Creation of correlated photon pairs is one of the key topics in contemporary quantum optics. Here, we theoretically describe the generation of photon pairs in the process of spontaneous parametric down-conversion in a resonant spherical nanoparticle made of a dielectric material with bulk $χ^{(2)}$ nonlinearity. We pick the nanoparticle size that satisfies the condition of resonant eigenmodes described by Mie theory. We reveal that highly directional photon-pair generation can be observed utilising the nonlinear Kerker-type effect, and that this regime provides useful polarisation correlations.
We demonstrate a spectrally broadband and effcient technique for collecting photoluminescence from a single InAs quantum dot directly into a standard single mode optical fiber. In this approach, an optical fiber taper waveguide is placed in contact with a suspended GaAs nanophotonic waveguide with embedded quantum dots, forming an effcient and broadband directional coupler with standard optical fiber input and output. Effcient photoluminescence collection over a wavelength range of tens of nanometers is demonstrated, and a maximum collection effciency of 6.05 % (corresponding single photon rat…
We experimentally show how a single Ag nanoparticle (NP) coupled to an Ag nanowire (NW) can convert propagating surface plasmon polaritons to directional photons. By employing dual-excitation Fourier microscopy with spatially filtered collection-optics, we show single- and dual-directional out-coupling of light from NW-NP junction for plasmons excited through glass-substrate and air-superstrate. Furthermore, we show NW-NP junction can influence the directionality of molecular-fluorescence emission, thus functioning as an optical antenna. The results discussed herein may have implications in re…
Controlling the dispersion and directionality of the emission of nanosources is one of the major goals of nanophotonics research. This control will allow the development of highly efficient nanosources even at the single photon level. One of the ways to achieve this goal is to couple the emission to Bloch modes of periodic structures. Here, we present the first measurements of the directional emission from nanowire photonic crystals by using Fourier microscopy. With this technique we efficiently collect and resolve the directional emission of nanowires within the numerical aperture of a micros…
Directional light scattering by spherical silicon nanoparticles in the visible spectral range is experimentally demonstrated for the first time. These unique scattering properties arise due to simultaneous excitation and mutual interference of magnetic and electric dipole resonances inside a single nanosphere. Directivity of the far-field radiation pattern can be controlled by changing light wavelength and the nanoparticle size. Forward-to-backward scattering ratio above 6 can be experimentally obtained at visible wavelengths. These unique properties of silicon nanoparticles make them promisin…
We study the angular scattering properties of individual core-shell nanoparticles that support simultaneously both electric and optically-induced magnetic resonances of different orders. In contrast to the approach to suppress the backward scattering and enhance the forward scattering relying on overlapping electric and magnetic dipoles, we reveal that the directionality of the forward scattering can be further improved through the interferences of higher order electric and magnetic modes. Since the major contributing electric and magnetic responses can be tuned to close magnitudes, ultra-dire…
An important source of innovation in nanophotonics is the idea to scale down known radio wave technologies to the optical regime. One thoroughly investigated example of this approach are metallic nanoantennas which employ plasmonic resonances to couple localized emitters to selected far-field modes. While metals can be treated as perfect conductors in the microwave regime, their response becomes Drude-like at optical frequencies. Thus, plasmonic nanoantennas are inherently lossy. Moreover, their resonant nature requires precise control of the antenna geometry. A promising way to circumvent the…
Controlling directional emission of nanophotonic radiation sources is fundamental to tailor radiation-matter interaction and to conceive highly efficient nanophotonic devices for on-chip wireless communication and information processing. Nanoantennas coupled to quantum emitters have proven to be very efficient radiation routers, while electrical control of unidirectional emission has been achieved through inelastic tunneling of electrons. Here we prove that the radiation emitted from the interaction of a high-energy electron beam with a graphene-nanoparticle composite has beaming directions wh…
In this paper, we describe the implementation of leakage radiation microscopy (LRM) to probe the chirality of plasmonic nanostructures. We demonstrate experimentally spin-driven directional coupling as well as vortex generation of surface plasmon polaritons (SPPs) by nanostructures built with T-shaped and $Λ$- shaped apertures. Using this far-field method, quantitative inspections, including directivity and extinction ratio measurements, are achieved via polarization analysis in both image and Fourier planes. To support our experimental findings, we develop an analytical model based on a multi…
We report on spiking dynamics of frequency up-converted emission at 420 nm generated on the 6P3/2-5S1/2 transition in Rb vapour two-photon excited to the 5D5/2 level with laser light at 780 and 776 nm. The spike duration is less than the natural lifetime of any excited level involved in the interaction with both continuous and pulsed pump radiation. The spikes at 420 nm are attributed to temporal properties of the directional emission at 5.23 μm generated on the population inverted 5D5/2-6P3/2 transition. A link between the spiking regime and cooperative effects is discussed. We suggest that t…
