We theoretically study the electrical transport properties of a single level quantum dot connected to two normal conducting leads, which is coupled to the lattice vibrations. We determine the current through the quantum dot in two different situations: time-independent and time-averaged. In all situations we consider three cases: when there is no electron-phonon interaction, when the dot electrons interact with optical phonons or when they interact with acoustic phonons. At finite temperatures we take into account the temperature dependence of the chemical potential. We treat the electron-phonon interaction by the canonical transformation method. In the case of electron-longitudinal optical phonon interaction the spectrum contains a subpeak. In the case of electron-acoustic phonon interaction the spectrum is continuous. In the time-averaged situation many parasite peaks appear in the spectrum, due to the external time-modulation.
Phonons strongly influence the optical control of semiconductor quantum dots. When modeling the electron-phonon interaction in several theoretical approaches the quantum dot geometry is approximated by a spherical structure, though typical self-assembled quantum dots are strongly lens-shaped. By explicitly comparing simulations of a spherical and a lens-shaped dot using a well-established correlation expansion approach we show that indeed lens-shaped dots can be exactly mapped to a spherical geometry when studying the phonon influence on the electronic system. We also give a recipe to reproduc…
Phonon-mediated spin dynamics in a two-electron double quantum dot under a phonon temperature gradient
Institute of Industrial Science, The University of Tokyo（东京大学工业科学研究所）；Center for Emergent Materials Science (CEMS), RIKEN（理化学研究所新兴材料科学中心）；RIKEN Center for Quantum Computing (RQC), RIKEN（理化学研究所量子计算中心）；Pure and Applied Sciences, University of Tsukuba（筑波大学自然系统工学研究科）
The effect of electron-phonon coupling on transport through a pair of strongly correlated quantum dots embedded in the Aharonov-Bohm ring is considered in the mean field slave boson Kotliar-Ruckenstein approach. It is shown that coupling with phonons opens transport gap in the region of double occupancy. Low-bias conductance and thermopower provide information on electron-phonon coupling strength.
We study phonon emission in a GaAs/AlGaAs double quantum dot by monitoring the tunneling of a single electron between the two dots. We prepare the system such that a known amount of energy is emitted in the transition process. The energy is converted into lattice vibrations and the resulting tunneling rate depends strongly on the phonon scattering and its effective phonon spectral density. We are able to fit the measured transition rates and see imprints of interference of phonons with themselves causing oscillations in the transition rates.
We report the inclusion of phonon scattering to our recently established numerical package QmeQ for transport in quantum dot systems. This enables straightforward calculations for a large variety of devices. As examples we show (i) transport in a double-dot structure, where energy relaxation is crucial to match the energy difference between the levels, and (ii) the generation of electrical power by contacting cold electric contacts with quantum dot states, which are subjected to heated phonons.
In semiconductor quantum dots the coupling to the environment, i.e. to phonons, plays a crucial role for optical state preparation. We analyze the phonon impact on two methods for a direct optical preparation of the dark exciton, which is enabled by a tilted magnetic field: the excitation with a chirped laser pulse and the excitation with a detuned pulse. Our study reveals that for both methods phonons either do not impede the proposed mechanism or are even useful by widening the parameter range where a dark state preparation is possible due to phonon-assisted dark exciton preparation. In view…
We present a theoretical study of the evolution of spatial coherence during relaxation between delocalized exciton states in a pair of vertically stacked semiconductor quantum dots coupled to acoustic phonons. We show that spatial coherence can be transferred to the ground state even in a system of uncoupled non-identical quantum dots if a particular kind of degeneracy between the inter-level energy splittings is present. The phonon-assisted mechanism of coherence transfer leads to a dependence of the amount of the resulting coherence on the inter-dot distance and temperature. We analyze also …
For many applications of semiconductor quantum dots in quantum technology a well controlled state preparation of the quantum dot states is mandatory. Since quantum dots are embedded in the semiconductor matrix, the interaction with phonons plays often a major role in the preparation process. In this review, we discuss the influence of phonons on three basically different optical excitation schemes which can be used for the preparation of exciton, biexciton, and superposition states: a resonant excitation leading to Rabi rotations in the excitonic system, an excitation with chirped pulses explo…
We calculate the conductance through strongly correlated T-shaped molecular or quantum dot systems under the influence of phonons. The system is modelled by the extended Anderson-Holstein Hamiltonian. The finite-U mean-field slave boson approach is used to study many-body effects. Phonons influence both interference and correlations. Depending on the dot unperturbed energy and the strength of electron-phonon interaction the system is occupied by a different number of electrons which effectively interact with each other repulsively or attractively. This leads together with the interference effe…
We demonstrate an approach to realize the population inversion of a single InGaAs/GaAs quantum dot, which is driven by a laser pulse tuned within the neutral exciton phonon sideband. The inversion is achieved by rapid thermalization of the optically dressed states via phonon-assisted relaxation. A maximum exciton population of 0.67 $\pm$ 0.06 is measured for a laser tuned 0.83 meV to higher energy and the phonon sideband is mapped using a two-color pump-probe technique. Our experiments reveal that, in accordance with theory, the phonon-bath provides additional functionality for an optically dr…
We study and compare two analytic models of graphene quantum dots for calculating charge relaxation times due to electron-phonon interaction. Recently, charge relaxation processes in graphene quantum dots have been probed experimentally and here we provide a theoretical estimate of relaxations times. By comparing a model with pure edge confinement to a model with electrostatic confinement, we find that the latter features much larger relaxation times. Interestingly, relaxation times in electrostatically defined quantum dots are predicted to exceed the experimentally observed lower bound of ~10…
