Frustration in magnetic systems is fertile ground for complex behaviour, including unconventional ground states with emergent symmetries, topological properties, and exotic excitations. A canonical example is the emergence of magnetic-charge-carrying quasiparticles in spin-ice compounds. Despite extensive work, a reliable experimental indicator of the density of these magnetic monopoles in spin-ice systems is yet to be found. Here, using measurements on single crystals of Ho$_{2}$Ir$_{2}$O$_{7}$ in combination with dipolar Monte Carlo simulations, we show that the magnetoresistance is highly sensitive to the density of monopoles. Moreover, we find that for the orientations of magnetic field in which the monopole density is enhanced, a strong coupling emerges between the magnetic charges on the holmium sublattice and the antiferromagnetically ordered iridium ions, leading to an ability to manipulate the antiferromagnetic domains via a uniform external field. Our results pave the way to a quantitative experimental measure of monopole density and provide a powerful illustration of the interplay between the various magnetic and electronic degrees of freedom in the frustrated pyrochlore iridates. This interdependence holds promise for potential functional properties arising from the link between magnetic and electric charges, as well as for the control of antiferromagnetic domain walls, a key goal in the design of next-generation spintronic devices.
We report experimental signatures of topological transitions among the Weyl semimetal states of pyrochlore Pr2Ir2O7, where the Kondo coupling between the Ir topological electrons and the spin-ice like orders of Pr moments plays a decisive role. The magnetic-field dependence of resistivity and the Hall conductivity exhibits a plateau and a sharp jump associated with a magnetic-field hysteresis, similar to a liquid-gas-like transition in dipolar spin ice system. Furthermore, the Kondo coupling is controlled by the hydrostatic pressure, revealing that the field-induced displacement of Weyl points…
Insulating magnetic rare-earth pyrochlores related to spin ice host emergent bosonic monopolar spinons, which obey a magnetic analogue of quantum electrodynamics and may open a route to a magnetic analogue of electronics. However, the energy scales of the interactions among rare-earth moments are so low as 1 K that the possible quantum coherence can only be achieved at a sub-Kelvin. Here, we desgin high-temperature quantum spin ice materials from first principles. It is shown that the A-site deintercalated spinel iridate Ir2O4, which has been experimentally grown as epitaxial thin films, is a …
Spin ice magnetic monopoles are fractionalized emergent excitations in a class of frustrated magnets called spin ices. The classical spin ice model has an extensive number of ground state spin configurations, whereas magnetic monopoles can be thought of as the endpoints of string operators applied to these ground states. Introducing quantum fluctuations into the model induces monopoles with dynamics, which would normally lift the degeneracy of the two-monopole energy level at the linear order of the perturbation. Contrary to this expectation, we find that quantum fluctuations in the form of a …
Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a prototypical example of the pyrochlore iridates. The density of states, the Fermi surface, and the near Fermi level band dispersion in the plane perpendicular to the (111) direction were all measured and found to be in overall agreement with our LDA + SOC density functional calculations. Our observations indicate the general validity of the LDA + SOC-based approach for the electronic structure of pyrochlore iridates, raising the possibility that some of the novel predicted phases such as quantum spin i…
Dunsiger and co-workers have criticised our paper on magnetic monopole dynamics spin ice [S. T. Bramwell et al., Nature, 461 956 (2009)]. We consider their criticisms and results but show that these do not warrant any revision of our earlier conclusions. In contrast, we point out that their conclusion of a `new' type of spin dynamics in spin ice is inconsistent with established facts.
