We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber design we show that generation of single photons with very high spectral purity is feasible even in the presence of large core-radius fluctuations. At the same time, contamination from spontaneous Raman scattering is greatly mitigated by separating the single-photon frequency by more than 32 THz from the pump frequency.
We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral f…
Heralded single photon source (HSPS) is an important way in generating genuine single photon, having advantages of experimental simplicity and versatility. However, HSPS intrinsically suffers from the trade-off between the heralded single photon rate and the single photon purity. To overcome this, one can apply multiplexing technology in different degrees of freedom to enhance the performance of HSPS. Here, by employing spectral multiplexing and active feed-forward spectral manipulating, we demonstrate a HSPS at 1.5 μm telecom-band. Our experimental results show that the spectral multiplexing …
Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We est…
We present an experiment of nonclassical interference between a pure heralded single-photon state and a weak coherent state. Our experiment is the first to demonstrate that spectrally pure single photons can have high interference visibility, 89.4 \pm 0.5%, with weak coherent photons. Our scheme lays the groundwork for future experiments requiring quantum interference between photons in nonclassical states and those in coherent states.
We present an experimental method for creating and verifying photon-number states created by non-degenerate, third-order nonlinear-optical photon-pair sources. By using spatially multiplexed, thresholding single-photon detectors and inverting a conditional probability matrix, we determine the photon-number probabilities created through heralded spontaneous four-wave-mixing. The deleterious effects of noise photons on reliable heralding are investigated and shown to degrade the conditional preparation of two-photon number states more than they degrade conditional single-photon states. We derive…
We present an experimental demonstration of heralded single photons prepared in pure quantum states from a parametric downconversion source. It is shown that, through controlling the modal structure of the photon pair emission, one can generate pairs in factorable states and thence eliminate the need for spectral filters in multiple-source interference schemes. Indistinguishable heralded photons were generated in two independent spectrally engineered sources, and, by performing a Hong-Ou-Mandel interference between them without spectral filters at a raw visibility of 94.4%, their purity was me…
Spectrally uncorrelated biphoton state generated from the spontaneous nonlinear optical process is an important resource for quantum information. Currently such spectrally uncorrelated biphoton state can only be prepared from limited kinds of nonlinear media, thus limiting their wavelengths. In order to explore wider wavelength range, here we theoretically study the generation of spectrally uncorrelated biphoton state from 14 isomorphs of potassium dihydrogen phosphate (KDP) crystal. We find that 11 crystals from the `KDP family' still maintain similar nonlinear optical properties of KDP, such…
Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family', including BBO…
A scheme for heralded generation of frequency-bin photonic qubits via spontaneous four-wave mixing in a system of coupled microring resonators (photonic molecule) is developed so that the qubit state is fully controlled by the frequency amplitude of the pump field. It is shown that coupling parameters of the photonic molecule can be optimized to provide generation of nearly pure heralded photons. The heralded qubit state does not depend on the microring resonator mode frequency, thereby allowing to take advantage of frequency multiplexing for improving efficiency of quantum information process…
A novel time-domain approach using the momentum operator is used to model spontaneous four-wave mixing in a lossless nonlinear waveguide. The effects of self- and cross-phase modulation on the photon-pair production rate and heralded photon purity are investigated. We show that in the special case where only one half of the photon-pair state is filtered that the generation rate and purity of the heralded photons are unmodified by the presence of self- and cross-phase modulation. The significance of this special case arises when we consider heralded single-photon sources, where future schemes a…
On-Chip Generation of Co-Polarized and Spectrally Separable Photon Pairs
National University of Singapore（新加坡国立大学）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）；A ∗ STAR Quantum Innovation Centre (Q.InC), Agency for Science, Technology and Research (A ∗ STAR)（新加坡科技研究局A*STAR量子创新中心）；Institute of Materials Research and Engineering (IMRE), Agency for Science, Technology and Research (A ∗ STAR)（新加坡科技研究局A*STAR材料研究与工程学院）
