Efficient manipulation of the emission direction of a chiral nanoscale light source is significant for information transmission and on-chip information processing. Here, we propose a scheme to control the directionality of nanoscale chiral light sources based on gap plasmons. The gap plasmon mode formed by a gold nanorod and a silver nanowire realizes the highly directional emission of chiral light sources. Based on the optical spin-locked light propagation, the hybrid structure enables the directional coupling of chiral emission to achieve a contrast ratio of 99.5%. The emission direction can be manipulated by tailoring the configuration of the structure, such as the positions, aspect ratios, and orientation of the nanorod. Besides, a great local field enhancement exists for highly enhanced emission rates within the nanogap. This chiral nanoscale light source manipulation scheme provides a way for chiral valleytronics and integrated photonics.
Observation of surface-plasmon phenomena that are dependent upon the handedness of the circularly polarized incident light (spin) is presented. The polarization-dependent near-field intensity distribution obtained in our experiment is attributed to the presence of a geometric phase arising from the interaction of light with an anisotropic and inhomogeneous nanoscale structure. A near-field vortex surface mode with a spin-dependent topological charge was obtained in a plasmonic microcavity. The remarkable phenomenon of polarization-sensitive focusing in a plasmonic structure was also demonstrat…
Focusing electromagnetic energy to sub-wavelength dimensions has become an increasingly active field of research for a variety of applications such as Heat Assisted Magnetic Recording (HAMR), nanolithography, and nanoscale optical characterization of biological cells and single molecules using near-field scanning optical microscopy (NSOM) technique. Double-sided surface plasmons in a metal-insulator-metal (MIM) geometry have been shown to have very small wavelengths for dielectric of thickness of less than 10 nm. A tapered dielectric structure sandwiched between metal, can be used to efficient…
To enable multiple functions of plasmonic nanocircuits, it is of key importance to control the propagation properties and the modal distribution of the guided optical modes such that their impedance matches to that of nearby quantum systems and desired light-matter interaction can be achieved. Here, we present efficient mode converters for manipulating guided modes on a plasmonic two-wire transmission line. The mode conversion is achieved through varying the path length, wire cross section and the surrounding index of refraction. Instead of pure optical interference, strong near-field coupling…
The research area of plasmonics promises devices with ultrasmall footprint operating at ultrafast speeds and with lower energy consumption compared to conventional electronics. These devices will operate with light and bridge the gap between microscale dielectric photonic systems and nanoscale electronics. Recent research advancements in nanotechnology and optics have led to the creation of a plethora of new plasmonic designs. Among the most promising are nanoscale antennas operating at optical frequencies, called nanoantennas. Plasmonic nanoantennas can provide enhanced and controllable light…
We experimentally show how a single Ag nanoparticle (NP) coupled to an Ag nanowire (NW) can convert propagating surface plasmon polaritons to directional photons. By employing dual-excitation Fourier microscopy with spatially filtered collection-optics, we show single- and dual-directional out-coupling of light from NW-NP junction for plasmons excited through glass-substrate and air-superstrate. Furthermore, we show NW-NP junction can influence the directionality of molecular-fluorescence emission, thus functioning as an optical antenna. The results discussed herein may have implications in re…
Controlling the directionality of surface plasmon polaritons (SPPs) has been widely studied, while the direction of SPPs was always switched by orthogonal polarizations in the reported methods. Here, we present a scheme to control the directionality of SPPs by arbitrary spin polarizations. Extremely, the device can split two quite adjacent polarization components to two opposite directions. The versatility of the presented design scheme can offer opportunities for polarization sensing, polarization splitting and polarization-controlled plasmonic devices.
