We study theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fiber. We show that it is possible to engineer two-photon states with specific spectral correlation (``entanglement'') properties suitable for quantum information processing applications. We focus on the case exhibiting no spectral correlations in the two-photon component of the state, which we call factorability, and which allows heralding of single-photon pure-state wave packets without the need for spectral post filtering. We show that spontaneous four wave mixing exhibits a remarkable flexibility, permitting a wider class of two-photon states, including ultra-broadband, highly-anticorrelated states.
We present an experiment of preparing Werner state via spontaneous parametric down-conversion and controlled decoherence of photons in this paper. In this experiment two independent BBO (beta-barium borate) crystals are used to produce down-conversion light beams, which are mixed to prepare Werner state.
We study the conditional preparation of single photons based on parametric downconversion, where the detection of one photon from a given pair heralds the existence of a single photon in the conjugate mode. We derive conditions on the modal characteristics of the photon pairs, which ensure that the conditionally prepared single photons are quantum-mechanically pure. We propose specific experimental techniques that yield photon pairs ideally suited for single-photon conditional preparation.
We propose a dissipative scheme to prepare a three-dimensional entangled state for two atoms trapped in separate coupled cavities. Our work shows that both atomic spontaneous emission and cavity decay, which are two typical obstacles in unitary-dynamics-based schemes, could be utilized as resources for high-dimensional entangled state preparation without specifying initial state and controlling time precisely. Final numerical simulation with one group of experimental parameters indicates that the performance of our scheme is better than the unitary-dynamics-based scheme.
We present theoretical and experimental study of preparing maximally entangled two-photon polarization states, or Bell states, using femtosecond pulse pumped spontaneous parametric down-conversion (SPDC). First, we show how the inherent distinguishability in femtosecond pulse pumped type-II SPDC can be removed by using an interferometric technique without spectral and amplitude post-selection. We then analyze the recently introduced Bell state preparation scheme using type-I SPDC. Theoretically, both methods offer the same results, however, type-I SPDC provides experimentally superior methods …
We study photon pair generation through scalar spontaneous four-wave mixing in single-mode fibre and for frequency-degenerate pumps; we concentrate on source geometries which fulfil full group velocity matching (GVM), i.e. where the pump, signal and idler propagate at identical group velocities. We discuss two experimental techniques which permit the attainment of full GVM, and discuss the resulting two-photon state properties. In particular, we show that full GVM can lead to sources which approach phasematching unconstrained by dispersion and therefore with a remarkably large bandwidth. We al…
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state prepared two-level atom in a high-$Q$ cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom--field interaction and short-term atom--field interaction, we have determined the spatio-temporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-p…
We present a study of the spectral properties of photon pairs generated through the process of spontaneous four wave mixing (SFWM) in single mode fiber. Our analysis assumes narrowband pumps, which are allowed to be frequency-degenerate or non-degenerate. Based on this analysis, we derive conditions on the pump frequencies and on the fiber dispersion parameters which guarantee the generation of ultra-broadband photon pairs. Such photon pairs are characterized by: i) a very large degree of entanglement, and ii) a very high degree of temporal synchronization between the signal and idler photons.…
We describe an experimentally straightforward method for preparing an entangled W state of up to 100 qubits. Our repeat-until-success protocol relies on detection of single photons from collective spontaneous emission in free space. Our method allows entanglement preparation in a wide range of qubit implementations that lack entangling qubit-qubit interactions. We give detailed numerical examples for entanglement of neutral atoms in optical lattices and of nitrogen-vacancy centres in diamond. The simplicity of our method should enable preparation of mesoscopic entangled states in a number of p…
We report interferometric schemes to prepare arbitrary states of four-dimensional qudits (ququarts) based on biphoton states of ultrafast-pumped frequency-nondegenerate spontaneous parametric down-conversion. Preparation and tomographic characterization of a few examples of general single-ququart states, a pure state, a completely mixed state, and a partially-mixed state, are experimentally demonstrated.
We experimentally demonstrate the first remote state preparation of arbitrary single-qubit states, encoded in the polarization of photons generated by spontaneous parametric downconversion. Utilizing degenerate and nondegenerate wavelength entangled sources, we remotely prepare arbitrary states at two wavelengths. Further, we derive theoretical bounds on the states that may be remotely prepared for given two-qubit resources.
A simple experimental setup consisting of a spontaneous parametric down-conversion source and passive linear optics is proposed for conditional preparation of a maximally entangled polarization state of two photons. Successful preparation is unambiguously heralded by coincident detection of four auxiliary photons. The proposed scheme utilizes the down-conversion term corresponding to the generation of three pairs of photons. We analyze imperfect detection of the auxiliary photons and demonstrate that its deleterious effect on the fidelity of the prepared state can be suppressed at the cost of …
Photon pairs produced in spontaneous parametric down-conversion are naturally entangled in their transverse spatial degrees of freedom including the orbital angular momentum. Pumping a non-linear crystal with a zero order Gaussian mode produces quantum correlated signal and idler photons with equal orbital angular momentum and opposite signs. Measurements performed on one of the photons prepares the state of the other remotely. We study the remote state preparation in this system from the perspective of its potential application to Quantum Thermodynamics.
