We perform experimental quantum polarimetry using a heralded single photon to analyze the optical activity of linearly polarized light traversing a chiral medium. Three kinds of estimators are considered to estimate the concentrations of sucrose solutions from measuring the rotation angle of the linear polarization of the output photons. Through repetition of independent and identical measurements performed for each individual scheme and different concentration sucrose solutions, we compare the estimation uncertainty among the three schemes. The results are also compared to classical benchmarks for which a coherent state of light is taken into account. The quantum enhancement in the estimation uncertainty is evaluated and the impact of experimental and technical imperfections is discussed. In this work, we lay out a route for future applications relying on quantum polarimetry.
We analyze the quantum-state purity of heralded single photons produced from frequency-anti-correlated biphotons. We find that the quantum-state purity in time-frequency domain depends strongly on the response time uncertainty of the trigger-photon detector that heralds the generation of its paired photon. If the trigger response time is much shorter than the two-photon coherence time, the time-frequency quantum-state purity of heralded single photons approaches unity and the heralded single photon is in a nearly pure state. If the trigger response time is much longer than the two-photon coher…
We derive calculations on the statistics of a heralded single photon source based on parametric photon pair generation. These calculations highlight fundamental and practical limits for these sources, and show which physical parameters can be optimized to improve the quality of a real source.
We present a heralded single-photon source with a much lower level of unwanted background photons in the output channel by using the herald photon to control a shutter in the heralded channel. The shutter is implemented using a simple field programable gate array controlled optical switch.
We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coi…
We report on the experimental realization and characterization of an asynchronous heralded single photon source based on spontaneous parametric down conversion. Photons at 1550nm are heralded as being inside a single-mode fiber with more than 60% probability, and the multi-photon emission probability is reduced by up to a factor 600 compared to poissonian light sources. These figures of merit, together with the choice of telecom wavelength for the heralded photons are compatible with practical applications needing very efficient and robust single photon sources.
We demonstrate the generation of rubidium-resonant heralded single photons for quantum memories. Photon pairs are created by cavity-enhanced down-conversion and narrowed in bandwidth to 7 MHz with a novel atom-based filter operating by "interaction-free measurement" principles. At least 94% of the heralded photons are atom-resonant as demonstrated by a direct absorption measurement with rubidium vapor. A heralded auto-correlation measurement shows $g_c^{(2)}(0)=0.040 \pm 0.012$, i.e., suppression of multi-photon contributions by a factor of 25 relative to a coherent state. The generated herald…
We present a multiplexed single photon source that re-synchronises heralded single photons generated by four-wave mixing in photonic crystal fibre using a fibre delay loop controlled by a single switch. By combining the probabilities of generating heralded single photons on four consecutive pump pulses we obtain an enhancement of the per-bin single-photon delivery probability. Our source demonstrates a way in which single-photon source multiplexing may be carried out with minimised resource overhead while retaining the benefits of a robust and alignment-free platform.
We propose a scheme to implement a heralded quantum memory for single-photon polarization qubits with a single atom trapped in an optical cavity. In this scheme, an injected photon only exchanges quantum state with the atom, so that the heralded storage can be achieved by detecting the output photon. We also demonstrate that the scheme can be used for realizing the heralded quantum state transfer, exchange and entanglement distribution between distant nodes. The ability to detect whether the operation has succeeded or not is crucial for practical application.
We present an experiment of nonclassical interference between a pure heralded single-photon state and a weak coherent state. Our experiment is the first to demonstrate that spectrally pure single photons can have high interference visibility, 89.4 \pm 0.5%, with weak coherent photons. Our scheme lays the groundwork for future experiments requiring quantum interference between photons in nonclassical states and those in coherent states.
In this paper we study the spectral (temporal) properties of heralded single photon wavepackets, triggered by the detection of an idler photon in the process of parametric downconversion. The generated single photons are studied within the framework of the chronocyclic Wigner function, from which the single photon spectral width and temporal duration can be computed. We derive specific conditions on the two-photon joint spectral amplitude which result in both pure and Fourier- transform limited heralded single photons. Likewise, we present specific source geometries which lead to the fulfilmen…
We report on experimental verification of quantum non-Gaussianity of a heralded single photon state with positive Wigner function. We unambiguously demonstrate that the generated state cannot be expressed as a mixture of Gaussian states. A sufficient information to witness the quantum non-Gaussianity is obtained from a standard photon anti-correlation measurement.
