We study realizations of spirals and skyrmions in two-dimensional antiferromagnets with a triangular lattice on an inversion-symmetry-breaking substrate. As a possible material realization, we investigate the adsorption of transition-metal atoms (Cr, Mn, Fe, or Co) on a monolayer of MoS$_2$, WS$_2$, or WSe$_2$ and obtain the exchange, anisotropy, and Dzyaloshinskii-Moriya interaction parameters using first-principles calculations. Using energy minimization and parallel-tempering Monte-Carlo simulations, we determine the magnetic phase diagrams for a wide range of interaction parameters. We find that skyrmion lattices can appear even with weak Dzyaloshinskii-Moriya interactions, but their stability is hindered by magnetic anisotropy. However, a weak easy plane magnetic anisotropy can be beneficial for stabilizing the skyrmion phase. Our results suggest that Cr$/$MoS$_2$, Fe$/$MoS$_2$, and Fe$/$WSe$_2$ interfaces can host spin spirals formed from the 120$^{\circ}$ antiferromagnetic states. Our results further suggests that for other interfaces, such as Fe$/$MoS$_2$, the Dzyaloshinskii-Moriya interaction is strong enough to drive the system into a three-sublattice skyrmion lattice in the presence of experimentally feasible external magnetic field.
The instability toward a magnetic skyrmion crystal in centrosymmetric trilayer magnets is investigated based on a spin model with layer-dependent Dzayloshinskii-Moriya interaction. We find various types of skyrmion crystal phases with different skyrmion numbers in a low-temperature phase diagram by performing the simulated annealing. In addition to the Néel skyrmion crystal phase that is expected to emerge in the presence of the polar-type Dzayloshinskii-Moriya interaction, we obtain the skyrmion crystal phases characteristics of the layered system: the twisted surface skyrmion crystal, anti-s…
We numerically examine a single skyrmion dynamics under the influence of triangular and honeycomb obstacle arrays at zero temperature. The skyrmion Hall angle $θ_{sk}$, that is the angle between the applied external drive and the direction of the skyrmion motion, increases in quantized steps or continuously as a function of the applied drive. For the obstacle arrays studied in this work, the skyrmion exhibits two main directional locking effects, where the skyrmion motion locks with $θ_{sk}=-30^\circ$ and $-60^\circ$. We show that these directions are privileged due to the obstacle landscape s…
We discuss distinctive features of spiral states in bulk chiral magnets such as MnSi and Cu$_2$OSeO$_3$ that stem from the effect of the cubic magneto-crystalline anisotropy. First of all, at both the helical-to-conical and the conical-to-ferromagnetic transitions, taking place at H$_{c1}$ and H$_{c2}$, respectively, the cubic anisotropy leads to reversible or irreversible jump-like reorientations of the spiral wavevectors. The subtle interplay between the easy and hard anisotropy axes gives rise to a phase transition between elliptically distorted conical states almost without any detectable …
The influence of in-plane and canted magnetic fields on spin spirals and skyrmions in atomic bilayer islands of palladium and iron on an Ir(111) substrate is investigated by scanning tunnelling microscopy at low temperatures. It is shown that the spin spiral propagation direction is determined by the island's border which can be explained by equilibrium state calculations on a triangular lattice. By application of in-plane fields, the spin spiral reorientates its propagation direction and becomes distorted, thereby allowing a proof for its cycloidal nature. Furthermore, it is demonstrated that…
Magnetic skyrmions are particle-like topological excitations that recently generated much interest as candidates for future spintronic devices based on skyrmion small size, enhanced topological stability, and/or mutual interaction. Here we examine the properties of isolated skyrmions in a frustrated chiral magnet with competing Dzyaloshinskii-Moriya and frustrated exchange interactions. We show that the skyrmion size drastically decreases even for small values of competing stabilization mechanisms. Skyrmion mutual interaction remains attracting as is inherent for frustrated skyrmions, but the …