We report a novel Bell state preparation experiment. High-purity Bell states are prepared by using femtosecond pulse pumped \emph{nondegenerate} collinear spontaneous parametric down-conversion. The use of femtosecond pump pulse {\em does not} result in reduction of quantum interference visibility in our scheme in which post-selection of amplitudes and other traditional mechanisms, such as, using thin nonlinear crystals or narrow-band spectral filters are not used. Another distinct feature of this scheme is that the pump, the signal, and the idler wavelengths are all distinguishable, which is …
We have proposed a simple scheme to entangle two distant qutrits trapped in separate optical cavities. The quantum information of each qutrit is skillfully encoded on the degenerate ground states of a pair of atoms, hence the entanglement between them is relatively stable against spontaneous emission. In Lamb-Dicke limits, it is not necessary to require coincidence detections, which will relax the conditions for the experimental realization. The scheme is robust against the inefficient detections.
We discuss the generation of entangled states of two two-level atoms inside an optical cavity. The cavity mode is supposed to be coupled to a white noise with adjustable intensity. We describe how the entanglement between the atoms inside the cavity arise in such a situation. The entanglement is maximized for intermediate values of the noise intensity, while it is a monotonic function of the spontaneous rate. This resembles the phenomenon of stochastic resonance and sheds more light on the idea to exploit white noise in quantum information processing.
We study theoretically the properties of a three-photon state prepared inside a semiconductor cavity, due to the interaction between a quantum dot and an electromagnetic field, and two consecutive spontaneous parametric downconversion (SPDC) processes. Thus, we consider a scheme involving three modes of the electromagnetic field, whose frequencies are given by the SPDC processes: $ω_0 \rightarrow ω_1 + ω_2$, and $ω_2 \rightarrow ω_1 + ω_1$. Furthermore, we study the low excitation regime, in which a three-photon state is accessible within the system's dynamics.
We propose two schemes for generating the Knill-Lafamme-Milburn (KLM) states of two distant polar molecules (PMs) ensembles respectively in two transmission-line resonators (TLRs) connected by a superconducting charge qutrit (SCQ), and of two SCQs in a TLR, respectively. Both of the schemes are robust against photon decay due to the virtual excitations of the microwave photons of the TLRs, and the spontaneous emission can be suppressed owing to the virtual transitions of the SCQs in the second scheme. In addition, the schemes have high controllability and feasibility under the current availabl…
We describe a protocol capable of preparing an arbitrary state of two photons in several spatial modes using pairs of photons generated by spontaneous parametric down-conversion, linear optical elements and single-photon detectors or post-selection. The protocol involves unitary and non-unitary transformations realizable by beam splitters and phase shifters. Non-unitary transformations are implemented by attenuation filters. The protocol contains several optimization capabilities with the goal of improving overall probability of its success. We also show how entangled two-photon states require…
This work presents a feasible design of an integrated photonic circuit performing as a device for single-qubit preparation and rotations through the third-order nonlinear process of difference frequency generation (DFG) and defined in the temporal mode basis. The first stage of our circuit includes the generation of heralded single photons by spontaneous four-wave mixing in a micro-ring cavity engineered for delivering a single-photon state in a unique temporal mode. The second stage comprises the implementation of DFG in a spiral waveguide with controlled dispersion properties for reaching co…
We consider conditional photonic non-Gaussian state preparation using multimode Gaussian states and photon-number-resolving detectors in the presence of photon loss. While simulation of such state preparation is often computationally challenging, we show that obtaining the required multimode Gaussian state Fock matrix elements can be reduced to the computation of matrix functions known as loop hafnians, and develop a tailored algorithm for their calculation that is faster than previously known methods. As an example of its utility, we use our algorithm to explore the loss parameter space for t…
Two novel schemes are proposed for the dissipative preparation of large W states, of the order of ten qubits, within the context of Cavity QED. By utilizing properties of the irreducible representations of su(3), we are able to construct protocols in which it is possible to restrict the open system dynamics to a fully symmetric irreducible subspace of the total Hilbert space, and hence obtain analytic solutions for effective ground state dynamics of arbitrary sized ensembles of $Λ$ atoms within an optical cavity. In the proposed schemes, the natural decay processes of spontaneous emission and …
We investigate the spontaneous emission from an inverted Y-type atomic system coupled by three coherent fields. We use the Schrödinger equation to calculate the probability amplitudes of the wave function of the system and derive an analytical expression of the spontaneous emission spectrum to trace the origin of the spectral features. Quantum interference effects, such as the spectral line narrowing, spectrum splitting and dark resonance are observed. The number of spectral components, the spectral linewidth, and relative heights can be very different depending on the physical parameters. A v…
We propose a scheme to prepare a maximally entangled state for two Lambda-type atoms trapped in separate optical cavities coupled through an optical fiber based on the combined effect of the unitary dynamics and the dissipative process. Our work shows that the fiber loss, as well as the atomic spontaneous emission and the cavity decay, is no longer undesirable, but requisite to prepare the distributed entanglement, which is meaningful for the long distance quantum information processing tasks. Originating from an arbitrary state, the desired state could be prepared without precise time control…
