The study of optical phenomena on the subwavelength scale is becoming increasingly important in photonics, particularly in the fields of nanoemitters, photonic crystals and plasmonics. Subwavelength field patterns are evanescent and must thus be investigated with near-field techniques. The light powers emitted by nanoscale sources are extremely low, undermining the traditional approach of scattering a near field to a large (thus noisy) far-field detector. Nanoscale detectors, providing direct sensing in the near-field with small noise due to a small active area, are needed in high-sensitivity, high-resolution near-field imaging and in quantum nanophotonic circuits. Here we report the first nanoscale ~50x50nm2) detector displaying single-photon sensitivity and a nanosecond response. These nanodetectors can also be operated in multi-photon mode, where the detection threshold can be set at N=1, 2, 3 or 4 photons, thus allowing the mapping of photon number statistics on the nanoscale.
Surface nanoscale axial photonics (SNAP) structures are fabricated with a femtosecond laser for the first time. The inscriptions introduced by the laser pressurize the fiber and cause its nanoscale effective radius variation. We demonstrate the subangstrom precise fabrication of individual and coupled SNAP microresonators having the effective radius variation of several nanometers. Our results pave the way to a novel ultraprecise SNAP fabrication technology based on the femtosecond laser inscription.
Recently introduced Surface Nanoscale Axial Photonics (SNAP) makes it possible to fabricate high Q-factor microresonators and other photonic microdevices by dramatically small deformation of the optical fiber surface. To become a practical and robust technology, the SNAP platform requires methods enabling reproducible modification of the optical fiber radius at nanoscale. In this Letter, we demonstrate super-accurate fabrication of high Q-factor microresonators by nanoscale modification of the optical fiber radius and refractive index using the CO2 laser and the UV excimer laser beam exposures…
We propose using the effective spin-orbit interaction of light in Bragg-modulated cylindrical waveguides for the effcient separation of spin-up and spin-down photons emitted by a single photon emitter. Due to the spin and directional dependence of photonic stopbands in the waveguides, spin-up (down) photon propagation in the negative (positive) direction along the waveguide axis is blocked while the same photon freely propagates in the opposite direction.
We experimentally demonstrate series of identical two, three, and five coupled high Q-factor Surface Nanoscale Axial Photonics (SNAP) microresonators formed by periodic nanoscale variation of the optical fiber radius. These microresonators are fabricated with a 100 \mum period along an 18 \mum radius optical fiber. The axial FWHM of these microresonators is 80 \mum and their Q-factor exceeds 107. In addition, we demonstrate a SNAP microresonator with the axial FWHM as small as 30 \mum and the axial FWHM of the fundamental mode as small as 10 \mum. These results may potentially enable the dense…
We report on an experimental technique to quantify the relative importance of electric and magnetic dipole luminescence from a single nanosource in structured environments. By attaching a $Eu^{3+}$-doped nanocrystal to a near-field scanning optical microscope tip, we map the branching ratios associated to two electric dipole and one magnetic dipole transitions in three dimensions on a gold stripe. The relative weight of the electric and magnetic radiative local density of states can be recovered quantitatively, based on a multilevel model. This paves the way towards the full electric and magne…
Integration of photon pairs nanosources is a major challenge for quantum technology. In this context, we develop a formalism for the investigation of Spontaneous Parametric Down Conversion in hybrid structures that combine plasmonic resonances and intrinsic nonlinearity. Using quantum and numerical approaches together, we quantitatively evaluate photon pair correlation measurements for realistic experimental configurations. Hybrid structures embedding a small nanocystal allow for a $10^{3}$ fold increase in pair production compared to the same nanocrystal alone and a photon pair production eff…
The critical properties of functional materials and nanoscale devices often originate from the coexistence of different thermodynamic phases and / or oxidization states, but sample makeup is seldom completely known a priori. Coherent diffractive imaging (CDI) provides the spatial resolution needed to observe nanoscale coexistence while returning the full amplitude and phase information of an object, but to date lacks the spectral information necessary for composition identification. Here we demonstrate CDI spectroscopy (CDIS), acquiring images of the prototypical quantum material vanadium oxid…
Fabricating nanocavities in which optically-active single quantum emitters are precisely positioned, is crucial for building nanophotonic devices. Here we show that self-assembly based on robust DNA-origami constructs can precisely position single molecules laterally within sub-5nm gaps between plasmonic substrates that support intense optical confinement. By placing single-molecules at the center of a nanocavity, we show modification of the plasmon cavity resonance before and after bleaching the chromophore, and obtain enhancements of $\geq4\times10^3$ with high quantum yield ($\geq50$%). By …
