We consider interaction of counter-propagating waves in a bi-directionally pumped ring microresonator with Kerr nonlinearity. We introduce a hierarchy of the mode expansions and envelope functions evolving on different time scales set by the cavity linewidth and nonlinearity, dispersion, and repetition rate, and provide a detailed derivation of the corresponding hierarchy of the coupled mode and of the Lugiato-Lefever-like equations. An effect of the washout of the repetition rate frequencies from the equations governing dynamics of the counter-propagating waves is elaborated in details.
Collimated directional emission is essentially required an asymmetric resonant cavity. In this paper, we theoretically investigate a type of peanut-shaped microcavity which can support highly directional emission with the emission divergence as small as 2.5o. The mechanism of the collimated emission is explained with the short-term ray trajectory and the intuitive lens model in detail. Wave simulation also confirms these results. This extremely narrow divergence of the emission holds a great potential in highly collimated lasing from on-chip microcavities.
The Kerr effect in optical microresonators plays an important role for integrated photonic devices and enables third harmonic generation, four-wave mixing, and the generation of microresonator-based frequency combs. Here we experimentally demonstrate that the Kerr nonlinearity can split ultra-high-Q microresonator resonances for two continuous-wave lasers. The resonance splitting is induced by self- and cross-phase modulation and counter-intuitively enables two lasers at different wavelengths to be simultaneously resonant in the same microresonator mode. We develop a pump-probe spectroscopy sc…
We use Maxwell's equations to derive several models describing the interaction of the multi-mode fundamental field and its second harmonic in a ring microresonator with quadratic nonlinearity and quasi-phase-matching. We demonstrate how multi-mode three-wave mixing sums entering nonlinear polarisation response can be calculated via Fourier transforms of products of the field envelopes. Quasi-phase-matching gratings with arbitrary profiles are incorporated seamlessly into our models. We also introduce several levels of approximations allowing to account for dispersion of nonlinear coefficients …
Whispering gallery mode (WGM) microresonators, benefitting from the ultrahigh quality (Q) factors and small mode volumes, could considerably enhance the light-matter interaction, making it an ideal platform for studying a broad range of nonlinear optical effects. In this review, the progress of optical nonlinear effects in WGM microresonators is comprehensively summarized. First, several basic nonlinear effects in WGM microresonator are reviewed, including not only Pockels effect and Kerr effect, but also harmonic generations, four-wave mixing and stimulated optical scattering effects. Apart f…
We investigate the single-photon transport problem in the system of a Whispering-Gallery mode microresonator directionally coupled with a two-level quantum emitter (QE). This QE-microresonator coupling system can usually be studied by cavity quantum electrodynamics and the single-photon transport methods. However, we find that if we treat a two-level QE as a single-photon phase-amplitude modulator, we can also deal with such systems using the transfer matrix method. Further, in theory, we prove that these three methods are equivalent. The corresponding relations of respective parameters among …
We numerically study, by means of the single envelope equation, the generation of optical frequency combs ranging from the visible to the mid-infrared spectral regions in resonators with quadratic and cubic nonlinearities. Phase-matched quadratic wave-mixing processes among the comb lines can be activated by low-power continuous wave pumping in the near infrared of a radially poled lithium niobate whispering gallery resonator (WGR). We examine both separate and co-existing intra-cavity doubly resonant second-harmonic generation and parametric oscillation processes, and find that modulation ins…
We present a theory of the frequency comb generation in the high-Q ring microresonators with quadratic nonlinearity and normal dispersion and demonstrate that the naturally large difference of the repetition rates at the fundamental and 2nd harmonic frequencies supports a family of the bright soliton frequency combs providing the parametric gain is moderated by tuning the index-matching parameter to exceed the repetition rate difference by a significant factor. This factor equals the sideband number associated with the high-order phase-matched sum-frequency process. The theoretical framework, …