A recent Brief Report [Phys. Rev. A 79, 035801 (2009)] investigates two figures of merit for heralded photon sources based on spontaneous parametric down-conversion with a continuous pump, namely the time-averaged temporal coherence between the signal and idler beams and the time-averaged conditioned second-order degree of coherence for photons in the heralded arm. However, contrary to what is claimed, no one-arm second-order effect is actually measured.
Optical quantum protocols are reliant on the production of highly pure single photons. However, most parametric heralded single photon sources possess spectral correlations, limiting the purity of the produced photon. The most common method for restoring the purity is with narrowband spectral filtering, which comes at the cost of reducing the rate of heralding detection. Here, we characterize this trade-off analytically for a large class of parametric sources. It is possible to achieve up to 20% heralding success probabilities with 90% heralded photon purities.
We present an all-fibre source of high-purity heralded single photons with an integrated conditional optical gate that reduces uncorrelated noise by almost an order of magnitude. Generating photon pairs by four-wave mixing in photonic crystal fibre, we observe with the noise gate active a factor of 7 reduction in the rate of single counts in the heralded channel with no measurable drop in coincidence count rate. In contrast to electronic post-selection of coincidence events, the real reduction in the flux of unwanted photons is beneficial for example to avoid bleaching light-sensitive samples …
We report on a source of heralded narrowband (3MHz) single photons compatible with solid-state spin-wave quantum memories based on praseodymium doped crystals. Widely non-degenerate narrow-band photon pairs are generated using cavity enhanced down conversion. One photon from the pair is at telecom wavelengths and serves as heralding signal, while the heralded single photon is at 606nm, resonant with an optical transition in Pr:YSO. The source offers a heralding efficiency of 28% and a generation rate exceeding 2000 pairs/mW in a single-mode. The single photon nature of the heralded field is co…
We report the experimental demonstration of efficient interaction of multi kilo electron Volt heralded x-ray photons with a beam splitter. The measured heralded photon rate at the outputs of the beam splitter is about 0.01 counts/s which is comparable to the rate in the absence of the beam splitter. We use this beam splitter together with photon number and photon energy resolving detectors to show directly that single x ray photons cannot split. Our experiment demonstrates the major advantage of x rays for quantum optics: the possibility to observe experimental results with high fidelity and w…
We propose a practical decoy state method with heralded single photon source for quantum key distribution (QKD). In the protocol, 3 intensities are used and one can estimate the fraction of single-photon counts. The final key rate over transmission distance is simulated under various parameter sets. Due to the lower dark count than that of a coherent state, it is shown that a 3-intensity decoy-state QKD with a heralded source can work for a longer distance than that of a coherent state.
We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral f…
We describe an experimental demonstration of a novel three-photon NOON state generator using a single source of photons based on spontaneous parametric down-conversion (SPDC). The three-photon number-entangled state is deterministically generated by the detection of a heralding photon. Interference fringes measured with an emulated three-photon absorber reveal the three-photon de Broglie wavelength and exhibit visibility > 70% without background subtraction.
High visibility on-chip quantum interference among indistinguishable single-photons from multiples sources is a key prerequisite for integrated linear optical quantum computing. Resonant enhancement in micro-ring resonators naturally enables brighter, purer and more indistinguishable single-photon production without any tight spectral filtering. The indistinguishability of heralded single-photons from multiple micro-ring resonators has not been measured in any photonic platform. Here, we report on-chip indistinguishability measurements of heralded single-photons generated from independent micr…
We present an experimental demonstration of heralded single photons prepared in pure quantum states from a parametric downconversion source. It is shown that, through controlling the modal structure of the photon pair emission, one can generate pairs in factorable states and thence eliminate the need for spectral filters in multiple-source interference schemes. Indistinguishable heralded photons were generated in two independent spectrally engineered sources, and, by performing a Hong-Ou-Mandel interference between them without spectral filters at a raw visibility of 94.4%, their purity was me…
We demonstrate a heralded quantum memory based on mapping of a photon polarization state onto a single collective-spin excitation (magnon) shared between two spatially overlapped atomic ensembles. The polarization fidelity is measured by quantum state tomography to be above 90(2)% for any input polarization, which far exceeds the classical limit of 2/3. The process also constitutes a quantum non-destructive probe that detects and regenerates a photon without touching its - potentially undetermined - polarization.