We study the generation of correlated photon pairs and heralded single photons via strongly non-degenerate spontaneous four-wave mixing (SFWM) in a series of identical micro-/nano fibers (MNF). Joint spectral intensity of the biphoton field generated at the wavelength of about 880 nm and 1310 nm has been measured under excitation by 100 ps laser pulses demonstrating good agreement with the theoretical prediction. The measured zero-time second-order autocorrelation function was about 0.2 when the emission rate of the heralded photons was of 4 Hz. The MNF-based source perfectly matches standard …
We interface a spontaneous parametric down conversion (SPDC) crystal and a cold atomic ensemble and demonstrate a highly efficient quantum memory through polarization-encoded single-photon qubits. Specifically, narrowband heralded single photons from a cavity-enhanced SPDC source is stored using cold atomic ensemble, with ~70% storage-and-retrieval efficiency and ~10$μ$s storage time at 50% efficiency. To prevent the degradation after storage, we also manipulate the single-photon wave profile so that the retrieved non-classical nature of single photon is preserved. On the other hand, the dual-…
A recent Brief Report [Phys. Rev. A 79, 035801 (2009)] investigates two figures of merit for heralded photon sources based on spontaneous parametric down-conversion with a continuous pump, namely the time-averaged temporal coherence between the signal and idler beams and the time-averaged conditioned second-order degree of coherence for photons in the heralded arm. However, contrary to what is claimed, no one-arm second-order effect is actually measured.
We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coi…
Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (sFWM), generate an entangled (so-called, continuous-variable) quantum state that contains contri…
When building a parametric downconversion photon-pair source with spectrally separable photons, e.g. for making high-purity heralded single photons, two practical issues must be accounted for: the design of the experiment, and its characterization. To address experiment design, we study the impact on spectral separability of realistic (sech shaped and chirped) pump fields, realistic nonlinear crystals with fabrication imperfections, and undesirable PDC generation far from the central PMF peak coming from nonlinearity shaping methods. To address experiment characterization, we study the effect …
The future of integrated quantum photonics relies heavily on the ability to engineer refined methods for preparing the quantum states needed to implement various quantum protocols. An important example of such states are quantum-correlated photon pairs, which can be efficiently generated using spontaneous nonlinear processes in integrated microring-resonator structures. In this work, we propose a method for generating spectrally unentangled photon pairs from a standard microring resonator. The method utilizes interference between a primary and a delayed secondary pump pulse to effectively incr…
We report on the experimental realization and characterization of an asynchronous heralded single photon source based on spontaneous parametric down conversion. Photons at 1550nm are heralded as being inside a single-mode fiber with more than 60% probability, and the multi-photon emission probability is reduced by up to a factor 600 compared to poissonian light sources. These figures of merit, together with the choice of telecom wavelength for the heralded photons are compatible with practical applications needing very efficient and robust single photon sources.
We describe an experimental demonstration of a novel three-photon NOON state generator using a single source of photons based on spontaneous parametric down-conversion (SPDC). The three-photon number-entangled state is deterministically generated by the detection of a heralding photon. Interference fringes measured with an emulated three-photon absorber reveal the three-photon de Broglie wavelength and exhibit visibility > 70% without background subtraction.
We demonstrate a method for time gating the standard heralded continuous- wave (cw) spontaneous parametric down-converted (SPDC) single photon source by using pulsed pumping of the optical parametric oscillator (OPO) below threshold. The narrow bandwidth, high purity, high spectral brightness and the pseudo-deterministic character make the source highly suitable for light-atom interfaces with atomic memories.
We describe a new scheme to fully control the joint spectrum of paired photons generated in spontaneous parametric down-conversion. We show the capability of this method to generate frequency-uncorrelated photon pairs that are pure and indistinguishable, and whose bandwidth can be readily tuned. Importantly, the scheme we propose here can be implemented in any nonlinear crystal and frequency band of interest.
