High-order optical vortices are inherently unstable, as they tend to split up under perturbation to a series of vortices with unity charge. Control over the perturbation opens up a new degree of freedom to control and tune their location in a 2D-space, with immediate implications on trapping, light-matter interactions and super-resolution imaging. Here, we present a continuous nano-scale tuning of the spatial location of plasmonic vortices on metal-air interface achieved by varying the polarization state of the light coupled to the surface plasmons through a spiral slit. We demonstrate such a control at nano-scale resolution using phase-resolved near-field microscopy.
We study paraxial beam propagation parallel to the screw axis of a dislocated amorphous medium that is optically weakly inhomogeneous and isotropic. The effect of the screw dislocation on the beam's orbital angular momentum is shown to change the optical vortex strength, rendering vortex annihilation or generation possible. Furthermore, the dislocation is shown to induce a weak \textit{biaxial} anisotropy in the medium due to the elasto-optic effect, which changes the beam's spin angular momentum as well as causing precession of the polarization. We derive the equations of motion of the beam a…
Here we demonstrate that giant transverse optical forces can be generated in nanoscale slot waveguides of hyperbolic metamaterials, with more than two orders of magnitude stronger compared to the force created in conventional silicon slot waveguides, due to the nanoscale optical field enhancement and the extreme optical energy compression within the air slot region. Both numerical simulation and analytical treatment are carried out to study the dependence of the optical forces on the waveguide geometries and the metamaterial permittivity tensors, including the attractive optical forces for the…
Nanoscale slot waveguides of hyperbolic metamaterials are proposed and demonstrated for achieving large optical field enhancement. The dependence of the enhanced electric field within the air slot on waveguide mode coupling and permittivity tensors of hyperbolic metamaterials is analyzed both numerically and analytically. Optical intensity in the metamaterial slot waveguide can be more than 25 times stronger than that in a conventional silicon slot waveguide, due to tight optical mode confinement enabled by the ultrahigh refractive indices supported in hyperbolic metamaterials. The electric fi…
The study of optical phenomena on the subwavelength scale is becoming increasingly important in photonics, particularly in the fields of nanoemitters, photonic crystals and plasmonics. Subwavelength field patterns are evanescent and must thus be investigated with near-field techniques. The light powers emitted by nanoscale sources are extremely low, undermining the traditional approach of scattering a near field to a large (thus noisy) far-field detector. Nanoscale detectors, providing direct sensing in the near-field with small noise due to a small active area, are needed in high-sensitivity,…
As any physical object, light undergoing a circular trajectory features a constant extrinsic angular momentum. Within strong curvatures, this angular momentum can match the spin momentum of a photon, thus providing the opportunity of a strong spin-orbit interaction. Using this effect, we demonstrate tunable symmetry breaking in the coupling of light in a curved nanoscale plasmonic waveguide. The helicity of the impinging optical wave controls the power distribution between the two counter-propagating guided modes, including unidirectional waveguiding. We found that up to 95 % of the incoupled …
To enable multiple functions of plasmonic nanocircuits, it is of key importance to control the propagation properties and the modal distribution of the guided optical modes such that their impedance matches to that of nearby quantum systems and desired light-matter interaction can be achieved. Here, we present efficient mode converters for manipulating guided modes on a plasmonic two-wire transmission line. The mode conversion is achieved through varying the path length, wire cross section and the surrounding index of refraction. Instead of pure optical interference, strong near-field coupling…
Optical response of artificial composite nanoscale molecules comprising a closely spaced noble metal nanoparticle and a semiconductor quantum dot have been studied theoretically. We consider a system composed of an Au particle and CdSe or CdSe/ZnSe quantum dot and predict optical bistability and hysteresis in its response, which suggests various applications, in particular, all-optical processing and optical memory.