Optical microresonators with high quality ($Q$) factors are essential to a wide range of integrated photonic devices. Steady efforts have been directed towards increasing microresonator $Q$ factors across a variety of platforms. With success in reducing microfabrication process-related optical loss as a limitation of $Q$, the ultimate attainable $Q$, as determined solely by the constituent microresonator material absorption, has come into focus. Here, we report measurements of the material-limited $Q$ factors in several photonic material platforms. High-$Q$ microresonators are fabricated from …
Microresonator frequency combs based on the $χ^{(3)}$ nonlinearity are nowadays well understood and making their way into different applications. Recently, microresonator frequency combs based on the $χ^{(2)}$ nonlinearity are receiving increasing attention, as they promise certain benefits, but still require further study. Here, we demonstrate the generation of a $χ^{(2)}$ frequency comb, initiated via optical parametric oscillation (OPO) in a lithium niobate mm-sized microresonator. By pumping at 532 nm with 30 $μ$W of power, we observe 1-THz-wide comb spectra around 1064 nm with degenerate …
Optical solitons are waveforms that preserve their shape while propagating, relying on a balance of dispersion and nonlinearity. Soliton-based data transmission schemes were investigated in the 1980s, promising to overcome the limitations imposed by dispersion of optical fibers. These approaches, however, were eventually abandoned in favor of wavelength-division multiplexing (WDM) schemes that are easier to implement and offer improved scalability to higher data rates. Here, we show that solitons may experience a comeback in optical communications, this time not as a competitor, but as a key e…
We describe the generation of stable mode-locked pulse trains from on-chip normal dispersion microresonators. The excitation of hyper-parametric oscillation is facilitated by the local dispersion disruptions induced by mode interactions. The system is then driven from hyper-parametric oscillation to the mode-locked state with over 200 nm spectral width by controlled pump power and detuning. With the continuous-wave driven nonlinearity, the pulses sit on a pedestal, akin to a cavity soliton. We identify the importance of pump detuning and wavelength-dependent quality factors in stabilizing and …
Herein, we report sub-wavelength propagation and directional out-coupling of whispering gallery modes (WGMs) of a fluorescent silica microsphere resonator mediated via plasmon polaritons in a single crystalline silver nanowire. Fluorescent spectral signatures of emission from the nanowire ends confirm efficient guiding of WGMs via nanowire plasmons. By employing Fourier plane optical microscopy, we reveal and quantify the directional fluorescence emission of WGMs from the ends of the nanowire. Given that the discussed geometry is self-assembled from a solution-phase, our results will find rele…
We demonstrate stable microresonator Kerr soliton frequency combs in a III-V platform (AlGaAs on SiO$_2$) through quenching of thermorefractive effects by cryogenic cooling to temperatures between 4~K and 20~K. This cooling reduces the resonator's thermorefractive coefficient, whose room-temperature value is an order of magnitude larger than that of other microcomb platforms like Si$_3$N$_4$, SiO$_2$, and AlN, by more than two orders of magnitude, and makes soliton states adiabatically accessible. Realizing such phase-stable soliton operation is critical for applications that fully exploit the…
Soliton microcombs based on Kerr nonlinearity in microresonators have been a prominent miniaturized coherent light source. Here, for the first time, we demonstrate the existence of Kerr solitons in an optomechanical microresonator, for which a nonlinear model is built by incorporating a single mechanical mode and multiple optical modes. Interestingly, an exotic vibrational Kerr soliton state is found, which is modulated by a self-sustained mechanical oscillation. Besides, the soliton provides extra mechanical gain through the optical spring effect, and results in phonon lasing with a red-detun…
Solitons occur in many physical systems when a nonlinearity compensates wave dispersion. Their recent formation in microresonators opens a new research direction for nonlinear optical physics and provides a platform for miniaturization of spectroscopy and frequency metrology systems. These microresonator solitons orbit around a closed waveguide path and produce a repetitive output pulse stream at a rate set by the round-trip time. In this work counter-propagating solitons that simultaneously orbit in an opposing sense (clockwise/counter-clockwise) are studied. Despite sharing the same spatial …