The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic p…
Surface plasmon polaritons have attracted varies of interests due to its special properties, especially in the polarization-controlled devices. Typically, the polarization-controlled devices include directional coupling, focusing lens and plasmonic vortex lens, and almost all of them are controlled by the input circularly polarized light or the linearly polarized light. We present a novel device that realize the functions of directional coupling and focusing with high polarization extinction ratio for arbitrary spin of input light. This device offers opportunities for polarization sensing, pol…
Infrared spectroscopy, especially for molecular vibrations in the fingerprint region between 600 and 1500 cm-1, is a powerful characterization method for bulk materials. However, molecular fingerprinting at the nanoscale level still remains a significant challenge, due to weak light-matter interaction between micron-wavelengthed infrared light and nano-sized molecules. Here, we demonstrate molecular fingerprinting at the nanoscale level using our specially designed graphene plasmonic structure on CaF2 nanofilm. This structure not only avoids the plasmon-phonon hybridization, but also provides …
We theoretically propose directional, low-threshold plasmon lasing in both the near-infrared and visible wavelengths by utilizing spatially coherent surface plasmon polaritons on a meta-surface. The gain strength required for threshold lasing can be tuned down to a large extent through compatible structural parameters. Our calculations show that no more than 65 cm$^{-1}$ at 193.5 THz (1.55 $μ$m) or 267 cm$^{-1}$at 474THz (0.633 $μ$m) of gain coefficient is sufficient to compensate for the dissipation of metal films for threshold lasing; these values are smaller than any reported studies at the…
As any physical object, light undergoing a circular trajectory features a constant extrinsic angular momentum. Within strong curvatures, this angular momentum can match the spin momentum of a photon, thus providing the opportunity of a strong spin-orbit interaction. Using this effect, we demonstrate tunable symmetry breaking in the coupling of light in a curved nanoscale plasmonic waveguide. The helicity of the impinging optical wave controls the power distribution between the two counter-propagating guided modes, including unidirectional waveguiding. We found that up to 95 % of the incoupled …
Open quantum systems consisting of coupled bound and continuum states have been studied in a variety of physical systems, particularly within the scope of nuclear, atomic and molecular physics. In the open systems, the effects of the continuum decay channels are accounted for by indirect non-Hermitian couplings among the quasi-bound states. Here we explore anti-Hermitian coupling in a plasmonic system for spatially manipulating light on the nano-scale. We show that by utilizing the anti-Hermitian coupling, plasmonic antennas closely packed within only λ/15 separations can be individually excit…
We develop a self-consistent finite element method to study spontaneous emission at nanoscale proximity of plasmonic waveguides. In the model, it is assumed that only one guided mode is dominatingly excited by the quantum emitter. With such one dominating mode assumption, the cross section of the plasmonic waveguide can be arbitrary. We apply our numerical method to calculate the coupling of a quantum emitter to a cylindrical nanowire and a rectangular waveguide, and compare the cylindrical nanowire to previous work valid in quasistatic approximation. The fraction of the energy coupled to the …
In this paper, we describe the implementation of leakage radiation microscopy (LRM) to probe the chirality of plasmonic nanostructures. We demonstrate experimentally spin-driven directional coupling as well as vortex generation of surface plasmon polaritons (SPPs) by nanostructures built with T-shaped and $Λ$- shaped apertures. Using this far-field method, quantitative inspections, including directivity and extinction ratio measurements, are achieved via polarization analysis in both image and Fourier planes. To support our experimental findings, we develop an analytical model based on a multi…
We demonstrate that an array of optical antennas may render a thin layer of randomly oriented semiconductor nanocrystals into an enhanced and highly directional source of polarized light. The array sustains collective plasmonic lattice resonances which are in spectral overlap with the emission of the nanocrystals over narrow angular regions. Consequently, different photon energies of visible light are enhanced and beamed into definite directions.
Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an analyte-induced modification of the dielectric properties of the medium surrounding the nanoparticle or an increase of the excitation and emission rates of an optically active analyte by the resonantly enhanced plasmon field. Either way, besides the nanoparticle geometry the dielectric properties of the metal and nanoscale surface roughness play an important role fo…
We show that a stack of metal-dielectric nanolayers, in addition to the long- and short-range plasmons, guides also an entire family of modes strongly confined within the multilayer - the bulk plasmon modes. We propose the classification scheme that reflects specific properties of these modes. We report experimental verification of the bulk plasmon modes by measuring modal indices in a structure made of three pairs of silica(29nm)/gold(25nm) layers.
This chapter discusses a hydrodynamics-inspired approach to trap and manipulate light in plasmonic nanostructures, which is based on steering optical powerflow around nano-obstacles. New insights into plasmonic nanofocusing mechanisms are obtained by invoking an analogy of the 'photon fluid' (PF). By proper nanostructure design, PF kinetic energy can be locally increased via convective acceleration and then converted into 'pressure' energy to generate localized areas of high field intensity. In particular, trapped light can be molded into optical vortices -tornado-like areas of circular motion…
In this study, we investigate plasmon-induced transparency (PIT) in a resonator structure consisting of two orthogonally-arranged metal-insulator-metal (MIM) nanocavities with the aim of spectral modulation of a specific resonant order of the resonator. Our FDTD simulations demonstrate that when both cavities in this structure resonate at the same frequency, the PIT effect can be used to induce spectral modulation. This spectral modulation depends on the resonance order of the cavity coupled directly to the external field, occurring when first-order resonance is exhibited, but not with second-…
Surface plasmon polariton is collective oscillation of the free electrons at metal dielectric interface. As a wave phenomenon, surface plasmon polaritons can be focused using appropriate excitation geometry of metallic structures. We theoretically demonstrate the possibility of controlling nanoscale short pulse superfocusing based on the generation of radially polarized surface plasmon polariton mode of conical metallic tip. Numerical simulation for femtosecond pulse propagation along a silver nano-needle is discussed. The spatial distribution for a near field strongly depends on a linear chir…
We propose a scheme to directionally couple light into graphene plasmons by placing a graphene sheet on a magneto-optical substrate. When a magnetic field is applied parallel to the surface, the graphene plasmon dispersion relation becomes asymmetric in the forward and backward directions. It is possible to achieve unidirectional excitation of graphene plasmons with normally incident illumination by applying a grating to the substrate. The directionality can be actively controlled by electrically gating the graphene, or by varying the magnetic bias. This scheme may have applications in graphen…
Surface plasmon polaritons (SPPs) have been widely exploited in various scientific communities, ranging from physics, chemistry to biology, due to the strong confinement of light to the metal surface. For many applications it is important that the free space photon can be coupled to SPPs in a controllable manner. In this Letter, we apply the concept of interfacial phase discontinuity for circularly polarizations on a metasurface to the design of a novel type of polarization dependent SPP unidirectional excitation at normal incidence. Selective unidirectional excitation of SPPs along opposite d…
Optical control of electronic properties is essential for future electric devices. Manipulating such properties has been limited to the microscale in spatial volume due to the wave nature of light; however, scaling down the volume is in extremely high demand. In this study, we demonstrate optical switching within a nanometric spatial volume in an organic electric material. Photochromic materials such as diarylethene derivatives exhibit semiconducting and insulating properties on ultraviolet (UV) and visible light, respectively, which are promising for optical switching and memory. To control t…
Plasmon-emitter interactions are of paramount importance in modern nanoplasmonics and are generally maximal at short emitter-surface separations. However, when the separation falls below 10-20 nm, the classical theory progressively deteriorates due to its neglect of quantum mechanical effects such as nonlocality, electronic spill-out, and Landau damping. Here, we show how this neglect can be remedied by presenting a unified theoretical treatment of mesoscopic electrodynamics grounded on the framework of Feibelman $d$-parameters. Crucially, our technique naturally incorporates nonclassical reso…