Dense photonic integration promises to revolutionize optical computing and communications. However, efforts towards this goal face unacceptable attenuation of light caused by surface roughness in microscopic devices. Here we address this problem by introducing Surface Nanoscale Axial Photonics (SNAP). The SNAP platform is based on whispering gallery modes circulating around the optical fiber surface and undergoing slow axial propagation readily described by the one-dimensional Schrödinger equation. These modes can be steered with dramatically small nanoscale variation of the fiber radius, whic…
As any physical object, light undergoing a circular trajectory features a constant extrinsic angular momentum. Within strong curvatures, this angular momentum can match the spin momentum of a photon, thus providing the opportunity of a strong spin-orbit interaction. Using this effect, we demonstrate tunable symmetry breaking in the coupling of light in a curved nanoscale plasmonic waveguide. The helicity of the impinging optical wave controls the power distribution between the two counter-propagating guided modes, including unidirectional waveguiding. We found that up to 95 % of the incoupled …
We demonstrate spatially-resolved measurements of spontaneous and stimulated electron-photon interactions in nanoscale optical near fields using electron energy-loss spectroscopy (EELS), cathodoluminescence spectroscopy (CL), and photon-induced near-field electron microscopy (PINEM). Specifically, we study resonant surface plasmon modes that are tightly confined to the tip apexes of an Au nanostar, enabling a direct correlation of EELS, CL, and PINEM on the same physical structure at the nanometer length scale. Complemented by numerical electromagnetic boundary-element method calculations, we …
Nanophotonics has been an active research field over the past two decades, triggered by the rising interests in exploring new physics and technologies with light at the nanoscale. As the demands of performance and integration level keep increasing, the design and optimization of nanophotonic devices become computationally expensive and time-inefficient. Advanced computational methods and artificial intelligence, especially its subfield of machine learning, have led to revolutionary development in many applications, such as web searches, computer vision, and speech/image recognition. The comple…
Classical electromagnetic boundary conditions (EMBCs) fail to describe quantum interface phenomena at nanoscale. Here, we construct the interface model with a transition layer describing the electromagnetic field inhomogeneity across the interface. Generalized nanoscale EMBCs are derived by introducing the magnetic interfacial response functions (IRFs) and are rewritten as three different forms based on Maxwell's equations in first order approximation. The corresponding Fresnel formula are further used to analyze the interfacial photonic phenomenon, demonstrating interesting behaviors of Brews…
Relativistic electrons in a structured medium generate radiative losses such as Cherenkov and transition radiation that act as a virtual light source, coupling to the photonic densities of states. The effect is most pronounced when the imaginary part of the dielectric function is zero, a regime where in a non-retarded treatment no loss or coupling can occur. Maps of the resultant energy losses as a sub-5nm electron probe scans across finite waveguide structures reveal spatial distributions of optical modes in a spectral domain ranging from near-infrared to far ultraviolet.
While nanoscale modal confinement radically enhances a variety of nonlinear light-matter interactions within silicon waveguides, traveling-wave stimulated Brillouin scattering nonlinearities have never been observed in silicon nanophotonics. Through a new class of hybrid photonic-phononic waveguides, we demonstrate tailorable traveling-wave forward stimulated Brillouin scattering in nanophotonic silicon waveguides for the first time, yielding 3000 times stronger forward SBS responses than any previous waveguide system. Simulations reveal that a coherent combination of electrostrictive forces a…
The emergence of two-dimensional transition metal chalcogenide materials has sparked an intense activity in valleytronics since their valley information can be directly encoded and detected by using the spin angular momentum of light. For their practical applications such as on-chip valley logic gates and chip-to-chip valley transport, the encoding and processing of valley pseudospin using light should be extended to an integrated, on-chip nanophotonic system. Here, we successfully demonstrate, at room temperature, the valley-dependent directional coupling of light using a plasmonic nanowire-W…
Novel time-resolved imaging techniques for the investigation of ultrafast nanoscale magnetization dynamics are indispensable for further developments in light-controlled magnetism. Here, we introduce femtosecond Lorentz microscopy, achieving a spatial resolution below 100 nm and a temporal resolution of 700 fs, which gives access to the transiently excited state of the spin system on femtosecond timescales and its subsequent relaxation dynamics. We demonstrate the capabilities of this technique by spatio-temporally mapping the light-induced demagnetization of a single magnetic vortex structure…
