Experimental Tuning of Transport Regimes in Hyperuniform Disordered Photonic Materials
Geoffroy J. Aubry, Luis S. Froufe-Pérez, Ulrich Kuhl, Olivier Legrand, Frank Scheffold, Fabrice Mortessagne
备注：
Main text (6 pages, 4 figures) + SI (4 pages, 7 figures); The SI videos are permanently stored on the Zenodo repository https://doi.org/10.5281/zenodo.3978032
We present wave transport experiments in hyperuniform disordered arrays of cylinders with high dielectric permittivity. Using microwaves, we show that the same material can display transparency, photon diffusion, Anderson localization, or a full band gap, depending on the frequency $ν$ of the electromagnetic wave. Interestingly, we find a second weaker band gap, which appears to be related to the second peak of the structure factor. Our results emphasize the importance of spatial correlations on different length scales for the formation of photonic band gaps.
We introduce the first designs for high-Q photonic cavities in slab architectures in hyperuniform disordered solids displaying isotropic band gaps. Despite their disordered character, hyperuniform disordered structures have the ability to tightly confine the TE-polarised radiation in slab configurations that are readily fabricable. The architectures are based on carefully designed local modifications of otherwise unperturbed hyperuniform dielectric structures. We identify a wide range of confined cavity modes, which can be classified according to their approximate symmetry (monopole, dipole, q…
The purpose of this work is to understand the fundamental connection between structural correlations and light localization in three-dimensional (3D) open scattering systems of finite size. We numerically investigate the transport of vector electromagnetic waves scattered by resonant electric dipoles spatially arranged in 3D space by stealthy hyperuniform disordered point patterns. Three-dimensional stealthy hyperuniform disordered systems (3D-SHDS) are engineered with different structural correlation properties determined by their degree of stealthiness $χ$. Such fine control of exotic states…
Hyperuniform disordered photonic materials have recently been shown to display large, complete photonic band gaps and isotropic optical properties, and are emerging as strong candidates for a plethora of optoelectronic applications, making them competitive with many of their periodic and quasiperiodic counterparts. In this work, high quality factor optical cavities in hyperuniform disordered architectures are fabricated through semiconductor slabs and experimentally addressed by scanning near-field optical microscopy. The wide range of confined cavity modes that we detect arise from carefully …
We demonstrate the existence of large phononic band gaps in designed hyperuniform (isotropic) disordered two-dimensional (2D) phononic structures of Pb cylinders in epoxy matrix. The phononic band gaps in hyperuniform disordered phononic structures are comparable to band gaps of similar periodic structures, for both out-of-plane and in-plane polarizations. A large number of localized modes is identified near the band edges, as well as, diffusive transmission throughout the rest of the frequency spectrum. Very high-Q cavity modes for both out-of-plane and in-plane polarizations are formed by se…
Hyperuniform disordered photonic materials (HDPM) are spatially correlated dielectric structures with unconventional optical properties. They can be transparent to long-wavelength radiation while at the same time have isotropic band gaps in another frequency range. This phenomenon raises fundamental questions concerning photon transport through disordered media. While optical transparency is robust against recurrent multiple scattering, little is known about other transport regimes like diffusive multiple scattering or Anderson localization. Here we investigate band gaps, and we report Anderso…
Structural and physical properties of gyromorphs and disordered stealthy hyperuniform media
Princeton Materials Institute, Princeton University（普林斯顿材料研究所，普林斯顿大学）；Department of Electrical & Computer Engineering, Boston University（波士顿大学电气与计算机工程系）；Department of Physics, Boston University（波士顿大学物理系）；Division of Materials Science & Engineering, Boston University（波士顿大学材料与工程分院）；Department of Chemistry, Princeton University（普林斯顿大学化学系）；Program in Applied and Computational Mathematics, Princeton University（普林斯顿大学应用与计算数学项目）
Disordered and hyperuniform structures of densely packed spheres near and at jamming are characterized by vanishing of long-wavelength density fluctuations, or equivalently by long-range power-law decay of the direct correlation function (DCF). We focus on previous simulation results that exhibit degradation of hyperuniformity in jammed structures while maintaining the long-range nature of the DCF to a certain length scale. Here we demonstrate that a field-theoretic formulation of the stochastic density functional theory is relevant to explore the degradation mechanism. The strong-coupling exp…
In this work we present a study on the characterization of ordered and disordered hyperuniform point distributions on spherical surfaces. In spite of the extensive literature on disordered hyperuniform systems in Euclidean geometries, to date few works have dealt with the problem of hyperuniformity in curved spaces. As a matter of fact, some systems that display disordered hyperuniformity, like the space distribution of photoreceptors in avian retina, actually occur on curved surfaces. Here we will focus on the local particle number variance and its dependence on the size of the sampling windo…
