Semiconductor quantum dots are a versatile source of single photons with tunable properties to be used in quantum-cryptographic applications. A crucial figure of merit of the emitted photons is photon number coherence (PNC), which impacts the security of many quantum communication protocols. In the process of single-photon generation, the quantum dot as a solid-state object is subject to an interaction with phonons, which can therefore indirectly affect the PNC. In this paper, we elaborate on the origin of PNC in optically excited quantum dots and how it is affected by phonons. In contrast to the expectation that phonons always deteriorate coherence, PNC can be increased in a quantum dot-cavity system due to the electron-phonon interaction.
Phonon-cavity electromechanics allows the manipulation of mechanical oscillations similar to photon-cavity systems. Many advances on this subject have been achieved in various materials. In addition, the coherent phonon transfer (phonon Rabi oscillations) between the phonon cavity mode and another oscillation mode has attracted many interest in nano-science. Here we demonstrate coherent phonon transfer in a carbon nanotube phonon-cavity system with two mechanical modes exhibiting strong dynamical coupling. The gate-tunable phonon oscillation modes are manipulated and detected by extending the …
An electron-phonon cavity consisting of a quantum dot embedded in a free-standing GaAs/AlGaAs membrane is characterized in Coulomb blockade measurements at low temperatures. We find a complete suppression of single electron tunneling around zero bias leading to the formation of an energy gap in the transport spectrum. The observed effect is induced by the excitation of a localized phonon mode confined in the cavity. This phonon blockade of transport is lifted at magnetic fields where higher electronic states with nonzero angular momentum are brought into resonance with the phonon energy.
Semiconductor quantum dots (QDs) in photonic nanocavities provide monolithic, robust platforms for both quantum information processing and cavity quantum electrodynamics (QED). An inherent feature of such solid-state cavity QED systems is the presence of electron-phonon interactions, which distinguishes these systems from conventional atomic cavity QED. Understanding the effects of electron-phonon interactions on these systems is indispensable for controlling and exploiting the rich physics that they exhibit. Here we investigate the effects of electron-phonon interactions on a QD-based cavity …
For a semiconductor quantum dot strongly coupled to a microcavity, we theoretically investigate phonon-assisted transitions from the exciton to a cavity photon, where the energy mismatch is compensated by phonon emission or absorption. By means of a Schrieffer-Wolff transformation we derive an effective Hamiltonian, which describes the combined effect of exciton-cavity and exciton-phonon coupling, and compute the scattering rates within a Fermi golden rule approach. The results of this approach are compared with those of a recently reported description scheme based on the independent Boson mod…
The concept of coherence is one of the fundamental phenomena in electronics and optics. In addition to electron and photon, phonon, is another important energy and information carrier in nature. Without any doubt, exploration of the phonon coherence and its impact on thermal conduction will markedly change many aspects in broad applications for heat control and management in the real world. So far, the application of coherent effect on manipulation of phonon transport is a challenge work. In this article, we review recent advances in the study of the phonon coherent transport in nanomaterials …
We study the resonance fluorescence spectra of a driven quantum dot placed inside a high $Q$ semiconductor cavity and interacting with an acoustic phonon bath. The dynamics is calculated using a time-convolutionless master equation obtained in the polaron frame. We demonstrate pronounced spectral broadening of the Mollow sidebands through cavity-emission which, for small cavity-coupling rates, increases quadratically with the Rabi frequency. However, for larger cavity coupling rates, this broadening dependence is found to be more complex. This field-dependent Mollow triplet broadening is prima…
We investigate the effect of electron-phonon interactions on the coherence properties of single photons emitted from a semiconductor cavity QED system, i.e. a quantum dot embedded in an optical cavity. The degree of indistinguishability, governing the quantum mechanical interference between two single photons, is calculated as a function of important parameters describing the cavity QED system and the phonon reservoir, e.g. cavity quality factor, light-matter coupling strength, temperature and phonon lifetime. We show that non-Markovian effects play an important role in determining the coheren…
We study the fundamental limit on single-photon indistinguishability imposed by decoherence due to phonon interactions in semiconductor quantum dot-cavity QED systems. Employing an exact diagonalization approach we find large differences compared to standard methods. An important finding is that short-time non-Markovian effects limit the maximal attainable indistinguishability. The results are explained using a polariton picture that yields valuable insight into the phonon-induced dephasing dynamics.
