Nuclear spins show long coherence times and are well isolated from the environment, which are properties making them promising for quantum information applications. Here, we present a method for nuclear spin readout by probing the transmission of a microwave resonator. We consider a single electron in a silicon quantum dot-donor device interacting with a microwave resonator via the electric dipole coupling and subjected to a homogeneous magnetic field and a transverse magnetic field gradient. In our scenario, the electron spin interacts with a $^{31}\mathrm{P}$ defect nuclear spin via the hyperfine interaction. We theoretically investigate the influence of the P nuclear spin state on the microwave transmission through the cavity and show that nuclear spin readout is feasible with current state-of-the-art devices. Moreover, we identify optimal readout points with strong signal contrast to facilitate the experimental implementation of nuclear spin readout. Furthermore, we investigate the potential for achieving coherent excitation exchange between a nuclear spin qubit and cavity photons.
In this work we perform direct single-shot readout of the singlet-triplet states in exchange coupled electrons confined to precision placed donor atoms in silicon. Our method takes advantage of the large energy splitting given by the Pauli-spin blockaded (2,0) triplet states, from which we can achieve a single-shot readout fidelity of 98.4$\pm$0.2%. We measure the triplet-minus relaxation time to be of the order 3s at 2.5T and observe its predicted decrease as a function of magnetic field, reaching 0.5s at 1T.
Electron readout contrast enhancement in the parallel nuclear regime of an exchange-coupled donor spin qubit system
Research Laboratory of Electronics, Massachusetts Institute of Technology（麻省理工学院电子研究实验室）；Quantum Machines（量子机器公司）；Intel Corporation（英特尔公司）；School of Electrical Engineering and Telecommunications, UNSW Sydney（新南威尔士大学悉尼分校电气与电信工程学院）；ARC Centre of Excellence for Quantum Computation and Communication Technology（ARC量子计算与通信技术卓越中心）；Diraq Pty. Ltd.（Diraq有限公司）；School of Fundamental Science and Technology, Keio University（庆应义塾大学基础科学与技术学院）；School of Physics, University of Melbourne（墨尔本大学物理学院）；School of Science, RMIT University（皇家墨尔本理工大学理学院）
We demonstrate optical readout of a single electron spin using cavity quantum electrodynamics. The spin is trapped in a single quantum dot that is strongly coupled to a nanophotonic cavity. Selectively coupling one of the optical transitions of the quantum dot to the cavity mode results in a spin-dependent cavity reflectivity that enables projective spin measurements by monitoring the reflected intensity of an incident optical field. Using this approach, we demonstrate spin readout fidelity of 0.61 for a quantum dot that has a poor branching ratio of 0.43. Achieving this fidelity using resonan…
We describe a method to control and detect in single-shot the electron spin state of an individual donor in silicon with greatly enhanced sensitivity. A silicon-based Single-Electron Transistor (SET) allows for spin-dependent tunneling of the donor electron directly into the SET island during the read-out phase. Simulations show that the charge transfer signals are typically Δq > 0.2 e - over an order of magnitude larger than achievable with metallic SETs on the SiO2 surface. A complete spin-based qubit structure is obtained by adding a local Electron Spin Resonance line for coherent spin cont…
We propose a realistic protocol for the preparation and readout of mechanical Bell states in an optomechanical system. The proposal relies on parameters characterizing a photonic crystal cavity mode, coupled to two localized flexural modes of the structure, but equally applies to other optomechanical systems in the same parameter range. The nonclassical states are heralded via optical postselection and revealed in specific interference patterns characterizing the emission at the cavity frequency.
