Using the zero time-delay second-order correlation function for studying the photon statistics, we investigate how the photon statistics of the field-modes generated by parametric down-conversion (PDC) process depends on the photon statistics of the pump field-mode. We derive general expressions for the zero time-delay second-order correlation function of the down-converted field-modes for both multi-mode and single-mode PDC processes. We further study these expressions in the weak down-conversion limit. We show that for a two-photon two-mode PDC process, in which a pump photon splits into two photons into two separate field-modes, the zero time-delay second-order correlation function of the individual down-converted field-modes is equal to twice that of the pump field-mode. Furthermore, for an $n$-photon $n$-mode down-conversion process, in which a pump photon splits into $n$ photons into $n$ separate field-modes, the zero time-delay second-order correlation function of the individual down-converted field-modes is equal to $2^{(n-1)}$ times that of the pump field-mode. However, in contrast to the multi-mode PDC processes, for a single-mode PDC process, in which a pump photons splits into two or more photons into a single mode, the zero time-delay second-order correlation function of the down-converted field-mode is not proportional to that of the pump in the weak down-conversion limit. Nevertheless, we find it to be inversely proportional to the average number of photons in the pump field-mode.
We numerically and experimentally show that all photons generated by spontaneous parametric down-conversion (SPDC) follow a transverse amplitude similar to that of the pump. This amplitude transfer from pump to SPDC is revealed in the Fourier image plane of the down-converted photons restricted by an aperture. We also observe a considerable shift of the image plane from the actual Fourier plane, when size of the aperture is gradually increased. The shift of the Fourier image of down-converted photons affects the quality of spatial mode-based projection in various quantum correlation experiment…
We report the efficient generation of high-gain parametric down-conversion, including pump depletion, with pump powers as low as 100 $μ$W (energies $0.1$~$μ$J/pulse) and conversion efficiencies up to 33\%. In our simple configuration, the pump beam is tightly focused into a bulk periodically poled lithium niobate crystal placed in free space. We also observe a change in the photon number statistics for both the pump and down-converted beams as the pump power increases to reach the depleted pump regime. The experimental results are a clear signature of the interplay between the pump and the dow…
In this article we investigate the orbital angular momentum spectrum of photons produced in parametric down conversion process. We study how the transverse profile of the pump mode affects the spectrum as compared to a gaussian pump beam. We show that using perfect optical vortex mode as pump the spectrum can be highly narrowed down. We further study the entanglement between the two down converted photons in the orbital angular momentum basis. We observe that photons entangled in Laguerre-Gaussian modes exhibit greater higher dimensional entanglement.
We show that in parametric down-conversion the coherence properties of a temporally partially coherent pump field get entirely transferred to the down-converted entangled two-photon field. Under the assumption that the frequency-bandwidth of the down-converted signal-idler photons is much larger than that of the pump, we derive the temporal coherence functions for the down-converted field, for both infinitely-fast and time-averaged detection schemes. We show that in each scheme the coherence function factorizes into two separate coherence functions with one of them carrying the entire statisti…
Photon modes have an important role in characterizing the quantum sources of light. Proper coupling of various photon modes obtained in spontaneous parametric down conversion (SPDC) process in optical fibers is essential to generate an effective source of entangled photons. The two main pre-detection factors affecting the biphoton mode coupling in SPDC are the pump beam focusing parameter and the crystal thickness. We present the numerical and experimental results on the effect of pump focusing on conditional down-converted photon modes for a Type-I BBO crystal. We experimentally verify that b…
We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields gives the signatures of a rich dynamic of multipa…
We demonstrate a hybrid approach to the generation of photon pairs of a short wavelength with high brightness, by combining parametric down-conversion (SPDC) and up-conversion techniques. Photon pairs were generated at the wavelength of 1550 nm via SPDC, and converted to 516.7 nm through up-conversion with the pump at 775 nm. The quantum sum-frequency interference of the up-converted photon pairs exhibited a fringe period of 258.3 nm, which was 6 times shorter than the original wavelength, demonstrating that the energy-time correlation of the photon pairs was preserved. The technique simultane…
We calculate the bi-photon state generated by spontaneous parametric down conversion in a thin crystal and under collinear phase matching conditions using a pump consisting of any superposition of Laguerre-Gauss modes. The result has no restrictions on the angular or radial momenta or, in particular, on the width of the pump, signal and idler modes. We demonstrate the strong effect of the pump to signal/idler width ratio on the composition of the down-converted entangled fields. Knowledge of the pump to signal/idler width ratio is shown to be essential when calculating the maximally entangled …
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