Simultaneous spatio-temporal confinement of energetic electron pulses to femtosecond and nanometer scales is a topic of great interest in the scientific community, given the potential impact of such development on a wide spectrum of scientific and industrial applications. For example, in ultrafast electron scattering, nanoscale probes would enable accurate maps of structural dynamics in materials with nanoscale heterogeneity, thereby understanding the role of boundaries and defects on macroscopic properties. On the other hand, advances in this field are mostly limited by the electron source br…
We investigate electromagnetic scattering and plasmonic cloaking in a system composed by a dielectric cylinder coated with a magneto-optical shell. In the long-wavelength limit we demonstrate that the application of an external magnetic field can not only switch on and off the cloaking mechanism but also mitigate losses, as the absorption cross-section is shown to be minimal precisely at the cloaking operation frequency band. We also show that the angular distribution of the scattered radiation can be effectively controlled by applying an external magnetic field, allowing for a swift change in…
Plasmon nanoantennas are extensively used with molecular systems for the chemical and biological ultra-sensing, for boosting the molecular emissive and energy transfer properties, for the nanoscale catalysis, and for building advanced hybrid nanoarchitectures. In this Perspective we focus on the latest developments of using plasmon nanoantennas for the nanoscale chiral chemistry and for advancing the molecular magnetism. We overview the decisive role nanoplasmonics and nano-optics can play in achieving the chirally-selective molecular synthesis and separation, and in the way such processes mig…
Electrically-driven optical antennas can serve as compact sources of electromagnetic radiation operating at optical frequencies. In the most widely explored configurations, the radiation is generated by electrons tunneling between metallic parts of the structure when a bias voltage is applied across the tunneling gap. Rather than relying on an inherently inefficient inelastic light emission in the gap, we suggest to use a ballistic nanoconstriction as the feed element of an optical antenna supporting plasmonic modes. We discuss the underlying mechanisms responsible for the optical emission, an…
Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale visualization of polaritons has remained an open challenge. Here, we demonstrate that plasmon-exciton polaritons, or plexcitons, generated by a hybrid system composed of an individual silver nanoparticle and a few-layer transition metal dichalcogenide can be spectroscopically mapped with nanometer spatial resolution using electron energy loss spectroscopy in …
Efficient delivery of light into nanoscale volumes by converting free photons into localized charge-density oscillations (surface plasmons) enables technological innovation in various fields from biosensing to photovoltaics and quantum computing. Conventional plasmonic nanostructures are designed as nanoscale analogs of radioantennas and waveguides. Here, we discuss an alternative approach for plasmonic nanocircuit engineering that is based on molding the optical powerflow through 'vortex nanogears' around a landscape of local phase singularities 'pinned' to plasmonic nanostructures. We show t…
We propose a plasmon-based reconfigurable antenna to controllably distribute emission from single quantum emitters in spatially separated channels. Our calculations show that crossed particle arrays can split the stream of photons from a single emitter into multiple narrow beams. We predict that beams can be switched on and off by switching host refractive index. The design method is based on engineering the dispersion relations of plasmon chains and is generally applicable to traveling wave antennas. Controllable photon delivery has potential applications in classical and quantum communicatio…
Ultrafast all-optical control of spins with femtosecond laser pulses is one of the hot topics at the crossroads of photonics and magnetism with a direct impact on future magnetic recording. Unveiling light-assisted recording mechanisms for an increase of the bit density beyond the diffraction limit without excessive heating of the recording medium is an open challenge. Here we show that surface plasmon-polaritons in hybrid metal-dielectric structures can provide spatial confinement of the inverse Faraday effect, mediating the excitation of localized coherent spin precession with 0.41 THz frequ…
High-order optical vortices are inherently unstable, as they tend to split up under perturbation to a series of vortices with unity charge. Control over the perturbation opens up a new degree of freedom to control and tune their location in a 2D-space, with immediate implications on trapping, light-matter interactions and super-resolution imaging. Here, we present a continuous nano-scale tuning of the spatial location of plasmonic vortices on metal-air interface achieved by varying the polarization state of the light coupled to the surface plasmons through a spiral slit. We demonstrate such a …