Electrical detection of spins is an essential tool in understanding the dynamics of spins in semiconductor devices, providing valuable insights for applications ranging from optoelectronics and spintronics to quantum information processing. For electron spins bound to shallow donors in silicon, bulk electrically-detected magnetic resonance has relied on coupling to spin readout partners such as paramagnetic defects or conduction electrons which fundamentally limits spin coherence times. Here we demonstrate electrical detection of phosphorus donor electron spin resonance by transport through a …
Quantum state transfer into a memory, state shuttling over long distances via a quantum bus, and high-fidelity readout are important tasks for quantum technology. Realizing these tasks is challenging in the presence of realistic couplings to an environment. Here, we introduce and assess protocols that can be used in cavity QED to perform high-fidelity quantum state transfer and fast quantum nondemolition qubit readout through Hamiltonian engineering. We show that high-fidelity state transfer between a cavity and a single qubit can be performed, even in the limit of strong dephasing due to inho…
Opto-Electrical Detection of Donor Bound Excitons in Silicon-on-Insulator Substrate
University of Jyväskylä（于韦斯屈莱大学）；QuTech（奎泰克）；Netherlands Organisation for Applied Scientific Research (TNO)（荷兰应用科学研究组织）；Kavli Institute of Nanoscience, Delft University of Technology（代尔夫特理工大学卡弗里纳米科学研究所）
Donor impurity spins in silicon-28 are highly competitive qubits for upcoming solid-state quantum technologies, yet a proven scalable strategy for multi-qubit devices remains conspicuously absent. These CMOS-compatible, atomically identical qubits offer significant advantages including 3-hour coherence ($T_2$) lifetimes, as well as simultaneous qubit initialization, manipulation and readout fidelities near $\sim\!99.9\%$. These properties meet the requirements for many modern quantum error correction protocols, which are essential for constructing large-scale universal quantum technologies. Ho…
An important requirement for spin-based quantum information processing is reliable and fast readout of electron spin states, allowing for feedback and error correction. However, common readout techniques often require additional gate structures hindering device scaling or impose stringent constraints on the tuning configuration of the sensed quantum dots. Here, we operate an in-line charge sensor within a triple quantum dot, where one of the dots is coupled to a microwave cavity and used to readout the charge states of the other two dots. Owing to the proximity of the charge sensor, we observe…
The dispersive coupling between a qubit and a cavity mode is widely used for performing non-destructive readout of the qubit state. In this approach, it is typically required that the dispersive strong coupling regime is achieved. Here we show that the use of an auxiliary cavity mode reduces by orders of magnitude the required value of the dispersive coupling, for a given decay rate of the cavity mode. The analysis is performed within the input-output formalism, in terms of the photon scattering matrix elements and of the signal-to-noise ratio. We derive simple analytical expressions for the o…
Shifts from the expected nuclear magnetic resonance frequencies of antimony and bismuth donors in silicon of greater than a megahertz are observed in electrically detected magnetic resonance spectra. Defects created by ion implantation of the donors are discussed as the source of effective electric field gradients generating these shifts via quadrupole interaction with the nuclear spins. The experimental results are modeled quantitatively by molecular orbital theory for a coupled pair consisting of a donor and a spin-dependent recombination readout center.
We use microwave radiation generated by a semiconductor double quantum dot (DQD) micromaser for charge state detection. A cavity is populated with n_c ~ 6000 photons by driving a current through an emitter DQD. These photons are used to sense the charge state of a target DQD that is located at the opposite end of the cavity. Charge dynamics in the target DQD influence the output power and emission frequency of the maser. Three different readout mechanisms are compared. The detection scheme requires no cavity input field and may potentially be used to improve the scalability of semiconductor an…
Donor spin states in silicon are a promising candidate for quantum information processing. One possible donor spin readout mechanism is the bound exciton transition that can be excited optically and creates an electrical signal when it decays. This transition has been extensively studied in bulk, but in order to scale towards localized spin readout, microfabricated structures are needed for detection. As these electrodes will inevitably cause strain in the silicon lattice, it will be crucial to understand how strain affects the exciton transitions. Here we study the phosphorous donor bound exc…
We present an analysis of electron transport through two weakly coupled precision placed phosphorus donors in silicon. In particular, we examine the (1,1) to (0,2) charge transition where we predict a new type of current blockade driven entirely by the nuclear spin dynamics. Using this nuclear spin blockade mechanism we devise a protocol to readout the state of single nuclear spins using electron transport measurements only. We extend our model to include realistic effects such as Stark shifted hyperfine interactions and multi-donor clusters. In the case of multi-donor clusters we show how nuc…
The readout of semiconductor spin qubits based on spin blockade is fast but suffers from a small charge signal. Previous work suggested large benefits from additional charge mapping processes, however uncertainties remain about the underlying mechanisms and achievable fidelity. In this work, we study the single-shot fidelity and limiting mechanisms for two variations of an enhanced latching readout. We achieve average single-shot readout fidelities > 99.3% and > 99.86% for the conventional and enhanced readout respectively, the latter being the highest to date for spin blockade. The signal amp…
We propose a quantum state readout mechanism of a weakly coupled qubit in dispersive regime. The hybrid system consists of ferromagnetic insulator and a superconducting qubit in a microwave cavity. The enhancement of the measurement sensitivity is achieved by exerting torque on the ferromagnetic insulator magnetization, which compensates the damping of the system leading to an exceptional point. The proposed machanism allows to measure the qubit state either via the transmission of the cavity or the FMR signal of the magnetic material.