The influence of electron--phonon interactions on the dynamics of a quantum dot coupled to a photonic cavity mode is investigated using a nonequilibrium Green's function approach. Within a polaron frame, the self-consistent-Born approximation is used to treat the phonon-assisted scattering processes between the quantum dot polaron and the cavity. Two-time correlators of the quantum dot-cavity system are calculated by solving the Kadanoff-Baym equations, giving access to photon spectra and photon indistinguishability. The non-Markovian nature of the interaction with the phonon bath is shown to …
We investigate the influence of electron-phonon interactions on the dynamical properties of a quantum-dot-cavity QED system. We show that non-Markovian effects in the phonon reservoir lead to strong changes in the dynamics, arising from photon-assisted dephasing processes, not present in Markovian treatments. A pronounced consequence is the emergence of a phonon induced spectral asymmetry when detuning the cavity from the quantum-dot resonance. The asymmetry can only be explained when considering the polaritonic quasi-particle nature of the quantum-dot-cavity system. Furthermore, a temperature…
We present a medium-dependent quantum optics approach to describe the influence of electron-acoustic phonon coupling on the emission spectra of a strongly coupled quantum-dot cavity system. Using a canonical Hamiltonian for light quantization and a photon Green function formalism, phonons are included to all orders through the dot polarizability function obtained within the independent Boson model. We derive simple user-friendly analytical expressions for the linear quantum light spectrum, including the influence from both exciton and cavity-emission decay channels. In the regime of semiconduc…
We present a theoretical study of the evolution of spatial coherence during relaxation between delocalized exciton states in a pair of vertically stacked semiconductor quantum dots coupled to acoustic phonons. We show that spatial coherence can be transferred to the ground state even in a system of uncoupled non-identical quantum dots if a particular kind of degeneracy between the inter-level energy splittings is present. The phonon-assisted mechanism of coherence transfer leads to a dependence of the amount of the resulting coherence on the inter-dot distance and temperature. We analyze also …
We present a semi-analytic and asymptotically exact solution to the problem of phonon-induced decoherence in a quantum dot-microcavity system. Particular emphasis is placed on the linear polarization and optical absorption, but the approach presented herein may be straightforwardly adapted to address any elements of the exciton-cavity density matrix. At its core, the approach combines Trotter's decomposition theorem with the linked cluster expansion. The effects of the exciton-cavity and exciton-phonon couplings are taken into account on equal footing, thereby providing access to regimes of co…
A signature of the scattering between microcavity polaritons and longitudinal optical phonons has been observed in the electroluminescence spectrum of an intersubband device operating in the light-matter strong coupling regime. By electrical pumping we resonantly populate the upper polariton branch at different energies as a function of the applied bias. The electroluminescent signal arising from these states is seconded by a phonon replica from the lower branch.
The generation of photons in a microcavity coupled to a laser-driven quantum dot interacting with longitudinal acoustic (LA) phonons is studied in the regime of simultaneously strong driving and strong dot-cavity coupling. The stationary cavity photon number is found to depend in a non-trivial way on the detuning between the laser and the exciton transition in the dot. In particular, the maximal efficiency of the cavity feeding is obtained for detunings corresponding to transition energies between cavity-dressed states with excitation numbers larger than one. Phonons significantly enhance the …
Phonon cavities are believed to be the next step towards a control of dephasing in semiconductor quantum dot `qubits'. In this paper, we discuss two models for phonon cavities - a surface acoustic wave (SAW) inter-digitated transducer on an infinite half-space, and an elastic thin slab. The inelastic current through double quantum dots in non-perfect SAW cavities exhibits a gap at small energies and is completely suppressed in a perfect, infinite system. In the free-standing slab model, van Hove singularities evolve in the phonon spectral density. We find that these singularities cause additio…
Negatively charged boron vacancies ($V_B^-$) in hexagonal boron nitride (hBN) exhibit a broad emission spectrum due to strong electron-phonon coupling and Jahn-Teller mixing of electronic states. As such, the direct measurement of zero-phonon line (ZPL) of $V_B^-$ has remained elusive. Here, we measure the room-temperature ZPL wavelength to be $773\pm2$ nm by coupling the hBN layer to the high-Q nanobeam cavity. As the wavelength of cavity mode is tuned, we observe a pronounced intensity resonance, indicating the coupling to $V_B^-$. Our observations are consistent with the spatial redistribut…
The phonon-induced spin relaxation in a two-dimensional quantum dot embedded inside a semiconductor slab is investigated theoretically. An enhanced relaxation rate is found due to the phonon van Hove singularities. Oppositely, a vanishing deformation potential may also result in a suppression of the spin relaxation rate. For larger quantum dots, the interplay between the spin orbit interaction and Zeeman levels causes the suppression of the relaxation at several points. Furthermore, a crossover from confined to bulk-like systems is obtained by varying the width of the slab.
