Role of disorder in plasmon-assisted near-field heat transfer between two-dimensional metals
Jonathan L. Wise, Denis M. Basko, Frank W. J. Hekking
备注：
Addition of Sec. IIC. discussing the generality of the results - in particular clarifying the validity conditions for the near-field limit. Addition of Sec. VI. comparing the theoretical results to experiments. Addition of an illustrative panel in Fig. 5(b)
We perform a theoretical study of the near-field heat transfer between two atomically thin metallic layers, isolated galvanically but coupled by the Coulomb interaction, within the framework of fluctuational electrodynamics in the Coulomb limit. We clarify the role of disorder and spatial dispersion, and identify several distinct regimes of the heat transfer. We find that the plasmon contribution to the heat current is suppressed both in the clean and diffusive limits, but dominates in a parametrically wide crossover region at sufficiently high temperatures.
We develop a theory of electron tunneling accompanied by carrier-carrier scattering in graphene - insulator - graphene heterostructures. Due to the dynamic screening of Coulomb interaction, the scattering-aided tunneling is resonantly enhanced if the transferred energy and momentum correspond to those of surface plasmons. We reveal the possible experimental manifestations of such plasmon-assisted tunneling in current-voltage curves and plasmon emission spectra of graphene-based tunnel junctions. We find that inelastic current and plasmon emission rates have sharp peaks at voltages providing eq…
Thermal relaxation of nanoscale magnetic islands, mimicking Ising macrospins, is indispensable for studies of geometrically frustrated artificial spin systems and low-energy nanomagnetic computation. Currently-used heating schemes based on contact to a thermal reservoir, however, lack the speed and spatial selectivity required for the implementation in technological applications. Applying a hybrid approach by combining a plasmonic nanoheater with a magnetic element, in this work we establish the robust and reliable control of local temperatures in nanomagnetic arrays by contactless optical mea…
Phononless plasmon assisted thermally activated transport through a long disordered array of finite length quantum wires is investigated analytically. Generically strong electron plasmon interaction in quantum wires results in a qualitative change of the temperature dependence of thermally activated resistance in comparison to phonon assisted transport. At high temperatures, the thermally activated resistance is determined by the Luttinger liquid interaction parameter of the wires.
In a proposed book chapter surface plasmon polariton assisted optical switching in noble metal nanoparticle systems is discussed in the sub-band gap formalism.
Reply to comment on "Thermal effects -- an alternative mechanism for plasmon-assisted photocatalysis" by P. Jain [Chem. Sci., 2020, 11, DOI: 10.1039/D0SC02914A]
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Majorana zero modes in one-dimensional topological superconductors obey non-Abelian braiding statistics. Braiding manipulations can be realized by controlling Coulomb couplings in hybrid Majorana-transmon devices. However, strong disorder may induce accidental Majorana modes, which are expected to have detrimental effects on braiding statistics. Nevertheless, we show that the Coulomb-assisted braiding protocol is efficiently realized also in the presence of accidental modes. The errors occurring during the braiding cycle are small if the couplings of the computational Majorana modes to the acc…
To study the effect of disorder on quantum phase slips (QPS) in superconducting wires, we consider the plasmon-only model where disorder can be incorporated into a first-principles instanton calculation. We consider weak but general finite-range disorder and compute the formfactor in the QPS rate associated with momentum transfer. We find that the system maps onto dissipative quantum mechanics, with the dissipative coefficient controlled by the wave (plasmon) impedance Z of the wire and with a superconductor-insulator transition at Z=6.5 kOhm. We speculate that the system will remain in this u…
The excitation spectrum and the collective modes of graphene antidot lattices (GALs) are studied in the context of a $π$-band tight-binding model. The dynamical polarizability and dielectric function are calculated within the random phase approximation. The effect of different kinds of disorder, such as geometric and chemical disorder, are included in our calculations. We highlight the main differences of GALs with respect to single-layer graphene (SLG). Our results show that, in addition to the well-understood bulk plasmon in doped samples, inter-band plasmons appear in GALs. We further show …
The current voltage (IV) characteristics for perpendicular transport through two sequentially coupled wires of finite length is calculated analytically. The transport within a Coulomb blockade step is assisted by plasmon resonances that appear as steps in the IV characteristics with positions and heights depending on inter- and intrawire interactions. In particular, due to the interwire interactions, the peak positions shift to lower voltages in comparison to the noninteracting wires which reflects the facilitation of current by interactions. The interwire interactions are also found to enhanc…
