Temperature chaos is present in off-equilibrium spin-glass dynamics
Janus Collaboration, M. Baity-Jesi, E. Calore, A. Cruz, L. A. Fernandez, J. M. Gil-Narvion, I. Gonzalez-Adalid Pemartin, A. Gordillo-Guerrero, D. Iñiguez, A. Ma… 展开作者
Janus Collaboration, M. Baity-Jesi, E. Calore, A. Cruz, L. A. Fernandez, J. M. Gil-Narvion, I. Gonzalez-Adalid Pemartin, A. Gordillo-Guerrero, D. Iñiguez, A. Maiorano, E. Marinari, V. Martin-Mayor, J. Moreno-Gordo, A. Muñoz-Sudupe, D. Navarro, I. Paga, G. Parisi, S. Perez-Gaviro, F. Ricci-Tersenghi, J. J. Ruiz-Lorenzo, S. F. Schifano, B. Seoane, A. Tarancon, R. Tripiccione, D. Yllanes
备注：
Version accepted for publication in Communication Physics 10 pages, 9 figures
We find a dynamic effect in the non-equilibrium dynamics of a spin glass that closely parallels equilibrium temperature chaos. This effect, that we name dynamic temperature chaos, is spatially heterogeneous to a large degree. The key controlling quantity is the time-growing spin-glass coherence length. Our detailed characterization of dynamic temperature chaos paves the way for the analysis of recent and forthcoming experiments. This work has been made possible thanks to the most massive simulation to date of non-equilibrium dynamics, carried out on the Janus~II custom-built supercomputer.
Spin glasses have competing interactions that lead to a rough energy landscape which is highly susceptible to small perturbations. These chaotic effects strongly affect numerical simulations and, as such, gaining a deeper understanding of chaos in spin glasses is of much importance. The use of thermal boundary conditions is an effective approach to study chaotic phenomena. Here, we generalize population annealing Monte Carlo, combined with thermal boundary conditions, to study bond chaos due to small perturbations in the spin-spin couplings of the three-dimensional Edwards-Anderson Ising spin …
We study the effects of small temperature as well as disorder perturbations on the equilibrium state of three-dimensional Ising spin glasses via an alternate scaling ansatz. By using Monte Carlo simulations, we show that temperature and disorder perturbations yield chaotic changes in the equilibrium state and that temperature chaos is considerably harder to observe than disorder chaos.
We present a finite size scaling analysis of Monte Carlo simulation results on a four dimensional Ising spin glass. We study chaos with both coupling and temperature perturbations, and find the same chaos exponent in each case. Chaos is investigated both at the critical temperature and below where it seems to be more efficient (larger exponent). Dimension four seems to be above the critical dimension where chaos with temperature is no more present in the critical region. Our results are consistent with the Gaussian and bimodal coupling distributions being in the same universality class.
Recently extended precise numerical methods and droplet scaling arguments allow for a coherent picture of the glassy states of two-dimensional Ising spin glasses to be assembled. The length scale at which entropy becomes important and produces "chaos", the extreme sensitivity of the state to temperature, is found to depend on the type of randomness. For the $\pm J$ model this length scale dominates the low-temperature specific heat. Although there is a type of universality, some critical exponents do depend on the distribution of disorder.
We calculate the finite size scaling of the sample-to-sample fluctuations of the free energy $ΔF$ of the $m$ component vector spin glass in the large-$m$ limit. This is accomplished using a variant of the interpolating Hamiltonian technique which is used to establish a connection between the free energy fluctuations and bond chaos. The calculation of bond chaos then shows that the scaling of the free energy fluctuaions with system size $N$ is $ΔF \sim N^μ$ with ${1/5}\leqμ<{3/10}$, and very likely $μ={1}{5}$ exactly.
