Post-compression of picosecond pulses into the few-cycle regime
Prannay Balla, Ammar Bin Wahid, Ivan Sytcevich, Chen Guo, Anne-Lise Viotti, Laura Silletti, Andrea Cartella, Skirmantas Alisauskas, Hamed Tavakol, Uwe Grosse-Wo… 展开作者
Prannay Balla, Ammar Bin Wahid, Ivan Sytcevich, Chen Guo, Anne-Lise Viotti, Laura Silletti, Andrea Cartella, Skirmantas Alisauskas, Hamed Tavakol, Uwe Grosse-Wortmann, Arthur Schönberg, Marcus Seidel, Andrea Trabattoni, Bastian Manschwetus, Tino Lang, Francesca Calegari, Arnaud Couairon, Anne L'Huillier, Cord L. Arnold, Ingmar Hartl, Christoph M. Heyl
In this work, we demonstrate post-compression of 1.2 picosecond laser pulses to 13 fs via gas-based multi-pass spectral broadening. Our results yield a single-stage compression factor of about 40 at 200 W in-burst average power and a total compression factor >90 at reduced power. The employed scheme represents a route towards compact few-cycle sources driven by industrial-grade Yb:YAG lasers at high average power.
We theoretically and experimentally demonstrate a new electro-optic linear approach to generate high repetition-rate picosecond pulse trains. This simple cavity-free method is based on a temporal sinusoidal phase modulation combined with a triangular spectral phase processing. Experimental results validate the concept at repetition rates ranging from 10 GHz up to 40 GHz with the generation of background-free pulse trains made of nearly Gaussian Fourier-transform limited pulses.
We report on the generation of a train of ~ 2 ps, 10 um laser pulses via multiple four-wave mixing and compression of an infrared laser beat-wave propagating in the negative group velocity dispersion region of bulk GaAs and a combination of GaAs and NaCl. The use of a 200 ps, 106 GHz beat-wave, produced by combining laser pulses amplified on the 10P(20) and 10P(16) transition of a CO2 laser, provides a novel method for generating high-power, picosecond, mid-IR laser pulses at a high repetition rate. By using 165 and 882 GHz beat-waves we show that cascaded phase-mismatched difference frequency…
We report on the generation of four spatially multiplexed picosecond 40-GHz pulse trains in a km-long 6-LP multimode optical fiber. The principle of operation is based on the parallel nonlinear compression of initial beat-signals into well separated pulse trains owing to intra-modal multiple four-wave mixings. A series of four 40-GHz dual-frequency beatings at different wavelengths are simultaneously injected into the LP01, LP11, LP02 and LP12 modes of a 1.8-km long graded-index few-mode fiber. The combined effects of Kerr nonlinearity and anomalous chromatic dispersion lead to the simultaneou…
We report the study and demonstration of a new laser pulse shaping system capable of generating linearly polarized picosecond laser pulses with variable temporal profiles including symmetric intensity distributions such as parabolic, flattop, elliptical, triangular, as well as non-symmetric distributions, which are highly desired by various applications. It is found that both high transmittance and high stability of the shaped pulse can be achieved simultaneously when crystals are set at a specific phase delay through fine control of the crystal temperature. Although multi-crystal pulse stacki…
This paper describes the demonstration of linearly polarized picosecond pulse shaping with variable profiles including symmetric and non-symmetric intensity distributions. Important characteristics such as stability and transmission were studied, resulting in highly reliable performance of this fan-type birefringent shaping system. This variable temporal shaping technique is applicable over a wide range of laser parameters and may lead to new opportunities for many potential applications. A new double-pass variable temporal shaping method that significantly reduces the required crystal quantit…
We report on the experimental generation of spatially multiplexed picosecond 40-GHz pulse trains at telecommunication wavelengths by simultaneous intra-modal multiple four wave mixing and intermodal cross-phase modulation in km-long bi-modal and 6-LP-mode graded-index few-mode fibers. More precisely, an initial beat-signal injected into the fundamental mode is first nonlinearly compressed into well-separated pulses by means of an intra-modal multiple four-wave mixing process, while several group-velocity matched continuous-wave probe signals are injected into higher-order modes in such a way t…
This paper reports the study and demonstration of a new variable temporal shaping method capable of generating linearly polarized picosecond laser pulses with arbitrary predefined shapes, which are highly desired by various applications including low emittance high brightness electron bunch generation in photocathode guns. It is found that both high transmittance and high stability of the shaped pulses can be achieved simultaneously when birefringent stages (BSs) are set at specific phase delay. Such variable temporal shaping technique may lead to new opportunities for many potential applicati…