Sources of photon pairs based on the spontaneous parametric down conversion process are commonly used for long distance quantum communication. The key feature for improving the range of transmission is engineering their spectral properties. Following two experimental papers [Opt. Lett., 38, 697 (2013)] and [Opt. Lett., 39, 1481 (2014)] we analytically and numerically analyze the characteristics of a source. It is based on a $β$-barium borate (BBO) crystal cut for type II phase matching at the degenerated frequencies 755 nm $\rightarrow$ 1550 nm + 1550 nm. Our analysis shows a way for full cont…
The time-energy entanglement of down-converted photon pairs is particularly difficult to characterize because direct measurements of photon arrival times are limited by the temporal resolution of photon detection. Here, we explore an alternative possibility of characterizing the temporal coherence of two-photon wavefunctions using single photon interference with weak coherent light. Specifically, this method makes use of the fact that down-conversion generates a coherent superposition of vacuum and two-photon states, so that the coincidence count rates for photon pairs after interference with …
The state of the spatially correlated down-converted photons is usually treated as a two-mode Gaussian entangled state. While intuitively this seems to be reasonable, it is known that new structures in the spatial distributions of these photons can be observed when the phase-matching conditions are properly taken into account. Here, we study how the variances of the near- and far-field conditional probabilities are affected by the phase-matching functions, and we analyze the role of the EPR-criterion regarding the non-Gaussianity and entanglement detection of the spatial two-photon state of sp…
We report on quantum frequency conversion of near-infrared photons from a wavelength of 854nm to the telecommunication O-band at 1310nm with 8% overall conversion efficiency. Entangled photon pairs at 854nm are generated via type-II spontaneous parametric down conversion. One photon is mixed with a strong pump field in a nonlinear ridge waveguide for its conversion to 1310nm. We demonstrate preservation of first and second order coherence of the photons in the conversion process. Based on this we infer the coherence function of the two-photon state and compare it with the actual measured one. …
We present a scheme for engineering the joint spectrum of photon pairs created via spontaneous parametric down conversion. Our method relies on customizing the poling configuration of a quasi-phase-matched crystal. We use simulated annealing to find an optimized poling configuration which allows almost arbitrary shaping of the crystal's phase-matching function. This has direct application in the creation of pure single photons---currently one of the most important goals of single-photon quantum optics. We describe the general algorithm and provide code, written in C++, that outputs an optimize…
We report on a new technique for entanglement distillation of the bipartite continuous variable state of spatially correlated photons generated in the spontaneous parametric down-conversion process (SPDC), where tunable non-Gaussian operations are implemented and the post-processed entanglement is certified in real-time using a single-photon sensitive electron multiplying CCD (EMCCD) camera. The local operations are performed using non-Gaussian filters modulated into a programmable spatial light modulator and, by using the EMCCD camera for actively recording the probability distributions of th…
Photons generated by spontaneous parametric down conversion (SPDC) are one of the most useful resources in quantum information science. Two of their most important characteristics are the purity and the indistinguishability, which determine just how useful they are as a resource. We show how these characteristics can both be accessed through Hong, Ou and Mandel (HOM) type interferences using a single pair source. We also provide simple and intuitive analytical formulas to extract their values from the depth of the resulting interference patterns. The validity of these expressions is demonstrat…
Coherence properties of the down-converted beams generated in spontaneous parametric down-conversion are investigated in detail using an iCCD camera. Experimental results are compared with those from a theoretical model developed for pulsed pumping with a Gaussian transverse profile. The results allow to tailor the shape of correlation area of the signal and idler photons using pump-field and crystal parameters. As an example, splitting of a correlation area caused by a two-peak pump-field spectrum is experimentally studied.
We make a source of entangled photons (SEP) using spontaneous parametric down-conversion (SPDC) in a non-linear crystal and study the spatial distribution of photon pairs obtained through the down-conversion of different modes of light including higher order vortices. We observe that for the Gaussian pump, the thickness of the SPDC ring varies linearly with the radius of pump beam. However, in case of vortex carrying beams, two concentric SPDC rings are formed for beams above a critical radius. The full width at half maximum (FWHM) of SPDC rings increase with increase in the order of optical v…
The correlation properties of the pump field in spontaneous parametric down-conversion are crucial in determining the degree of entanglement of generated signal and idler photons. We find theoretically that continuous-variable entanglement of the transverse positions and momenta of these photons can be achieved only if the coherence of the pump beam is sufficiently high. The positions of signal and idler photons are found to be correlated, even for an incoherent pump. However, the momenta of the signal and idler photons are not anti-correlated, even though transverse momentum is conserved.