Controlling directionality of optical emitters is of utmost importance for their application in communication and biosensing devices. Metallic nanoantennas have been proven to affect both excitation and emission properties of nearby emitters, including directionality of their emission. In this regard, optical directional nanoantennas based on a Yagi-Uda design have been demonstrated in the visible range. Despite this impressive proof of concept, their overall size and considerable number of elements represent obstacles for the exploitation of these antennas in nanophotonic applications and for…
A structure based on a dimer of silicon nanoparticles, presenting directional scattering in the visible range, was studied as a new design of an all-optical switch. The combination of spherical nanoparticles satisfying, at the same incident wavelength, the zero-backward and the minimum-forward scattering conditions, can produce either a maximum or a minimum of the scattered field in the area between the nanoparticles. The modulation of the incident wavelength can be used as switching parameter, due to the sensitivity of these conditions to it. An optimization of the dimer setup, both in the di…
Optical surface waves, highly localized modes bound to the surface of media, enable manipulation of light at nanoscale, thus impacting a wide range of areas in nanoscience. By applying metamaterials, artificially designed optical materials, as contacting media at the interface, we can significantly ameliorate surface wave propagation and even generate new types of waves. Here, we demonstrate that high aspect ratio (1:20) grating structures with plasmonic lamellas in deep nanoscale trenches function as a versatile platform supporting both surface and volume infrared waves. The surface waves exh…
Influencing spectral and directional features of exciton emission characteristics from 2D transition metal dichalcogenides by coupling it to plasmonic nano-cavities has emerged as an important prospect in nanophotonics of 2D materials. In this paper we experimentally study the directional photoluminescence emission from Tungsten disulfide (WS2) monolayer sandwiched between a single-crystalline plasmonic silver nanowire (AgNW) waveguide and a gold (Au) mirror, thus forming an AgNW-WS2-Au cavity. By employing polarization-resolved Fourier plane optical microscopy, we quantify the directional emi…
We report on the experimental observation of mirror enhanced directional surface enhanced Raman scattering (SERS) from a self-assembled monolayer of molecules coupled to a nanowire-nanoparticle (NW-NP) junction on a mirror in remote excitation configuration. Placing NW-NP junction on a metallic mirror generates multiple gap plasmon modes which have unique momentum space scattering signatures. We perform Fourier plane imaging of SERS from NW-NP on a mirror to understand the effect of multiple hotspots on molecular emission. We systematically study the effect of ground plane on the directionalit…
The resonant modes observed in semiconductor nanoparticles and the coherence interaction between them, producing directional light scattering, may be very interesting for CMOS integrated all-optical devices. In these systems the control over the light scattering should be crucial, as well as the strength of this control. Fabrication parameters such as the size and shape of the nanoparticles and the optical properties of the environment can strongly affect to the emergence of these phenomena. In this work, we numerically explore the size dependence of the directional scattering conditions of se…
A fundamental building block in nano-photonics is the ability to directionally excite highly squeezed optical mode dynamically, particularly with an electrical bias. Such capabilities would enable the active manipulation of light propagation for information processing and transfer. However, when the optical source is built-in, it remains challenging to steer the excitation directionality in a flexible way. Here, we reveal a novel mechanism for tunable directional excitation of highly squeezed polaritons in graphene-hexagonal boron nitride (hBN) heterostructures. The effect relies on controllin…
Chiral emission, where the handedness of a transition dipole determines the direction in which a photon is emitted, has recently been observed from atoms and quantum dots coupled to nanophotonic waveguides. Here, we consider the case of chiral light-matter interactions in resonant nanophotonic structures, deriving closed-form expressions for the fundamental quantum electrodynamic quantities that describe these interactions. We show how parameters such as the position dependent, directional Purcell factors and mode volume can be calculated using computationally efficient two dimensional eigenmo…
The strong electric and magnetic resonances in dielectric subwavelength structures have enabled unique opportunities for efficient manipulation of light-matter interactions. Besides, the dramatic enhancement of nonlinear light-matter interactions near so-called bound states in the continuum (BICs) has recently attracted enormous attention due to potential advancements in all-optical and quantum computing. However, the experimental realizations and the applications of high- Q factor resonances in dielectric resonances in the visible regime have thus far been considerably limited. In this work, …
We demonstrate that an array of optical antennas may render a thin layer of randomly oriented semiconductor nanocrystals into an enhanced and highly directional source of polarized light. The array sustains collective plasmonic lattice resonances which are in spectral overlap with the emission of the nanocrystals over narrow angular regions. Consequently, different photon energies of visible light are enhanced and beamed into definite directions.