It is shown theoretically that an optical bottle resonator with a nanoscale radius variation can perform a multi-nanosecond long dispersionless delay of light in a nanometer-order bandwidth with minimal losses. Experimentally, a 3 mm long resonator with a 2.8 nm deep semi-parabolic radius variation is fabricated from a 19 micron radius silica fiber with a sub-angstrom precision. In excellent agreement with theory, the resonator exhibits the impedance-matched 2.58 ns (3 bytes) delay of 100 ps pulses with 0.44 dB/ns intrinsic loss. This is a miniature slow light delay line with the record large …
Recently introduced Surface Nanoscale Axial Photonics (SNAP) makes it possible to fabricate high Q-factor microresonators and other photonic microdevices by dramatically small deformation of the optical fiber surface. To become a practical and robust technology, the SNAP platform requires methods enabling reproducible modification of the optical fiber radius at nanoscale. In this Letter, we demonstrate super-accurate fabrication of high Q-factor microresonators by nanoscale modification of the optical fiber radius and refractive index using the CO2 laser and the UV excimer laser beam exposures…
We demonstrate the measurement of laterally induced optical forces using an Atomic Force Microscope (AFM). The lateral electric field distribution between a gold coated AFM probe and a nano-aperture in a gold film is mapped by measuring the lateral optical force between the apex of the AFM probe and the nano-aperture. Torsional eigenmodes of an AFM cantilever probe were used to detect the laterally induced optical forces. We engineered the cantilever shape using a focused ion beam to enhance the torsional eigenmode resonance. The measured lateral optical force agrees well with simulations. Thi…
On-chip photonic networks have the potential to transmit and route information more efficiently than electronic circuits. Recently, a number of silicon-based optical devices including modulators, buffers, and wavelength converts have been reported. However, a number of technical challenges need to be overcome before these devices can be combined into network-level architectures. In particular, due to the high refractive index contrast between the core and cladding of semiconductor waveguides, nanoscale defects along the waveguide often scatter light into the backward-propagating mode. These re…
We propose a design concept for tailoring the local density of optical states (LDOS) in dielectric nanostructures, based on the phase distribution of the scattered optical fields induced by point-like emitters. First we demonstrate that the LDOS can be expressed in terms of a coherent summation of constructive and destructive contributions. By using an iterative approach, dielectric nanostructures can be designed to effectively remove the destructive terms. In this way dielectric Mie resonators, featuring low LDOS for electric dipoles, can be reshaped to enable enhancements of three orders of …
We experimentally demonstrate series of identical two, three, and five coupled high Q-factor Surface Nanoscale Axial Photonics (SNAP) microresonators formed by periodic nanoscale variation of the optical fiber radius. These microresonators are fabricated with a 100 \mum period along an 18 \mum radius optical fiber. The axial FWHM of these microresonators is 80 \mum and their Q-factor exceeds 107. In addition, we demonstrate a SNAP microresonator with the axial FWHM as small as 30 \mum and the axial FWHM of the fundamental mode as small as 10 \mum. These results may potentially enable the dense…
Optical beams carrying orbital angular momentum (OAM) can find tremendous applications in several fields. In order to apply these particular beams in photonic integrated devices innovative optical elements have been proposed. Here we are interested in the generation of OAM-carrying beams at the nanoscale level. We design and experimentally demonstrate a plasmonic optical vortex emitter, based on a metal-insulator-metal holey plasmonic vortex lens. Our plasmonic element is shown to convert impinging circularly polarized light to an orbital angular momentum state capable of propagating to the fa…
While the thermal and electromagnetic properties of plasmonic nanostructures are well understood, nanoscale thermometry still presents an experimental and theoretical challenge. Plasmonic structures can confine electromagnetic energy at the nanoscale, resulting in local, inhomogeneous, controllable heating. But reading out the temperature with nanoscale precision using optical techniques poses a difficult challenge. Here we report on the optical thermometry of individual gold nanorod trimers that exhibit multiple wavelength-dependent plasmon modes resulting in measurably different local temper…
This chapter discusses a hydrodynamics-inspired approach to trap and manipulate light in plasmonic nanostructures, which is based on steering optical powerflow around nano-obstacles. New insights into plasmonic nanofocusing mechanisms are obtained by invoking an analogy of the 'photon fluid' (PF). By proper nanostructure design, PF kinetic energy can be locally increased via convective acceleration and then converted into 'pressure' energy to generate localized areas of high field intensity. In particular, trapped light can be molded into optical vortices -tornado-like areas of circular motion…