Dissipative temporal Kerr solitons in optical microresonators enable to convert a continuous wave laser into a train of femtosecond pulses. Of particular interest are single soliton states, whose $\mathrm{sech}^{2}$ spectral envelope provides a spectrally smooth and low noise optical frequency comb, and that recently have been generated in crystalline, silica, and silicon-nitride resonators. Here, we study the dynamics of multiple soliton states containing ${N}$ solitons and report the discovery of a novel, yet simple mechanism which makes it possible to reduce deterministically the number of …
We present measurements of silicon nitride nonlinear microresonators and frequency comb generation at cryogenic temperatures as low as 7~K. The resulting two orders of magnitude reduction in the thermo-refractive coefficient relative to room-temperature enables direct access to single bright Kerr soliton states through adiabatic frequency tuning of the pump laser while remaining in thermal equilibrium. Our experimental results, supported by theoretical modeling, show that single solitons are easily accessible at temperatures below 60~K for the microresonator device under study. We further demo…
The repetition rate of a Kerr comb comprising a single soliton in an anomalous dispersion silicon nitride microcavity is measured as a function of pump frequency tuning. The contributions from the Raman soliton self-frequency shift (SSFS) and from thermal effects are evaluated both experimentally and theoretically; the SSFS is found to dominate the changes in repetition rate. The relationship between the changes in repetition rate and pump frequency detuning is found to be independent of the nonlinearity coefficient and dispersion of the cavity. Modeling of the repetition rate change by using …
We demonstrate fully crystalline, single-mode ultrahigh quality factor integrated microresonators comprising epitaxially grown Si$_{0.86}$Ge$_{0.14}$ waveguide cores with silicon claddings. These waveguides support resonances with internal $Q >10^8$ for both polarization modes, a nearly order-of-magnitude improvement over that seen in prior integrated Si photonics platforms. The maximum $Q$ is $1.71\pm0.06 \times 10^8$ for the transverse magnetic (TM) polarization mode, corresponding to a loss of $0.39\pm0.02$ dB/m. Together with silicon's strong Kerr nonlinearity and low losses in the optical…
The transportation of photons and phonons typically obeys the principle of reciprocity. Breaking reciprocity of these bosonic excitations will enable the corresponding non-reciprocal devices, such as isolators and circulators. Here, we use two optical modes and two mechanical modes in a microresonator to form a four-mode plaquette via radiation pressure force. The phase-controlled non-reciprocal routing between any two modes with completely different frequencies is demonstrated, including the routing of phonon to phonon (MHz to MHz), photon to phonon (THz to MHz), and especially photon to phot…
We consider a high-Q microresonator with $χ^{(2)}$ nonlinearity under conditions when the coupling rates between the sidebands around the pump and second harmonic exceed the damping rates, implying the strong coupling regime (SC). Using the dressed-resonator approach we demonstrate that this regime leads to the dominance of the Hermitian part of the operator driving the side-band dynamics over its non-Hermitian part responsible for the parametric gain. This has allowed us to introduce and apply the cross-area concept of the polariton quasi-particles and define their effective masses in the con…
We address the problem of directional mobility of discrete solitons in two-dimensional rectangular lattices, in the framework of a discrete nonlinear Schrödinger model with saturable on-site nonlinearity. A numerical constrained Newton-Raphson method is used to calculate two-dimensional Peierls-Nabarro energy surfaces, which describe a pseudopotential landscape for the slow mobility of coherent localized excitations, corresponding to continuous phase-space trajectories passing close to stationary modes. Investigating the two-parameter space of the model through independent variations of the no…
I derive unidirectional wave equations for fields propagating in materials with both electric and magnetic dispersion and nonlinearity. The derivation imposes no conditions on the pulse profile except that the material modulates the propagation slowly, that is, that loss, dispersion, and nonlinearity have only a small effect over the scale of a wavelength. It also allows a direct term-to-term comparison of the exact bidirectional theory with its approximate unidirectional counterpart.
In materials that do not allow birefringent phase-matching or periodic poling we propose to use waveguides to exploit the tensor structure of the second order nonlinearity for quasi-phase matching of nonlinear interactions. In particular, we concentrate on curved waveguides in which the interplay between the propagation direction, electric field polarizations and the nonlinearity can change the strength and sign of the nonlinear interaction periodically to achieve quasi-phase matching.
