals the split of Fermi surfaces induced by the nonsymmetric spin-orbit interacti…
We have studied the magnetic, magnetocaloric and magnetotransport properties of RSn1+xGe1-x(R=Gd, Tb, Er; x=0.1) series by means of magnetization, heat capacity and resistivity measurements. It has been found that all the compounds crystallize in the orthorhombic crystal structure described by the centrosymmetric space group Cmcm (No. 63). The magnetic susceptibility and heat capacity data suggest that all the compounds are antiferromagnetic. Large negative values of θp in case of GdSn1.1Ge0.9 and TbSn1.1Ge0.9 indicate that strong antiferromagnetic interactions are involved, which is also refl…
We present a theoretical mapping to show that a ferromagnet with gain (loss) is equivalent to an antiferromagnet with an equal amount of loss (gain). Our finding indicates a novel first-order ferromagnet-antiferromagnet phase transition by tuning the gain-loss parameter. As an appealing application, we demonstrate the realization as well as the manipulation of the antiferromagnetic skyrmion, a stable topological quasiparticle not yet observed experimentally, in a chiral ferromagnetic thin film with gain. We also consider ferromagnetic bilayers with balanced gain and loss, and show that the ant…
While in most ferro or antiferromagnetic materials there is a unique crystallographic direction, including crystallographically equivalent directions, in which the moments like to point due to spin-orbit coupling, in some, the direction of the spin reorients as a function of a certain physical parameter such as temperature, pressure etc. Fe3Sn2 is a kagome ferromagnet with an onset of ferromagnetism below 650 K, and undergoes a spin reorientation near 150 K. While it is known that the moments in Fe3Sn2 point perpendicular to the kagome plane at high temperatures and parallel to the kagome plan…
We report on the magnetic and magnetotransport properties of ferromagnetic semiconductor (Ga,Mn)As modified by Ga$^{+}$ ion irradiation using focused ion beam. A marked reduction in the conductivity and the Curie temperature is induced after the irradiation. Furthermore, an enhanced negative magnetoresistance (MR) and a change in the magnetization reversal process are also demonstrated at 4 K. Raman scattering spectra indicate a decrease in the concentration of hole carriers after the irradiation, and a possible origin of the change in the magnetic properties is discussed.
Magnetic and magnetotransport properties of oriented polycrystalline Pr0.58Ca0.42MnO3 thin films prepared in flowing oxygen and air ambient has been investigated. The magnetic ground state of both the films is a frozen cluster glass. In the air annealed film charge order (CO) is quenched and ferromagnetic (FM) transition, which appears at TC=148 K is followed by antiferromagnetic (AFM) transition at TN=104 K. This film shows self-field hysteretic insulator-metal transition (IMT) at TIMC=89 K and TIMW=148 K in the cooling and warming cycle, respectively. Application of magnetic field (H) gradua…
We report the effect of La-substitution on the magnetic and magnetotransport properties of Brownmillerite-like bilayered compounds Ca2.5-xLaxSr0.5GaMn2O8 (x = 0, 0.05, 0.075, and 0.1) by using dc-magnetization, resistivity and magnetoresistance techniques. The Rietveld analysis of the room temperature x-ray diffraction patterns confirms no observable change of average crystal structure with the La-substitution. Both magnetic and magnetotransport properties are found to be very sensitive to the La-substitution. Interestingly, the La-substituted compounds show ferromagnetic-like behavior (due to…
We study the problem of controlling spin waves propagation through an antiferromagnet/ferromagnet interface via tuning material parameters. It is done by introducing the degree of sublattice noncompensation of antiferromagnet (DSNA), which is a physical characteristic of finite-thickness interfaces. The DSNA value can be varied by designing interfaces with a particular disorder or curvilinear geometry. We describe a spin-wave propagation through any designed antiferromagnet/ferromagnet interface considering a variable DSNA and appropriate boundary conditions. As a result, we calculate the phys…
Magnetotransport properties of ferromagnetic semiconductor (Ga,Mn)As have been investigated. Measurements at low temperature (50 mK) and high magnetic field (<= 27 T) have been employed in order to determine the hole concentration p = 3.5x10^20 cm ^-3 of a metallic (Ga0.947Mn0.053)As layer. The analysis of the temperature and magnetic field dependencies of the resistivity in the paramagnetic region was performed with the use of the above value of p, which gave the magnitude of p-d exchange energy |N0beta | ~ 1.5 eV.