Heralding of single photon at 1550 nm from pump pulsed non degenerate spontaneous parametric downconversion is demonstrated. P(1) and P(2) of our source are 0.1871 and 2.4 x 10 ^-3 respectively. Triggering of our source is 2.16 x 10^5 trigger.s^-1. This source may be used in QKD system.
We demonstrate a monolithically integrable heralded photon source in a femtosecond laser direct written glass waveguide. The generation of photon pairs with a wide wavelength separation requires a concomitant large birefringence in the normal dispersion regime. Here, by incorporation of side-stress tracks, we produce a waveguide with a birefringence of $1.64\times~10^{-4}$ and propagation loss as low as 0.21 dB/cm near 980~nm. We measure photon pairs with 300~nm wavelength separation at an internal generation rate exceeding $5.05\times10^6$/s. The second order correlations indicate that the ge…
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
For advanced quantum information technology, sources of photon pairs in quantum mechanically factorable states are of great importance for realizing high-fidelity photon-photon quantum gate operations. Here we experimentally demonstrate a technique to produce spectrally factorable photon pairs utilizing multi-order quasi-phase-matching (QPM) conditions in spontaneous parametric downconversion (SPDC). In our scheme, a spatial nonlinearity profile of a nonlinear optical crystal is shaped with current standard poling techniques, and the associated phase-matching function can be approximated to a …
We present the optimal design for an on-chip single-photon source based on spontaneous four-wave mixing in a system of coupled ring microresonators, which provides frequency uncorrelated joint spectral amplitude of the biphoton field and thereby generation of pure single-photon heralded states. A simple method is proposed for suppressing negative dispersion effects by optimizing the controlled spectroscopic parameters of the system. It shown that the optimal coupling parameters, in combination with the optimal spectral width of the pump pulse, give rise to the highest purity of the heralded ph…
We analyze theoretically performance of four-state quantum key distribution protocols implemented with a realistic heralded single-photon source. The analysis assumes a noisy model for the detector heralding generation of individual photons via spontaneous parametric down-conversion, including dark counts and imperfect photon number resolution. We identify characteristics of the heralding detector that defines the attainable cryptographic key rate and the maximum secure distance. Approximate analytical formulas are applied to multiplexed detection and compared with results of numerical calcula…
The heralded generation of entangled states is a long-standing goal in quantum information processing, because it is indispensable for a number of quantum protocols. Polarization entangled photon pairs are usually generated through spontaneous parametric down-conversion, but the emission is probabilistic. Their applications are generally accompanied by post-selection and destructive photon detection. Here, we report a source of entanglement generated in an event-ready manner by conditioned detection of auxiliary photons. This scheme benefits from the stable and robust properties of spontaneous…
A simple, room-temperature, cavity- and vacuum-free interface for a photon-matter interaction is implemented. In the experiment, a heralded single photon generated by the process of spontaneous parametric down-conversion is absorbed by an ensemble of nitrogen-vacancy color centers. The broad absorption spectrum associated with the phonon sideband solves the mismatch problem of a narrow absorption bandwidth in a typical atomic medium and broadband spectrum of quantum light. The heralded single photon source is tunable in the spectral range 452-575 nm, which overlaps well with the absorption spe…
We propose and experimentally demonstrate a novel approach to a heralded single photon source based on spectral multiplexing (SMUX) and feed-forward-based spectral manipulation of photons created by means of spontaneous parametric down-conversion in a periodically-poled LiNbO3 crystal. As a proof-of-principle, we show that our 3-mode SMUX increases the heralded single-photon rate compared to that of the individual modes without compromising the quality of the emitted single-photons. We project that by adding further modes, our approach can lead to a deterministic SPS.