The emergence of two-dimensional transition metal chalcogenide materials has sparked an intense activity in valleytronics since their valley information can be directly encoded and detected by using the spin angular momentum of light. For their practical applications such as on-chip valley logic gates and chip-to-chip valley transport, the encoding and processing of valley pseudospin using light should be extended to an integrated, on-chip nanophotonic system. Here, we successfully demonstrate, at room temperature, the valley-dependent directional coupling of light using a plasmonic nanowire-W…
We propose deep-subwavelength optical waveguides based on metal-dielectric multilayer indefinite metamaterials with ultrahigh effective refractive indices. Waveguide modes with different mode orders are systematically analyzed with numerical simulations based on both metal-dielectric multilayer structures and the effective medium approach. The dependences of waveguide mode indices, propagation lengths and mode areas on different mode orders, free space wavelengths and sizes of waveguide cross sections are studied. Furthermore, waveguide modes are also illustrated with iso-frequency contours in…
Precise control and manipulation of optical fields on a nanoscale is one of the most important and challenging problems in "nanophotonics". Since optical wavelength is on a much larger microscale, it is impossible to employ conventional focusing for that purpose. We show the strong optically-induced interactions between discrete meta-molecules in a metamaterial system and coherent monochromatic continuous light beam with a spatially-tailored phase profile can be used to prepare a sub-wavelength scale energy localization. Well isolated energy hot-spots as small as $λ/10$ can be created and posi…
Fabricating nanocavities in which optically-active single quantum emitters are precisely positioned, is crucial for building nanophotonic devices. Here we show that self-assembly based on robust DNA-origami constructs can precisely position single molecules laterally within sub-5nm gaps between plasmonic substrates that support intense optical confinement. By placing single-molecules at the center of a nanocavity, we show modification of the plasmon cavity resonance before and after bleaching the chromophore, and obtain enhancements of $\geq4\times10^3$ with high quantum yield ($\geq50$%). By …
A light beam with phase singularity (PS) characterized with azimuthally symmetric angular positions (APs) can be constructed by the rotationally symmetric superposition of n (n is N) fractional vortex light beams with identical charges. The profile of this light beam deforms after propagation owing to its orbital angular momentum (OAM) noneigenvalue, and the deformation degree can be evaluated by the degree of phase dislocation associated with the PS. The expectation value of the mean deviation of its OAM from its characteristic charge value and the variation of the degree of phase dislocation…
Recent progress in nanotechnology has enabled us to fabricate subwavelength architectures that function as antennas for improving the exchange of optical energy with nanoscale matter. We describe the main features of optical antennas for enhancing quantum emitters and review designs that increase the spontaneous emission rate by orders of magnitude from the ultraviolet up to the near-infrared spectral range. To further explore how optical antennas may lead to unprecedented regimes of light-matter interaction, we draw a relationship between metal nanoparticles, radio-wave antennas and optical r…
By applying the optical nanocircuit concepts to metasurfaces, we propose an effective route to locally control light transmission over a deeply subwavelength scale. This concept realizes the optical equivalent of a transmitarray, whose use is demonstrated for light bending and focusing with unprecedented efficiency over a subwavelength distance, with crucial benefits for nano-optics applications. These findings may lead to large improvements in the manipulation of optical transmission and processing of nanoscale optical signals over conformal and Si-compatible substrates.
We study theoretically and experimentally the process of Brillouin light scattering on an array of silicon disks on a thin Permalloy layer. We show that phase-resolved Brillouin light scattering microscopy performed on an array of weakly interacting dielectric nanoresonators can detect nanoscale waves and measure their dispersion. In our experiment, we were able to map the evolution of the phase of the spin wave with a wavelength of 209 nm with a precision of 6 nm. These results demonstrate the feasibility of all-optical phase-resolved characterization of nanoscale spin waves.
Employing plasmonic antennas for subdiffraction focusing of light on recording media requires to take into account the complete structure of the medium, including dielectric cover layers. We find, with finite difference time domain simulations, that optical energy transfer to the magnetic recording layer is most efficient for an off-resonant antenna. Furthermore, we show that the focal spot in the magnetic film is well below the diffraction limit, making nanoscale all-optical magnetic data recording achievable.
Strong-field photoemission from metal nanostructures enabled fundamental discoveries recently. Here, we deliver theoretical demonstration of the electric field control of electrons in the closest nanoscale vicinity of plasmonic nanoparticles with the help of few-cycle laser waveforms. We analyze the effect of plasmonic resonance on photoemission properties and show that it is only off-resonant nanoparticles that can provide electron control on a true sub-fs timescale.