A major achievement of the past decade has been the realization of macroscopic quantum systems by exploiting interactions between optical cavities and mechanical resonators. In these systems, phonons are coherently annihilated or created in exchange for photons. Similar phenomena have recently been observed through "phonon cavity" coupling -- energy exchange between modes of a single system as mediated by intrinsic material nonlinearity. To date, this has been demonstrated primarily for bulk crystalline, high-quality-factor (Q>100,000) mechanical systems operated at cryogenic temperatures. Her…
We present a fully quantum theory describing the cooling of a cantilever coupled via radiation pressure to an illuminated optical cavity. Applying the quantum noise approach to the fluctuations of the radiation pressure force, we derive the opto-mechanical cooling rate and the minimum achievable phonon number. We find that reaching the quantum limit of arbitrarily small phonon numbers requires going into the good cavity (resolved phonon sideband) regime where the cavity linewidth is much smaller than the mechanical frequency and the corresponding cavity detuning. This is in contrast to the com…
A theoretical model for the phonon-mediated off-resonant coupling between a quantum dot and a cavity, under resonant excitation of the quantum dot, is presented. We show that the coupling is caused by electron-phonon interaction in the quantum dot and is enhanced by the cavity. We analyze recently observed resonant quantum dot spectroscopic data by our theoretical model.
Mechanical resonators are promising systems for storing and manipulating information. To transfer information between mechanical modes, either direct coupling or an interface between these modes is needed. In previous works, strong coupling between different modes in a single mechanical resonator and direct interaction between neighboring mechanical resonators have been demonstrated. However, coupling between distant mechanical resonators, which is a crucial request for long-distance classical and quantum information processing using mechanical devices, remains an experimental challenge. Here,…
The energy transport of acoustic phonons generated by the optical excitation of a quantum dot as well as the coherence properties of these phonons are studied theoretically both for the case of a pulsed excitation and for a continuous wave (cw) excitation switched on instantaneously. For a pulsed excitation, depending on pulse area and pulse duration, a finite number of phonon wave packets is emitted, while for the case of a cw excitation a sequence of wave packets with decreasing amplitude is generated after the excitation has been switched on. We show that the energy flow associated with the…
We present a comprehensive theoretical study of the resonance fluorescence spectra of an exciton-driven quantum dot (QD) placed inside a high-$Q$ semiconductor cavity and interacting with an acoustic phonon bath. We derive a quantum master equation (ME) in the polaron frame which includes exciton-phonon and exciton-cavity coupling to all orders. This work details and extends the theory used in a recent issue of {\em Physical Review Letters} (C. Roy and S. Hughes 2011: Phys. Rev. Lett. {\bf 106} 247403) to describe the QD Mollow triplet in the regime of semiconductor cavity-QED. Here we introdu…
We present measurements at millikelvin temperatures of the microwave-frequency acoustic properties of a crystalline silicon nanobeam cavity incorporating a phononic bandgap clamping structure for acoustic confinement. Utilizing pulsed laser light to excite a co-localized optical mode of the nanobeam cavity, we measure the dynamics of cavity acoustic modes with single-phonon sensitivity. Energy ringdown measurements for the fundamental $5$~GHz acoustic mode of the cavity shows an exponential increase in phonon lifetime versus number of periods in the phononic bandgap shield, increasing up to $τ…
Quantum confinement leads to the formation of discrete electronic states in quantum dots. Here we probe electron-phonon interactions in a suspended InAs nanowire double quantum dot (DQD) that is electric-dipole coupled to a microwave cavity. We apply a finite bias across the wire to drive a steady state population in the DQD excited state, enabling a direct measurement of the electron-phonon coupling strength at the DQD transition energy. The amplitude and phase response of the cavity field exhibit features that are periodic in the DQD energy level detuning due to the phonon modes of the nanow…