Current proposals for scalable photonic quantum technologies require on-demand sources of indistinguishable single photons with very high efficiency (having unheralded loss below $1\%$). Even with recent progress in the field there is still a significant gap between the requirements and state of the art performance. Here, we propose an on-chip source of multiplexed, heralded photons. Using quantum feedback control on a photon storage cavity with an optimized driving protocol, we estimate an on-demand efficiency of $99\%$ and unheralded loss of order $1\%$, assuming high efficiency detectors an…
Heralded single photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal and signal-signal-idler coincidences of photons generated by continuous wave pumped cavity-enhanced spontaneous pa…
Hong-Ou-Mandel (HOM) interference between independent photon sources (HOMI-IPS) is the fundamental block for quantum information processing, such as quantum gate, Shor's algorithm, Boson sampling, etc. All the previous HOMI-IPS experiments were carried out in time-domain, however, the spectral information during the interference was lost, due to technical difficulties. Here, we investigate the HOMI-IPS in spectral domain using the recently developed fast fiber spectrometer, and demonstrate the spectral distribution during the HOM interference between two heralded single-photon sources, and two…
Efficient heralded generation of entanglement together with its manipulation is of great importance for quantum communications. In addition, states generated with bandwidths naturally compatible with atomic transitions allow a more efficient mapping of light into matter which is an essential requirement for long distance quantum communications. Here we propose a scheme where the indistinguishability between two spontaneous four-wave mixing processes is engineered to herald generation of single-photon frequency-bin entangled states, i.e., single-photons shared by two distinct frequency modes. W…
Heralded single photon sources are often implemented using spontaneous parametric downconversion, but their quality can be restricted by optical loss, double pair emission and detector dark counts. Here, we show that the performance of such sources can be improved using cascaded downconversion, by providing a second trigger signal to herald the presence of a single photon, thereby reducing the effects of detector dark counts. We find that for a setup with fixed detectors, an improved heralded second-order correlation function $g^{(2)}$ can always be achieved with cascaded downconversion given …
Photons have proven to be excellent carriers of quantum information, and play essential roles in numerous quantum information processing (QIP) applications. In particular, heralded single- photon sources via spontaneous parametric-down conversion (SPDC) have been a key technology for demonstrating small-scale QIP, yet their low generation efficiency is a critical limitation for further scaling up optical QIP technology. In order to efficiently overcome the probabilistic nature of SPDC, here we demonstrate time multiplexing for up to 30 time slots of a periodically pumped heralded single-photon…
We report the experimental realization of heralded distribution of single-photon path entanglement at telecommunication wavelengths in a repeater-like architecture. The entanglement is established upon detection of a single photon, originating from one of two spontaneous parametric down conversion photon pair sources, after erasing the photon's which-path information. In order to certify the entanglement, we use an entanglement witness which does not rely on post-selection. We herald entanglement between two locations, separated by a total distance of 2 km of optical fiber, at a rate of 1.6 kH…
We report a bright and tunable source of spectrally pure heralded single photons in the telecom O-Band, based on cross-polarized four wave mixing in a commercial birefringent optical fiber. The source can achieve a purity of 85%, heralding efficiency of 30% and high coincidences to accidentals ratio of 108. Furthermore, the possibility of building multiple identical sources is explored. Through the measurements of joint spectral intensities, we find that the fiber is homogeneous over atleast 45 centimeters and can potentially realize 4 identical sources. This paves the way for a cost-effective…
We demonstrate a way to prepare single photons with a temporal envelope that resembles the time reversal of photons from the spontaneous decay process. We use the photon pairs generated from a time-ordered atomic cascade decay: the detection of the first photon of the cascade is used as a herald for the ground-state transition resonant second photon. We show how the interaction of the heralding photon with an asymmetric Fabry-Perot cavity reverses the temporal shape of its twin photon from a decaying to a rising exponential envelope. This single photon is expected to be ideal for interacting w…