Optical control of electronic properties is essential for future electric devices. Manipulating such properties has been limited to the microscale in spatial volume due to the wave nature of light; however, scaling down the volume is in extremely high demand. In this study, we demonstrate optical switching within a nanometric spatial volume in an organic electric material. Photochromic materials such as diarylethene derivatives exhibit semiconducting and insulating properties on ultraviolet (UV) and visible light, respectively, which are promising for optical switching and memory. To control t…
Optical polaritons appear when a material excitation strongly couples to the optical mode. Such strong coupling between molecular transitions and optical cavities results in far-reaching opportunities in modifying fundamental properties of chemical matter. More recently an exciting prospect of cavity-free polaritons has emerged by matter sustaining the optical mode with its geometry. Here we show how strong coupling of the interband transition and surface plasmons can be engineered in nickel at the nanoscale to realize cavity-free optical polaritons inside metals. Using electron energy-loss sp…
The plasma membrane of living cells is compartmentalized at multiple spatial scales ranging from the nano- to the meso-scale. This non-random organization is crucial for a large number of cellular functions. At the nanoscale, cell membranes organize into dynamic nano-assemblies enriched by cholesterol, sphingolipids and certain types of proteins. Investigating these nano-assemblies known as lipid rafts is of paramount interest in fundamental cell biology. However, this goal requires simultaneous nanometer spatial precision and microsecond temporal resolution which is beyond the reach of common…
Optical dielectric resonances have the ability to modulate optical energy, and by coupling multiple resonators into photonic molecules, new opportunities emerge in spectral engineering. Using electron-beam spectroscopy, in a 300-keV scanning transmission electron microscope, we probe optical modes of photonic molecules at the nanometer scale. Monochromated electron energy-loss spectra of 400nm-silica-sphere monomers, dimers and trimers display series of sharp peaks in the ultraviolet region. For monomers, the peaks are assigned to low angular number optical whispering gallery modes. For dimers…
Relativistic electrons in a structured medium generate radiative losses such as Cherenkov and transition radiation that act as a virtual light source, coupling to the photonic densities of states. The effect is most pronounced when the imaginary part of the dielectric function is zero, a regime where in a non-retarded treatment no loss or coupling can occur. Maps of the resultant energy losses as a sub-5nm electron probe scans across finite waveguide structures reveal spatial distributions of optical modes in a spectral domain ranging from near-infrared to far ultraviolet.
Observation of linear and nonlinear light trapping on topological dislocations
Universidad de Valencia（瓦伦西亚大学）；Institute of Spectroscopy, Russian Academy of Sciences（俄罗斯科学院光谱学研究所）；Moscow Institute of Physics and Technology (National Research University)（莫斯科物理技术学院（国立研究型大学））；Quantum Technology Centre, Faculty of Physics, M. V. Lomonosov Moscow State University（莫斯科罗蒙诺索夫国立大学物理学院量子技术中心）
Electrically-driven optical antennas can serve as compact sources of electromagnetic radiation operating at optical frequencies. In the most widely explored configurations, the radiation is generated by electrons tunneling between metallic parts of the structure when a bias voltage is applied across the tunneling gap. Rather than relying on an inherently inefficient inelastic light emission in the gap, we suggest to use a ballistic nanoconstriction as the feed element of an optical antenna supporting plasmonic modes. We discuss the underlying mechanisms responsible for the optical emission, an…
A significant challenge in the development of chip-scale cavity-optomechanical devices as testbeds for quantum experiments and classical metrology lies in the coupling of light from nanoscale optical mode volumes to conventional optical components such as lenses and fibers. In this work we demonstrate a high-efficiency, single-sided fiber-optic coupling platform for optomechanical cavities. By utilizing an adiabatic waveguide taper to transform a single optical mode between a photonic crystal zipper cavity and a permanently mounted fiber, we achieve a collection efficiency for intracavity phot…
We demonstrate highly efficient coupling of light from an optical fiber to a silicon photonic crystal optomechanical cavity. The fiber-to-cavity coupling utilizes a compact (L ~ 25 um) intermediate adiabatic coupler. The optical coupling is lithographically controlled, broadband, relatively insensitive to fiber misalignment, and allows for light to be transferred from an optical fiber to, in principle, any photonic chip with refractive index greater than that of the optical fiber. Here we demonstrate single-sided cavity coupling with a total fiber-to-cavity optical power coupling efficiency of…