We study theoretically the dynamics of the spin textures, i.e., Skyrmion crystal (SkX) and spiral structure (SS), in two-dimensional helical magnets under external current. By numerically solving the Landau-Lifshitz-Gilbert equation, it is found that (i) the critical current density of the motion is much lower for SkX compared with SS in agreement with the recent experiment, (ii) there is no intrinsic pinning effect for SkX and the deformation of the internal structure of Skyrmion reduces the pinning effect dramatically, (iii) the Bragg intensity of SkX shows strong time-dependence as can be o…
Spin waves in antiferromagnetic materials have great potential for next-generation magnonic technologies. However, their properties and their dependence on the type of ground-state antiferromagnetic structure are still open questions. Here, we investigate theoretically spin waves in one- and two-dimensional model systems with a focus on noncollinear antiferromagnetic textures such as spin spirals and skyrmions of opposite topological charges. We address in particular the nonreciprocal spin excitations recently measured in bulk antiferromagnet $α$--$\text{Cu}_2\text{V}_2\text{O}_7$ utilizing in…
We investigate the existence of spiral ordering in the planar spin orientation of skyrmions localised on a face centered rectangular lattice (FCRL). We use the non-linear sigma model (NLSM) to numerically calculate the minimum energy configurations of this lattice around the $ν=1$ quantum Hall ground state. Our variational ansatz contains an angle $θ$, characterising the FCRL and an angle $q$, characterising the orientational order. As $ν$ is increased towards one, there is a smooth transition from the triangular lattice (TL) characterised by $(θ,q) = (120^o,120^o)$ to FCRLs with spiral orient…
We study the equilibrium and dynamical properties of skyrmions in thin films of chiral magnets with oblique magnetic field. The shape of an individual skyrmion is non-circular and the skyrmion density decreases with the tilt angle from the normal of films. As a result, the interaction between two skyrmions depends on the relative angle between them in addition to their separation. The triangular lattice of skyrmions under a perpendicular magnetic field is distorted into a centered rectangular lattice for a tilted magnetic field. For a low skyrmion density, skyrmions form a chain like structure…
Spin waves are the low-energy excitations of magnetically ordered materials. They are key elements in the stability analysis of the ordered phase and have a wealth of technological applications. Recently, we showed that spin waves of a magnetic nanowire may carry a definite amount of orbital angular momentum components along the propagation direction. This helical, in addition to the chiral, character of the spin waves is related to the spatial modulations of the spin wave phase across the wire. It, however, remains a challenge to generate and control such modes with conventional magnetic fiel…
We study inter-skyrmion interactions and stable spin configurations in a 2D chiral magnet with in-plane anisotropies of a tilted magnetic field and the magneto-crystalline anisotropy on a (011) thin film. We find that in both cases a small deformation of a skyrmion shape makes the inter-skyrmion interaction anisotropic, and that the skyrmions are weakly bounded along a certain direction due to an emergent attractive interaction. Furthermore, when the magneto-crystalline anisotropy is comparable to the Zeeman energy, skyrmions embedded in a uniform magnetization are tightly bound by creating a …
Skyrmions dynamics in the approximation of point-particle skyrmions is considered in the multiferroic insulators, where the spiral magnetic structure is accompanied by finite electric dipole moment. The skyrmion motion is studied in the gradients of perpendicular magnetic and electric fields. The nonuniform magnetic field with a fixed gradient magnitude leads to the spiral motion, where skyrmion circulates in the plane perpendicular to the direction of magnetic field. The frequency of circulation is fixed by the derivative of the external magnetic field and the magnitude of the dipole moment. …
Spin-polarized scanning tunneling microscopy has been applied to study non-collinear spin textures of a Mn monolayer on a four-fold symmetric W(001) substrate revealing a zero-field spin spiral ground state and two different types of rotational domain walls. With an applied magnetic field of 9 T, we observe a coexistence of the spin spiral and the skyrmion phase, even though a previous theoretical study reported that the phase transition occurs at 18 T. The skyrmions show a roughly hexagonal arrangement despite the square lattice symmetry of the W(001) substrate. Based on a reduced set of ener…