We report resonant Raman spectroscopy of neutral excitons X$^0$ and intravalley trions X$^-$ in hBN-encapsulated MoS$_2$ monolayer embedded in a nanobeam cavity. By temperature tuning the detuning between Raman modes of MoS$_2$ lattice phonons and X$^0$/X$^-$ emission peaks, we probe the mutual coupling of excitons, lattice phonons and cavity vibrational phonons. We observe an enhancement of X$^0$-induced Raman scattering and a suppression for X$^-$-induced, and explain our findings as arising from the tripartite exciton-phonon-phonon coupling. The cavity vibrational phonons provide intermedia…
Entangled photon pairs are essential for many applications in quantum technologies. Recent theoretical studies demonstrated that different types of entangled Bell states can be created in a constantly driven four-level quantum emitter-cavity system. Unlike other candidates for the realization of the four-level emitter, semiconductor quantum dots unavoidably interact with their environment, resulting in carrier-phonon interactions. Surprisingly, phonons change the entanglement of emitted photon pairs in a qualitative way, already at low temperatures on the order of 4 K. While one type of Bell s…
A dielectric body couples with electromagnetic fields through radiation pressure and electrostrictive forces, which mediate phonon-photon coupling in cavity optomechanics. In a magnetic medium, according to Korteweg-Helmholtz formula, magnetostrictive forces should arise and lead to phonon-magnon interaction. Here we report such a coupled phonon-magnon system based on ferrimagnetic spheres, which we term as cavity magnomechanics, by analogy to cavity optomechanics. Coherent phonon-magnon interactions, including electromagnetically induced transparency and absorption, are demonstrated. Exciting…
The phonon analog of an optical laser has become the focus of research. We theoretically study phonon laser in a cavity magnomechanical system, which consist of a microwave cavity, a small ferromagnetic sphere and an uniform external bias magnetic field. This system can realize the phonon-magnon coupling and the cavity photon-magnon coupling via magnetostrictive interaction and magnetic dipole interaction respectively, the magnons are driven directly by a strong microwave field simultaneously. Frist, the intensity of driving magnetic field which can reach the threshold condition of phonon lase…
We investigate pump-induced exciton inversion in a quantum-dot cavity system with continuous wave drive. Using a polaron-based master equation, we demonstrate excited-state populations above 0.9 for an InAs dot at a phonon bath temperature of 4K. In an exciton-driven system, the dominant mechanism is incoherent excitation from the phonon bath. For cavity driving, the mechanism is phonon-mediated switching between ground- and excited-state branches of the ladder of photon states, as quantum trajectory simulations clearly show. The exciton inversion as a function of detuning is found to be quali…
We report on simulations of the degree of polarization entanglement of photon pairs simultaneously emitted from a quantum dot-cavity system that demand revisiting the role of phonons. Since coherence is a fundamental precondition for entanglement and phonons are known to be a major source of decoherence, it seems unavoidable that phonons can only degrade entanglement. In contrast, we demonstrate that phonons can cause a degree of entanglement that even surpasses the corresponding value for the phonon-free case. In particular, we consider the situation of comparatively small biexciton binding e…
Arrays of coupled phonon cavities each including an impurity qubit in silicon are considered. We study experimentally feasible architectures that can exhibit quantum many-body phase transitions of phonons, e.g. Mott insulator and superfluid states, due to a strong phonon-phonon interaction (which is mediated by the impurity qubit-cavity phonon coupling). We investigate closed equilibrium systems as well as driven dissipative non-equilibrium systems at zero and non-zero temperatures. Our results indicate that quantum many-body phonon systems are achievable both in on-chip nanomechanical systems…
We develop a theoretical frame to investigate the single-photon emission spectral efficiency of a solid-state nano-emitter embedded in a high quality factor micro-cavity. This study encompasses the case of localized excitons embedded in a one, two or three-dimensional matrix. The populations evolutions are calculated based on a spin-boson model, using the non-interacting blip approximation (NIBA). We find that the single-photon spectral efficiency of the cavity-coupled emitter can be expressed by a simple formula, taking as inputs the free-space emission and absorption spectra of the emitter a…