The close connection of electricity and magnetism is one of the cornerstones of modern physics. This connection plays crucial role from the fundamental point of view and in practical applications, including spintronics and multiferroic materials. A breakthrough was a recent proposal that in magnetic materials called spin ice the elementary excitations have a magnetic charge and behave as magnetic monopoles. I show that, besides magnetic charge, there should be an electric dipole attached to each magnetic monopole. This opens new possibilities to study and to control such monopoles by electric …
We present a proposal for applying nanoscale magnetometry to the search for magnetic monopoles in the spin ice materials holmium and dysprosium titanate. Employing Monte Carlo simulations of the dipolar spin ice model, we find that when cooled to below $1.5\,$K these materials exhibit a sufficiently low monopole density to enable the direct observation of magnetic fields from individual monopoles. At these temperatures we demonstrate that noise spectroscopy can capture the intrinsic fluctuations associated with monopole dynamics, allowing one to isolate the qualitative effects associated with …
At low temperatures, spin dynamics in ideal spin ice is due mainly to dilute, thermally excited magnetic monopole excitations. I consider how these will affect the dynamics of a nuclear spin (the same theory applies to muon spin resonance if implanted muons do not diffuse). Up to the time scale for nearby monopoles to be rearranged, a stretched-exponential form of the relaxation functions is expected. I work out the expected exponent in that exponential and the formulas for the $T_1$ (longitudinal) and $T_2$ (dephasing) relaxations, as a function of the monopole density. Experimental NMR is in…
Elementary excitations in the spin-ice compound Dy$_2$Ti$_2$O$_7$ can be described as magnetic monopoles propagating independently within the pyrochlore lattice formed by magnetic Dy ions. We studied the magnetic-field dependence of the thermal conductivity κ(B) for B || [001] and observe clear evidence for magnetic heat transport originating from the monopole excitations. The magnetic contribution κ_{mag} is strongly field-dependent and correlates with the magnetization M(B). The diffusion coefficient obtained from the ratio of κ_{mag} and the magnetic specific heat is strongly enhanced below…
Magnetic monopoles are hypothesised elementary particles connected by Dirac strings that behave like infinitely thin solenoids. Despite decades of searches, free magnetic monopoles and their Dirac strings have eluded experimental detection, although there is substantial evidence for deconfined magnetic monopole quasiparticles in spin ice materials. Here we report the detection of a hierarchy of unequally-spaced magnetic excitations \emph{via} high resolution inelastic neutron spectroscopic measurements on the quantum spin ice candidate Pr$_{2}$Sn$_{2}$O$_{7}$. These excitations are well-descri…
We report on the non-equilibrium monopole dynamics in the classical spin ice Dy$_2$Ti$_2$O$_7$ detected by means of high-resolution magnetostriction measurements. Significant lattice changes occur at the transition from the kagome-ice to the saturated-ice phase, visible in the longitudinal and transverse magnetostriction. A hysteresis opening at temperatures below 0.6 K suggests a first-order transition between the kagome and saturated state. Extremely slow lattice relaxations, triggered by changes of the magnetic field, were observed. These lattice-relaxation effects result from non-equilibri…
Magnetic monopoles are hypothetical particles that may exist as quantized sources and sinks of the magnetic field. In materials, they may appear in an emergent quantum electrodynamics described by a U(1) lattice gauge theory. Particularly, quantum spin ice hosts monopoles as bosonic spinons coupled to emergent gauge fields in a U(1) quantum spin liquid, namely, a deconfined Coulomb phase. When monopoles are condensed to form a long-range order, monopoles and gauge fields are screened and confined. Here we show, however, that monopole supercurrent flows across a junction of two ferromagnets tha…
An analysis is presented of the behaviour of muons in the low-temperature state in spin ice. It is shown in detail how the behavior observed in some previous muon experiments on spin ice in a weak transverse field may result from the macroscopic stray field of magnetized spin ice. A model is presented which allows these macroscopic field effects to be simulated and the results agree with experiment. The persistent spin dynamics at low temperature originate from the sample and could be a muon-induced implantation effect that is operative in out-of-equilibrium systems with long relaxation times.