The magnetization reversal in 330 nm triangular prismatic magnetic nanoelements with variable magnetocrystalline anisotropy similar to that of partially chemically ordered FePt is studied using micromagnetic simulations employing Finite Element discretizations. Several magnetic properties including the evaluation of the magnetic skyrmion number $S$ are computed in order to characterize magnetic configurations exhibiting vortex-like formations. Magnetic vortices and skyrmions are revealed in different systems generated by the variation of the magnitude and relative orientation of the magnetocry…
Quantization of topological charges determines the various topological spin textures that are expected to play a key role in future spintronic devices. While the magnetic skyrmion with a unit topological charge Q has been extensively studied, spin textures with other integer valued have not been verified well so far. Here, we report the real-space image, creation, and manipulation of a type of multi Q three-dimensional skyrmionic texture, where a circular spin spiral ties a bunch of skyrmion tubes. We define these objects as skyrmion bundles, and show they have arbitrarily integer values Q fro…
We study the high-temperature phase diagram of the chiral magnetic insulator Cu$_2$OSeO$_3$ by measuring the spin-Hall magnetoresistance (SMR) in a thin Pt electrode. We find distinct changes in the phase and amplitude of the SMR signal at critical lines separating different magnetic phases of bulk Cu$_2$OSeO$_3$. The skyrmion lattice state appears as a strong dip in the SMR phase. A strong enhancement of the SMR amplitude is observed in the conical spiral state, which we explain by an additional symmetry-allowed contribution to the SMR present in non-collinear magnets. We demonstrate that the…
The recent discovery of tunable Dzyaloshinskii-Moriya interactions in layered magnetic materials with perpendicular magnetic anisotropy makes them promising candidates for stabilization and manipulation of skyrmions at elevated temperatures. In this article, we use Monte Carlo simulations to investigate the robustness of skyrmions in these materials against thermal fluctuations and finite-size effects. We find that in confined geometries and at finite temperatures skyrmions are present in a large part of the phase diagram. Moreover, we find that the confined geometry favors the skyrmion over t…
We demonstrate a fast numerical method of theoretical studies of skyrmion lattice or spiral order in magnetic materials with Dzyaloshinsky-Moriya interaction. The method is based on the Fourier expansion of the magnetization combined with a minimization of the free energy functional of the magnetic material in Fourier space, yielding the optimal configuration of the system for any given set of parameters. We employ a Lagrange multiplier technique in order to satisfy micromagnetic constraints. We apply this method to a system that exhibits, depending on the parameter choice, ferromagnetic, skyr…
We have employed spin-polarized scanning tunneling microscopy and Monte-Carlo simulations to investigate the effect of lateral confinement onto the nanoskyrmion lattice in Fe/Ir(111). We find a strong coupling of one diagonal of the square magnetic unit cell to the close-packed edges of Fe nanostructures. In triangular islands this coupling in combination with the mismatching symmetries of the islands and of the square nanoskyrmion lattice leads to frustration and triple-domain states. In direct vicinity to ferromagnetic NiFe islands, the surrounding skyrmion lattice forms additional domains. …
We investigate the impact of the local spin texture on the differential conductance by scanning tunneling microscopy. In the focus is the previously found non-collinear magnetoresistance, which originates from spin mixing effects upon electron hopping between adjacent sites with canted magnetic moments. In the present work it is studied with lateral resolution both for the zero magnetic field spin spiral state as well as for individual magnetic skyrmions at different magnetic field values. We analyze in detail the response of the differential conductance and find different dependencies of peak…