We obtain the local density of states (LDOS) for any nanoplasmonic system in the frequency range dominated by a localized surface plasmon. By including the Ohmic losses in a consistent way, we show that the plasmon LDOS is proportional to the local field intensity normalized by the absorbed power. We obtain explicit formulas for the energy transfer (ET) between quantum emitters and plasmons as well as between donors and acceptors situated near a plasmonic structure. In the latter case, we find that the plasmon-assisted ET rate is proportional to the LDOS product at the donor and acceptor posit…
Dirac Fermion, which is the low energy collective excitation near the Dirac cone in monolayer graphene, have gained great attention by low energy Terahertz probe. In the case of undoped graphene, it has been generally understood that the ultrafast terahertz thermal relaxation is mostly driven by the electron-phonon coupling (EOP), which can be prolonged to tens and hundreds of picoseconds. However, for the high doped graphene, which manifests the negative photoinduced terahertz conductivity, there is still no consensus on the dominant aspects of the cooling process on a time scale of a few pic…
Understanding the interplay between disorder, environment and interactions is key to elucidating the transport properties of open quantum systems, from excitons in photosynthetic networks to qubits in ion traps. This interplay is studied here theoretically in the context of environment-assisted quantum transport (ENAQT), a unique situation in open system where an environment-induced dephasing can, counter-intuitively, enhance transport. First, we show a surprising situation where the particle current grows with increasing disorder, even without dephasing. Then, we suggest a specific mechanism …
We evaluate the rate of energy loss of a plasmon in a disorder-free carbon nanotube. The plasmon decays into neutral bosonic excitations of the electron liquid. The process is mediated either by phonon-assisted backscattering of a single electron, or Umklapp backscattering of two electrons. To lowest order in the backscattering interactions the partial decay rates are additive. At zero doping the corresponding decay rates scale as power-laws of the temperature with positive and negative exponents for the two mechanisms, respectively. The precise values of the exponents depend on the Luttinger …
The electric conductance of a strip of undoped graphene increases in the presence of a disorder potential, which is smooth on atomic scales. The phenomenon is attributed to impurity-assisted resonant tunneling of massless Dirac fermions. Employing the transfer matrix approach we demonstrate the resonant character of the conductivity enhancement in the presence of a single impurity. We also calculate the two-terminal conductivity for the model with one-dimensional fluctuations of disorder potential by a mapping onto a problem of Anderson localization.
We describe the process of Foerster transfer between semiconductor nanoparticles in the presence of a metal subsystem (metal nanocrystals). In the presence of metal nanocrystals, the Foerster process can become faster and more long-range. The enhancement of Foerster transfer occurs due to the effect of plasmon-assisted amplification of electric fields inside the nanoscale assembly. Simultaneously, metal nanocrystals lead to an increase of energy losses during the Foerster transfer process. We derive convenient equations for the energy transfer rates, photoluminescence intensities, and energy d…
One-dimensional quantum emitters with chiral couplings can exhibit nonreciprocal decay channels, along with light-induced dipole-dipole interactions mediated via an atom-waveguide interface. When the position disorders are introduced to such atomic array, we are able to identify the dynamical phase transition from excitation delocalization to localization, with an interplay between the directionality of decay rates and the strength of light-induced dipole-dipole interactions. Deep in the localization phase, its characteristic length decreases and saturates toward a reciprocal coupling regime, …
We investigate in a fully quantum-mechanical manner how the many-body excitation spectrum of topological insulators is affected by the presence of long-range Coulomb interactions. In the one-dimensional Su-Schrieffer-Heeger model and its mirror-symmetric variant strongly localized plasmonic excitations are observed which originate from topologically non-trivial single-particle states. These \textit{"topological plasmons"} inherit some of the characteristics of their constituent topological single-particle states, but they are not equally well protected against disorder due to the admixture of …
Plasmon decay via the surface or interface is a critical process for practical energy conversion and plasmonic catalysis. However, the relationship between plasmon damping and the coupling between the plasmon and 2D materials is still unclear. The spectral splitting due to plasmon-exciton interaction impedes the conventional single-particle method to evaluate the plasmon damping rate by the spectral linewidth directly. Here, we investigated the interaction between a single gold nanorod (GNR) and 2D materials using the single-particle spectroscopy method assisted with in situ nanomanipulation t…
Here we present the theoretical foundation of the strong coupling phenomenon between quantum emitters and propagating surface plasmons observed in two-dimensional metal surfaces. For that purpose, we develop an ab-initio quantum framework that accounts for the coherent coupling be- tween emitters and surface plasmons and incorporates the presence of dissipation and dephasing. For both a single emitter and a disordered ensemble of emitters, our formalism is able to reveal the key physical mechanisms that explain the reported phenomenology and also to determine the physical parameters that optim…