We produce transmission and reflection spectra of the anti-directional coupler (ADC) composed of linearly-coupled positive- and negative-refractive-index arms, with intrinsic Kerr nonlinearity. Both reflection and transmission feature two highly amplified peaks at two distinct wavelengths in a certain range of values of the gain, making it possible to design a wavelength-selective mode-amplification system. We also predict that a blend of gain and loss in suitable proportions can robustly enhance reflection spectra which are detrimentally affected by the attenuation, in addition to causing red…
Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have triggered major advances in optical frequency metrology and precision measurements and in applications such as broadband laser-based gas sensing8 and molecular fingerprinting. Early work generated frequency combs by intra-cavity phase modulation while to date frequency combs are generated utilizing the comb-like mode structure of mode-locked lasers, whose repetiti…
The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically-poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second harmonic conversion efficiency---almost 20-fold enhancement over the state-of-the-art---by accessing its largest $χ^{(2)}$ tensor component $d_{33}$ via quasi-phase matching. The corresponding single photon coupling rate $g/2π$ is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rat…
The Kerr nonlinearity can be a key enabler for many digital photonic circuits as it allows access to bistable states needed for all-optical memories and switches. A common technique is to use the Kerr shift to control the resonance frequency of a resonator and use it as a bistable, optically-tunable filter. However, this approach works only in a narrow power and frequency range or requires the use of an auxiliary laser. An alternative approach is to use the asymmetric bistability between counterpropagating light states resulting from the interplay between self- and cross-phase modulation, whic…
I calculate the limitations on the widely-used forward-only (uni-directional) propagation assumption by considering the effects of transverse effects (e.g. diffraction). The starting point is the scalar second order wave equation, and simple predictions are made which aim to clarify the forward-backward coupling limits on diffraction strength. The result is unsurprising, being based on the ratio of transverse and total wave vectors, but the intent is to present a derivation directly comparable to a recently published \emph{nonlinearity} constrained limits on the uni-directional approximation […
Microresonator Kerr frequency combs, which rely on third-order nonlinearity ($χ^{(3)}$), are of great interest for a wide range of applications including optical clocks, pulse shaping, spectroscopy, telecommunications, light detection and ranging (LiDAR) and quantum information processing. Many of these applications require further spectral and temporal control of the generated frequency comb signal, which is typically accomplished using additional photonic elements with strong second-order nonlinearity ($χ^{(2)}$). To date these functionalities have largely been implemented as discrete off-ch…
Solitons, ubiquitous in nonlinear sciences, are wavepackets which maintain their characteristic shape upon propagation. In optics, they have been observed and extensively studied in optical fibers. The spontaneous generation of a dissipative Kerr soliton (DKS) train in an optical microresonator pumped with continuous wave (CW) coherent light has placed solitons at the heart of optical frequency comb research in recent years. The commonly observed soliton has a ``sech''-shaped envelope resulting from resonator cubic nonlinearity balanced by its quadratic anomalous group velocity dispersion (GVD…
Stimulated Brillouin interaction between sound and light, known to be the strongest optical nonlinearity common to all amorphous and crystalline dielectrics, has been widely studied in fibers and bulk materials but rarely in optical microresonators. The possibility of experimentally extending this principle to excite mechanical resonances in photonic microsystems, for sensing and frequency reference applications, has remained largely unexplored. The challenge lies in the fact that microresonators inherently have large free spectral range, while the phase matching considerations for the Brillou…
Bridging high-Q and Kerr-nonlinear photonics using modal phase matching
National Institute for Standards and Technology（国家标准与技术研究院）；Whiting School of Engineering, Johns Hopkins University（约翰斯·霍普金斯大学惠廷工程学院）；Beacon Photonics（灯塔光子学）；Joint Quantum Institute, NIST/University of Maryland（NIST/马里兰大学联合量子研究所）
Advances in microresonator-based soliton generation promise chip-scale integration of optical frequency comb for applications spanning from time keeping to frequency synthesis. Miniaturized cavities harness Kerr nonlinearity and enable terahertz soliton repetition rates. However, such high repetition rates are not amenable to direct electronic detection. Here, we demonstrate hybrid Kerr and electro-optic microcombs using the lithium niobate thin film that exhibits both Kerr and Pockels nonlinearities. By interleaving the high-repetition-rate Kerr soliton comb with the low-repetition-rate elect…