We measure singlet-triplet mixing in a precision fabricated double donor dot comprising of 2 and 1 phosphorus atoms separated by $16{\pm}1$ nm. We identify singlet and triplet-minus states by performing sequential independent spin readout of the two electron system and probe its dependence on magnetic field strength. The relaxation of singlet and triplet states are measured to be $12.4{\pm}1.0$ s and $22.1{\pm}1.0$ s respectively at $B_z{=}2.5$ T.
We show how to realize high-fidelity quantum non-demolition qubit readout using longitudinal qubit-oscillator interaction. This is realized by modulating the longitudinal coupling at the cavity frequency. The qubit-oscillator interaction then acts as a qubit-state dependent drive on the cavity, a situation that is fundamentally different from the standard dispersive case. Single-mode squeezing can be exploited to exponentially increase the signal-to-noise ratio of this readout protocol. We present an implementation of this idea in circuit quantum electrodynamics and a possible multi-qubit arch…
We present the realization of a cavity quantum electrodynamics setup in which photons of strongly different lifetimes are engineered in different harmonic modes of the same cavity. We achieve this in a superconducting transmission line resonator with superconducting qubits coupled to the different modes. One cavity mode is strongly coupled to a detection line for qubit state readout, while a second long lifetime mode is used for photon storage and coherent quantum operations. We demonstrate sideband based measurement of photon coherence, generation of n photon Fock states and the scaling of th…
We investigate spin and charge dynamics of a quantum dot of phosphorus atoms coupled to a radio-frequency single-electron transistor (rf-SET) using full counting statistics. We show how the magnetic field plays a role in determining the bunching or anti-bunching tunnelling statistics of the donor dot and SET system. Using the counting statistics we show how to determine the lowest magnetic field where spin-readout is possible. We then show how such a measurement can be used to investigate and optimise single electron spin-readout fidelity.
Light trapping is a crucial mechanism for synchronization in optical communication. Especially on the level of single photons, control of the exact emission time is desirable. In this paper, we theoretically propose a single-photon buffering device composed of a quantum dot doped with a single Mn atom in a cavity. We present a method to detain a single cavity photon as an excitation of the dot. The storage scheme is based on bright to dark exciton conversion performed with an off-resonant external optical field and mediated via a spin-flip with the magnetic ion. The induced Stark shift brings …
Robust, high-fidelity readout is central to quantum device performance. Overcoming poor readout is an increasingly urgent challenge for devices based on solid-state spin defects, particularly given their rapid adoption in quantum sensing, quantum information, and tests of fundamental physics. Spin defects in solids combine the repeatability and precision available to atomic and cryogenic systems with substantial advantages in compactness and range of operating conditions. However, in spite of experimental progress in specific systems, solid-state spin sensors still lack a universal, high-fidel…
We consider a quantum network of mid-infrared, graphene plasmons coupled to the hydrogen-like excited states of group-V donors in silicon. First, we show how to use plasmon-enhanced light-matter interactions to achieve single-shot spin readout of the donor qubits via optical excitation and electrical detection of the emitted plasmons. We then show how plasmons in high mobility graphene nanoribbons can be used to achieve high-fidelity, two-qubit gates and entanglement of distant Si donor qubits. The proposed device is readily compatible with existing technology and fabrication methods.