We study the chronocyclic character, i.e. the joint temporal and spectral properties, of the single-photon constituents of photon pairs generated by spontaneous parametric down conversion. In particular we study how single photon properties, including purity and single-photon chirp, depend on photon pair properties, including the type of signal-idler spectral and correlations and the level of pump chirp.
We study the quantum correlations induced by spontaneous parametric down-conversion (SPDC) of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the adva…
The amount of entanglement that exists in a parametric down-converted state is investigated in terms of all the degrees of freedom of the state. We quantify the amount of entanglement by the Schmidt number of the state, represented as a pure bipartite state by tagging the down-converted photons in terms of orthogonal states of polarization with the aid of type II phase-matching. To facilitate our calculations, we use a Wigner functional approach, which allows the incorporation of the full infinite dimensional spatiotemporal degrees of freedom. A quantitative example with reasonably achievable …
Most investigations of multipartite entanglement have been concerned with temporal modes of the electromagnetic field, and have neglected its spatial structure. We present a simple model which allows to generate tripartite entanglement between spatial modes by parametric down-conversion with two symmetrically-tilted plane waves serving as a pump. The characteristics of this entanglement are investigated. We also discuss the generalization of our scheme to 2N+1-partite entanglement using 2N symmetrically-tilted plane pump waves. Another interesting feature is the possibility of entanglement loc…
We experimentally investigate the parametric down-conversion process in a nonlinear bulk crystal, driven by two non-collinear pump modes. The experiment shows the emergence of bright hot-spots in modes shared by the two pumps, in analogy with the phenomenology recently observed in 2D nonlinear photonic crystals. By exploiting the spatial walk-off between the two extraordinary pump modes we have been able to recreate a peculiar resonance condition, reported by a local enhancement of the parametric gain, which corresponds to a transition from a three-mode to a four-mode coupling. From a quantum …
Correlated photon pairs produced by a spontaneous parametric down conversion (SPDC) process can be used for secure quantum communication over long distances including free space transmission over a link through turbulent atmosphere. We experimentally investigate the possibility to utilize the intrinsic strong correlation between the pump and output photon spatial modes to mitigate the negative targeting effects of atmospheric beam wander. Our approach is based on a demonstration observing the deflection of the beam on a spatially resolved array of single photon avalanche diodes (SPAD-array).
A novel two-mode non-degenerate squeezed light is generated based on a four-wave mixing (4WM) process driven by two pump fields crossing at a small angle. By exchanging the roles of the pump beams and the probe and conjugate beams, we have demonstrated the frequency-degenerate two-mode squeezed light with separated spatial patterns. Different from a 4WM process driven by one pump field, the refractive index of the corresponding probe field $n_{p}$ can be converted to a value that is greater than $1$ or less than $1$ by an angle adjustment. In the new region with $n_{p}<1$, the bandwidth of the…
Strong correlations in two conjugate variables are the signature of quantum entanglement and have played a key role in the development of modern physics. Entangled photons have become a standard tool in quantum information and foundations. An impressive example is position-momentum entanglement of photon pairs, explained heuristically through the correlations implied by a common birth zone and momentum conservation. However, these arguments entirely neglect the importance of the `quantumness', i.e. coherence, of the driving force behind the generation mechanism. We study theoretically and expe…
We consider novel method for implementation of hybrid entanglement between microscopic and macroscopic states on output of spontaneous parametric down converter through the depletion of the pump wave. The generated signal, idler and pumping fields show weak entanglement. We characterize it and show the limits of applicability of the depleted pump regime. Testing method of the hybrid entanglement is proposed. The hybrid entanglement is tested by conditional generation of maximally entangled states of two qubits and qutrits regardless of its smallness. Possibilities to enhance the hybrid entangl…
We investigate the up-conversion process of broadband light from parametric down-conversion (PDC), focusing on the spatio-temporal spectral properties of the sum-frequency generated (SFG) radiation. We demonstrate that the incoherent component of the SFG spectrum is characterized by a skewed cigar-shaped geometry in space-time due to the compensation of spatial walk-off and group-velocity mismatch between the fundamental and the generated SFG fields. The results are illustrated both by a theoretical modeling of the optical system and by experimental measurements.