Excitations in a spin ice behave as magnetic monopoles, and their population and mobility control the dynamics of a spin ice at low temperature. CdEr$_2$Se$_4$ is reported to have the Pauling entropy characteristic of a spin ice, but its dynamics are three-orders of magnitude faster than the canonical spin ice Dy$_2$Ti$_2$O$_7$. In this letter we use diffuse neutron scattering to show that both CdEr$_2$Se$_4$ and CdEr$_2$S$_4$ support a dipolar spin ice state -- the host phase for a Coulomb gas of emergent magnetic monopoles. These Coulomb gases have similar parameters to that in Dy$_2$Ti$_2$O…
The generalised longitudinal susceptibility $χ({\bf q}, ω)$ affords a sensitive measure of the spatial and temporal correlations of magnetic monopoles in spin ice. Starting with the monopole model, a mean field expression for $χ({\bf q}, ω)$ is derived as well as expressions for the mean square longitudinal field and induction at a point. Monopole motion is shown to be strongly correlated, and both spatial and temporal correlations are controlled by the dimensionless monopole density $x$ which defines the ratio of the magnetization relaxation rate and the monopole hop rate. Thermal effects and…
We respond to the comment of Bramwell et al (arXiv:1111.4168v1) to our original publication (S. R. Dunsiger et al, Phys. Rev. Lett. 107, 207207 (2011)), detailing muon spin rotation measurements of the Spin Ice compound Dy2Ti2O7.
During recent years the interest to frustrated magnets has grown considerably. Such systems reveal very peculiar properties which distinguish them from standard paramagnets, magnetically ordered regular systems (like ferro-, ferri-, and antiferromagnets), or spin glasses. In particular great amount of attention has been devoted to the so-called spin ices, in which magnetic frustration together with the large value of the single-ion magnetic anisotropy of a special kind, yield peculiar behavior. One of the most exciting features of spin ices is related to low-energy emergent excitations, which,…
Competing interactions in the so-called spin-ice compounds stabilize a frustrated ground-state with finite zero-point entropy and, interestingly, emergent magnetic monopole excitations. The properties of these monopoles are at the focus of recent research with particular emphasis on their quantum dynamics. It is predicted that each monopole also possesses an electric dipole moment, which allows to investigate their dynamics via the dielectric function ε(ν). Here, we report on broadband spectroscopic measurements of ε(ν) in Dy2Ti2O7 down to temperatures of 200mK with a specific focus on the cri…
An important and continuing theme of modern solid state physics is the realization of exotic excitations in materials (e.g. quasiparticles) that have no analogy (or have not yet been observed) in the actual physical vacuum of free space. Although they are not fundamental particles, such quasiparticles do constitute the most basic description of the excited states of the "vacuum" in which they reside. In this regard the magnetic textures of the excited states of spin ices, magnetic pyrochlore oxides with dominant Ising interactions, are proposed to be modeled as effective magnetic charge monopo…
We present magnetization and Hall effect measurements on the pyrochlore iridate Nd2Ir2O7. Previous muon spin rotation measurements have shown that the system undergoes an unusual transition at T$_M$ = 110 K into a magnetic phase lacking long-range order, followed by a transition at T$_LRO$ = 6 K into a state with long-range magnetic order. We observe a small remnant magnetization when cycling through zero magnetic field at temperatures below T$_M$. Below T$_LRO$, this remnant magnetization increases sharply, and new hysteresis effects appear at a higher field B$_c$ = 2.5 T, while the Hall resi…
Theory predicts the low-temperature magnetic excitations in spin ices consist of deconfined magnetic charges, or monopoles. A recent transverse-field (TF) muon spin rotation (muSR) experiment [S T Bramwell et al, Nature 461, 956 (2009)] reports results claiming to be consistent with the temperature and magnetic field dependence anticipated for monopole nucleation - the so-called second Wien effect. We demonstrate via a new series of muSR experiments in Dy_2Ti_2O_7 that such an effect is not observable in a TF muSR experiment. Rather, as found in many highly frustrated magnetic materials, we ob…
A non-Ohmic current that grows exponentially with the square root of applied electric field is well known from thermionic field emission (the Schottky effect), electrolytes (the second Wien effect) and semiconductors (the Poole-Frenkel effect). It is a universal signature of the attractive Coulomb force between positive and negative electrical charges, which is revealed as the charges are driven in opposite directions by the force of an applied electric field. Here we apply thermal quenches to spin ice to prepare metastable populations of bound pairs of positive and negative emergent magnetic …