We investigate chaotic, memory and cooling rate effects in the three dimensional Edwards-Anderson model by doing thermoremanent (TRM) and AC susceptibility numerical experiments and making a detailed comparison with laboratory experiments on spin glasses. In contrast to the experiments, the Edwards-Anderson model does not show any trace of re-initialization processes in temperature change experiments (TRM or AC). A detailed comparison with AC relaxation experiments in the presence of DC magnetic field or coupling distribution perturbations reveals that the absence of chaotic effects in the Edw…
New low frequency ac susceptibility measurements on two different spin glasses show that cooling/heating the sample at a constant rate yields an essentially reversible (but rate dependent) X(T) curve; a downward relaxation of X occurs during a temporary stop at constant temperature (ageing). Two main features of our results are: (i)when cooling is resumed after such a stop, X goes back to the reversible curve (chaos) (ii) upon re-heating, X perfectly traces the previous ageing history (memory). We discuss implications of our results for a real space (as opposed to phase space) picture of spin …
Spin glasses have competing interactions and complex energy landscapes that are highly-susceptible to perturbations, such as the temperature or the bonds. The thermal boundary condition technique is an effective and visual approach for characterizing chaos, and has been successfully applied to three dimensions. In this paper, we tailor the technique to partial thermal boundary conditions, where thermal boundary condition is applied in a subset (3 out of 4 in this work) of the dimensions for better flexibility and efficiency for a broad range of disordered systems. We use this method to study b…
This thesis pretends to be another step in the development of numerical research in disordered systems. Specifically, we will focus on spin glasses which have demonstrated to be a fertile field from both, experimental and theoretical approaches. Throughout this thesis, we will discuss a variety of interesting phenomenons and we will also open new avenues to previously unexplored effects in the context of spin glasses. However, without a doubt, the leitmotiv conducting this thesis is the role of numerical simulations as a valuable tool to explore spin-glass physics. This thesis is organized int…
Temperature chaos has often been reported in literature as a rare-event driven phenomenon. However, this fact has always been ignored in the data analysis, thus erasing the signal of the chaotic behavior (still rare in the sizes achieved) and leading to an overall picture of a weak and gradual phenomenon. On the contrary, our analysis relies on a large-deviations functional that allows to discuss the size dependencies. In addition, we had at our disposal unprecedentedly large configurations equilibrated at low temperatures, thanks to the Janus computer. According to our results, when temperatu…
Reentrance and temperature chaos in the $p$-spin Ising spin glass
Institute of Integrated Research, Institute of Science Tokyo（东京科学大学综合研究 institute）；Graduate School of Information Sciences, Tohoku University（东北大学情报科学研究院）
Temperature chaos plays a role in important effects, like for example memory and rejuvenation, in spin glasses, colloids, polymers. We numerically investigate temperature chaos in spin glasses, exploiting its recent characterization as a rare-event driven phenomenon. The peculiarities of the transformation from periodic to anti-periodic boundary conditions in spin glasses allow us to conclude that temperature chaos is non-local: no bounded region of the system causes it. We precise the statistical relationship between temperature chaos and the free-energy changes upon varying boundary conditio…
The aging in a Heisenberg-like spin glass Ag(11 at% Mn) is investigated by measurements of the zero field cooled magnetic relaxation at a constant temperature after small temperature shifts $|ΔT/T_g| < 0.012$. A crossover from fully accumulative to non-accumulative aging is observed, and by converting time scales to length scales using the logarithmic growth law of the droplet model, we find a quantitative evidence that positive and negative temperature shifts cause an equivalent restart of aging (rejuvenation) in terms of dynamical length scales. This result supports the existence of a unique…
Temperature chaos is an extreme sensitivity of the equilibrium state to a change of temperature. It arises in several disordered systems that are described by the so called scaling theory of spin glasses, while it seems to be absent in mean field models. We consider a model spin glass on a tree and show that although it has mean field behavior with replica symmetry breaking, it manifestly has ``strong'' temperature chaos. We also show why chaos appears only very slowly with system size.