Mode-locked fiber laser technology to date has been limited to sub-3 μm wavelengths, despite significant application-driven demand for compact picosecond and femtosecond pulse sources at longer wavelengths. Erbium- and holmium-doped fluoride fiber lasers incorporating a saturable absorber are emerging as promising pulse sources for 2.7--2.9 μm, yet it remains a major challenge to extend this coverage. Here, we propose a new approach using dysprosium-doped fiber with frequency shifted feedback (FSF). Using a simple linear cavity with an acousto-optic tunable filter, we generate 33 ps pulses wit…
A long sought-after goal for photocathode electron sources has been to improve performance by temporally shaping the incident exitation laser pulse. The narrow bandwidth, short wavelength, and picosecond pulse duration make it challenging to employ conventional spectral pulse shaping techniques. We present a novel and efficient intensity-envelope shaping technique achieved during nonlinear upconversion through opposite-chirp sum-frequency mixing. We also present a numerical case-study of the LCLS-II photoinjector where transverse electron emittance is improved by at least 25%.
Recent experiments demonstrating storage of optical pulses in acoustic phonons based on stimulated Brillouin scattering raise a number of questions about the spectral and temporal capacities of such protocols and the limitations of the theoretical frameworks routinely used to describe them. In this work, we consider the dynamics of photon-phonon scattering induced by optical pulses with temporal widths comparable to the period of acoustic oscillations. We revisit the widely adopted classical formalism of coupled modes and demonstrate its breakdown. We propose a simple extension to generalise t…
The generation of mid-infrared pulses in monolithic and electrically pumped devices is of great interest for mobile spectroscopic instruments. The gain dynamics of interband cascade lasers (ICL) are promising for mode-locked operation at low threshold currents. Here, we present conclusive evidence for the generation of picosecond pulses in ICLs via active mode-locking. At small modulation power, the ICL operates in a linearly chirped frequency comb regime characterized by strong frequency modulation. Upon increasing the modulation amplitude, the chirp decreases until broad pulses are formed. C…
Few-picosecond pulse generation featuring ultrafast spectral dynamics in gain-switched surface-grating DFB lasers via impulsive optical pumping
Institute for Solid State Physics, The University of Tokyo（东京大学固体物理研究所）；State Key Laboratory of Precision Spectroscopy, Department of Electronic Engineering, East China Normal University（华东师范大学精密光谱科学国家重点实验室电子工程系）；LDseed Co., Ltd.（LDseed有限公司）
The propagation of intense picosecond laser pulses in air in the presence of strong nonlinear self-action effects and air ionization is investigated experimentally and numerically. The model used for numerical analysis is based on the nonlinear propagator for the optical field coupled with the rate equations for the production of various ionic species and plasma temperature. Our results show that the phenomenon of plasma-driven intensity clamping, which is paramount in femtosecond laser filamentation, holds for picosecond pulses. Furthermore, the temporal pulse distortions are limited and the …
Optical quadratic nonlinearity is ultrafast in nature, while parametric interaction usually manifests only the broadband characteristic. Enormous progress has been made toward broadband phase-matching for parametric amplification and wide applications. In existing devices of broadband parametric amplification, the power efficiency of conversion is restricted to approximately the energy efficiency, and the desire for the signal power enhancement necessitates additional pulse compression after amplification. Here, we demonstrate ultrafast parametric amplification having an extraordinary power ef…
The ability to generate phase-stabilised trains of ultrafast laser pulses by mode-locking underpins photonics research in fields such as precision metrology and spectroscopy. However, the complexity of conventional mode-locked laser systems, combined with the need for a mechanism to induce active or passive phase locking between resonator modes, has hindered their realisation at the nanoscale. Here, we demonstrate that GaAs-AlGaAs nanowire lasers are capable of emitting pairs of phase-locked picosecond laser pulses when subject to non-resonant pulsed optical excitation with a repetition freque…