We consider electron transport in ferromagnets or antiferromagnets sandwiched between metals. When spins in the magnetic materials precess, they emit currents into the surrounding conductors. Generally, adiabatic pumping in mesoscopic systems also enhances current fluctuations. We generalize the description of current fluctuations driven by spin dynamics in three ways using scattering theory. First, our theory describes a general junction with any given electron scattering properties. Second, we consider antiferromagnets as well as ferromagnets. Third, we treat multiterminal devices. Using sho…
By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much more efficiently manipulated by optical excitation than its ferromagnetic counterpart. We assign the fast and extremely efficient process in the antiferromagnet to an interatomic transfer of angular momentum within the spin system. Our findings do not only reveal this angular momentum transfer channel effective in antiferromagnets and other magnetic structur…
We propose to use ferromagnetic insulator MnBi2Se4/Bi2Se3/antiferromagnetic insulator Mn2Bi2Se5 heterostructures for the realization of the axion insulator state. Importantly, the axion insulator state in such heterostructures only depends on the magnetization of the ferromagnetic insulator and hence can be observed in a wide range of external magnetic field. Using density functional calculations and model Hamiltonian simulations, we find that the top and bottom surfaces have opposite half-quantum Hall conductance, with a sizable global spin gap of 5.1 meV opened for the topological surface st…
The oxygen-deficient perovskite cobaltite SrCo1-xNbxO3-d was synthesized by direct solid-state reaction and its magnetotransport properties were investigated. This cobaltite exhibits an unusual ferromagnetic behavior with a transition temperature Tm = 130-150 K and a spin glass like behavior below Tm. Importantly, this phase reaches a large magnetoresistance (MR) value, MR = -(rH - r0) / r0 = 30% at 5 K in 7 T. The large MR effect is believed to be related to the disordered magnetic state induced by the Nb-for-Co substitution.
We have been able to synthesize Lu+3 substituted La0.67Ca0.33MnO3 (LCMO) by an auto-combustion method. Synthesis of this compound is not successful by conventional ceramic or other chemical methods. Magnetic and electrical transport properties of the Lu substituted LCMO [(La1-xLux)0.67Ca0.33MnO3 (0 < x < 0.12)] system have been investigated and compared with those of the Y+3, Pr+3, Dy+3 and Tb+3 substituted LCMO systems. All the compounds show a ferromagnetic metal to paramagnetic insulator transition at TC. The tolerance factor reduces from 0.917 for x = 0 to 0.909 for x = 0.12 and for this r…
Magnetic lanthanide half-Heuslers ($R$PtBi; $R$ being the lanthanide) represent an attractive subgroup of the Heusler family and have been identified as ideal candidates for time reversal symmetry breaking topological Weyl semimetals. In this paper, we present the detailed analysis of the magnetotransport properties of frustrated antiferromagnet TbPtBi. This material shows large, non-saturating magnetoresistance (MR) with unusual magnetic field dependence. The MR of TbPtBi is significantly anisotropic with respect to the magnetic field, applied along different crystallographic directions and i…
Recent works aiming at understanding magnetotransport phenomena in ferromagnetic III-V and II-VI semiconductors are described. Theory of the anomalous Hall effect in p-type magnetic semiconductors is discussed, and the relative role of side-jump and skew-scattering mechanisms assessed for (Ga,Mn)As and (Zn,Mn)Te. It is emphasized that magnetotransport studies of ferromagnetic semiconductors in high magnetic fields make it possible to separate the contributions of the ordinary and anomalous Hall effects, to evaluate the role of the spins in carrier scattering and localization as well as to dete…
We have compared and contrasted magnetic, magnetocaloric and magnetoresistive properties of Gd and Dy members of the rare-earth (R) series RFe5Al7, crystallizing in ThMn12 structure, known to order antiferromagnetically. Among other observations, we would like to emphasize on the following novel findings: (i) There are multiple sign-crossovers in the temperature (T) dependence of isothermal entropy change (DeltaS) in the case of Dy compound; in addition to nil DeltaS at the magnetic compensation point known for two-magnetic-sublattice systems, there is an additional sign-crossover at low tempe…
Spin-polarized current effect is studied on the static and dynamic magnetization of the antiferromagnet in a ferromagnet - antiferromagnet junction. The macrospin approximation is generalized to antiferromagnets. Canted antiferromagnetic configuration and resulting magnetic moment are induced by an external magnetic field. The resonance frequency and damping are calculated, as well as the threshold current density corresponding to instability appearance. A possibility is shown of generating low-damping magnetization oscillations in terahertz range. The fluctuation effect is discussed on the ca…
We report two-dimensional quantum transport and Dirac fermions in YbMnBi2 single crystals. YbMnBi2 is a layered material with anisotropic conductivity and magnetic order below 290 K. Magnetotransport properties, nonzero Berry phase and small cyclotron mass indicate the presence of quasi two dimensional Dirac fermions. Quantum oscillations in Hall resistivity suggest the presence of both electron and hole parts of the Fermi surface whereas the Berry phase suggests spin-orbit coupling.