We analyze theoretically how to use the radiation pressure coupling between a mechanical oscillator and an optical cavity field to generate in a heralded way a single quantum of mechanical motion (a Fock state), and release on-demand the stored excitation as a single photon. Starting with the oscillator close to its ground state, a laser pumping the upper motional sideband leads to dynamical backaction amplification and to the creation of correlated photon-phonon pairs. The detection of one Stokes photon thus projects the macroscopic oscillator into a single-phonon Fock state. The non-classica…
For some cavity-quantum-electrodynamics systems, such as a single electron spin coupled to a passive cavity, it is challenging to reach the strong-coupling regime. In such a weak-coupling regime, the conventional dispersive readout technique cannot be used to resolve the quantum states of the spin. Here we propose an improved dispersive readout method to measure the quantum states of a weakly coupled qubit by harnessing either one or two auxiliary cavities linearly coupled to the passive cavity containing the qubit. With appropriate parameters in both cases, the system excluding the qubit can …
Substitutional donor atoms in silicon are promising qubits for quantum computation with extremely long relaxation and dephasing times demonstrated. One of the critical challenges of scaling these systems is determining inter-donor distances to achieve controllable wavefunction overlap while at the same time performing high fidelity spin readout on each qubit. Here we achieve such a device by means of scanning tunnelling microscopy lithography. We measure anti-correlated spin states between two donor-based spin qubits in silicon separated by 16${\pm}1$ nm. By utilizing an asymmetric system with…
Operating the cavity-embedded Cooper pair transistor (cCPT) in the Kerr bistable regime, we demonstrate single-shot resolution between two charge states that are $0.09e$ apart. The measurement is performed with 94$\%$ fidelity in a duration of 3 $μ$s. The drive power at which the measurement is performed corresponds to only 20 intracavity photons on average in the high oscillation amplitude state of the cCPT, which is orders-of-magnitude smaller than that in rf-SETs. We find that the limiting factor for this mode of operation of the cCPT is the spontaneous fluctuation-induced switching between…
We show how to use two-mode squeezed light to exponentially enhance cavity-based dispersive qubit measurement. Our scheme enables true Heisenberg-limited scaling of the measurement, and crucially, is not restricted to small dispersive couplings or unrealistically long measurement times. It involves coupling a qubit dispersively to two cavities, and making use of a symmetry in the dynamics of joint cavity quadratures (a so-called quantum-mechanics-free subsystem). We discuss the basic scaling of the scheme and its robustness against imperfections, as well as a realistic implementation in circui…
For solid-state spin qubits, single-gate RF readout can help minimise the number of gates required for scale-up to many qubits since the readout sensor can integrate into the existing gates required to manipulate the qubits (Veldhorst 2017, Pakkiam 2018). However, a key requirement for a scalable quantum computer is that we must be capable of resolving the qubit state within single-shot, that is, a single measurement (DiVincenzo 2000). Here we demonstrate single-gate, single-shot readout of a singlet-triplet spin state in silicon, with an average readout fidelity of $82.9\%$ at a $3.3~\text{kH…
The bandstructure of bulk silicon has a six-fold valley degeneracy. Strain in the Si/SiGe quantum well system partially lifts the valley degeneracy, but the materials factors that set the splitting of the two lowest lying valleys are still under intense investigation. We propose a method for accurately determining the valley splitting in Si/SiGe double quantum dots embedded into a superconducting microwave resonator. We show that low lying valley states in the double quantum dot energy level spectrum lead to readily observable features in the cavity transmission. These features generate a "fin…
Resonant interaction between excitonic transitions of molecules and localized electromagnetic field allows the formation of hybrid light-matter polaritonic states. This hybridization of the light and the matter states has been shown to be able to significantly alter the intrinsic properties of molecular ensembles placed inside the optical cavity. Here, we have achieved strong coupling between the excitonic transition in typical oligonucleotide-based molecular beacons labelled with a pair of organic dye molecules, demonstrating an efficient donor to acceptor resonance energy transfer, and the t…
We investigate coupling an encoded spin qubit to a microwave resonator via qubit energy level curvature versus gate voltage. This approach enables quantum non-demolition readout with strength of tens to hundred MHz all while the qubit stays at its full sweet-spot to charge noise, with zero dipole moment. A "dispersive-like" spin readout approach similar to circuit-QED but avoiding the Purcell effect is proposed. With the addition of gate voltage modulation, selective longitudinal readout and n-qubit entanglement-by-measurement are possible.