The revisited theoretical phase diagrams for thin films of cubic helimagnets with the easy-plane anisotropy are shown to have different topology as previously reported [Phys. Rev. B 85, 094429 (2012)]. For both in-plane and out-of-plane directions of an applied magnetic field, the phase diagrams exhibit extensive areas of stable skyrmions, which overlap for a wide range of anisotropy parameters. Although the existence of the out-of-plane skyrmions was contradicted within the previous theoretical models, we prove that additional surface twists lead to their stability, while the moderate easy-pl…
We determined the parameters of a classical spin Hamiltonian describing an Fe monolayer on Pd(111) surface with a Pt_{1-x}Ir_{x} alloy overlayer from ab initio calculations. While the ground state of the system is ferromagnetic for x=0.00, it becomes a spin spiral state as Ir is intermixed into the overlayer. Although the Dzyaloshinsky-Moriya interaction is present in the system, we will demonstrate that the frustrated isotropic exchange interactions play a prominent role in creating the spin spiral state, and these frustrated couplings lead to an attractive interaction between skyrmions at sh…
We study the equilibrium phase diagram of ultrathin chiral magnets with easy-plane anisotropy $A$. The vast triangular skyrmion lattice phase that is stabilized by an external magnetic field evolves continuously as a function of increasing $A$ into a regime in which nearest-neighbor skyrmions start overlapping with each other. This overlap leads to a continuous reduction of the skyrmion number from its quantized value $Q=1$ and to the emergence of antivortices at the center of the triangles formed by nearest-neighbor skyrmions. The antivortices also carry a small "skyrmion number" $Q_A \ll 1$ …
We study the impact of an exchange-reducing defect on a skyrmion for a thin film of finite thickness. Attraction of the skyrmion to a defect is demonstrated in a lattice model by computing the micromagnetic energy accounting for the exchange, Dzyaloshinskii-Moriya interaction, magnetic anisotropy, and dipole-dipole coupling. The spiraling dynamics of the skyrmion towards the defect is illustrated by solving numerically the full Landau-Lifshitz-Gilbert equations on a lattice and, independently, the Thiele equation, with the two methods in agreement with each other. We find that the skyrmion def…
The ground states of square lattice two-dimensional antiferromagnets with anisotropy in an external magnetic field are determined using Monte Carlo simulations and compared to theoretical analysis. We find a new phase in between the spin-flop and spiral phase that shows strong similarity to skyrmions in ferromagnetic thin films. We show that this phase arises as a result of the competition between Zeeman and Dzyaloshinskii-Moriya interaction energies of the magnetic system. Moreover, we find that isolated (anti-)skyrmions are stabilized in finite-sized systems, even at higher temperatures. The…
In bulk non-centrosymmetric magnets the chiral Dzyaloshinskii-Moriya exchange stabilizes tubular skyrmions with a reversed magnetization in their centers. While the double-twist is favorable in the center of a skyrmion, it gives rise to an excess of the energy density at the outskirt. Therefore, magnetic anisotropies are required to make skyrmions more favorable than the conical spiral state in bulk materials. Using Monte Carlo simulations, we show that in magnetic nanowires unusual skyrmions with a doubly twisted core and a number of concentric helicoidal undulations (target-skyrmions) are th…
We study the spin waves of the triangular skyrmion crystal that emerges in a two dimensional spin lattice model as a result of the competition between Heisenberg exchange, Dzyalonshinkii-Moriya interactions, Zeeman coupling and uniaxial anisotropy. The calculated spin wave bands have a finite Berry curvature that, in some cases, leads to non-zero Chern numbers, making this system topologically distinct from conventional magnonic systems. We compute the edge spin-waves, expected from the bulk-boundary correspondence principle, and show that they are chiral, which makes them immune to elastic ba…
Spin-polarized scanning tunneling microscopy is used to identify the magnetic state of different thin films on a Re(0001) substrate, which becomes superconducting below 1.7 K. All magnetic films contain an Fe/Ir interface, which is known to facilitate the emergence of non-collinear magnetic order. For Fe monolayers on ultra-thin Ir films of different thickness we find several different atomic-scale magnetic states. For Pd/Fe bilayers we find nano-scale spin spirals as magnetic ground states for Ir thicknesses of three and four atomic layers. In applied magnetic fields skyrmions emerge, and in …