Electron-phonon coupling is known to play an important role in the charge dynamics of semiconductor quantum dots. Here we explore its role in the combined charge-photon dynamics of cavity-coupled double quantum dots. Previous work on these systems has shown that strong electron-phonon coupling leads to a large contribution to photoemission and gain from phonon-assisted emission and absorption processes. We compare the effects of this phonon sideband in three commonly investigated gate-defined quantum dot material systems: InAs nanowires and GaAs and Si two-dimensional electron gases (2DEGs). W…
Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted emission. Here, we study theoretically and experimentally the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity as a function of temperature. We show that a large coupling to a high quality factor cavity can simultaneously reduce the effect of both phonon-induced sources of decoherence. It first limits the effect of pure dephasi…
A quantum dot strongly coupled to a single high finesse optical microcavity mode constitutes a new fundamental system for quantum optics. Here, the effect of exciton-phonon interactions on reversible quantum-dot cavity coupling is analysed without making Born-Markov approximation. The analysis is based on techniques that have been used to study the ``spin boson'' Hamiltonian. Observability of vacuum-Rabi splitting depends on the strength and the frequency dependence of the spectral density function characterizing the interactions with phonons, both of which can be influenced by phonon confinem…
Coupled electromechanical resonators that can be independently driven/detected and easily integrated with external circuits are essential for exploring mechanical modes based signal processing. Here, we present a room temperature phonon-cavity electromechanical system, consisting of two distinct resonators: a silicon nitride electromechanical drum capacitively coupled to an aluminum one. We demonstrate electromechanically induced transparency and amplification in a two-tone driving scheme and observe the phonon-cavity force affecting the mechanical damping rates of both movable objects. We als…
A quantum mechanical superposition of a long-lived, localized phonon and a matter excitation is described. We identify a realization in strained silicon: a low-lying donor transition (P or Li) driven solely by acoustic phonons at wavelengths where high-Q phonon cavities can be built. This phonon-matter resonance is shown to enter the strongly coupled regime where the "vacuum" Rabi frequency exceeds the spontaneous phonon emission into non-cavity modes, phonon leakage from the cavity, and phonon anharmonicity and scattering. We introduce a micropillar distributed Bragg reflector Si/Ge cavity, w…
We describe a chip-based, solid-state analogue of cavity-QED utilizing acoustic phonons instead of photons. We show how long-lived and tunable acceptor impurity states in silicon nanomechanical cavities can play the role of a matter non-linearity for coherent phonons just as, e.g., the Josephson qubit plays in circuit-QED. Both strong coupling (number of Rabi oscillations ~ 100) and strong dispersive coupling (0.1-2 MHz) regimes can be reached in cavities in the 1-20 GHz range, enabling the control of single phonons, phonon-phonon interactions, dispersive phonon readout of the acceptor qubit, …
For a single semiconductor quantum dot embedded in a microcavity, we theoretically and experimentally investigate phonon-assisted transitions between excitons and the cavity mode. Within the framework of the independent boson model we find that such transitions can be very efficient, even for relatively large exciton-cavity detunings of several millielectron volts. Furthermore, we predict a strong detuning asymmetry for the exciton lifetime that vanishes for elevated lattice temperature. Our findings are corroborated by experiment, which turns out to be in good quantitative and qualitative agr…
Two main mechanisms dictate the tunneling process in a double quantum dot: overlap of excited wave functions, effectively described as a tunneling rate, and phonon-assisted tunneling. In this paper, we study different regimes of tunneling that arise from the competition between these two mechanisms in a double quantum dot molecule immersed in a unimodal optical cavity. We show how such regimes affect the mean number of excitations in each quantum dot and in the cavity, the spectroscopic resolution and emission peaks of the photoluminescence spectrum, and the second-order coherence function whi…
We propose a realistic protocol for the preparation and readout of mechanical Bell states in an optomechanical system. The proposal relies on parameters characterizing a photonic crystal cavity mode, coupled to two localized flexural modes of the structure, but equally applies to other optomechanical systems in the same parameter range. The nonclassical states are heralded via optical postselection and revealed in specific interference patterns characterizing the emission at the cavity frequency.