We experimentally demonstrate temporal reshaping of optical waveforms in the telecom wavelength band using the principle of quantum frequency conversion. The reshaped optical pulses do not undergo any wavelength translation. The interaction takes place in a nonlinear $χ^{(2)}$ waveguide using an appropriately designed pump pulse programmed via an optical waveform generator. We show reshaping of a single-peak pulse into a double-peak pulse and vice versa. We also show that exponentially decaying pulses can be reshaped into near Gaussian shape, and vice versa, which is a useful functionality for…
Generation of 480 nm picosecond pulses for ultrafast excitation of Rydberg atoms
Institute for Molecular Science, National Institutes of Natural Sciences（国立自然科学研究所分子科学研究所）；SOKENDAI (The Graduate University for Advanced Studies)（综合研究大学院大学）
Synchrotrons are powerful and productive in revealing the spatiotemporal complexities in matter. However, X-ray pulses produced by the synchrotrons are predetermined in specific patterns and widths, limiting their operational flexibility and temporal resolution. Here, we introduce the on-chip picosecond synchrotron pulse shaper that shapes the sub-nm-wavelength hard X-ray pulses at individual beamlines, flexibly and efficiently beyond the synchrotron pulse limit. The pulse shaper is developed using the widely available silicon-on-insulator technology, oscillates in torsional motion at the same…
Experimental measurements and calculations of STIRAP transfer efficiencies were made on a sodium gas starting from the $3^2{\rm S}_{1/2}$ electronic ground state, passing through the $3^2{\rm P}_{1/2}$ and/or the $3^2{\rm P}_{3/2}$ to the $5^2{\rm S}_{1/2}$ state. The lasers used in the experiments had a pulse width of several picoseconds and were close to the Fourier transform limit. Although the linewidth of the laser was much smaller than the spin orbit splitting between the $3^2{\rm P}_{1/2}$ and $3^2{\rm P}_{3/2}$ states, Experiments and calculations reveal that both 3p states play a role…
We report on the creation of angle-independent colors on silver using closely time-spaced laser bursts. The use of burst mode, compared to traditional non-burst is shown to increase the Chroma (color saturation) by ~50% and to broaden the lightness range by up to ~60%. Scanning electron microscope analysis of the surfaces created using burst mode, reveal the creation of 3 distinct sets of laser induced periodic surface structures (LIPSS): low spatial frequency LIPSS (LSFL), high spatial frequency LIPSS (HSFL) and large laser-induced periodic surface structures (LLIPSS) that are 10 times the la…
The thermal lensing effects in the lasing crystal appear to be dominant when the pump laser focused on the lasing crystal which causes the local heating effect. The spatial refractive index variations observed if the crystal has non-uniform temperature distribution. In the present study, the demonstration of thermal lensing effect of Brewster-cut Ti: Sapphire crystal carried out when pumped by 25 ps pulses at 80 MHz repetition rate with 532 nm central wavelength, while the average pump power controlled by the attenuator. The thermal lensing effects measured first at the ~293 K temperature and …
The quantum cascade laser (QCL) has evolved to be a compact, powerful source of coherent mid-infrared (mid-IR) light. However, its fast gain dynamics strongly restricts the formation of ultrashort pulses. As such, the shortest pulses reported so far were limited to a few picoseconds with some hundreds of milliwatts of peak power, strongly narrowing their applicability for time-resolved and nonlinear experiments. Here, we demonstrate an alternative approach capable of producing near-transform-limited sub-picosecond pulses with several watts of peak power. Starting from a frequency modulated pha…
It is well known that when the fused silica is irradiated with focused femtosecond laser beams, space selective chemical etching can be achieved. The etching rate depends sensitively on the polarization of the laser. Surprisingly, we observe that by chirping the Fourier-transform-limited femtosecond laser pulses to picosecond pulses, the polarization dependence of the etching rate disappears, whereas an efficient etching rate can still be maintained. Observation with a scanning electron microscope reveals that the chirped pulses can induce interconnected nanocracks in the irradiated areas whic…