In an antiferromagnet (AF) with uniaxial anisotropy, spin-up and spin-down magnons coexist and form an intrinsic degree of freedom resembling electrons. When polarized by an adjacent ferromagnet (F), a magnonic pure spin current can be thermally generated in an AF. We explore thermal magnon transport in an insulating F/AF/F trilayer where propagating magnons inside the AF spacer can transfer angular momenta between the two Fs. We find that a sufficiently large temperature gradient can switch the downstream F via magnonic spin-transfer torque if it is initially antiparallel with the upstream F.…
By means of micromagnetic spin dynamics calculations, a quantitative calculation is carried out to explore the mechanism of exchange bias (EB) in ferromagnetic (FM)/compensated antiferromagnetic (AFM) bilayers. The antiferromagnets with low and high Neel temperatures have been both considered, and the crossover from negative to positive EB is found only in the case with low Neel temperature. We propose that the mechanism of EB in FM/compensated AFM bilayers is due to the symmetry broken of AFM that yields some net ferromagnetic components.
ThCr2Si2-type Ce2O2Bi epitaxial thin films were grown by recently developed multilayer solid phase epitaxy. The ionic state of Ce was confirmed to be 3+ by x-ray photoelectron spectroscopy, corresponding to the electronic configuration of [Xe]4f1. Electrical resistivity showed the nonmonotonic temperature dependence with a sharp resistivity maximum, concomitant with a magnetization kink at 10 K, suggesting antiferromagnetic transition. In addition, magnetoresistance showed a large angular-dependent magnetoresistance. These results imply that carrier transport in the Bi2- square net could be in…
We calculate the response of a ferromagnet - antiferromagnet junction to a high-frequency magnetic field as a function of the spin-polarized current through the junction. Conditions are choused under which the response is zero in absence of such a current. It is shown that increasing in the current density leads to proportional increase in the resonance frequency and resonant absorption. A principal possibility is indicated of using ferromagnet - antiferromagnet junction as a terahertz radiation detector.
Fermi level dependence of magnetism and magnetotransport in the magnetic topological insulators Bi$_{2}$Te$_{3}$ and BiSbTe$_{3}$ containing self-organized MnBi$_{2}$Te$_{4}$ septuple layers
The dc magnetization (M) and electrical resistivity (ρ) as functions of magnetic field and temperature are reported for a series of lightly electron dopedCa(1-x)La(x)MnO(3) (0<=x<=0.10) specimens for which magnetization [Phys. Rev. B {\bf 61}, 14319 (2000)] and scattering studies [Phys. Rev. B {\bf 68}, 134440 (2003)] indicate an inhomogeneous magnetic ground state composed of ferromagnetic (FM) droplets embedded in a G-type antiferromagnetic matrix. A change in the magnetic behavior near x=0.02 has been suggested to be the signature of a crossover to a long-ranged spin-canted phase. The data …
We report on the exchange bias between antiferromagnetic and ferroelectric hexagonal YMnO3 epitaxial thin films sandwiched between a metallic electrode (Pt) and a soft ferromagnetic layer (Py). Anisotropic magnetoresistance measurements are performed to monitor the presence of an exchange bias field. When the heteroestructure is biased by an electric field, it turns out that the exchange bias field is suppressed. We discuss the dependence of the observed effect on the amplitude and polarity of the electric field. Particular attention is devoted to the role of current leakage across the ferroel…
Hydrogenation and posthydrogenation annealings have been used as a very efficient tool to tune the hole density over a wide range, at fixed magnetic moment concentration, in thin GaMnAs layers. Reduction of the hole density resulted in strong modifications of their ferromagnetic properties. In particular, we observed in magnetotransport experiments the decrease of the Curie temperature, along with modifications of the magnetic anisotropy, a behavior consistent with the mean-field theory.