A single nuclear spin holds the promise of being a long-lived quantum bit or quantum memory, with the high fidelities required for fault-tolerant quantum computing. We show here that such promise could be fulfilled by a single phosphorus (31P) nuclear spin in a silicon nanostructure. By integrating single-shot readout of the electron spin with on-chip electron spin resonance, we demonstrate the quantum non-demolition, electrical single-shot readout of the nuclear spin, with readout fidelity better than 99.8% - the highest for any solid-state qubit. The single nuclear spin is then operated as a…
We propose a quantum computer architecture involving substitutional donors in photonic-crystal silicon cavities and the optical initialization, manipulation, and detection processes already demonstrated in ion traps and other atomic systems. Our scheme considerably simplifies the implementation of the building blocks for the successful operation of silicon-based solid-state quantum computers, including positioning of the donors, realization of one- and two-qubit gates, initialization and readout of the qubits. Detailed consideration of the processes involved, using state-of-the-art values for …
We report fabrication of transistors in a FinFET geometry using isotopically purified silicon-28 -on-insulator (28-SOI) substrates. Donor electron spin coherence in natural silicon is limited by spectral diffusion due to the residual $^{29}$Si nuclear spin bath, making isotopically enriched nuclear spin-free $^{28}$Si substrates a promising candidate for forming spin quantum bit devices. The FinFET architecture is fully compatible with single-ion implant detection for donor-based qubits, and the donor spin-state readout through electrical detection of spin resonance. We describe device process…
Ultrafast initialization enables fault-tolerant processing of quantum information while QND readout enables scalable quantum computation. By spatially assembling photon resonators and wave-guides around an n-doped nanodot and by temporally designing optical pump pulses, an efficient quantum pathway can be established from an electron spin to a charged exciton to a cavity photon and finally to a flying photon in the waveguide. Such control of vacuum-nanodot coupling can be exploited for ultrafast initialization and QND readout of the spin, which are particularly compatible with the optically dr…
We propose a method for the measurement of adiabatic phases of periodically driven quantum systems coupled to an open cavity that enables dispersive readout. It turns out that the cavity transmission exhibits peaks at frequencies determined by a resonance condition that involves the dynamical and the geometric phase. Since these phases scale differently with the driving frequency, one can determine them by fitting the peak positions to the theoretically expected behavior. For the derivation of the resonance condition and for a numerical study, we develop a Floquet theory for the dispersive rea…
Two-electron states bound to donors in silicon are important for both two qubit gates and spin readout. We present a full configuration interaction technique in the atomistic tight-binding basis to capture multi-electron exchange and correlation effects taking into account the full bandstructure of silicon and the atomic scale granularity of a nanoscale device. Excited $s$-like states of $A_1$-symmetry are found to strongly influence the charging energy of a negative donor centre. We apply the technique on sub-surface dopants subjected to gate electric fields, and show that bound triplet state…
We propose a scheme to perform single-shot quantum non-demolition (QND) readout of the spin of an electron trapped in a semiconductor quantum dot (QD). Our proposal relies on the interaction of the QD electron spin with optically excited, quantum well (QW) microcavity exciton-polaritons. The spin-dependent Coulomb exchange interaction between the QD electron and cavity polaritons causes the phase and intensity response of left circularly polarized light to be different to that of the right circularly polarized light, in such a way that the QD electron's spin can be inferred from the response t…
We present a unified picture of dispersive readout of quantum systems in and out of equilibrium. A cornerstone of the approach is the backaction of the measured system to the cavity obtained with non-equilibrium linear-response theory. It provides the dispersive shift of the cavity frequency in terms of a system susceptibility. It turns out that already effortless computations of the susceptibility allow one to generalize former results beyond a rotating-wave approximation. Examples are the readout of detuned qubits and thermally excited multi-level systems. For ac-driven quantum systems, we i…
We demonstrate a qubit readout scheme that exploits the Jaynes-Cummings nonlinearity of a superconducting cavity coupled to transmon qubits. We find that in the strongly-driven dispersive regime of this system, there is the unexpected onset of a high-transmission "bright" state at a critical power which depends sensitively on the initial qubit state. A simple and robust measurement protocol exploiting this effect achieves a single-shot fidelity of 87% using a conventional sample design and experimental setup, and at least 61% fidelity to joint correlations of three qubits.