The physical mechanisms of the laser-induced periodic surface structures (LIPSS) formation are studied in this paper for single-pulse irradiation regimes. The change in the LIPSS period with wavelength of incident laser radiation is investigated experimentally, using a picosecond laser system, which provides 7-ps pulses in near-IR, visible, and UV spectral ranges. The experimental results are compared with predictions made under the assumption that the surface-scattered waves are involved in the LIPSS formation. Considerable disagreement suggests that hydrodynamic mechanisms can be responsible…
Pulse self-compression followed by the generation of resonant radiation is a well known phenomenon in non-linear optics. Resonant radiation is important as it allows for efficient and tunable wavelength conversion. We vary the chirp of the initial pulse and find in simulations and experiments that a small positive chirp enhances the pulse compression and strongly increases the generation of resonant radiation. This result corroborates previously published simulation results indicating an improved degree of pulse compression for a small positive chirp [1]. It also demonstrates how pulse evoluti…
The efficiency of photo-conductive switches, which continue to be used for the generation and detection of THz waves, has been overlooked for a long time. The so far 'optics-dominated' devices are making their way through to new and emerging fields of research that require ultrafast picosecond voltage pulses, as well as to new applications where power efficiency is of uttermost importance. To address the efficiency problems, in this article we present a novel photo-conductive switch that is based on a 3-dimensional design. In contrast to conventional planar designs, our photo-conductive switch…
Ghost imaging (GI) lidar, as a novel remote sensing technique,has been receiving increasing interest in recent years. By combining pulse-compression technique and coherent detection with GI, we propose a new lidar system called pulse-compression GI lidar. Our analytical results, which are backed up by numerical simulations, demonstrate that pulse-compression GI lidar can obtain the target's spatial intensity distribution, range and moving velocity. Compared with conventional pulsed GI lidar system, pulse-compression GI lidar, without decreasing the range resolution, is easy to obtain high sing…
We present a free-running 80-MHz dual-comb polarization-multiplexed solid-state laser which delivers 1.8 W of average power with 110-fs pulse duration per comb. With a high-sensitivity pump-probe setup, we apply this free-running dual-comb laser to picosecond ultrasonic measurements. The ultrasonic signatures in a semiconductor multi-quantum-well structure originating from the quantum wells and superlattice regions are revealed and discussed. We further demonstrate ultrasonic measurements on a thin-film metalized sample and compare these measurements to ones obtained with a pair of locked femt…
We demonstrate the use of hybrid rotational femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman spectroscopy (HR-CARS) as a technique for temperature measurements in nitrogen gas at high pressures and temperatures. A broadband pulse shaper-adjusted 42 fs pulse interacts with a narrow-bandwidth, frequency-upconverted 5.5 ps pulse in a cell containing nitrogen at pressures of 1-70 atm and temperatures of 300-1000 K. A computational code is used to model spectra and fit experimental results to obtain best-fit temperatures. We demonstrate good qualitative fits as well as good accuracy and pr…
Comparative study of second harmonic generation at 1030 nm in BiBO and LBO crystals using a 100 W-class picosecond laser
HiLASE Centre, FZU - Institute of Physics of the Czech Academy of Sciences（捷克科学院物理研究所 HiLASE 中心）；Department of Laser Physics and Photonics, Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University in Prague（布拉格捷克理工大学核科学与物理工程学院激光物理与光子学系）；Faculty of Mathematics and Physics, Charles University（查理大学数学与物理学院）
Post-compression of ultra-short laser pulses via self-phase modulation is routinely employed for the generation of laser pulses with optical bandwidths reaching far beyond the laser gain limitations. While high compression factors can be routinely achieved, the compressed pulses typically suffer from temporal quality degradation. We numerically and experimentally analyze the deterioration of different measures of temporal quality with increasing compression factor and show how appropriate dispersion management and cascading of the post-compression process can be employed to limit the impact of…
We report on the nonlinear temporal compression of mJ energy pulses from a Ti:Sa chirped pulse amplifier system in a multipass cell filled with argon. The pulses are compressed from 30 fs down to 5.3 fs, corresponding to two optical cycles. The post-compressed beam exhibits excellent spatial quality and homogeneity. These results pave the way to robust and energy-scalable compression of Ti:Sa pulses down to the few-cycle regime.