We propose and experimentally demonstrate a novel approach to a heralded single photon source based on spectral multiplexing (SMUX) and feed-forward-based spectral manipulation of photons created by means of spontaneous parametric down-conversion in a periodically-poled LiNbO3 crystal. As a proof-of-principle, we show that our 3-mode SMUX increases the heralded single-photon rate compared to that of the individual modes without compromising the quality of the emitted single-photons. We project that by adding further modes, our approach can lead to a deterministic SPS.
Due to their strict photon-number correlation, the twin beams produced in parametric down-conversion (PDC) work well for heralded state generation. Often, however, this state manipulation is distorted by the optical losses in the herald and by the higher photon-number contributions inevitable in the PDC process. In order to find feasible figures of merit for characterizing the heralded states, we investigate their normalized factorial moments of the photon number that can be accessed regardless of the optical losses in the detection. We then perform a measurement of the joint photon statistics…
Heralded single photon source (HSPS) is an important way in generating genuine single photon, having advantages of experimental simplicity and versatility. However, HSPS intrinsically suffers from the trade-off between the heralded single photon rate and the single photon purity. To overcome this, one can apply multiplexing technology in different degrees of freedom to enhance the performance of HSPS. Here, by employing spectral multiplexing and active feed-forward spectral manipulating, we demonstrate a HSPS at 1.5 μm telecom-band. Our experimental results show that the spectral multiplexing …
A simple, room-temperature, cavity- and vacuum-free interface for a photon-matter interaction is implemented. In the experiment, a heralded single photon generated by the process of spontaneous parametric down-conversion is absorbed by an ensemble of nitrogen-vacancy color centers. The broad absorption spectrum associated with the phonon sideband solves the mismatch problem of a narrow absorption bandwidth in a typical atomic medium and broadband spectrum of quantum light. The heralded single photon source is tunable in the spectral range 452-575 nm, which overlaps well with the absorption spe…
Photons have proven to be excellent carriers of quantum information, and play essential roles in numerous quantum information processing (QIP) applications. In particular, heralded single- photon sources via spontaneous parametric-down conversion (SPDC) have been a key technology for demonstrating small-scale QIP, yet their low generation efficiency is a critical limitation for further scaling up optical QIP technology. In order to efficiently overcome the probabilistic nature of SPDC, here we demonstrate time multiplexing for up to 30 time slots of a periodically pumped heralded single-photon…
Based on the signal and idler photon pairs produced in a piece of high nonlinear fiber by a pulsed pump, we characterize the heralded single photon source from both the theoretical and experimental aspects. In the theory model, started from the derived expression of Bogoliubov transformation for a broadband pulsed pump, the second-order intensity correlation function $g_c^{(2)}(0)$, heralding efficiency $H$, indistinguishability and brightness of the heralded single photons as a function of source parameters are analyzed and discussed. In the experiments, using several kinds of combinations of…
Heralded noiseless amplifcation of photons has recently been shown to provide a means to overcome losses in complex quantum communication tasks. In particular, to overcome transmission losses that could allow for the violation of a Bell inequality free from the detection loophole, for Device Independent Quantum Key Distribution (DI-QKD). Several implementations of a heralded photon amplifier have been proposed and the first proof of principle experiments realised. Here we present the first full characterisation of such a device to test its functional limits and potential for DI-QKD. This devic…
We analyze theoretically performance of four-state quantum key distribution protocols implemented with a realistic heralded single-photon source. The analysis assumes a noisy model for the detector heralding generation of individual photons via spontaneous parametric down-conversion, including dark counts and imperfect photon number resolution. We identify characteristics of the heralding detector that defines the attainable cryptographic key rate and the maximum secure distance. Approximate analytical formulas are applied to multiplexed detection and compared with results of numerical calcula…
We present, characterize, and apply a photonic quantum interface between the near infrared and telecom spectral regions. A singly resonant optical parametric oscillator (OPO) operated below threshold, in combination with external filters, generates high-rate ($>2.5\cdot10^6~{\rm s}^{-1}$) narrowband photon pairs ($\sim 7$ MHz bandwidth); the signal photons are tuned to resonance with an atomic transition in Ca$^+$, while the idler photons are at telecom wavelength. Quantum interface operation is demonstrated through high-rate absorption of single photons by a single trapped ion ($\sim 670~{\rm…
We report on an experiment demonstrating entanglement swapping of time-frequency entangled photons. We perform a frequency-resolved Bell-state measurement on the idler photons from two independent entangled photon pairs, which projects the signal photons onto a two-color Bell state. We verify entanglement in this heralded state using two-photon interference and observing quantum beating without the use of filters, indicating the presence of two-color entanglement. Our method could lend itself to use as a highly-tunable source of frequency-bin entangled single photons.
