We present the optimal design for an on-chip single-photon source based on spontaneous four-wave mixing in a system of coupled ring microresonators, which provides frequency uncorrelated joint spectral amplitude of the biphoton field and thereby generation of pure single-photon heralded states. A simple method is proposed for suppressing negative dispersion effects by optimizing the controlled spectroscopic parameters of the system. It shown that the optimal coupling parameters, in combination with the optimal spectral width of the pump pulse, give rise to the highest purity of the heralded photons for a given pump linewidth.
Chirality is an important concept that describes the asymmetry property of a system, which usually emerges spontaneously due to mirror symmetry breaking. Such spontaneous chirality manifests predominantly as parity breaking in modern physics, which has been studied extensively, for instance, in Higgs physics, double-well Bose-Einstein condensates, topological insulators and superconductors. In the optical domain, spontaneous chiral symmetry breaking has been elusive experimentally, especially for micro- and nano-photonics which demands multiple identical subsystems, such as photonic nanocaviti…
Synchronization is of importance in both fundamental and applied physics, but their demonstration at the micro/nanoscale is mainly limited to low-frequency oscillations like mechanical resonators. Here, we report the synchronization of two coupled optical microresonators, in which the high-frequency resonances in optical domain are aligned with reduced noise. It is found that two types of synchronization emerge with either the first- or second-order transition, both presenting a process of spontaneous symmetry breaking. In the second-order regime, the synchronization happens with an invariant …
Composite optical systems can show compelling collective dynamics. For instance, the cooperative decay of quantum emitters into a common radiation mode can lead to superradiance, where the emission rate of the ensemble is larger than the sum of the rates of the individual emitters. Here, we report experimental evidence of super spontaneous four-wave mixing (super SFWM), an analogous effect for the generation of photon pairs in a parametric nonlinear process on an integrated photonic device. We study this phenomenon in an array of microring resonators on a silicon photonic chip coupled to bus w…
Generation of heralded single photons has recently been demonstrated using spontaneous four-wave mixing in integrated microresonators. While the results of coincidence measurements on the generated photon pairs from these systems show promise for their utility in heralding applications, such measurements do not reveal all of the effects of photon losses within the resonator. These effects, which include a significant degradation of the heralding efficiency, depend strongly on the relative strengths of the coupling of the ring modes to loss modes and channel modes. We show that the common choic…
We consider chaotic dynamics of a system of two coupled ring resonators with a linear gain and a nonlinear absorption. Such a structure can be implemented in various settings including microresonator nanostructures, polariton condensates, optical waveguides or atomic Bose-Einstein condensates of ultra-cold atoms placed in a circular-shaped trap. From the theoretical point of view this system is attractive due to its modulational instability and rich structure, including various types of spontaneous symmetry breaking, period doubling bifurcations, eventually leading to chaotic regime. It is des…
Filter-Free Indistinguishable Photon Generation from Continuous-Wave-Driven Integrated Microresonators
University of Science and Technology of China（中国科学技术大学）；Hefei National Laboratory（合肥国家实验室）；International Quantum Academy（国际量子科学院）；Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering（深圳福田南方科技大学量子技术与工程研究所）；Southern University of Science and Technology（南方科技大学）
On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limit…
We study the conditional preparation of single photons based on parametric downconversion, where the detection of one photon from a given pair heralds the existence of a single photon in the conjugate mode. We derive conditions on the modal characteristics of the photon pairs, which ensure that the conditionally prepared single photons are quantum-mechanically pure. We propose specific experimental techniques that yield photon pairs ideally suited for single-photon conditional preparation.
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber desig…
The characteristics of a single-photon emitter based on a semiconductor quantum dot, such as their indistinguishability and brightness, depend on the stability of the recombination channel, which can switch spontaneously between exciton and trion. We show that dominant recombination through neutral exciton states can be achieved by careful control of the doping profile near an epitaxial InAs/GaAs quantum dot placed in a columnar microcavity with distributed Bragg reflectors. The Hong-Ou-Mandel experiments carried out in the fabricated device demonstrate the degree of indistinguishability of 91…
We report on recent developments in the integration of optical microresonators into atom chips and describe some fabrication and implementation challenges. We also review theoretical proposals for quantum computing with single atoms based on the observation of photons leaking through the cavity mirrors. The use of measurements to generate entanglement can result in simpler, more robust and scalable quantum computing architectures. Indeed, we show that quantum computing with atom-cavity systems is feasible even in the presence of relatively large spontaneous decay rates and finite photon detect…
We show that under the influence of pure vacuum noise two entangled qubits become completely disentangled in a finite time, and in a specific example we find the time to be given by $\ln \Big(\frac{2 +\sqrt 2}{2}\Big)$ times the usual spontaneous lifetime.