The effects caused by phonon-assisted tunnelling (PhAT) in a double quantum dot (QD) molecule immersed in a cavity were studied under the quantum Markovian master equation formalism in order to account for dissipation phenomena. We explain how for higher PhAT rates, a stronger interaction between a QD and the cavity at off-resonance takes place through the resonant interaction of another QD and the cavity, where the QDs interact through tunnelling. A closer look at the system's allowed optical transitions as a function of PhAT rates showed coalescence of the transition energies, leading to a l…
We resolve phonon number states in the spectrum of a superconducting qubit coupled to a multimode acoustic cavity. Crucial to this resolution is the sharp frequency dependence in the qubit-phonon interaction engineered by coupling the qubit to surface acoustic waves in two locations separated by $\sim40$ acoustic wavelengths. In analogy to double-slit diffraction, the resulting self-interference generates high-contrast frequency structure in the qubit-phonon interaction. We observe this frequency structure both in the coupling rate to multiple cavity modes and in the qubit spontaneous emission…
We show how to create quantum squeezed states of magnons and phonons in a cavity magnomechanical system. The magnons are embodied by a collective motion of a large number of spins in a macroscopic ferrimagnet, and couple to cavity microwave photons and phonons (vibrational modes of the ferrimagnet) via the magnetic dipole interaction and magnetostrictive interaction, respectively. The cavity is driven by a weak squeezed vacuum field generated by a flux-driven Josephson parametric amplifier, which is essential to get squeezed states of the magnons and phonons. We show that the magnons can be pr…
We show how to generate tripartite entanglement in a cavity magnomechanical system which consists of magnons, cavity microwave photons, and phonons. The magnons are embodied by a collective motion of a large number of spins in a macroscopic ferrimagnet, and are driven directly by an electromagnetic field. The cavity photons and magnons are coupled via magnetic dipole interaction, and the magnons and phonons are coupled via magnetostrictive (radiation pressure-like) interaction. We show optimal parameter regimes for achieving the tripartite entanglement where magnons, cavity photons, and phonon…
We investigate the influence of the electron-phonon interaction on the decay dynamics of a quantum dot coupled to an optical microcavity. We show that the electron-phonon interaction has important consequences on the dynamics, especially when the quantum dot and cavity are tuned out of resonance, in which case the phonons may add or remove energy leading to an effective non-resonant coupling between quantum dot and cavity. The system is investigated using two different theoretical approaches: (i) a second-order expansion in the bare phonon coupling constant, and (ii) an expansion in a polaron-…
The mechanical properties of light have found widespread use in the manipulation of gas-phase atoms and ions, helping create new states of matter and realize complex quantum interactions. The field of cavity-optomechanics strives to scale this interaction to much larger, even human-sized mechanical objects. Going beyond the canonical Fabry-Perot cavity with a movable mirror, here we explore a new paradigm in which multiple cavity-optomechanical elements are wired together to form optomechanical circuits. Using a pair of optomechanical cavities coupled together via a phonon waveguide we demonst…
In spite of their importance for understanding phonon transport phenomena in thin films and polycrystalline solids, the effects of boundary roughness scattering on phonon specularity and coherence are poorly understood because there is no general method for predicting their dependence on phonon momentum, frequency, branch and boundary morphology. Using the recently formulated atomistic S-matrix method, we develop a theory of boundary roughness scattering to determine the mode-resolved phonon coherence and specularity parameters from the scattering amplitudes. To illustrate the theory, we apply…
Pump-probe experiments have suggested the possibility to control electronic correlations by driving infrared-active phonons with resonant midinfrared laser pulses. In this work we study two possible microscopic nonlinear electron-phonon interactions behind these observations, namely coupling of the squared lattice displacement either to the electronic density or to the double occupancy. We investigate whether photon-phonon coupling to quantized light in an optical cavity enables similar control over electronic correlations. We first show that inside a dark cavity electronic interactions increa…
Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and analysis of emission spectra from artificial atoms or quantum dots coupled to structured photon reservoirs and acoustic phonons, when excited with incoherent pump fields. As specific examples of structured reservoirs, we chose a Lorentzian cavity and a coupled cavity waveguide, which are of current experimental interest. For the case of optical cavities, we dir…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
Generating and detection coherent high-frequency heat-carrying phonons has been a great topic of interest in recent years. While there have been successful attempts in generating and observing coherent phonons, rigorous techniques to characterize and detect these phonon coherence in a crystalline material have been lagging compared to what has been achieved for photons. One main challenge is a lack of detailed understanding of how detection signals for phonons can be related to coherence. The quantum theory of photoelectric detection has greatly advanced the ability to characterize photon cohe…