Spin-glass phases and phase transitions for q-state clock models and their q $\rightarrow \infty$ limit the XY model, in spatial dimension d=3, are studied by a detailed renormalization-group study that is exact for the d=3 hierarchical lattice and approximate for the cubic lattice. In addition to the now well-established chaotic rescaling behavior of the spin-glass phase, each of the two types of spin-glass phase boundaries displays, under renormalization-group trajectories, their own distinctive chaotic behavior. These chaotic renormalization-group trajectories subdivide into two categories,…
We study the problem of chaos in temperature in some mean-field spin-glass models by means of a replica computation over a model of coupled systems. We propose a set of solutions of the saddle point equations which are intrinsically non-chaotic and solve a general problem regarding the consistency of their structure. These solutions are relevant in the case of uncoupled systems too, therefore they imply a non-trivial overlap distribution $P(q_{T1T2})$ between systems at different temperatures. The existence of such solutions is checked to fifth order in an expansion near the critical temperatu…
The analytical solution of a many-body localization problem in a quantum Sherrington-Kirkpatrick spin glass model in a random longitudinal field is proposed matching the problem with a model of Anderson localization in a Bethe lattice. The localization transition is dramatically sensitive to the relationship between interspin interaction and random field revealing different regimes in which the interaction can either suppress or enhance the delocalization. The localization is enhanced by decreasing the temperature and the localization transition shows a remarkable universality in a spin glass …
Dynamics of spin-glasses subjected to slow continuous changes of working enviroment such as slow changes of temperature or interaction bonds are studied based on scaling arguments and numerical simulations of continuous bond changes. Such perturbations lead to a glassy stationary state where the age or domain size of the system are pinned to macroscopic but finite values due to competition between relaxation and chaos effects (rejuvenation). Flutuation-dissipation relation is also pinned to that of a finite age. The scenario explains the anomalously weak cooling rate dependece of spin glasses.
We discuss temperature chaos in mean field and realistic 3D spin glasses. Our numerical simulations show no trace of a temperature chaotic behavior for the system sizes considered. We discuss the experimental and theoretical implications of these findings.
The temperature ($T$)-shift protcol of aging in the 3 dimensional (3D) Edwards- Anderson (EA) spin-glass (SG) model is studied through the out-of-phase component of the ac susceptibility simulated by the Monte Carlo method. For processes with a small magnitude of the $T$-shift, $ΔT$, the memory imprinted before the $T$-shift is preserved under the $T$-change and the SG short-range order continuously grows after the $T$-shift, which we call the cumulative memory scenario. For a negative $T$-shift process with a large $ΔT$ the deviation from the cumulative memory scenario has been observed for t…
We consider the problem of temperature chaos in mean-field spin-glass models defined on random lattices with finite connectivity. By means of an expansion in the order parameter we show that these models display a much stronger chaos effect than the fully connected Sherrington-Kirkpatrick model with the exception of the Bethe lattice with bimodal distribution of the couplings.
We address the problem of chaotic temperature dependence in disordered glassy systems at equilibrium by following states of a random-energy random-entropy model in temperature; of particular interest are the crossings of the free-energies of these states. We find that this model exhibits strong, weak or no temperature chaos depending on the value of an exponent. This allows us to write a general criterion for temperature chaos in disordered systems, predicting the presence of temperature chaos in the Sherrington-Kirkpatrick and Edwards-Anderson spin glass models, albeit when the number of spin…
The overlap length of a three-dimensional Ising spin glass on a cubic lattice with Gaussian interactions has been estimated numerically by transfer matrix methods and within a Migdal-Kadanoff renormalization group scheme. We find that the overlap length is large, explaining why it has been difficult to observe spin glass chaos in numerical simulations and experiment.