We verified operational approach based on direct measurement of entanglement degree for bipartite systems. In particular spectral distributions of single counts and coincidence for pure biphoton states generated by train of short pump pulses have been measured and entanglement quantifier calculated. The approach gives upper bound of entanglement stored in total biphoton states, which can reach extremely high value up to $10^{4}-10^{5}$.
We report on the efficient generation of single photons, making use of spontaneous Raman scattering in a single trapped ion. The photons are collected through in-vacuum high-NA objectives. Photon frequency, polarization and temporal shape are controlled through appropriate laser parameters, allowing for photons in a pure quantum state.
We describe a new scheme to fully control the joint spectrum of paired photons generated in spontaneous parametric down-conversion. We show the capability of this method to generate frequency-uncorrelated photon pairs that are pure and indistinguishable, and whose bandwidth can be readily tuned. Importantly, the scheme we propose here can be implemented in any nonlinear crystal and frequency band of interest.
A scheme for heralded generation of frequency-bin photonic qubits via spontaneous four-wave mixing in a system of coupled microring resonators (photonic molecule) is developed so that the qubit state is fully controlled by the frequency amplitude of the pump field. It is shown that coupling parameters of the photonic molecule can be optimized to provide generation of nearly pure heralded photons. The heralded qubit state does not depend on the microring resonator mode frequency, thereby allowing to take advantage of frequency multiplexing for improving efficiency of quantum information process…
How to prepare deterministically non-Gaussian entangled states is a fundamental question for continuous-variable quantum information technology. Here, we theoretically demonstrate through numerical methods that the triple-photon state generated by three-photon spontaneous parametric down-conversion is a pure super-Gaussian resource of non-Gaussian entanglement. Interestingly, the degree of entanglement between the modes of the triple-photon state is stronger than that corresponding to the two-mode squeezed vacuum state produced by a quadratic Hamiltonian with the same parameters. Furthermore, …
We investigate the possibility of generating pure heralded single photons through spontaneous parametric down-conversion comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. We estimate the Schmidt number associated to the temporal modes as a function of the pump pulse duration for three particular configurations, showing how the different phase-matching conditions influences the degree of separability that can be achieved.
We study theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fiber. We show that it is possible to engineer two-photon states with specific spectral correlation (``entanglement'') properties suitable for quantum information processing applications. We focus on the case exhibiting no spectral correlations in the two-photon component of the state, which we call factorability, and which allows heralding of single-photon pure-state wave packets without the need for spectral post filtering. We show that spontaneous four wave mixing exhibit…
Exploiting semiconductor fabrication techniques, natural carriers of quantum information such as atoms, electrons, and photons can be embedded in scalable integrated devices. Integrated optics provides a versatile platform for large-scale quantum information processing and transceiving with photons. Scaling up the integrated devices for quantum applications requires highperformance single-photon generation and photonic qubit-qubit entangling operations. However, previous demonstrations report major challenges in producing multiple bright, pure and identical single-photons, and entangling multi…
We demonstrate a Hong-Ou-Mandel interference between two independent, intrinsically pure, heralded single photons from spontaneous parametric down conversion (SPDC) at telecom wavelength. A visibility of $85.5\pm8.3%$ was achieved without using any bandpass filter. Thanks to the group-velocity-matched SPDC and superconducting nanowire single photon detectors (SNSPDs), the 4-fold coincidence counts are one order higher than that in the previous experiments. The combination of bright single photon sources and SNSPDs is a crucial step for future practical quantum info-communication systems at tel…
We demonstrate extraction of randomness from spontaneous-emission events less than 36 ns in the past, giving output bits with excess predictability below $10^{-5}$ and strong metrological randomness assurances. This randomness generation strategy satisfies the stringent requirements for unpredictable basis choices in current "loophole-free Bell tests" of local realism [Hensen et al., Nature (London) 526, 682 (2015); Giustina et al., Phys. Rev. Lett. 115, 250401 (2015); Shalm et al., Phys. Rev. Lett. 115, 250402 (2015)].
