The hyperuniformity concept provides a unified means to classify all perfect crystals, perfect quasicrystals, and exotic amorphous states of matter according to their capacity to suppress large-scale density fluctuations. While the classification of hyperuniform point configurations has received considerable attention, much less is known about the classification of hyperuniform heterogeneous two-phase media, which include composites, porous media, foams, cellular solids, colloidal suspensions and polymer blends. The purpose of this article is to begin such a program for certain two-dimensional models of hyperuniform two-phase media by ascertaining their local volume-fraction variances $σ^2_{_V}(R)$ and the associated hyperuniformity order metrics $\overline{B}_V$. This is a highly challenging task because the geometries and topologies of the phases are generally much richer and more complex than point-configuration arrangements and one must ascertain a broadly applicable length scale to make key quantities dimensionless. Therefore, we focus on a certain class of two-dimensional periodic cellular networks, periodic and disordered/irregular packings, some of which maximize their effective transport and elastic properties. Among the cellular networks considered, the honeycomb networks have a minimal value of $\overline{B}_V$ across all volume fractions. On the other hand, among all packings considered, the triangular-lattice packings have the smallest values of $\overline{B}_V$ for the possible range of volume fractions. Among all structures studied here, the triangular-lattice packing has the minimal order metric for almost all volume fractions. Our study provides a theoretical foundation for the establishment of hyperuniformity order metrics for general two-phase media and a basis to discover new hyperuniform two-phase systems by inverse design procedures.
Disordered hyperuniform systems are exotic states of matter that completely suppress large-scale density fluctuations like crystals, and yet possess no Bragg peaks similar to liquids or glasses. Such systems have been discovered in a variety of equilibrium and non-equilibrium physical and biological systems, and are often endowed with novel physical properties. The mechanisms associated with the emergence of disordered hyperuniformity in nonequilibrium systems, in particular inherent structures are often not well understood, which we will address from a topological perspective in this work. Sp…
Disordered hyperuniformity is a description of hidden correlations in point distributions revealed by an anomalous suppression in fluctuations of local density at various coarse-graining length scales. In the absorbing phase of models exhibiting an active-absorbing state transition, this suppression extends up to a hyperuniform length scale that diverges at the critical point. Here, we demonstrate the existence of additional many-body correlations beyond hyperuniformity. These correlations are hidden in the higher moments of the probability distribution of the local density, and extend up to a…
Carbon nanotubes are quasi-one-dimensional systems that possess superior transport, mechanical, optical, and chemical properties. In this work, we generalize the notion of disorder hyperuniformity, a recently discovered exotic state of matter with hidden long-range order, to quasi-one-dimensional materials. As a proof of concept, we then apply the generalized framework to quantify the density fluctuations in amorphous carbon nanotubes containing randomly distributed Stone-Wales defects. We demonstrate that all of these amorphous nanotubes are hyperuniform, i.e., the infinite-wavelength density…
Disordered and hyperuniform structures of densely packed spheres near and at jamming are characterized by vanishing of long-wavelength density fluctuations, or equivalently by long-range power-law decay of the direct correlation function (DCF). We focus on previous simulation results that exhibit degradation of hyperuniformity in jammed structures while maintaining the long-range nature of the DCF to a certain length scale. Here we demonstrate that a field-theoretic formulation of the stochastic density functional theory is relevant to explore the degradation mechanism. The strong-coupling exp…
The recently developed concept of spreadability, $\mathcal{S}(t)$, provides a direct link between time-dependent diffusive transport and the microstructure of two-phase media across length scales. We explicitly compute $\mathcal{S}(t)$ for well-known two-dimensional and three-dimensional model structures, including nonhyperuniform fully penetrable spheres and equilibrium hard spheres, as well as hyperuniform sphere packings derived from perfect glasses, uniformly randomized lattices (URL), disordered stealthy point processes and Bravais lattices. We further confirm that the small-, intermediat…
Disordered hyperuniformity (DHU) is a recently discovered novel state of many-body systems that is characterized by vanishing normalized infinite-wavelength density fluctuations similar to a perfect crystal, yet possesses an amorphous structure like a liquid or glass. Here we investigate equilibrium DHU states of Brownian particles induced by external potentials. In particular, we analytically derive sufficient conditions on the external potentials in order to achieve distinct classes of DHU density distributions of Brownian particles in thermal equilibrium, based on the stationary-state solut…
We investigate numerically and theoretically the precursory intermittent activity characterizing the preliminary phase of damage accumulation prior to failure of quasi-brittle solids. We use a minimal but thermodynamically consistent model of damage growth and localization developed by Berthier et al. (2017). The approach accounts for both microstructural disorder and non-local interactions and permits inferring a complete scaling description of the spatio-temporal structure of failure precursors. By developing a theoretical model of damage growth in disordered elasto-damageable specimen, we d…