Spin-glass and chiral-glass orderings in three-dimensional Heisenberg spin glasses are studied both by equilibrium and off-equilibrium Monte Carlo simulations. Fully isotropic model is found to exhibit a finite-temperature chiral-glass transition without the conventional spin-glass order. Although chirality is an Ising-like quantity from symmetry, universality class of the chiral-glass transition appears to be different from that of the standard Ising spin glass. In the off-equilibrium simulation, while the spin autocorrelation exhibits only an interrupted aging, the chirality autocorrelation …
Domain-wall free-energy $δF$, entropy $δS$, and the correlation function, $C_{\rm temp}$, of $δF$ are measured independently in the four-dimensional $\pm J$ Edwards-Anderson (EA) Ising spin glass. The stiffness exponent $θ$, the fractal dimension of domain walls $d_{\rm s}$ and the chaos exponent $ζ$ are extracted from the finite-size scaling analysis of $δF$, $δS$ and $C_{\rm temp}$ respectively well inside the spin-glass phase. The three exponents are confirmed to satisfy the scaling relation $ζ=d_{\rm s}/2-θ$ derived by the droplet theory within our numerical accuracy. We also study bond ch…
The left-right chiral and ferromagnetic-antiferromagnetic double spin-glass clock model, with the crucially even number of states q=4 and in three dimensions d=3, has been studied by renormalization-group theory. We find, for the first time to our knowledge, four different spin-glass phases, including conventional, chiral, and quadrupolar spin-glass phases, and phase transitions between spin-glass phases. The chaoses, in the different spin-glass phases and in the phase transitions of the spin-glass phases with the other spin-glass phases, with the non-spin-glass ordered phases, and with the di…
We study temperature chaos in a two-dimensional Ising spin glass with random quenched bimodal couplings, by an exact computation of the partition functions on large systems. We study two temperature correlators from the total free energy and from the domain wall free energy: in the second case we detect a chaotic behavior. We determine and discuss the chaos exponent and the fractal dimension of the domain walls.
We identify simple mechanisms that prevents the onset of disorder chaos for the Ising spin glass model on $\mathbb Z^d$. This was first shown by Chatterjee in the case of Gaussian couplings. We present three proofs of the theorem for general couplings with continuous distribution based on the presence in the coupling realization of stabilizing features of positive density.
For the long-range one-dimensional Ising spin-glass with random couplings decaying as $J(r) \propto r^{-σ}$, the scaling of the effective coupling defined as the difference between the free-energies corresponding to Periodic and Antiperiodic boundary conditions $J^R(N) \equiv F^{(P)}(N)-F^{(AP)}(N) \sim N^{θ(σ)}$ defines the droplet exponent $θ(σ)$. Here we study numerically the instability of the renormalization flow of the effective coupling $J^R(N)$ with respect to magnetic, disorder and temperature perturbations respectively, in order to extract the corresponding chaos exponents $ζ_H(σ)$, …
We argue that the chaotic temperature effect predicted in Ising spin glasses should be stronger when one considers continuous (XY, Heisenberg) kind of spins, due to bigger entropic fluctuations. We then discuss the behavior of 3d spin glasses using the Migdal-Kadanoff Renormalization Group for Ising and XY spins, where we show explicitly that the chaotic length scale, the length beyond which equilibrium configurations are completly reshuffled when one changes temperature, could be far smaller for XY than for Ising spins. These results could thus explain why experiments are seeing a stronger re…
We approximate a 2D Ising spin glass by tiling an infinite square lattice with large identical unit cells. The interactions within the unit cell are random. Each such sample shows one or more critical points. We examine the scaling of the critical temperatures with unit cell size. Due to chaos, the correlations between unit cells can change sign with changing temperature. We also examine the scaling of this chaos. This chaos causes many samples to have multiple phase transitions, because the interaction between adjacent unit cells changes sign within the ordered phases.
We study the fragility of spin glasses to small temperature perturbations numerically using population annealing Monte Carlo. We apply thermal boundary conditions to a three-dimensional Edwards-Anderson Ising spin glass. In thermal boundary conditions all eight combinations of periodic versus antiperiodic boundary conditions in the three spatial directions are present, each appearing in the ensemble with its respective statistical weight determined by its free energy. We show that temperature chaos is revealed in the statistics of crossings in the free energy for different boundary conditions.…
We investigate numerically disorder chaos in spin glasses, i.e. the sensitivity of the ground state to small changes of the random couplings. Our study focuses on the Edwards-Anderson model in d=1,2,3 and in mean-field. We find that in all cases, simple scaling laws, involving the size of the system and the strength of the perturbation, are obeyed. We characterize in detail the distribution of overlap between ground states and the geometrical properties of flipped spin clusters in both the weak and strong chaos regime. The possible relevance of these results to temperature chaos is discussed.
