The amount of entanglement that exists in a parametric down-converted state is investigated in terms of all the degrees of freedom of the state. We quantify the amount of entanglement by the Schmidt number of the state, represented as a pure bipartite state by tagging the down-converted photons in terms of orthogonal states of polarization with the aid of type II phase-matching. To facilitate our calculations, we use a Wigner functional approach, which allows the incorporation of the full infinite dimensional spatiotemporal degrees of freedom. A quantitative example with reasonably achievable experimental conditions is considered to demonstrate that extremely large Schmidt numbers are achievable.
We numerically and experimentally show that all photons generated by spontaneous parametric down-conversion (SPDC) follow a transverse amplitude similar to that of the pump. This amplitude transfer from pump to SPDC is revealed in the Fourier image plane of the down-converted photons restricted by an aperture. We also observe a considerable shift of the image plane from the actual Fourier plane, when size of the aperture is gradually increased. The shift of the Fourier image of down-converted photons affects the quality of spatial mode-based projection in various quantum correlation experiment…
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
Degenerate optomechanical parametric oscillators are optical resonators in which a mechanical degree of freedom is coupled to a cavity mode that is nonlinearly amplified via parametric down-conversion of an external pumping laser. Below a critical pumping power the down-converted field is purely quantum-mechanical, making the theoretical description of such systems very challenging. Here we introduce a theoretical approach that is capable of describing this regime, even at the critical point itself. We find that the down-converted field can induce significant mechanical cooling and identify th…
We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields gives the signatures of a rich dynamic of multipa…
In this article we investigate the orbital angular momentum spectrum of photons produced in parametric down conversion process. We study how the transverse profile of the pump mode affects the spectrum as compared to a gaussian pump beam. We show that using perfect optical vortex mode as pump the spectrum can be highly narrowed down. We further study the entanglement between the two down converted photons in the orbital angular momentum basis. We observe that photons entangled in Laguerre-Gaussian modes exhibit greater higher dimensional entanglement.
Creation of correlated photon pairs is one of the key topics in contemporary quantum optics. Here, we theoretically describe the generation of photon pairs in the process of spontaneous parametric down-conversion in a resonant spherical nanoparticle made of a dielectric material with bulk $χ^{(2)}$ nonlinearity. We pick the nanoparticle size that satisfies the condition of resonant eigenmodes described by Mie theory. We reveal that highly directional photon-pair generation can be observed utilising the nonlinear Kerker-type effect, and that this regime provides useful polarisation correlations…
We report the efficient generation of high-gain parametric down-conversion, including pump depletion, with pump powers as low as 100 $μ$W (energies $0.1$~$μ$J/pulse) and conversion efficiencies up to 33\%. In our simple configuration, the pump beam is tightly focused into a bulk periodically poled lithium niobate crystal placed in free space. We also observe a change in the photon number statistics for both the pump and down-converted beams as the pump power increases to reach the depleted pump regime. The experimental results are a clear signature of the interplay between the pump and the dow…
A detailed analysis of the stimulated parametric down-conversion (PDC) process is performed to investigate the effects of the spatiotemporal degrees of freedom. The analysis provides information that would be useful for PDC-based metrology applications. Using a Wigner functional approach, we obtain the parametric down-converted state as the Bogoliubov transformed input state, in terms of Bogoliubov kernel functions. The result is used to consider the case for a coherent state seeding stimulated PDC. We also compute the background which is obtained from spontaneous PDC.
We show that in parametric down-conversion the coherence properties of a temporally partially coherent pump field get entirely transferred to the down-converted entangled two-photon field. Under the assumption that the frequency-bandwidth of the down-converted signal-idler photons is much larger than that of the pump, we derive the temporal coherence functions for the down-converted field, for both infinitely-fast and time-averaged detection schemes. We show that in each scheme the coherence function factorizes into two separate coherence functions with one of them carrying the entire statisti…
In this work, we provide a means to quantify genuine tripartite entanglement in arbitrary (pure and mixed) continuous-variable states as measured by the Tripartite Entanglement of formation -- a resource-based measure quantifying genuine multi-partite entanglement in units of elementary Greenberger-Horne-Zeilinger (GHZ) states called gebits. Furthermore, we predict its effectiveness in quantifying the tripartite spatial and energy-time entanglement in photon triplets generated in cascaded spontaneous parametric down-conversion (SPDC), and find that ordinary nonlinear optics can be a substantia…
We study polarization effects in the nonlinear interference of photons generated via frequency non-degenerate spontaneous parametric down conversion. Signal and idler photons generated in the visible and infrared (IR) range, are split in different arms of a nonlinear Michelson interferometer. The interference pattern for signal photons is detected, and it is shown to be dependent on the polarization rotation of idler photons, introduced by a birefringent sample. Based on this concept, we realize two new methods for measurement of sample retardation in the IR range by using well-developed and i…
Spontaneous parametric down-conversion (SPDC) is widely used in quantum applications based on photonic entanglement. The efficiency of photon pair generation is often characterized by means of a $sinc(LΔk/2)$-function, where $L$ is the length of the nonlinear medium and $Δk$ the phase mismatch between the pump and down-converted fields. In theoretical investigations, the \textit{sinc} behavior of the phase mismatch has often been approximated by a Gaussian function $\exp{(-αx^2)}$ in order to derive analytical expressions for the SPDC process. Different values have been chosen in the literatur…
We present a novel yet simple approach to produced multiple entangled photon pairs through spontaneous parametric downconversion. We have developed Gaussian masks to subdivide the pump beam before passing it through a nonlinear medium. In this way, we are able to observe simultaneous separate down-converted emission cones with spatial overlap. The technique we employ can be used to greatly increase the dimensionality of entangled photonic systems generated from spontaneous parametric down conversion, affording greater scalability to optical quantum computing than previously explored.