Carbon nanotubes are quasi-one-dimensional systems that possess superior transport, mechanical, optical, and chemical properties. In this work, we generalize the notion of disorder hyperuniformity, a recently discovered exotic state of matter with hidden long-range order, to quasi-one-dimensional materials. As a proof of concept, we then apply the generalized framework to quantify the density fluctuations in amorphous carbon nanotubes containing randomly distributed Stone-Wales defects. We demonstrate that all of these amorphous nanotubes are hyperuniform, i.e., the infinite-wavelength density…
Disordered hyperuniformity (DHU) is a recently proposed new state of matter, which has been observed in a variety of classical and quantum many-body systems. DHU systems are characterized by vanishing infinite-wavelength density fluctuations and are endowed with unique novel physical properties. Here we report the first discovery of disordered hyperuniformity in atomic-scale 2D materials, i.e., amorphous silica composed of a single layer of atoms, based on spectral-density analysis of high-resolution transmission electron microscope images. Subsequent simulations suggest that the observed DHU …
The hyperuniformity concept provides a unified means to classify all perfect crystals, perfect quasicrystals, and exotic amorphous states of matter according to their capacity to suppress large-scale density fluctuations. While the classification of hyperuniform point configurations has received considerable attention, much less is known about the classification of hyperuniform heterogeneous two-phase media, which include composites, porous media, foams, cellular solids, colloidal suspensions and polymer blends. The purpose of this article is to begin such a program for certain two-dimensional…
Theoretical Prediction of the Effective Dynamic Dielectric Constant of Disordered Hyperuniform Anisotropic Composites Beyond the Long-Wavelength Regime
The creation of disordered hyperuniform materials with potentially extraordinary optical properties requires a capacity to synthesize large samples that are effectively hyperuniform down to the nanoscale. Motivated by this challenge, we propose a fabrication protocol using binary superparamagnetic colloidal particles confined in a 2D plane. The strong and long-ranged dipolar interaction induced by a tunable magnetic field is free from screening effects that attenuates long-ranged electrostatic interactions in charged colloidal systems. Specifically, we find a family of optimal size ratios that…
Two-dimensional stealthy hyperuniform distributions of rigid scatterers embedded in a waveguide are experimentally characterized the wave transport properties for scalar waves in airborne audible acoustics. The non resonant nature of the scatterers allows us to directly links the these properties to the geometric distribution of points through the structure factor. The transport properties are analyzed as a function of the stealthiness $χ$ of their hyperuniform point pattern and compared to those of a disordered material in the diffusive regime, which are characterized by the Ohm's law through…
We study the distribution of eigenfrequency spacings (the so-called level spacing statistics) for light in a two-dimensional (2D) disordered photonic crystal composed of circular dielectric (silicon) rods in air. Disorder introduces localized transverse-magnetic (TM) modes into the band gap of the ideal crystal. The level spacing statistics is found to approach the Poisson distribution for these modes. In contrast, for TM modes outside the band gap and for transverse-electric (TE) modes at all frequencies, the level spacing statistics follows the Wigner-Dyson distribution.
We study the density of states (DOS) in band gaps of ideal and disordered three-dimensional photonic crystals of finite size. The ideal crystal is a diamond lattice of resonant point scatterers (atoms) whereas the disordered one is obtained from it by displacing the scatterers by random distances in random directions. We find that DOS inside a band gap of the ideal crystal decreases as the inverse of the crystal size. Disorder narrows the band gap and DOS exhibits enhanced fluctuations near the new band edges. However, the average DOS still exhibits the same scaling with the crystal size withi…
Local Geometric and Transport Properties of Networks that are Generated from Hyperuniform Point Patterns
University of California, Los Angeles（加州大学洛杉矶分校）；University of North Carolina at Chapel Hill（北卡罗来纳大学教堂山分校）；Tandon School of Engineering, New York University（纽约大学坦登工程学院）；Santa Fe Institute（圣塔菲研究所）；Nordita（北欧理论天体物理学研究所）；KTH Royal Institute of Technology（瑞典皇家理工学院）；Stockholm University（斯德哥尔摩大学）；Uppsala University（乌普萨拉大学）
Predictive Formulas for Scattering Mean Free Path for General Disordered Dielectric Media Beyond the Long-Wavelength Regime
Princeton Materials Institute, Princeton University（普林斯顿大学材料研究所）；Department of Chemistry, Princeton University（普林斯顿大学化学系）；Department of Physics, Princeton University（普林斯顿大学物理系）；Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST)（韩国科学技术院化学与生物分子工程系）；GIST InnoCORE AI-Nano Convergence Institute for Early Detection of Neurodegenerative Diseases, Gwangju Institute of Science and Technology（光州科学技术研究院GIST InnoCORE神经退行性疾病早期检测AI-纳米融合研究所）；Program in Applied and Computational Mathematics, Princeton University（普林斯顿大学应用与计算数学项目）
We present experimental evidence for the different mechanisms driving the fluctuations of the local density of states (LDOS) in disordered photonic systems. We establish a clear link between the microscopic structure of the material and the frequency correlation function of LDOS accessed by a near-field hyperspectral imaging technique. We show, in particular, that short- and long-range frequency correlations of LDOS are controlled by different physical processes (multiple or single scattering processes, respectively) that can be---to some extent---manipulated independently. We also demonstrate…