Pyrochlore iridates and pyrochlore ices are two families of materials where novel quantum phenomena are intertwined with strong spin-orbit coupling, substantial electron correlation and geometrical frustration. Motivated by the puzzling experiments on two pyrochlore systems Pr2Ir2O7 and Yb2Ti2O7, we study the proximate Ising orders and the quantum phase transition out of quantum spin ice U(1) quantum spin liquid (QSL). We apply the electromagnetic duality of the compact quantum electrodynamics to analyze the "magnetic monopoles" condensation for U(1) QSL. The monopole condensation transition r…
The single-ion anisotropy and magnetic interactions in spin-ice systems give rise to unusual non-collinear spin textures, such as Pauling states and magnetic monopoles. The effective spin correlation strength ($J_{eff}$) determines the relative energies of the different spin-ice states. With this work, we display the capability of capacitive torque magnetometry in characterizing the magneto-chemical potential associated with monopole formation. We build a magnetic phase diagram of Ho$_2$Ti$_2$O$_7$, and show that the magneto-chemical potential depends on the spin-sublattice ($α$ or $β$), i.e.,…
We report a study of the thermal conductivity $κ$ of the spin-ice material Dy$_2$Ti$_2$O$_7$. From the anisotropic magnetic-field dependence of κ$ and by additional measurements on the phononic reference compounds Y$_2$Ti$_2$O$_7$ and DyYTi$_2$O$_7$, we are able to separate the phononic and the magnetic contributions to the total heat transport, i.e. $κ_{ph}$ and $κ_{mag}$, respectively, which both depend on the magnetic field. The field dependent $κ_{ph}$ arises from lattice distortions due to magnetic-field induced torques on the non-collinear magnetic moments of the Dy ions. For $κ_{mag}$, …
Here we calculate the dynamic susceptibility and dynamic correlation function in spin ice using the model of emergent magnetic monopoles. Calculations are based on a method originally suggested for the description of dynamic processes in water ice (non-equilibrium thermodynamics approach). We show that for zero temperature the dynamic correlation function reproduces the transverse dipole correlations (static correlation function) characteristic of spin ice in its ground state. At non-zero temperatures the dynamic correlation function includes an additional longitudinal component which decrease…
Quantum spin ice, modeled for magnetic rare-earth pyrochlores, has attracted great interest for hosting a U(1) quantum spin liquid, which involves spin-ice monopoles as gapped deconfined spinons, as well as gapless excitations analogous to photons. However, the global phase diagram under a [111] magnetic field remains open. Here we uncover by means of unbiased quantum Monte-Carlo simulations that a supersolid of monopoles, showing both a superfluidity and a partial ionization, intervenes the kagomé spin ice and a fully ionized monopole insulator, in contrast to classical spin ice where a direc…
The spin ice materials Ho$_{2}$Ti$_{2}$O$_{7}$ and Dy$_{2}$Ti$_{2}$O$_{7}$ are by now perhaps the best-studied classical frustrated magnets. A crucial step towards the understanding of their low temperature behaviour -- both regarding their unusual dynamical properties and the possibility of observing their quantum coherent time evolution -- is a quantitative understanding of the spin-flip processes which underpin the hopping of magnetic monopoles. We attack this problem in the framework of a quantum treatment of a single-ion subject to the crystal, exchange and dipolar fields from neighbourin…
While there is compelling evidence for the existence of magnetic monopoles in spin ice, the direct observation of a point-like source of magnetic field in these systems remains an open challenge. One promising approach is electron holography, which combines atomic-scale resolution with extreme sensitivity to magnetic vector potentials, through the Aharonov-Bohm effect. Here we explore what holography can teach us about magnetic monopoles in spin ice, through experiments on artificial spin ice, and numerical simulations of pyrochlore spin ice. In the case of artificial spin ice, we show that ho…
Designing Quantum Matter in Pyrochlore Iridates: A Perspective on Recent Thin-Film Advances
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；Department of Physics and Astronomy, Rutgers University（罗格斯大学）；School of Physics and Astronomy, University of Minnesota（明尼苏达大学）；Department of Chemical Engineering and Materials Science, University of Minnesota（明尼苏达大学）；School of Physical Sciences, University of Chinese Academy of Sciences（中国科学院大学）
It has been proposed recently \cite{son} that excitations in Spin Ice can be of the form of magnetic monopoles that does not obey the Dirac Quantization Condition. It is also well known \cite{rj} that the above scenario leads to non-associativity among translation generators. It will be interesting to see how the monopole picture in Spin Ice survives in the light of the latter observation.