The emergence of two-dimensional transition metal chalcogenide materials has sparked an intense activity in valleytronics since their valley information can be directly encoded and detected by using the spin angular momentum of light. For their practical applications such as on-chip valley logic gates and chip-to-chip valley transport, the encoding and processing of valley pseudospin using light should be extended to an integrated, on-chip nanophotonic system. Here, we successfully demonstrate, at room temperature, the valley-dependent directional coupling of light using a plasmonic nanowire-W…
Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial dependence of the strong coupling on various properties of the cavity and emitter, as well as the subwavelength scale of the interaction. In this work, we develop a methodology for obtaining hybrid nanostructures consisting of plasmonic metasurfaces coupled to atomically thin WS2 layers, exhibiting extreme values of Rabi splitting, by inverse design of the ne…
Optical polaritons appear when a material excitation strongly couples to the optical mode. Such strong coupling between molecular transitions and optical cavities results in far-reaching opportunities in modifying fundamental properties of chemical matter. More recently an exciting prospect of cavity-free polaritons has emerged by matter sustaining the optical mode with its geometry. Here we show how strong coupling of the interband transition and surface plasmons can be engineered in nickel at the nanoscale to realize cavity-free optical polaritons inside metals. Using electron energy-loss sp…
Optical computing uses photons as information carriers, opening up the possibility for ultrahigh-speed and ultrawide-band information processing. Integrated all-optical logic devices are indispensible core components of optical computing systems. However, up to now, little experimental progress has been made in nanoscale all-optical logic discriminators, which have the function of discriminating and encoding incident light signals according to wavelength. Here, we report a strategy to realize a nanoscale all-optical logic discriminator based on plasmonic bandgap engineering in a planar plasmon…
We propose and demonstrate a new approach for achieving strong light-matter interactions with quantum emitters. Our approach makes use of a plasmon resonator composed of defect-free, highly crystalline silver nanowires surrounded by patterned dielectric distributed Bragg reflectors (DBRs). These resonators have an effective mode volume (Veff) two orders of magnitude below the diffraction limit and quality factor (Q) approaching 100, enabling enhancement of spontaneous emission rates by a factor exceeding 75 at the cavity resonance. We also show that these resonators can be used to convert a br…
Nanoscale pulsed light is highly desirable in nano-integrated optics. In this letter, we obtained femtosecond pulses with THz repetition frequency via the strong coupling between quantum emitters (QEs) and plasmonic resonators. Our structure consists of a V-groove (VG) plasmonic resonator and a nanowire embedded with two-level QEs. The influences of the incident light intensity and QE number density on the transmission response for this hybrid system are investigated through semi-classical theory and simulation. It is found that the transmission response can be modulated to the pulse form. The…
Controlling directional emission of nanophotonic radiation sources is fundamental to tailor radiation-matter interaction and to conceive highly efficient nanophotonic devices for on-chip wireless communication and information processing. Nanoantennas coupled to quantum emitters have proven to be very efficient radiation routers, while electrical control of unidirectional emission has been achieved through inelastic tunneling of electrons. Here we prove that the radiation emitted from the interaction of a high-energy electron beam with a graphene-nanoparticle composite has beaming directions wh…
Influencing spectral and directional features of exciton emission characteristics from 2D transition metal dichalcogenides by coupling it to plasmonic nano-cavities has emerged as an important prospect in nanophotonics of 2D materials. In this paper we experimentally study the directional photoluminescence emission from Tungsten disulfide (WS2) monolayer sandwiched between a single-crystalline plasmonic silver nanowire (AgNW) waveguide and a gold (Au) mirror, thus forming an AgNW-WS2-Au cavity. By employing polarization-resolved Fourier plane optical microscopy, we quantify the directional emi…
Efficient manipulation and long distance transport of single-photons is a key component in nanoscale quantum optics. In this letter, we study the emission properties of an individual light emitter placed into a nanofiber and coupled to a metallic nanoparticle. We find that plasmonic field enhancement together with the nanofiber optical confinement uniquely and synergistically contribute to an overall increase of emission rates as well as quantum yields.