We present an experimental method for creating and verifying photon-number states created by non-degenerate, third-order nonlinear-optical photon-pair sources. By using spatially multiplexed, thresholding single-photon detectors and inverting a conditional probability matrix, we determine the photon-number probabilities created through heralded spontaneous four-wave-mixing. The deleterious effects of noise photons on reliable heralding are investigated and shown to degrade the conditional preparation of two-photon number states more than they degrade conditional single-photon states. We derive…
We demonstrate a method for time gating the standard heralded continuous- wave (cw) spontaneous parametric down-converted (SPDC) single photon source by using pulsed pumping of the optical parametric oscillator (OPO) below threshold. The narrow bandwidth, high purity, high spectral brightness and the pseudo-deterministic character make the source highly suitable for light-atom interfaces with atomic memories.
Single photon sources (SPS) are a fundamental building block for optical implementations of quantum information protocols. Among SPSs, multiple crystal heralded single photon sources seem to give the best compromise between high pair production rate and low multiple photon events. In this work, we study their performance in a practical quantum key distribution experiment, by evaluating the achievable key rates. The analysis focuses on the two different schemes, symmetric and asymmetric, proposed for the practical implementation of heralded single photon sources, with attention on the performan…
Heralded noiseless amplification based on single-photon sources and linear optics is ideally suited for long-distance quantum communication tasks based on discrete variables. We experimentally demonstrate such an amplifier, operating at telecommunication wavelengths. Coherent amplification is performed with a gain of G=1.98+/-0.2, for a state with a maximum expected gain G=2. We also demonstrate that there is no need for a stable phase reference between the initial signal state and the local auxiliary photons used by the amplifier. These results highlight the potential of heralded quantum ampl…
We experimentally demonstrate a source of nearly pure single photons in arbitrary temporal shapes heralded from a parametric down-conversion (PDC) source at telecom wavelengths. The technology is enabled by the tailored dispersion of in-house fabricated waveguides with shaped pump pulses to directly generate the PDC photons in on-demand temporal shapes. We generate PDC photons in Hermite-Gauss and frequency-binned modes and confirm a minimum purity of 0.81, even for complex temporal shapes.
Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronising stochastic events. We recently interfaced a Raman-type quantum memory with a travelling-wave heralded photon source. Here we discuss the trade-space for the spectral characteristics of such sources, and we present measurements of our source, which represents a practical compromise enabling passive stab…
Combining techniques of cavity quantum electrodynamics, quantum measurement, and quantum feedback, we have realized the heralded transfer of a polarization qubit from a photon onto a single atom with 39% efficiency and 86% fidelity. The reverse process, namely, qubit transfer from the atom onto a given photon, is demonstrated with 88% fidelity and an estimated efficiency of up to 69%. In contrast to previous work based on two-photon interference, our scheme is robust against photon arrival-time jitter and achieves much higher efficiencies. Thus, it constitutes a key step toward the implementat…
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber desig…
We describe a new scheme to fully control the joint spectrum of paired photons generated in spontaneous parametric down-conversion. We show the capability of this method to generate frequency-uncorrelated photon pairs that are pure and indistinguishable, and whose bandwidth can be readily tuned. Importantly, the scheme we propose here can be implemented in any nonlinear crystal and frequency band of interest.