We present non-equilibrium physics in spin ice as a novel setting which combines kinematic constraints, emergent topological defects, and magnetic long range Coulomb interactions. In spin ice, magnetic frustration leads to highly degenerate yet locally constrained ground states. Together, they form a highly unusual magnetic state -- a "Coulomb phase" -- whose excitations are pointlike defects -- magnetic monopoles -- in the absence of which effectively no dynamics is possible. Hence, when they are sparse at low temperature, dynamics becomes very sluggish. When quenching the system from a monop…
We present the full phase diagram of the dumbbell model of spin ice as a function of temperature, chemical potential and staggered chemical potential which breaks the translational lattice symmetry in favour of charge crystal ordering. We observe a double winged structure with five possible phases, monopole fluid (spin ice), fragmented single monopole crystal phases and double monopole crystal, the zinc blend structure. Our model provides a skeleton for liquid-liquid phase transitions and for the winged structures observed for itinerant magnets under pressure and external field. We relate our …
We study quantum spin ice in an external magnetic field applied along a $<100>$ direction. When quantum spin fluctuations are weak, elementary excitations are quantum strings with monopoles at their ends manifested as multiple spin-wave branches in the dynamical structure factor. Strong quantum fluctuations make the string tension negative and give rise to the deconfinement of monopoles. We discuss our results in the light of recent neutron scattering experiments in $\mathrm{Yb_2Ti_2O_7}$
The complexity embedded in condensed matter fertilizes the discovery of new states of matter, enriched by ingredients like frustration. Illustrating examples in magnetic systems are Kitaev spin liquids, skyrmions phases, or spin ices. These unconventional ground states support exotic excitations, for example the magnetic charges in spin ices, also called monopoles. Beyond their discovery, an important challenge is to be able to control and manipulate them. Here, we propose a new mechanism to inject monopoles in a spin ice through a staggered magnetic field. We show theoretically, and demonstra…
Extensive work on single molecule magnets has identified a fundamental mode of relaxation arising from the nuclear-spin assisted quantum tunnelling of nearly independent and quasi-classical magnetic dipoles. Here we show that nuclear-spin assisted quantum tunnelling can also control the dynamics of purely emergent excitations: magnetic monopoles in spin ice. Our low temperature experiments were conducted on canonical spin ice materials with a broad range of nuclear spin values. By measuring the magnetic relaxation, or monopole current, we demonstrate strong evidence that dynamical coupling wit…
While sources of magnetic fields - magnetic monopoles - have so far proven elusive as elementary particles, several scenarios have been proposed recently in condensed matter physics of emergent quasiparticles resembling monopoles. A particularly simple proposition pertains to spin ice on the highly frustrated pyrochlore lattice. The spin ice state is argued to be well-described by networks of aligned dipoles resembling solenoidal tubes - classical, and observable, versions of a Dirac string. Where these tubes end, the resulting defect looks like a magnetic monopole. We demonstrate, by diffuse …
Condensed matter in the low temperature limit reveals much exotic physics associated with unusual orders and excitations, examples ranging from helium superfluidity to magnetic monopoles in spin ice. The far-from-equilibrium physics of such low temperature states may be even more exotic, yet to access it in the laboratory remains a challenge. Here we demonstrate a simple and robust technique, the 'magnetothermal avalanche quench', and its use in the controlled creation of nonequilibrium populations of magnetic monopoles in spin ice at millikelvin temperatures. These populations are found to ex…