We propose a framework that unifies the description of light transport in three-dimensional amorphous dielectric materials that exhibit both localization and a photonic bandgap. To this end, we argue that coherent reflection near and in the bandgap attenuates the generation of diffuse or localized photons. Using the self-consistent theory of localization and considering the density of states of photons, we can quantitatively describe all transport regimes: Transparency, light diffusion, localization, and bandgap. Comparing the model with numerical data on optical transport in hyperuniform diel…
In disordered two dimensional Chern insulators, a single bulk extended mode is predicted to exist per band, up to a critical disorder strength; all the other bulk modes are localized. This behavior contrasts strongly with topologically trivial two-dimensional phases, whose modes all become localized in the presence of disorder. Using a tight-binding model of a realistic photonic Chern insulator, we show that delocalized bulk eigenstates can be observed in an experimentally realistic setting. This requires the selective use of resonator losses to suppress topological edge states, and acquiring …
We demonstrate that disorder in photonic crystals could lead to pronounced modification of spontaneous emission rate in the frequency region corresponding to the photonic band gap (PBG). Depending on the amount of disorder, two different regimes of the Purcell effect occurs. For the moderate disorder, an enhancement of spontaneous emission occurs at the edge of PBG due to modification of the properties of the edge state. This effect is responsible for recently observed mirrorless lasing in photonic crystals at the edge of PBG. When the level of disorder increases, the spontaneous emission rate…
We investigate numerically and experimentally the influence of coupling disorder on the self-trapping dynamics in nonlinear one-dimensional optical waveguide arrays. The existence of a lower and upper bound of the effective average propagation constant allows for a generalized definition of the threshold power for the onset of soliton localization. When compared to perfectly ordered systems, this threshold is found to decrease in the presence of coupling disorder.
We studied lasing modes in a disordered photonic crystal. The scaling of the lasing threshold with the system size depends on the strength of disorder. For sufficiently large size, the minimum of the lasing threshold occurs at some finite value of disorder strength. The highest random cavity quality factor was comparable to that of an intentionally introduced single defect. At the minimum, the lasing threshold showed a super-exponential decrease with the size of the system. We explain it through a migration of the lasing mode frequencies toward the photonic bandgap center, where the localizati…
We discover two distinct topological pathways through which the pentagonal Cairo tiling (P5), a structural model for single-layer $AB_2$ pyrite materials, respectively transforms into a crystalline rhombus-hexagon (C46) tiling and random rhombus-pentagon-hexagon (R456) tilings, by continuously introducing the Stone-Wales (SW) topological defects. We find these topological transformations are controlled by the orientation correlations among neighboring $B$-$B$ bonds, and exhibit a phenomenological analogy of the (anti)ferromagnetic to paramagnetic transition in two-state Ising systems. Unlike t…
We report on the mesoscale fabrication and characterization of polymeric templates for isotropic photonic materials derived from hyper- uniform point patterns using direct laser writing in a polymer photoresist. We study experimentally the microscopic structure by electron microscopy and small angle light scattering. Reducing the refractive index mismatch by liquid infiltration we find good agreement between the scattering data and numerical calculations based on a discrete dipole approximation. Our work demonstrates the feasibility of fabricating such random designer materials on technologica…
By using two ab initio numerical methods we study the effects that disorder has on the spectral gaps and on wave localization in two-dimensional photonic band gap materials. We find that there are basically two different responses depending on the lattice realization (solid dielectric cylinders in air or vise versa), the wave polarization, and the particular form under which disorder is introduced. Two different pictures for the photonic states are employed, the ``nearly free'' photon and the ``strongly localized'' photon. These originate from the two different mechanisms responsible for the f…
Inferring stealthy hyperuniform correlations from quantum transport
Instituto de Física, Universidade Federal do Rio de Janeiro（里约热内卢联邦大学物理研究所）；Institut für Theoretische Physik und Astrophysik, Universität Würzburg（维尔茨堡大学理论物理与天体物理研究所）；School of Physics, Trinity College Dublin（都柏林圣三一学院物理学院）；Centre for Research on Adaptive Nanostructures and Nanodevices (CRANN) & Advanced Materials and Bioengineering Research (AMBER) Centre, Trinity College Dublin（都柏林圣三一学院自适应纳米结构与纳米器件研究中心及先进材料与生物工程技术研究中心）；Department of Physics, Princeton University（普林斯顿大学物理系）；Department of Chemistry, Princeton University（普林斯顿大学化学系）；Princeton Institute for the Science and Technology of Materials, Princeton University（普林斯顿大学材料科学与工程研究所）；Program in Applied and Computational Mathematics, Princeton University（普林斯顿大学应用与计算数学项目）
We propose an efficient numerical method to compute configuration averages of observables in disordered open quantum systems whose dynamics can be unraveled via stochastic trajectories. We prove that the optimal sampling of trajectories and disorder configurations is simply achieved by considering one random disorder configuration for each individual trajectory. As a first application, we exploit the present method to the study the role of disorder on the physics of the driven-dissipative Bose-Hubbard model in two different regimes: (i) for strong interactions, we explore the dissipative physi…