Ultrafast manipulation of magnetic skyrmions by microwave fields
School of Materials and Physics, China University of Mining and Technology（中国矿业大学材料科学与工程学院）；Center for Quantum Matter, School of Physics, Zhejiang University（浙江大学物理学院量子物质研究中心）
We report the application of the nonlinear $σ$ model to study the multi-skyrmion problem in the quantum Hall ferromagnet system. We show that the ground state of the system can be described by a ferromagnet triangular Skyrme lattice near $ν=1$ where skyrmions are extremely dilute. We find a transition into antiferromagnet square lattice by increasing the skyrmion density and therefore $|ν-1|$. We investigate the possibility that the square Skyrme lattice deforms to a single skyrmion with the same topological charge when the Zeeman energy is extremely smaller than the Coulomb energy. We explici…
By introducing biquadratic together with usual bilinear ferromagnetic nearest neighbor exchange interaction in a square lattice, we find that the energy of the spin-wave mode is minimized at a finite wavevector for a vanishingly small Dzyaloshinskii-Moriya interaction (DMI), supporting a ground state with spin-spiral structure whose pitch length is unusually short as found in some of the experiments. Apart from reproducing the magnetic structures that can be obtained in a canonical model with nearest neighbor exchange interaction only, a numerical simulation of this model with further introduc…
We study the Thiele equation for current-induced motion in a skyrmion lattice through two soluble models of the pinning potential. Comprised by a Magnus term, a dissipative term and a pinning force, Thiele's equation resembles Newton's law but in virtue of the topological character of the first two, it differs significantly from Newtonian mechanics and because the Magnus force is dominant, unlike its mechanical counterpart, the Coriolis force, skyrmion trajectories do not necessarily have mechanical counterparts. This is important if we are to understand skykrmion dynamics and tap into its pot…
We study two-body interactions of magnetic skyrmions on the plane and apply them to a (mostly) analytic description of a skyrmion lattice. This is done in the context of the solvable line, a particular choice of a potential for magnetic anisotropy and Zeeman terms, where analytic expressions for skyrmions are available. The energy of these analytic single skyrmion solutions is found to become negative below a critical point, where the ferromagnetic state is no longer the lowest energy state. This critical value is determined exactly without the ambiguities of numerical simulations. Along the s…
We study quantum Hall ferromagnets with a finite density topologically charged spin textures in the presence of internal degrees of freedom such as spin, valley, or layer indices, so that the system is parametrised by a $d$-component complex spinor field. In the absence of anisotropies, we find formation of a hexagonal Skyrmion lattice which completely breaks the underlying SU(d) symmetry. The ground state charge density modulation, which inevitably exists in these lattices, vanishes exponentially in $d$. We compute analytically the complete low-lying excitation spectrum, which separates into …
A continuum model of frustrated ferromagnets is analyzed in detail in the regime of low applied magnetic field, $H_0<1/4$, where the ground state is a spatially varying conical spiral. By changing variables to a corotating spin field, the model is reformulated as a gauged sigma model in a fixed background gauge, allowing the construction of stable isolated Skyrmions, and stable multi-Skyrmion clusters, which approach the conical ground state at spatial infinity. Owing to the spatial anisotropy induced by the ground state, these Skyrmions exhibit only discrete symmetries, and are of neither Née…
We demonstrate the emergence of an anomalous Hall effect in chiral magnetic textures which is neither proportional to the net magnetization nor to the well-known emergent magnetic field that is responsible for the topological Hall effect. Instead, it appears already at linear order in the gradients of the magnetization texture and exists for one-dimensional magnetic textures such as domain walls and spin spirals. It receives a natural interpretation in the language of Alain Connes' noncommutative geometry. We show that this chiral Hall effect resembles the familiar topological Hall effect in e…