We study the three-dimensional Kasteleyn transition in both nearest neighbours and dipolar spin ice models using an algorithm that conserves the number of excitations. We first limit the interactions range to nearest neighbours to test the method in the presence of a field applied along $[100]$, and then focus on the dipolar spin ice model. The effect of dipolar interactions, which is known to be greatly self screened at zero field, is particularly strong near full polarization. It shifts the Kasteleyn transition to lower temperatures, which decreases $\approx 0.4 K$ for the parameters corresp…
We consider the effect of adding quantum dynamics to a classical topological spin liquid, with particular view to how best to detect its presence in experiment. For the Coulomb phase of spin ice, we find quantum effects to be most visible in the gauge-charged monopole excitations. In the presence of weak dilution with nonmagnetic ions we find a particularly crisp phenomenon, namely the emergence of hydrogenic excited states in which a magnetic monopole is bound to a vacancy at various distances. Via a mapping to an analytically tractable single particle problem on the Bethe lattice, we obtain …
Electrically charged particles, such as the electron, are ubiquitous. By contrast, no elementary particles with a net magnetic charge have ever been observed, despite intensive and prolonged searches. We pursue an alternative strategy, namely that of realising them not as elementary but rather as emergent particles, i.e., as manifestations of the correlations present in a strongly interacting many-body system. The most prominent examples of emergent quasiparticles are the ones with fractional electric charge e/3 in quantum Hall physics. Here we show that magnetic monopoles do emerge in a class…
We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of different field regimes. In particular, we observe a prominent feature at approximately 1.0 T that is a precursor of the low-temperature metamagnetic transition out of field-induced kagome ice, below which the kinetic constraints imposed by the ice rules manifest themselves in a substantial frequency-dependence of the susceptibility. Despite the relatively hi…
We study the quantum dynamics of fractional excitations in quantum spin ice. We focus on the density of states in the two-monopole sector, $ρ(ω)$, as this can be connected to the wavevector-integrated dynamical structure factor accessible in neutron scattering experiments. We find that $ρ(ω)$ exhibits a strikingly characteristic singular and asymmetric structure which provides a useful fingerprint for comparison to experiment. $ρ(ω)$ obtained from exact diagonalisation of a finite cluster agrees well with that from the analytical solution of a hopping problem on a Husimi cactus representing co…
A magnetic monopole in spin ice is a novel quasiparticle excitation in condensed matter physics, and we found that the ac frequency dependent magnetic susceptibility $χ(ω)$ in the two-dimensional (2D) spin ice (so-called kagomé ice) of Dy$_2$Ti$_2$O$_7$ shows a single scaling form. This behavior can be understood in terms of the dynamical scaling law for 2D Coulomb gas (CG) systems [Phys. Rev. B 90, 144428 (2014)], characterized by the charge correlation length $ξ(\propto1/\sqrt{ω_1})$, where $ω_{1}$ is a characteristic frequency proportional to the peak position of the imaginary part of $χ(ω)…
Classical symmetry enriched topological orders and distinct monopole charges for dipole-octupole spin ices
International Center for Quantum Materials, Peking University（北京大学量子材料中心）；Tsung-Dao Lee Institute, Shanghai Jiao Tong University（上海交通大学李政道研究所）；Collaborative Innovation Center of Quantum Matter（量子物质协同创新中心）；The University of Hong Kong, Shenzhen Institute of Research and Innovation（香港大学深圳研究院）；Beijing Key Laboratory of Quantum Devices, Peking University（北京大学量子器件北京市重点实验室）