We report the anomalous magnetocaloric behavior in the polycrystalline compound Tb2Ni2Sn. The magnetization measurements show that this compound shows multiple magnetic transitions, which are attributed to the coexistence of ferromagnetic and antiferromagnetic phases at low temperatures. With increase in field and temperature, the compound undergoes a metamagnetic transition to a ferromagnetic state. In the temperature range where the antiferromagnetic phase is dominant, it exhibits inverse (negative) magnetocaloric effect. At temperatures close to the Neel temperature, the compound shows posi…
We report on the effects of spin fluctuations, magnetic ordering, and external magnetic field on the dielectric constant of the ferromagnet SeCuO3, and the antiferromagnet TeCuO3. A model based on the coupling between uniform polarization and the q-dependent spin-spin correlation function is presented to explain the different behaviors for these isostructural compounds. The large magnetocapacitance near the transition temperature in the ferromagnet SeCuO3 suggests routes to enhancing the magnetodielectric response for practical applications.
Spin-polarized current effect is studied on the static and dynamic magnetization of the antiferromagnet in a ferromagnet - antiferromagnet nanojunction. The macrospin approximation is generalized to antiferromagnets. Canted antiferromagnetic configuration and resulting magnetic moment are induced by an external magnetic field. The resonance frequency and damping are calculated, as well as the threshold current density corresponding to instability appearance. A possibility is shown of generating low-damping magnetization oscillations in terahertz range. The fluctuation effect is discussed on th…
Magnetic properties of the pyrovanadate CaCoV$_2$O$_7$ have been studied by means of the bulk magnetization and neutron powder diffraction measurements. Magnetic susceptibility in the paramagnetic phase shows Curie-Weiss behavior with negative Weiss temperature $Θ\simeq -22.5$ K, indicating dominant antiferromagnetic interactions. At $T_{\rm N} = 3.44$ K, CaCoV$_2$O$_7$ shows antiferromagnetic order, accompanied by a weak net ferromagnetic moment of $\sim 0.05$~$μ_{\rm B}/{\rm Co}^{2+}$. Neutron powder diffraction confirms the formation of antiferromagnetic order below $T_{\rm N}$. It was furt…
Using density functional theory combined with a Hubbard model (DFT+U ), the electronic band structure of CrI3 multilayers, both free-standing and enclosed between graphene contacts, is calculated. We show that the DFT+U approach, together with the 'around mean field' correction scheme, is able to describe the vertical magnetotransport in line with the experimental measurements of magnetoresistance in multi-layered CrI3 enclosed between graphene contacts. Moreover, by interpolating between different double-counting correction schemes, namely the 'around mean field' correction and the fully loca…
Using density functional theory, we study the magnetic stability of the Ga$_{1-x}$Mn$_x$N alloy system. We show that unlike Ga$_{1-x}$Mn$_x$As, which shows only ferromagnetic (FM) phase, Ga$_{1-x}$Mn$_x$N can be stable in either FM or antiferromagnetic phases depending on the alloy concentration. The magnetic order can also be altered by applying pressure or with charge compensation. A unified model is used to explain these behaviors.
The unusual thermodynamic properties of the Ising antiferromagnet supplemented with a ferromagnetic, mean-field term are outlined. This simple model is inspired by more realistic models of spin-crossover materials. The phase diagram is estimated using Metropolis Monte Carlo methods, and differences with preliminary Wang-Landau Monte Carlo results for small systems are noted.
We present a Monte Carlo study of the magnetic properties of thin cylindrical nanowires composed of a ferromagnetic core and an antiferromagnetic shell implementing a classical spin Hamiltonian. We address systematically the impact of interface exchange coupling on the loop characteristics and the magnetization reversal mechanism. We study the effect of shell polycrystallinity on the characteristic fields of the isothermal hysteresis loop (coercivity, exchange-bias). We demonstrate that coupling to a polycrystalline antiferromagnetic shell increases the critical core diameter for transition fr…