Controlling light emission from quantum emitters has important applications ranging from solid-state lighting and displays to nanoscale single-photon sources. Optical antennas have emerged as promising tools to achieve such control right at the location of the emitter, without the need for bulky, external optics. Semiconductor nanoantennas are particularly practical for this purpose because simple geometries, such as wires and spheres, support multiple, degenerate optical resonances. Here, we start by modifying Mie scattering theory developed for plane wave illumination to describe scattering …
Angstrom precision localization of a single nanoantenna is a crucial step towards advanced nanometrology, medicine and biophysics. Here, we show that single nanoantenna displacements down to few Angstroms can be resolved with sub-Angstrom precision using an all-optical method. We utilize the tranverse Kerker scattering scheme where a carefully structured light beam excites a combination of multipolar modes inside a dielectric nanoantenna, which then upon interference, scatters directionally into the far-field. We spectrally tune our scheme such that it is most sensitive to the change in direct…
Efficient photon-pair emission from a nanostructured resonator and its theoretical description
Friedrich-Alexander-Universität Erlangen-Nürnberg（埃尔朗根-纽伦堡弗里德里希·亚历山大大学）；INRiM（意大利国家计量研究院）；Politecnico di Milano（米兰理工大学）；Max Planck Institute for the Science of Light（马克斯·普朗克光科学研究所）；University of Brescia（布雷西亚大学）；Istituto Italiano di Tecnologia（意大利理工学院）
Deterministic GHz-rate single photon sources at room-temperature would be essential components for various quantum applications. However, both the slow intrinsic decay rate and the omnidirectional emission of typical quantum emitters are two obstacles towards achieving such a goal which are hard to overcome simultaneously. Here we solve this challenge by a hybrid approach, using a complex monolithic photonic resonator constructed of a gold nanocone responsible for the rate enhancement, and a circular Bragg antenna for emission directionality. A repeatable process accurately binds quantum dots …
Directional lasing, with a low threshold and high quality factor, in active dielectric nanoantenna arrays is demonstrated. This is achieved through a leaky resonance excited in coupled gallium arsenide (GaAs) nanopillars. The leaky resonance is formed by partially breaking a bound state in the continuum (BIC) generated by the collective, vertical electric dipole resonances excited in the nanopillars for sub-diffractive arrays. By opening an unprotected, diffractive channel along one of the periods of the array one can control the directionality of the emitted light without sacrificing the high…
We design and fabricate an on-chip laser source that produces a directional beam with low spatial coherence. The lasing modes are based on the axial orbit in a stable cavity and have good directionality. To reduce the spatial coherence of emission, the number of transverse lasing modes is maximized by fine-tuning the cavity geometry. Decoherence is reached in a few nanoseconds. Such rapid decoherence will facilitate applications in ultrafast speckle-free full-field imaging.
We experimentally demonstrate plasmonic nano-circuits operating as sub-diffraction directional couplers optically excited with high efficiency from free-space using optical Yagi-Uda style antennas at λ= 1550 nm. The optical Yagi-Uda style antennas are designed to feed channel plasmon waveguides with high efficiency (45 % in coupling, 60 % total emission), narrow angular directivity (< 40°) and low insertion loss. SPP gap waveguides exhibit propagation lengths as large as 34 μm with adiabatically tuned confinement, and are integrated with ultra-compact (5 μm x 10 μm), highly dispersive directio…
We report the design of highly efficient optical antennas employing a judicious synthesis of metallic and dielectric materials. In the proposed scheme, a pair of metallic coupled nanoparticles permits large enhancements in both excitation strength and radiative decay rates, while a high refractive index dielectric microsphere is employed to efficiently collect light without spoiling the emitter quantum efficiency. Our simulations indicate potential fluorescence rate enhancements of 3 orders of magnitude over the entire optical frequency range.
Designing directional optical antennas without compromising the field enhancement requires specially designed optical cavities. Herein, we report on the experimental observations of directional photoluminescence emission from a monolayer Tungsten Disulfide using a bent-plasmonic nanowire on a mirror cavity. The geometry provides field enhancement and directivity to photoluminescence by sandwiching the monolayer between an extended cavity formed by dropcasting bent silver nanowire and a gold mirror. We image the photoluminescence emission wavevectors by using the Fourier plane imaging technique…
Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In addition to this, the molecules excite multiple guided modes of the nanowire which were imaged using leakage radiation Fourier microscopy. We further characterize the emission wavevectors as a function of output polarization. The excited guided modes of the wire show interesting polarization signatures. All the results were corroborated using finite element…
In this manuscript, we demonstrate the design and experimental proof of an optical cloaking structure which multi-directionally conceals a perfectly electric conductor (PEC) object from an incident plane wave. The dielectric modulation around the highly reflective scattering PEC object is determined by an optimization process for multi-directional cloaking purposes. And to obtain the multi-directional effect of the cloaking structure, an optimized slice is mirror symmetrized through a radial perimeter. Three-dimensional (3D) finite-difference time-domain method is integrated with genetic optim…
Herein, we report sub-wavelength propagation and directional out-coupling of whispering gallery modes (WGMs) of a fluorescent silica microsphere resonator mediated via plasmon polaritons in a single crystalline silver nanowire. Fluorescent spectral signatures of emission from the nanowire ends confirm efficient guiding of WGMs via nanowire plasmons. By employing Fourier plane optical microscopy, we reveal and quantify the directional fluorescence emission of WGMs from the ends of the nanowire. Given that the discussed geometry is self-assembled from a solution-phase, our results will find rele…
Rapid development of Fabry-Perot quantum cascade laser frequency combs has converted them from laboratory devices to key components of next-generation fast molecular spectrometers. Recently, free-running ring quantum cascade lasers allowed generation of new frequency comb states induced by phase turbulence. In absence of efficient light outcoupling, ring quantum cascade lasers are not suited for applications as they are limited in their power output to microwatt levels. Here we demonstrate electrically pumped ring quantum cascade lasers with integrated active directional couplers. These device…