All-optical switching (AOS) of magnetic domains by femtosecond laser pulses was first observed in the transition metal-rare earth (TM-RE) alloy GdFeCo1-5; this phenomenon demonstrated the potential for optical control of magnetism for the development of ever faster future magnetic recording technologies. The technological potential of AOS has recently increased due to the discovery of the same effect in other materials, including RE-free magnetic multilayers6,7. However, to be technologically meaningful, AOS must compete with the bit densities of conventional storage devices, restricting optic…
We develop a general framework of evaluating the gain coefficient of Stimulated Brillouin Scattering (SBS) in optical waveguides via the overlap integral between optical and elastic eigen-modes. We show that spatial symmetry of the optical force dictates the selection rules of the excitable elastic modes. By applying this method to a rectangular silicon waveguide, we demonstrate the spatial distributions of optical force and elastic eigen-modes jointly determine the magnitude and scaling of SBS gain coefficient in both forward and backward SBS processes. We further apply this method to inter-m…
Near-field infrared spectroscopy by elastic scattering of light from a probe tip resolves optical contrasts in materials at dramatically sub-wavelength scales across a broad energy range, with the demonstrated capacity for chemical identification at the nanoscale. However, current models of probe-sample near-field interactions still cannot provide a sufficiently quantitatively interpretation of measured near-field contrasts, especially in the case of materials supporting strong surface phonons. We present a model of near-field spectroscopy derived from basic principles and verified by finite-e…
Recent experiments showed that unity-order index change in a transparent conducting oxide (TCO) can be achieved in a metal-oxide-semiconductor (MOS) structure by accumulation charge. However, the ultrathin (~5nm) accumulation layer and inherent absorption of TCOs impede the practical applications of this effect. Herein, we propose and explore a novel waveguide, namely "TCO-slot waveguide", which combines both the tunable property of a TCO and field enhancement of a slot waveguide. In particular, light absorption can be sharply enhanced when the slot dielectric constant is tuned close to zero. …
Herein we describe a novel spinning pump-probe photoacoustic technique developed to study nonlinear absorption in thin films. As a test case, an organic polycrystalline thin film of quinacridone, a well-known pigment, with a thickness in the tens of nanometers range, is excited by a femtosecond laser pulse which generates a time-domain Brillouin scattering signal. This signal is directly related to the strain wave launched from the film into the substrate and can be used to quantitatively extract the nonlinear optical absorption properties of the film itself. Quinacridone exhibits both quadrat…
Optical nanoantennas can efficiently confine light into nanoscopic hotspots, enabling single-molecule detection sensitivity at biological relevant conditions. This innovative approach to breach the diffraction limit offers a versatile platform to investigate the dynamics of individual biomolecules in living cell membranes and their partitioning into cholesterol-dependent lipid nanodomains. Here, we present optical nanoantenna arrays with accessible surface hotspots to study the characteristic diffusion dynamics of phosphoethanolamine (PE) and sphingomyelin (SM) in the plasma membrane of living…
By using nanoscale energy-transfer dynamics and density matrix formalism, we demonstrate theoretically and numerically that chaotic oscillation and random-number generation occur in a nanoscale system. The physical system consists of a pair of quantum dots (QDs), with one QD smaller than the other, between which energy transfers via optical near-field interactions. When the system is pumped by continuous-wave radiation and incorporates a timing delay between two energy transfers within the system, it emits optical pulses. We refer to such QD pairs as nano-optical pulsers (NOPs). Irradiating an…
All optical nanothermometry has become a powerful, noninvasive tool for measuring nanoscale temperatures in applications ranging from medicine to nanooptics and solid-state nanodevices. The key features of any candidate nanothermometer are sensitivity and resolution. Here, we demonstrate a real time, diamond based nanothermometry technique with sensitivity and resolution much larger than those of any existing all optical method. The distinct performance of our approach stems from two factors. First, temperature sensors nanodiamonds cohosting two Group IV colour centers engineered to emit spect…
The quest to improve density, speed and energy efficiency of magnetic memory storage has led to exploration of new ways of optically manipulating magnetism at the ultrafast time scale, in particular in ferrimagnetic alloys. While all-optical magnetization switching is well-established on the femtosecond timescale, lateral nanoscale confinement and thus potential significant reduction of the size of the magnetic element remains an outstanding challenge. Here we employ resonant electromagnetic energy-funneling plasmon nanoantennas to influence the demagnetization dynamics of a ferrimagnetic TbCo…