We study the relationship between the collective phenomena of super and subradiance and spontaneous synchronization of quantum systems. To this aim we revisit the case of two detuned qubits interacting through a pure dissipative bosonic environment, which contains the minimal ingredients for our analysis. By using the Liouville formalism, we are able to find analytically the ultimate connection between these phenomena. We find that dynamical synchronization is due to the presence of long standing coherence between the ground state of the system and the subradiant state. We finally show that, u…
Polarization-entangled photon pairs can be efficiently prepared into pure Bell states with a high fidelity via type-II spontaneous parametric down-conversion (SPDC) of narrow-band pump light. However, the use of femtosecond pump pulses to generate multi-photon states with precise timing often requires spectral filtering to maintain a high quality of polarization entanglement. This typically reduces the efficiency of photon pair collection. We experimentally map the polarization correlations of photon pairs from such a source over a range of down-converted wavelengths with a high spectral resol…
We suggest and demonstrate a scheme for coherent nonlocal compensation of pure phase objects based on two-photon polarization and momentum entangled states. The insertion of a single phase object on one of the beams reduces the purity of the state and the amount of shared entanglement, whereas the original entanglement can be retrieved by adding a suitable phase object on the other beam. In our setup polarization and momentum entangled states are generated by spontaneous parametric downconversion and then purified using a programmable spatial light modulator, which may be also used to impose a…
We investigate different strategies suitable to generate pure heralded single photons through spontaneous parametric down-conversion, comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. Our analysis is based on the correlation of twin photons in the temporal domain,a non-standard approach that provides a physical view of the mechanisms that permit to eliminate the temporal entanglement of the state and to generate high-purity heralde…
Nonclassical motional states of matter are of interest both from a fundamental perspective but also for their potential technological applications as resources in various quantum processing tasks such as quantum teleportation, sensing, communication, and computation. In this work we explore the motional effects of a harmonically trapped, excited two-level emitter coupled to a one-dimensional (1D) photonic system. As the emitter decays it experiences a momentum recoil that entangles its motion with the emitted photon pulse. In the long-time limit the emitter relaxes to its electronic ground sta…
We demonstrate experimentally and theoretically that a coherent image of a pure phase object may be obtained by use of a spatially incoherent illumination beam. This is accomplished by employing a two-beam source of entangled photons generated by spontaneous parametric down-conversion. Though each of the beams is, in and of itself, spatially incoherent, the pair of beams exhibits higher-order inter-beam coherence. One of the beams probes the phase object while the other is scanned. The image is recorded by measuring the photon coincidence rate using a photon-counting detector in each beam. Usi…
While integrated photonics is a robust platform for quantum information processing, architectures for photonic quantum computing place stringent demands on high quality information carriers. Sources of single photons that are highly indistinguishable and pure, that are either near-deterministic or heralded with high efficiency, and that are suitable for mass-manufacture, have been elusive. Here, we demonstrate on-chip photon sources that simultaneously meet each of these requirements. Our photon sources are fabricated in silicon using mature processes, and exploit a novel dual-mode pump-delaye…
We present a detailed study on the properties of single photons generated by spontaneous parametric down conversion (SPDC) when both the spectral and spatial degrees of freedom are controlled by means of filters. Our results show that it is possible to obtain pure heralded single photons with high heralding efficiency despite the use of filters. Moreover, we report an asymmetry on the single photon properties exhibited in type-II SPDC sources that depends on choosing the signal or the idler photon as the heralding one.
We demonstrate the presence of parity-time (PT) symmetry for the non-Hermitian two-state Hamiltonian of a dissipative microwave billiard in the vicinity of an exceptional point (EP). The shape of the billiard depends on two parameters. The Hamiltonian is determined from the measured resonance spectrum on a fine grid in the parameter plane. After applying a purely imaginary diagonal shift to the Hamiltonian, its eigenvalues are either real or complex conjugate on a curve, which passes through the EP. An appropriate basis choice reveals its PT symmetry. Spontaneous symmetry breaking occurs at th…
We have computed the spectrum emitted spontaneously by a quantum dot coupled to an arbitrarily detuned single mode cavity, taking into account pure dephasing processes. We show that if the emitter is incoherent, the cavity can efficiently emit photons with its own spectral characteristics. This effect opens unique opportunities for the development of devices exploiting both cavity quantum electrodynamics effects and pure dephasing, such as wavelength stabilized single photon sources robust against spectral diffusion.
Strong-to-Weak Spontaneous Symmetry Breaking in a $(2+1)$D Transverse-Field Ising Model under Decoherence
Westlake University（西湖大学）；Westlake Institute for Advanced Study（西湖高等研究院）；Fudan University（复旦大学）；University of Tokyo（东京大学）；The Pennsylvania State University（宾夕法尼亚州立大学）
We present a source of polarization entangled photon pairs based on spontaneous parametric downconversion engineered for frequency uncorrelated telecom photon generation. Our source provides photon pairs that display, simultaneously, the key properties for high-performance quantum information and fundamental quantum science tasks. Specifically, the source provides for high heralding efficiency, high quantum state purity and high entangled state fidelity at the same time. Among different tests we apply to our source we observe almost perfect non-classical interference between photons from indep…