Photonics is a promising platform for quantum technologies. However, photon sources and two-photon gates currently only operate probabilistically. Large-scale photonic processing will therefore be impossible without a multiplexing strategy to actively select successful events. High time-bandwidth-product quantum memories - devices that store and retrieve single photons on-demand - provide an efficient remedy via active synchronisation. Here we interface a GHz-bandwidth heralded single-photon source and a room-temperature Raman memory with a time-bandwidth product exceeding 1000. We store heral…
Beyond the use of genuine monolithic integrated optical platforms, we report here a hybrid strategy enabling on-chip generation of configurable heralded two-photon states. More specifically, we combine two different fabrication techniques, \textit{i.e.}, non-linear waveguides on lithium niobate for efficient photon-pair generation and femtosecond-laser-direct-written waveguides on glass for photon manipulation. Through real-time device manipulation capabilities, a variety of path-coded heralded two-photon states can be produced, ranging from product to entangled states. Those states are engine…
We establish heralded interaction between two remotely trapped single 40Ca+ ions through the exchange of single photons. In the sender ion, we release single photons with controlled temporal shape on the P_3/2 to D_5/2 transition and transmit them to the distant receiver ion. Individual absorption events in the receiver ion are detected by quantum jumps. For continuously generated photons, the absorption reduces significantly the lifetime of the long-lived D_5/2 state. For triggered single-photon transmission, we observe coincidence between the emission at the sender and quantum jump events at…
We propose a method to produce pure single photons with an arbitrary designed temporal shape in a heralded, lossless and scalable way. As the indispensable resource, the method uses pairs of time-energy entangled photons. To accomplish the shaping, one photon of a pair undergoes temporal modulation according to the desired shape. Subsequent frequency-resolving detection of the photon heralds its entangled counterpart in a pure quantum state with a temporal shape non-locally affected by the modulation. We found conditions for the shape of the heralded photon to reproduce the modulation function…
We propose a scheme to generate two-photon, two-atom, or atom-photon entangledstates with a coupled system of two cavities. In our scheme, two cavity photonsare exchanged by the direct inter-cavity coupling, while atoms in the cavitiessimply play the role of generating and probing them. By virtue of the highefficiency of atomic state measurement, this method enables the realization ofefficient heralded entanglement generation robust against photon loss, whichgreatly facilitates applications in quantum information processing.
We demonstrate heralded qubit amplification for Time-Bin and Fock-state qubits in an all-fibre, telecom-wavelength, scheme that highlights the simplicity, the stability and potential for fully integrated photonic solutions. Exploiting high-efficiency superconducting detectors, the gain, the fidelity and the performance of the amplifier are studied as a function of loss. We also demonstrate the first heralded Fock-state qubit amplifier without post-selection. This provides a significant advance towards demonstrating Device-Independent Quantum Key Distribution as well as fundamental tests of qua…
Heralded entangling quantum gates are an essential element for the implementation of large-scale optical quantum computation. Yet, the experimental demonstration of genuine heralded entangling gates with free-flying output photons in linear optical system, was hindered by the intrinsically probabilistic source and double-pair emission in parametric down-conversion. Here, by using an on-demand single-photon source based on a semiconductor quantum dot embedded in a micro-pillar cavity, we demonstrate a heralded controlled-NOT (CNOT) operation between two single photons for the first time. To cha…
In this paper, we investigate the long-standing gap of quantum key rate between the Weak Coherent Pulse (WCP) and Heralded Single Photon Sources(HSPS) implementation of quantum cryptographical protocol. We prove that, by utilizing the Heralded Pair Coherent State (HPCS) photon sources, such a gap can be actually filled in both BB84 and SARG quantum key distribution. Thus, a universal photon source which achieves the up-to-date optimal key rate for each transmission distance is obtained.
Heralded single photon sources are often implemented using spontaneous parametric downconversion, but their quality can be restricted by optical loss, double pair emission and detector dark counts. Here, we show that the performance of such sources can be improved using cascaded downconversion, by providing a second trigger signal to herald the presence of a single photon, thereby reducing the effects of detector dark counts. We find that for a setup with fixed detectors, an improved heralded second-order correlation function $g^{(2)}$ can always be achieved with cascaded downconversion given …
Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multi-photon events. We propose a scheme to overcome this purity-yield trade-off by suppressing multi-photon events in a cavity-enhanced SPDC via the photon blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon …
Heralding of single photon at 1550 nm from pump pulsed non degenerate spontaneous parametric downconversion is demonstrated. P(1) and P(2) of our source are 0.1871 and 2.4 x 10 ^-3 respectively. Triggering of our source is 2.16 x 10^5 trigger.s^-1. This source may be used in QKD system.