Nanoscale thermally assisted hydrodynamic melt perturbations induced by ultrafast laser energy deposition in noble-metal films produce irreversible nanoscale translative mass redistributions and results in formation of radially-symmetric frozen surface structures. We demonstrate that the final three-dimensional (3D) shape of the surface structures formed after resolidification of the molten part of the film is shown to be governed by incident laser fluence and, more importantly, predicted theoretically via molecular dynamics modeling. Considering the underlying physical processes associated wi…
Topological states of light represent counterintuitive optical modes localized at boundaries of finite-size optical structures that originate from the properties of the bulk. Being defined by bulk properties, such boundary states are insensitive to certain types of perturbations, thus naturally enhancing robustness of photonic circuitries. Conventionally, the N-dimensional bulk modes correspond to (N-1)-dimensional boundary states. The higher-order bulk-boundary correspondence relates N-dimensional bulk to boundary states with dimensionality reduced by more than 1. A special interest lies in m…
The optical absorption of nanoscale thickness semiconductor films on top of light-trapping structures based on optical interference effects combined with spectrum-splitting structures is theoretically investigated. Nearly perfect absorption over a broad spectrum range can be achieved in $<100$ nm thick films on top of one-dimensional photonic crystal or metal films. This phenomenon can be attributed to interference induced photonic localization, which enhances the absorption and reduces the reflection of the films. Perfect solar absorption and low carrier thermalization loss can be achieved wh…
Deterministically integrating single solid-state quantum emitters with photonic nanostructures serves as a key enabling resource in the context of photonic quantum technology. Due to the random spatial location of many widely-used solid-state quantum emitters, a number of positoning approaches for locating the quantum emitters before nanofabrication have been explored in the last decade. Here, we review the working principles of several nanoscale positioning methods and the most recent progress in this field, covering techniques including atomic force microscopy, scanning electron microscopy, …
Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi…
A number of applications in basic science and technology would benefit from high fidelity photon number resolving photodetectors. While some recent experimental progress has been made in this direction, the requirements for true photon number resolution are stringent, and no design currently exists that achieves this goal. Here we employ techniques from fundamental quantum optics to demonstrate that detectors composed of subwavelength elements interacting collectively with the photon field can achieve high-performance photon number resolution. We propose a new design that simultaneously achiev…
We explore the possibility of achieving a significant nonlinear phase shift among photons propagating in nanoscale waveguides exploiting interactions among photons that are mediated by vibrational modes and induced through Stimulated Brillouin Scattering (SBS). We introduce a configuration that allows slowing down the photons by several orders of magnitude via SBS involving sound waves and two pump fields. We extract the conditions for maintaining vanishing amplitude gain or loss for slowly propagating photons while keeping the influence of thermal phonons to the minimum. The nonlinear phase a…
The integration of nanoscale electronics with conventional optical devices is restricted by the diffraction limit of light. Metals can confine light at the subwavelength scales needed, but they are lossy, while dielectric materials do not confine evanescent waves outside a waveguide or resonator, leading to cross talk between components. We introduce a paradigm shift in light confinement strategy and show that light can be confined below the diffraction limit using completely transparent artificial media. Our approach relies on controlling the optical momentum of evanescent waves, an important…
Topological photonics provides an ideal platform for demonstrating novel band topology concepts, which are also promising for robust waveguiding, communication and computation applications. However, many challenges such as extremely large device footprint and functionality at short wavelengths remain to be solved which are required to make practical and useful devices that can also couple to electronic excitations in many important organic and inorganic semiconductors. In this letter, we report an experimental realization of Z_2 photonic topological insulators with their topological edge state…
Photonic quantum technologies have been extensively studied in quantum information science, owing to the high-speed transmission and outstanding low-noise properties of photons. However, applications based on photonic entanglement are restricted due to the diffraction limit. In this work, we demonstrate for the first time the maintaining of quantum polarization entanglement in a nanoscale hybrid plasmonic waveguide composed of a fiber taper and a silver nanowire. The transmitted state throughout the waveguide has a fidelity of 0.932 with the maximally polarization entangled state Φ+. Furthermo…