Reply to the Comment by L. Berthier and J.-P. Bouchaud, Phys. Rev. Lett. 90, 059701 (2003), also cond-mat/0209165, on our paper Phys. Rev. Lett. 89, 097201 (2002), also cond-mat/0203444
We use simulations within the Migdal-Kadanoff real space renormalization approach to probe the scales relevant for rejuvenation and memory in spin glasses. One of the central questions concerns the role of temperature chaos. First we investigate scaling laws of equilibrium temperature chaos, finding super-exponential decay of correlations but no chaos for the total free energy. Then we perform out of equilibrium simulations that follow experimental protocols. We find that: (1) rejuvenation arises at a length scale smaller than the ``overlap length'' l(T,T'); (2) memory survives even if equilib…
The properties of discrete two-dimensional spin glasses depend strongly on the way the zero-temperature limit is taken. We discuss this phenomenon in the context of the Migdal-Kadanoff renormalization group. We see, in particular, how these properties are connected with the presence of a cascade of fixed points in the renormalization group flow. Of particular interest are two unstable fixed points that correspond to two different spin-glass phases at zero temperature. We discuss how these phenomena are related with the presence of entropy fluctuations and temperature chaos, and universality in…
We investigate partition-function zeros of the many-body interacting spherical spin glass, the so-called $p$-spin spherical model, with respect to the complex temperature in the thermodynamic limit. We use the replica method and extend the procedure of the replica symmetry breaking ansatz to be applicable in the complex-parameter case. We derive the phase diagrams in the complex-temperature plane and calculate the density of zeros in each phase. Near the imaginary axis away from the origin, there is a replica symmetric phase having a large density. On the other hand, we observe no density in t…
Using the decay of the out equilibrium spin-spin correlation function we compute the equilibrium Edward-Anderson order parameter in the three dimensional binary Ising spin glass in the spin glass phase. We have checked that the Edward-Anderson order parameter computed from out of equilibrium numerical simulations follows with good precision the critical law as determined in experiments and in numerical studies at equilibrium. We have also studied the dependence of the order parameter with the lattice size. Finally we present a large time study of the scaling of the off-equilibrium fluctuation-…
We have introduced a variational method to improve the computation of integrated correlation times in the Parallel Tempering Dynamics, obtaining a better estimate (a lower bound, at least) of the exponential correlation time. Using this determination of the correlation times, we revisited the problem of the characterization of the chaos in temperature in finite dimensional spin glasses by means of the study of correlations between different chaos indicators computed in the static and the correlation times of the Parallel Tempering dynamics. The sample-distribution of the characteristic time fo…
We derive lower bounds for the variance of the difference of energies between incongruent ground states, i.e., states with edge overlaps strictly less than one, of the Edwards-Anderson model on ${\mathbb Z}^d$. The bounds highlight a relation between the existence of incongruent ground states and the absence of edge disorder chaos. In particular, it suggests that the presence of disorder chaos is necessary for the variance to be of order less than the volume. In addition, a relation is established between the scale of disorder chaos and the size of critical droplets. The results imply a long-c…
Non-equilibrium dynamics in a Ag(11%Mn) spin-glass has been studied by low frequency ac-susceptibility and magnetic relaxation experiments. The results unequivocally show that spin structures that memorize the cooling process are imprinted in the system. These imprinted structures disclose themselves through dramatic changes of the dynamics on re-heating the spin-glass through the temperatures where intermittent stops or changes of the cooling rate have been imposed. We can qualitatively interpret our results in terms of the droplet spin-glass model developed by Fisher and Huse [Phys. Rev. B 3…
In spin-glass systems, frustration can be adjusted continuously and considerably, without changing the antiferromagnetic bond probability p, by using locally correlated quenched randomness, as we demonstrate here on hypercubic lattices and hierarchical lattices. Such overfrustrated and underfrustrated Ising systems on hierarchical lattices in d=3 and 2 are studied. With the removal of just 51 % of frustration, a spin-glass phase occurs in d=2. With the addition of just 33 % frustration, the spin-glass phase disappears in d=3. Sequences of 18 different phase diagrams for different levels of fru…