We report on quantum frequency conversion of near-infrared photons from a wavelength of 854nm to the telecommunication O-band at 1310nm with 8% overall conversion efficiency. Entangled photon pairs at 854nm are generated via type-II spontaneous parametric down conversion. One photon is mixed with a strong pump field in a nonlinear ridge waveguide for its conversion to 1310nm. We demonstrate preservation of first and second order coherence of the photons in the conversion process. Based on this we infer the coherence function of the two-photon state and compare it with the actual measured one. …
We show how to reach high fidelity NOON states with a high count rate inside optical interferometers. Recently it has been shown that by mixing squeezed and coherent light at a beamsplitter it is possible to generate NOON states of arbitrary N with a fidelity as high as 94%. (Afek I. et al. Science 328, 879 (2010)). The scheme is based on higher order interference between "quantum" down-converted light and "classical" coherent light. However, this requires optimizing the amplitude ratio of classical to quantum light thereby limiting the overall count rate for the interferometric super-resoluti…
We present a scheme for engineering the joint spectrum of photon pairs created via spontaneous parametric down conversion. Our method relies on customizing the poling configuration of a quasi-phase-matched crystal. We use simulated annealing to find an optimized poling configuration which allows almost arbitrary shaping of the crystal's phase-matching function. This has direct application in the creation of pure single photons---currently one of the most important goals of single-photon quantum optics. We describe the general algorithm and provide code, written in C++, that outputs an optimize…
Recent advances in the development of modern quantum technologies have opened the possibility of studying the interplay between spontaneous parametric down-conversion and optomechanics, two of the most fundamental nonlinear optical processes. Apart from practical reasons, such scenario is very interesting from a fundamental point of view, because it allows exploring the optomechanical interaction in the presence of a strongly quantum-correlated field, the spontaneously down-converted mode. In this work we analyze such problem from two approximate but valuable perspectives: the classical limit …
We report on a new technique for entanglement distillation of the bipartite continuous variable state of spatially correlated photons generated in the spontaneous parametric down-conversion process (SPDC), where tunable non-Gaussian operations are implemented and the post-processed entanglement is certified in real-time using a single-photon sensitive electron multiplying CCD (EMCCD) camera. The local operations are performed using non-Gaussian filters modulated into a programmable spatial light modulator and, by using the EMCCD camera for actively recording the probability distributions of th…
As a tutorial, we examine the absolute brightness and number statistics of photon pairs generated in Spontaneous Parametric Down-Conversion (SPDC) from first principles. In doing so, we demonstrate how the diverse implementations of SPDC can be understood through a single common framework, and use this to derive straightforward formulas for the biphoton generation rate (pairs per second) in a variety of different circumstances. In particular, we consider the common cases of both collimated and focused gaussian pump beams in a bulk nonlinear crystal, as well as in nonlinear waveguides and micro…
Using the zero time-delay second-order correlation function for studying the photon statistics, we investigate how the photon statistics of the field-modes generated by parametric down-conversion (PDC) process depends on the photon statistics of the pump field-mode. We derive general expressions for the zero time-delay second-order correlation function of the down-converted field-modes for both multi-mode and single-mode PDC processes. We further study these expressions in the weak down-conversion limit. We show that for a two-photon two-mode PDC process, in which a pump photon splits into two…
Quantifying entanglement in a quantum system generally requires a complete quantum tomography followed by the NP-hard computation of an entanglement monotone --- requirements that rapidly become intractable at higher dimensions. Observing entanglement in large quantum systems has consequently been relegated to witnesses that only verify its existence. In this article, we show that the violation of recent entropic witnesses of the Einstein-Podolsky-Rosen paradox also provides tight lower bounds to multiple entanglement measures, such as the entanglement of formation and the distillable entangle…
Full-field mapping of spatially varying polarization entanglement generated from spontaneous parametric down-conversion
Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；University of Ottawa（渥太华大学）；Indian Institute of Technology Ropar（印度理工学院罗帕尔分校）；National Research Council（国家研究委员会）；Czech Technical University（捷克理工大学）；Florida International University（佛罗里达国际大学）；Institute for Quantum Studies, Chapman University（查普曼大学量子研究所）
Autocorrelation is a common method to estimate the duration of ultra-short laser pulses. In the ultra-violet (UV) regime it is increasingly challenging to employ the standard process of second harmonic generation, most prominently due to absorption in nonlinear crystals at very short wavelengths. Here we show how to utilize spontaneous parametric down-conversion (SPDC) to generate an autocorrelation signal for UV pulses in the infrared. Our method utilizes the $n^{\text{th}}$ order emission of the SPDC process, which occurs for low pumping powers proportional to the $n^{\text{th}}$ power of th…
Third order parametric down-conversion describes a class of nonlinear processes in which a pump photon can be down-converted into triplets of photons. It has been identified as a source of non-classical light, with capabilities beyond those offered by better-established processes such as spontaneous four-wave mixing. Here we discuss the implementation of TOPDC in integrated photonic systems. We derive equations for the rates of TOPDC in a non-resonant (waveguide) and resonant (microring) platform, such that the scaling with experimental parameters can be plainly seen. We find that generally no…
We show how to quantify tri-partite entanglement using entropies derived from experimental correlations. We use a multi-partite generalization of the entanglement of formation that is greater than zero if and only if the state is genuinely multi-partite entangled. We develop an entropic witness for tripartite entanglement, and show that the degree of violation of this witness places a lower limit on the tripartite entanglement of formation. We test our results in the three-qubit regime using the GHZ-Werner state and the W-Werner state, and in the high-dimensional pure-state regime using the tr…