Emergent quasiparticles that arise from the fractionalization of the microscopic degrees of freedom have been one of the central themes in modern condensed matter physics. The notion of magnetic monopoles, freely moving quasiparticles fragmented from local dipole excitations, has enjoyed much success in understanding the thermodynamic, static, and transport properties of the so-called spin-ice materials. The artificial version of spin ice, where a lattice of nanoscale magnetic dipoles is sculpted out of a ferromagnetic film, provides a unique opportunity to study these unusual quasiparticles i…
We study the U(1) quantum spin liquid on the pyrochlore spin ice systems. For the non-Kramers doublets such as Pr$^{3+}$ and Tb$^{3+}$, we point out that the inelastic neutron scattering not only detects the low-energy gauge photon, but also contains the continuum of the "magnetic monopole" excitations. Unlike the spinons, these "magnetic monopoles" are purely of quantum origin and have no classical analogue. We further point out that the "magnetic monopole" experiences a background dual "$π$" flux due to the spin-1/2 nature of the local moment when the "monopole" hops on the dual diamond latt…
We consider quantum spin ice in a temperature regime in which its response is dominated by the coherent motion of a dilute gas of monopoles. The hopping amplitude of a monopole is sensitive to the configuration of its surrounding spins, taken to be quasi-static on the relevant timescales. This leads to well-known blocked directions in the monopole motion; we find that these are sufficient to reduce the coherent propagation of monopoles to quantum diffusion. This result is robust against disorder, as a direct consequence of the ground-state degeneracy, which disrupts the quantum interference pr…
The monopole picture for spin ice offers a natural description for a confounding class of materials. A paper published in Nature Physics in 2009 applied it to study the dynamical properties of these systems -- sparking intense experimental and theoretical efforts in the years that followed.
Exploring possible magnetic monopoles-induced magneto-electricity in spin ices
University of Geneva（日内瓦大学）；Institut Néel, CNRS and Université Grenoble Alpes（内勒研究所，法国国家科学研究中心与格勒诺布尔阿尔卑斯大学）；ICMMO, Université Paris-Saclay, CNRS（物质化学与分子和超分子研究所，巴黎萨克雷大学，法国国家科学研究中心）
We study Ising pyrochlores by means of Monte Carlo simulations. We cover a set of exchange constants ranging from the frustrated ferromagnetic case (spin-ice) to the fully-ordered "all-in--all-out" antiferromagnet in the dipolar model, reinterpreting the results --as in an ionic system-- in terms of a temperature vs. magnetic charge density phase diagram. In spite of its spin nature and the presence of both double and single non-conserved magnetic charges, the dipolar model gives place to a phase diagram which is quite comparable with those previously obtained for on-lattice systems of electri…
We study the band structure topology and engineering from the interplay between local moments and itinerant electrons in the context of pyrochlore iridates. For the metallic iridate Pr$_2$Ir$_2$O$_7$, the Ir $5d$ conduction electrons interact with the Pr $4f$ local moments via the $f$-$d$ exchange. While the Ir electrons form a Luttinger semimetal, the Pr moments can be tuned into an ordered spin ice with a finite ordering wavevector, dubbed "Melko-Hertog-Gingras" state, by varying Ir and O contents. We point out that the ordered spin ice of the Pr local moments generates an internal magnetic …
Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we have re-analyzed the field-induced magnetic structure previously determined by neutron diffraction in Tb2Ti2O7. We show that under a high field applied along a [110] direction, Tb2Ti2O7 orders as a three dimensional arrangement of monopole and antimonopole double layers. In contrast, Ho2Ti2O7 spin ice in the same conditions behaves as a monopole-free state.…
We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to each other, in unusual ways, making possible to lift the degeneracy underpinning the spin liquid and to potentially stabilize novel forms of charge crystals, opening the path to a "magnetic crystallography". In developing the general phase diagram including nearest-neighbour coupling, Zeeman energy, electric and magnetic dipolar interactions, we uncover the em…