The influence of a saturable nonlinearity on the modulation instability in oppositely directed coupler in the presence of high-order effects is investigated. By using the standard linear stability analysis, we obtain the instability gain that exhibits a significant change in the bands of instability due to the effects of a saturable nonlinearity. We also show that even in the presence of saturation there is no change in instability gain when we compare the results obtained for both channels not influenced by self-steepening effect or for both channels influenced by self-steepening effect but o…
Spontaneous symmetry breaking is an important concept in many areas of physics. A fundamentally simple symmetry breaking mechanism in electrodynamics occurs between counter-propagating electromagnetic waves in ring resonators, mediated by the Kerr nonlinearity. The interaction of counter-propagating light in bi-directionally pumped microresonators finds application in the realisation of optical non-reciprocity (for optical diodes), studies of PT-symmetric systems, and the generation of counter-propagating solitons. Here, we present comprehensive analytical and dynamical models for the nonlinea…
Optical microresonators with low quality factor ($Q$) can be efficiently excited by and scatter freely propagating optical waves, but those with high $Q$ typically cannot. Here, we present a universal model for resonators interacting with freely propagating waves and show that the stored energy of a resonator excited by a plane wave is proportional to the product of its $Q$ and directivity. Guided by this result, we devise a microdisk with periodic protrusions in its circumference that couples efficiently to normally incident plane waves. We experimentally demonstrate several microdisk designs…
We report the observation of a parametric instability in the out-of-equilibrium steady state of two coupled Kerr microresonators coherently driven by a laser. Using a resonant excitation, we drive the system into an unstable regime, where we observe the appearance of intense and well resolved sideband modes in the emission spectrum. This feature is a characteristic signature of self-sustained oscillations of the intracavity field. We comprehensively model our findings using semiclassical Langevin equations for the cavity field dynamics combined with a linear stability analysis. The inherent sc…
We theoretically investigate the solitary waves and their switching dynamics in a $\mathcal{PT}$-symmetric directional fiber coupler, exhibiting Kerr nonlinearity, by developing a variational analysis. We analyze the fundamental switching characteristics of the $\mathcal{PT}$-symmetric Kerr coupler in the picosecond timescale by considering the coupled-mode equation for the unperturbed nonlinear Schrödinger equation, which we compare to its conventional counterpart. The impacts of higher-order perturbations (intrapulse Raman scattering, self-steepening, and third-order dispersion) are investig…
We derive a general theory of linear coupling and Kerr nonlinear coupling between modes of dielectric optical resonators from first principles. The treatment is not specific to a particular geometry or choice of mode basis, and can therefore be used as a foundation for describing any phenomenon resulting from any combination of linear coupling, scattering and Kerr nonlinearity, such as bending and surface roughness losses, geometric backscattering, self- and cross-phase modulation, four-wave mixing, third-harmonic generation and Kerr frequency comb generation. The theory is then applied to a t…
Light is generally expected to travel through isotropic media independent of its direction. This makes it challenging to develop non-reciprocal optical elements like optical diodes or circulators, which currently rely on magneto-optical effects and birefringent materials. Here we present measurements of non-reciprocal transmission and spontaneous symmetry breaking between counter-propagating light in dielectric microresonators. The symmetry breaking corresponds to a resonance frequency splitting that allows only one of two counter-propagating (but otherwise identical) light waves to circulate …
Dissipative Kerr solitons are self-organized optical waves arising from the interplay between Kerr effect and dispersion. They can form spontaneously in nonlinear microresonators pumped with an external continuous-wave laser, which provides the parametric gain for the proliferation of an ultrastable frequency comb. These miniaturized and battery driven microcombs have become a disruptive technology for precision metrology, broadband telecommunication and ultrafast optical ranging. In this work, we report on the first experimental observation of dissipative Kerr solitons generated in a ring cav…