Flash memory technology is widely common in modern microelectronics, and is essentially affecting our daily life. Considering the recent progress in photonic circuitry, and in particular silicon photonics circuitry, there is now an opportunity to embed the flash memory technology in photonic applications. A particularly promising candidate that can benefit from such integration is the photonic resonator. As of today, chip scale resonators are essential building blocks in modern silicon photonic platform. However, their properties, and in particular their resonance frequencies deviate from thei…
The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic p…
Optical forces in guided-wave nanostructures have recently been proposed as an effective means of mechanically actuating and tuning optical components. In this work, we study the properties of a photonic crystal optomechanical cavity consisting of a pair of patterned silicon nitride nanobeams. Internal stresses in the stoichiometric silicon nitride thin-film are used to produce inter-beam slot-gaps ranging from 560 to 40nm. A general pump-probe measurement scheme is described which determines, self-consistently, the contributions of thermo-mechanical, thermo-optic, and radiation pressure effec…
Interferometric measurement of nuclear resonant phase shift with a nanoscale Young double waveguide
The Hamburg Centre for Ultrafast Imaging, Universität Hamburg（汉堡超快成像中心，汉堡大学）；Georg-August-Universität Göttingen（格奥尔格-奥古斯特哥廷根大学）；Deutsches Elektronen-Synchrotron DESY（德国电子同步加速器中心 DESY）；ESRF – The European Synchrotron（欧洲同步辐射装置 ESRF）；Helmholtz-Institut Jena（亥姆霍兹耶拿研究所）；GSI Helmholtzzentrum für Schwerionenforschung GmbH（GSI 亥姆霍兹重离子研究中心有限公司）；Friedrich-Schiller-Universität Jena（弗里德里希-席勒耶拿大学）
A new algorithmic framework is presented for holographic phase retrieval via maximum likelihood optimization, which allows for practical and robust image reconstruction. This framework is especially well-suited for holographic coherent diffraction imaging in the \textit{low-photon regime}, where data is highly corrupted by Poisson shot noise. Thus, this methodology provides a viable solution towards the advent of \textit{low-photon nanoscale imaging}, which is a fundamental challenge facing the current state of imaging technologies. Practical optimization algorithms are derived and implemented…
Strain has a strong effect on the properties of materials and the performance of electronic devices. Their ever shrinking size translates into a constant demand for accurate and precise measurement methods with very high spatial resolution. In this regard, transmission electron microscopes are key instruments thanks to their ability to map strain with sub-nanometer resolution. Here we present a novel method to measure strain at the nanometer scale based on the diffraction of electron Bessel beams. We demonstrate that our method offers a strain sensitivity better than $2.5 \cdot 10^{-4}$ and an…
Photonic metasurfaces are ultrathin electromagnetic wave-molding metamaterials providing the missing link for the integration of nanophotonic chips with nanoelectronic circuits. An extra twist in this field originates from spin-optical metasurfaces providing the photon spin (polarization helicity) as an additional degree of freedom in light-matter interactions at the nanoscale. Here we report on a generic concept to control the photonic transport by disordered (random) metasurfaces with a custom-tailored geometric phase. This approach combines the peculiarity of random patterns to support extr…
We propose and theoretically analyze a new vibrational spectroscopy, termed electron- and light-induced stimulated Raman (ELISR) scattering, that combines the high spatial resolution of electron microscopy with the molecular sensitivity of surface-enhanced Raman spectroscopy. With ELISR, electron-beam excitation of plasmonic nanoparticles is utilized as a spectrally-broadband but spatially-confined Stokes beam in the presence of a diffraction-limited pump laser. To characterize this technique, we develop a numerical model and conduct full-field electromagnetic simulations to investigate two di…
Focusing electromagnetic energy to sub-wavelength dimensions has become an increasingly active field of research for a variety of applications such as Heat Assisted Magnetic Recording (HAMR), nanolithography, and nanoscale optical characterization of biological cells and single molecules using near-field scanning optical microscopy (NSOM) technique. Double-sided surface plasmons in a metal-insulator-metal (MIM) geometry have been shown to have very small wavelengths for dielectric of thickness of less than 10 nm. A tapered dielectric structure sandwiched between metal, can be used to efficient…
Visible wavelengths of light control the quantum matter of atoms and molecules and are foundational for quantum technologies, including computers, sensors, and clocks. The development of visible integrated photonics opens the possibility for scalable circuits with complex functionalities, advancing both the scientific and technological frontiers. We experimentally demonstrate an inverse design approach based on superposition of guided-mode sources, allowing the generation and full control of free-space radiation directly from within a single 150 nm layer Ta2O5, showing low loss across visible …
We demonstrate the application of Atomic Force Microscopy (AFM) based optical force microscopy to map the optical near-fields with nanometer resolution, limited only by the AFM probe geometry. We map the electric field distributions of tightly focused laser beams with different polarizations and show that the experimentally measured data agrees well with the theoretical predictions from a dipole-dipole interaction model, thereby validating our approach. We further validate the proposed technique by evaluating the optical electric field scattered by a spherical nanoparticle by measuring the opt…