Glassy behavior is one of the main open problems in condensed matter physics. In this thesis, we approach the problem by studying spin-glasses and colloids, using several complementary strategies. From the point of view of model building, we propose a new model, the hypercube model, which is mean-field but defined in a metric space. We show that, also in Mean Field, the spin-glass non-equilibrium dynamics is a domain-growth process very similar to its three-dimensional counterpart. We also consider spin-glasses in three spatial dimensions, focusing on temperature chaos. Thanks to the low-tempe…
Using ground state computations, we study the transition from a spin glass to a ferromagnet in 3-d spin glasses when changing the mean value of the spin-spin interaction. We find good evidence for replica symmetry breaking up till the critical value where ferromagnetic ordering sets in, and no ferromagnetic spin glass phase. This phase diagram is in conflict with the droplet/scaling and mean field theories of spin glasses. We also find that the exponents of the second order ferromagnetic transition do not depend on the microscopic Hamiltonian, suggesting universality of this transition.
Chaotic quantum systems with Lyapunov exponent $λ_\mathrm{L}$ obey an upper bound $λ_\mathrm{L}\leq 2πk_\mathrm{B}T/\hbar$ at temperature $T$, implying a divergence of the bound in the classical limit $\hbar\to 0$. Following this trend, does a quantum system necessarily become `more chaotic' when quantum fluctuations are reduced? Moreover, how do symmetry breaking and associated non-trivial dynamics influence the interplay of quantum mechanics and chaos? We explore these questions by computing $λ_\mathrm{L}(\hbar,T)$ in the quantum spherical $p$-spin glass model, where $\hbar$ can be continuou…
We study aging phenomena of Migdal-Kadanoff spin glasses in order to clarify relevancy of temperature chaos to rejuvenation and memory. By exploiting renormalization, we do efficient dynamical simulations in very wide time/length scales including the chaos length. As a consequence, we find that temperature chaos and temperature dependence of speed of equilibration cause two significantly different effects against temperature variations, i.e., rejuvenation for positive temperature variation and memory for negative temperature variation, as are observed experimentally in spin glasses.
We report new experimental results obtained onthe insulating spin glass CdCrInS_4. Our experimental setup allows a quantitative comparison between thethermo-remanent magnetization and the autocorrelation of spontaneous fluctuations of magnetization, yielding acomplete determination of the fluctuation-dissipationrelation. The dynamics can be studied both in thequasi-equilibrium regime, where the fluctuation-dissipation theorem holds, and in the deeply aging regime. The limit of separation of time-scales, as used in analytical calculations, can be approached by use of a scaling procedure.
The dynamics of the 2D Coulomb glass model is investigated by kinetic Monte Carlo simulation. An exponential divergence of the relaxation time signals a zero-temperature freezing transition. At low temperatures the dynamics of the system is glassy. The local charge correlations and the response to perturbations of the local potential show aging. The dynamics of formation of the Coulomb gap is slow and the density of states at the Fermi level decays in time as a power law. The relevance of these findings for recent transport experiments in Anderson-insulating films is pointed out.
We investigate the question of temperature chaos in the Sherrington-Kirkpatrick spin glass model, applying to existing Monte Carlo data a recently proposed rare events based data analysis method. Thanks to this new method, temperature chaos is now observable for this model, even with the limited size systems that can be currently simulated.
Using Monte Carlo simulations, we have studied isothermal aging of three-dimensional Ising spin-glass model focusing on quasi-equilibrium behavior of the spin auto-correlation function. Weak violation of the time translational invariance in the quasi-equilibrium regime is analyzed in terms of {\it effective stiffness} for droplet excitations in the presence of domain walls. Within the range of computational time window, we have confirmed that the effective stiffness follows the expected scaling behavior with respect to the characteristic length scales associated with droplet excitations and do…