Spectrally unentangled biphotons with high single-spatiotemporal-mode purity are highly desirable for many quantum information processing tasks. We generate biphotons with an inferred heralded-state spectral purity of 99%, the highest to date without any spectral filtering, by pulsed spontaneous parametric downconversion in a custom-fabricated periodically-poled KTiOPO$_4$ crystal under extended Gaussian phase-matching conditions. To efficiently characterize the joint spectral intensity of the generated biphotons at high spectral resolution, we employ a commercially available dispersion compen…
We report on quantum frequency conversion of near-infrared photons from a wavelength of 854nm to the telecommunication O-band at 1310nm with 8% overall conversion efficiency. Entangled photon pairs at 854nm are generated via type-II spontaneous parametric down conversion. One photon is mixed with a strong pump field in a nonlinear ridge waveguide for its conversion to 1310nm. We demonstrate preservation of first and second order coherence of the photons in the conversion process. Based on this we infer the coherence function of the two-photon state and compare it with the actual measured one. …
Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multi-photon events. We propose a scheme to overcome this purity-yield trade-off by suppressing multi-photon events in a cavity-enhanced SPDC via the photon blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon …
Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order tem…
We report on the quantum storage of a heralded frequency-multiplexed single photon in an integrated laser-written rare-earth doped waveguide. The single photon contains 15 discrete frequency modes separated by 261 MHz and spaning across 4 GHz. It is obtained from a non-degenerate photon pair created via cavity-enhanced spontaneous down conversion, where the heralding photon is at telecom wavelength and the heralded photon is at 606 nm. The frequency-multimode photon is stored in a praseodymium-doped waveguide using the atomic frequency comb (AFC) scheme, by creating multiple combs within the i…
We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching con…
Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous p…
The generation of heralded pure Fock states via spontaneous parametric down conversion (PDC) relies on perfect photon-number correlations in the output modes. Correlations in any other degree of freedom, however, degrade the purity of the heralded state. In this paper, we investigate spectral entanglement between the two output modes of a periodically poled waveguide. With the intent of generating heralded 1- and 2-photon Fock states, we expand the output state of the PDC to second order in photon number. We explore the effects of spectral filtering and inefficient detection, of the heralding …
We investigate different strategies suitable to generate pure heralded single photons through spontaneous parametric down-conversion, comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. Our analysis is based on the correlation of twin photons in the temporal domain,a non-standard approach that provides a physical view of the mechanisms that permit to eliminate the temporal entanglement of the state and to generate high-purity heralde…
We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely non-degenerate narrow-band ($\approx 2\,\mathrm{MHz}$) photon-pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr$^{3+}$ transition. The signal photons are stored and retrieved using the atomic frequency comb pr…
Single photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum optics. However, their non-determinism presents a bottleneck to scaling up photonic and hybrid quantum-enhanced technologies. Furthermore, photon pairs are typically emitted into many correlated frequency modes, producing an undesirable mixed state on heralding. Here we present a complete fibre-integrated heralded single photon source that addresses both these difficulties simultaneously. We use active switching to provide a path to deterministic operation by multiplexing separate s…
Interference between independent single photons is perhaps the most fundamental interaction in quantum optics. It has become increasingly important as a tool for optical quantum information science, as one of the rudimentary quantum operations, together with photon detection, for generating entanglement between non-interacting particles. Despite this, demonstrations of large-scale photonic networks involving more than two independent sources of quantum light have been limited due to the difficulty in constructing large arrays of high-quality single photon sources. Here, we solve the key challe…
We make a thorough analysis of heralded single photon sources regarding how factors such as the detector gate-period, the photon rates, the fiber coupling efficiencies, and the system losses affect the performance of the source. In the course of this we give a detailed description of how to determine fiber coupling efficiencies from experimentally measurable quantities. We show that asynchronous sources perform, under most conditions, better than synchronous sources with respect to multiphoton events, but only for nearly perfect coupling efficiencies. We apply the theory to an asynchronous sou…