The ability to drive a system with an external input is a fundamental aspect of light-matter interaction. The coherent perfect absorption (CPA) phenomenon extends to the general multibeam interference phenomenology the well known critical coupling concepts. This interferometric control of absorption can be employed to reach full delivery of optical energy to nanoscale systems such as plasmonic nanoparticles, and multi-port interference can be used to enhance the absorption of a nanoscale device when it is embedded in a strongly scattering system, with potential applications to nanoscale sensin…
Humankind has long endeavored to control the propagation direction of light. Since time immemorial, shades, lenses and mirrors have been used to control the flow of light. In modern society, with the rapid development of nanotechnology, the control of light is moving toward devices at micrometer and even nanometer scales. At such scales, traditional devices based on geometrical optics reach their fundamental direction limits and cease to work. Nano photonics, on the other hand, has attracted wide attention from researchers, especially in the last decade, due to its ability to manipulate light …
In our former work (Sci. Rep. 4: 6039, 2014), we theoretically and numerically demonstrated that chaotic oscillation can be induced in a nanoscale system consisting of quantum dots between which energy transfer occurs via optical near-field interactions. Furthermore, in addition to the nanoscale implementation of oscillators, it is intriguing that the chaotic behavior is associated with probability derived via a density matrix formalism. Indeed, in our previous work (Sci. Rep. 6: 38634, 2016) we examined such oscillating probabilities via diffusivity analysis by constructing random walkers dri…
Topological states of light represent counterintuitive optical modes localized at boundaries of finite-size optical structures that originate from the properties of the bulk. Being defined by bulk properties, such boundary states are insensitive to certain types of perturbations, thus naturally enhancing robustness of photonic circuitries. Conventionally, the N-dimensional bulk modes correspond to (N-1)-dimensional boundary states. The higher-order bulk-boundary correspondence relates N-dimensional bulk to boundary states with dimensionality reduced by more than 1. A special interest lies in m…
Modern semiconductor integrated circuits are increasingly fabricated at untrusted third party foundries. There now exist myriad security threats of malicious tampering at the hardware level and hence a clear and pressing need for new tools that enable rapid, robust and low-cost validation of circuit layouts. Optical backside imaging offers an attractive platform, but its limited resolution and throughput cannot cope with the nanoscale sizes of modern circuitry and the need to image over a large area. We propose and demonstrate a multi-spectral imaging approach to overcome these obstacles by id…
Optical dielectric resonances have the ability to modulate optical energy, and by coupling multiple resonators into photonic molecules, new opportunities emerge in spectral engineering. Using electron-beam spectroscopy, in a 300-keV scanning transmission electron microscope, we probe optical modes of photonic molecules at the nanometer scale. Monochromated electron energy-loss spectra of 400nm-silica-sphere monomers, dimers and trimers display series of sharp peaks in the ultraviolet region. For monomers, the peaks are assigned to low angular number optical whispering gallery modes. For dimers…
Spin models arise in the microscopic description of magnetic materials, where the macroscopic characteristics are governed by exchange interactions among the constituent magnetic moments. Recently, there has been a growing interest in complex systems with spin Hamiltonians, largely due to the rich behaviors exhibited by such interactions at the macroscale. Along these lines, it has been shown that certain classes of optimization problems involving large degrees of freedom can be effectively mapped into classical spin models. In this vein, the respective extremum can be found by identifying the…
Light is a union of electric and magnetic fields, and nowhere is their complex relationship more evident than in the near fields of nanophotonic structures. There, complicated electric and magnetic fields varying over subwavelength scales are generally present, leading to photonic phenomena such as extraordinary optical momentum, super-chiral fields, and a complex spatial evolution of optical singularities. An understanding of such phenomena requires nanoscale measurements of the complete optical field vector. However, while it was recently demonstrated that near-field scanning optical microsc…
We measure the local near-field spin in topological edge state waveguides that emulate the quantum spin Hall effect. We reveal a highly structured spin density distribution that is not linked to a unique pseudospin value. From experimental near-field real-space maps and numerical calculations, we confirm that this local structure is essential in understanding the properties of optical edge states and light-matter interactions. The global spin is reduced by a factor of 30 in the near field and, for certain frequencies, flipped compared to the pseudospin measured in the far-field. We experimenta…