Research on graphene has revealed its unique optical properties, including strong coupling with light, high-speed operation, and gate-variable optical conductivity, which promise to satisfy the needs of future electro-optic (EO) modulators. In particular, recent work demonstrated a broadband EO modulator based on the interband absorption of graphene with overall length only 40μm. However, compared with the size of on-chip electronic components it is still bulky. On-chip optical interconnects require EO modulation at the nanoscale. The key to achieve nanoscale graphene EO modulation is to great…
We present an optical investigation of surface plasmon polaritons propagating along nanoscale Au-wires, lithographically defined on GaAs substrates. A two-axis confocal microscope was used to perform spatially and polarization resolved measurements in order to confirm the guiding of surface plasmon polaritons over lengths ranging from $5-20 μm$ along nanowires with a lateral dimension of only $\approx 100 nm$. Finite difference time domain simulations are used to corroborate our experimental observations and highlight the potential to couple proximal quantum dot emitters to propagating plasmon…
Strong light-matter interactions in both the single-emitter and collective strong coupling regimes attract significant attention due to emerging quantum and nonlinear optics applications, as well as opportunities for modifying material-related properties. Further exploration of these phenomena requires an appropriate theoretical methodology, which is demanding since polaritons are at the intersection between quantum optics, solid state physics and quantum chemistry. Fortunately, however, nanoscale polaritons can be realized in small plasmon-molecule systems, which in principle allows treating …
Experimental approaches to manipulate light-matter interaction at nanoscale have quickly advanced in recent years, leading to the demonstration of spaser (surface plasmon amplification by stimulated emission of radiation) in plasmonic nanocavities. Yet, a well-understood analytical theory to better understand and quantitatively explain the connotation of spaser system is urgently needed. Here we develop an all-analytical semiclassical theory to investigate the energy exchange between active materials and fields and the spaser performance in a plasmonic nanocavity. The theory can be commonly us…
We theoretically investigate the spontaneous emission process of an optical, dipolar emitter in metal-dielectric-metal slab and slot waveguide structures. We find that both structures exhibit strong off-resonant emission enhancements due to the tight confinement of modes between two metallic plates. The large enhancement of surface plasmon-polariton excitation enables dipole emission to be preferentially coupled into plasmon waveguide modes. These structures find applications in creating nanoscale local light sources or in generating guided single plasmons in integrated optical circuits.
Plasmonic waveguides are key elements in nanophotonic devices serving as optical interconnects between nanoscale light sources and detectors. Multimode operation in plasmonic two-wire transmission lines promises important degrees of freedom for near-field manipulation and information encoding. However, highly confined plasmon propagation in gold nanostructures is typically limited to the near-infrared region due to ohmic losses, excluding all visible quantum emitters from plasmonic circuitry. Here, we report on top-down fabrication of complex plasmonic nanostructures in single-crystalline silv…
Directional Dark Field for Nanoscale Full-Field Transmission X-Ray Microscopy
Helmholtz-Zentrum Hereon（赫姆霍兹海雷恩中心）；Technical University of Munich（慕尼黑工业大学）；Paul Scherrer Institut（保罗谢尔研究所）；ShanghaiTech University（上海科技大学）；Hamburg University of Technology（汉堡工业大学）；Deutsches Elektronen-Synchrotron DESY（德国电子同步加速器）；Fraunhofer IAPT（弗劳恩霍夫应用聚合物研究 institute）；Medical University of Vienna（维也纳医科大学）；Austrian Cluster for Tissue Regeneration（奥地利组织再生集群）