We present the experimental observation of a large exchange coupling $J \approx 300$ $μ$eV between two $^{31}$P electron spin qubits in silicon. The singlet and triplet states of the coupled spins are monitored in real time by a Single-Electron Transistor, which detects ionization from tunnel-rate-dependent processes in the coupled spin system, yielding single-shot readout fidelities above 95%. The triplet to singlet relaxation time $T_1 \approx 4$ ms at zero magnetic field agrees with the theoretical prediction for $J$-coupled $^{31}$P dimers in silicon. The time evolution of the 2-electron s…
A quantum mechanical superposition of a long-lived, localized phonon and a matter excitation is described. We identify a realization in strained silicon: a low-lying donor transition (P or Li) driven solely by acoustic phonons at wavelengths where high-Q phonon cavities can be built. This phonon-matter resonance is shown to enter the strongly coupled regime where the "vacuum" Rabi frequency exceeds the spontaneous phonon emission into non-cavity modes, phonon leakage from the cavity, and phonon anharmonicity and scattering. We introduce a micropillar distributed Bragg reflector Si/Ge cavity, w…
We compare charge transitions on a deterministic single P donor in silicon using radio frequency reflectometry measurements with a tunnel coupled reservoir and DC charge sensing using a capacitively coupled single electron transistor (SET). By measuring the conductance through the SET and comparing this with the phase shift of the reflected RF excitation from the reservoir, we can discriminate between charge transfer within the SET channel and tunneling between the donor and reservoir. The RF measurement allows observation of donor electron transitions at every charge degeneracy point in contr…
We study the physics of a magnetic molecule described by a "giant" spin with multiple ($d > 2$) spin states interacting with the quantized cavity field produced by a superconducting resonator. By means of the input-output formalism, we derive an expression for the output modes in the dispersive regime of operation. It includes the effect of magnetic anisotropy, which makes different spin transitions addressable. We find that the measurement of the cavity transmission allows to uniquely determine the spin state of the qudits. We discuss, from an effective Hamiltonian perspective, the conditions…
The size of silicon transistors used in microelectronic devices is shrinking to the level where quantum effects become important. While this presents a significant challenge for the further scaling of microprocessors, it provides the potential for radical innovations in the form of spin-based quantum computers and spintronic devices. An electron spin in Si can represent a well-isolated quantum bit with long coherence times because of the weak spin-orbit coupling and the possibility to eliminate nuclear spins from the bulk crystal. However, the control of single electrons in Si has proved chall…
We present a superconducting device that realizes the sequential measurement of a transmon qubit. The device disables common limitations of dispersive readout such as Purcell effect or transients in the cavity mode by turning on and off the coupling to the measurement channel on demand. The qubit measurement begins by loading a readout resonator that is coupled to the qubit. After an optimal interaction time with negligible loss, a microwave pump releases the content of the readout mode by upconversion into a measurement line in a characteristic time as low as 10~ns, which is 400 times shorter…