Creation of correlated photon pairs is one of the key topics in contemporary quantum optics. Here, we theoretically describe the generation of photon pairs in the process of spontaneous parametric down-conversion in a resonant spherical nanoparticle made of a dielectric material with bulk $χ^{(2)}$ nonlinearity. We pick the nanoparticle size that satisfies the condition of resonant eigenmodes described by Mie theory. We reveal that highly directional photon-pair generation can be observed utilising the nonlinear Kerker-type effect, and that this regime provides useful polarisation correlations…
We derive an analytical form of the Schmidt modes of spontaneous parametric down-conversion (SPDC) biphotons in both Cartesian and polar coordinates. We show that these correspond to Hermite-Gauss (HG) or Laguerre-Gauss (LG) modes only for a specific value of their width, and we show how such value depends on the experimental parameters. The Schmidt modes that we explicitly derive allow one to set up an optimised projection basis that maximises the mutual information gained from a joint measurement. The possibility of doing so with LG modes makes it possible to take advantage of the properties…
We investigate the quantum state generated by optical parametric down-conversion in a $χ^{(2) } $ medium driven by two noncollinear light modes. The analysis shows the emergence of multipartite, namely 3- or 4-partite, entangled states in a subset of the spatio-temporal modes generated by the process. These appear as bright spots against the background fluorescence, providing an interesting analogy with the phenomenology recently observed in two-dimensional nonlinear photonic crystals. We study two realistic setups: i) Non-critical phase-matching in a periodically poled Lithium Tantalate slab,…
We discuss the Bloch-Messiah decomposition for the broadband squeezed light generated by type-I parametric down-conversion with monochromatic pump. Using an exact solution for this process, we evaluate the squeezing parameters and the corresponding squeezing eigenmodes. Next, we consider the Magnus expansion of the quantum-mechanical evolution operator for this process and obtain its first three approximation orders. Using these approximated solutions, we evaluate the corresponding approximations for the Bloch-Messiah decomposition. Our results allow us to conclude that the first-order approxi…
We study how one-particle correlations transfer to manifest as two-particle correlations in the context of parametric down-conversion (PDC), a process in which a pump photon is annihilated to produce two entangled photons. We work in the polarization degree of freedom and show that for any two-qubit generation process that is both trace-preserving and entropy-nondecreasing, the concurrence $C(ρ)$ of the generated two-qubit state $ρ$ follows an intrinsic upper bound with $C(ρ)\leq (1+P)/2$, where $P$ is the degree of polarization of the pump photon. We also find that for the class of two qubit …
Nonclassical states of light are an important resource in today's quantum communication and metrology protocols. Quantum up-conversion of nonclassical states is a promising approach to overcome frequency differences between disparate subsystems within a quantum information network. Here, we present the generation of heralded narrowband single photons at 1550 nm via cavity enhanced spontaneous parametric downconversion (SPDC) and their subsequent up-conversion to 532 nm. Quantum non-Gaussianity (QNG), which is an important feature for applications in quantum information science, was experimenta…
We study polarization effects in the nonlinear interference of photons generated via frequency non-degenerate spontaneous parametric down conversion. Signal and idler photons generated in the visible and infrared (IR) range, are split in different arms of a nonlinear Michelson interferometer. The interference pattern for signal photons is detected, and it is shown to be dependent on the polarization rotation of idler photons, introduced by a birefringent sample. Based on this concept, we realize two new methods for measurement of sample retardation in the IR range by using well-developed and i…
We investigate the effect of the cumulative phase on the photon statistics of the three-mode state whose evolution is described by the trilinear Hamiltonian $\hat{H}_{I}=i\hbarκ\big(\hat{a}\hat{b}\hat{c}^{\dagger}-\hat{a}^{\dagger}\hat{b}^{\dagger}c\big)$, wherein the pump is taken to be quantized (and prepared in a coherent state) and the signal and idler modes are initially seeded with coherent states. We provide a brief review of the two-mode squeezed coherent states generated by non-degenerate coherently-stimulated parametric down-conversion, whereby the nonlinear crystal is driven by a st…
Quantum frequency conversion (QFC), a critical technology in photonic quantum information science, requires that the quantum characteristics of the frequency-converted photon must be the same as the input photon except for the color. In nonlinear optics, the wave mixing effect far away from the resonance condition is often used to realize QFC because it can prevent the vacuum field reservoir from destroying the quantum state of the converted photon effectively. Under conditions far away from resonance, experiments typically require strong pump light to generate large nonlinear interactions to …