We propose a simple technique for the generation of arbitrary-sized Dicke states in a chain of trapped ions. The method uses global addressing of the entire chain by two pairs of delayed but partially overlapping laser pulses to engineer a collective adiabatic passage along a multi-ion dark state. Our technique, which is a many-particle generalization of stimulated Raman adiabatic passage (STIRAP), is decoherence-free with respect to spontaneous emission and robust against moderate fluctuations in the experimental parameters. Furthermore, because the process is very rapid, the effects of heati…
Spontaneous parametric down-conversion (SPDC) is a widely used source for photonic entanglement. Years of focused research have led to a solid understanding of the process, but a cohesive analytical description of the paraxial biphoton state has yet to be achieved. We derive a general expression for the spatio-temporal biphoton state that applies universally across common experimental settings and correctly describes the non-separability of spatial and spectral modes. We formulate a criterion on how to decrease the coupling of the spatial from the spectral degree of freedom by taking into acco…
Heralded spontaneous parametric down-conversion (SPDC) has become the mainstay for single-photon state preparation in present-day photonics experiments. Because they are heralded, in principle one knows when a single photon has been prepared. However, the heralding efficiencies in experimentally realistic SPDC sources are typically very low. To overcome this, multiplexing techniques have been proposed which employ a bank of SPDC sources in parallel, and route successfully heralded photons to the output, thereby effectively boosting the heralding efficiency. However, running a large bank of ind…
We experimentally control the spectral structure of photon pairs created via spontaneous four-wave mixing in microstructured fibers. By fabricating fibers with designed dispersion, one can manipulate the photons' wavelengths, joint spectrum, and, thus, entanglement. As an example, we produce photon-pairs with no spectral correlations, allowing direct heralding of single photons in pure-state wave packets without filtering. We achieve an experimental purity of $85.9\pm1.6%$, while theoretical analysis and preliminary tests suggest 94.5% purity is possible with a much longer fiber.
We have built a quantum light source capable of producing different types of quantum states. The quantum light source is based on entangled state preparation in the process of spontaneous parametric down-conversion. The single-photon detection rate of eight-hundred thousand per second demonstrates that we have created a bright state-of-the-art quantum light source. As a part of the characterization we measured two-photon quantum interference in a Hong-Ou-Mandel interferometer.
We present an experimental method for creating and verifying photon-number states created by non-degenerate, third-order nonlinear-optical photon-pair sources. By using spatially multiplexed, thresholding single-photon detectors and inverting a conditional probability matrix, we determine the photon-number probabilities created through heralded spontaneous four-wave-mixing. The deleterious effects of noise photons on reliable heralding are investigated and shown to degrade the conditional preparation of two-photon number states more than they degrade conditional single-photon states. We derive…
Single-photon sources based on the process of spontaneous parametric down-conversion play a key role in various applied disciplines of quantum optics. We characterize intrinsic luminescence of BBO crystals as a source of non-removable noise in quantum-optics experiments. By analysing its spectral and temporal properties together with its intensity, we evaluate the impact of luminescence on single-photon state preparation using spontaneous parametric down-conversion.
We present protocols for dissipative entanglement of three trapped-ion qubits and discuss a scheme that uses sympathetic cooling as the dissipation mechanism. This scheme relies on tailored destructive interference to generate any one of six entangled W states in a three-ion qubit space. Using a beryllium-magnesium ion crystal as an example system, we theoretically investigate the protocol's performance and the effects of likely error sources, including thermal secular motion of the ion crystal, calibration imperfections, and spontaneous photon scattering. We estimate that a fidelity of $\sim$…
By using quantum Zeno dynamics, we propose a controllable approach to deterministically generate tripartite GHZ states for three atoms trapped in spatially separated cavities. The nearest-neighbored cavities are connected via optical fibers and the atoms trapped in two ends are tunably driven. The generation of the GHZ state can be implemented by only one step manipulation, and the EPR entanglement between the atoms in two ends can be further realized deterministically by Von Neumann measurement on the middle atom. Note that the duration of the quantum Zeno dynamics is controllable by switchin…
The heralded generation of entangled states is a long-standing goal in quantum information processing, because it is indispensable for a number of quantum protocols. Polarization entangled photon pairs are usually generated through spontaneous parametric down-conversion, but the emission is probabilistic. Their applications are generally accompanied by post-selection and destructive photon detection. Here, we report a source of entanglement generated in an event-ready manner by conditioned detection of auxiliary photons. This scheme benefits from the stable and robust properties of spontaneous…
We report on the experimental characterization of a novel nonlinear liquid-filled hollow-core photonic-crystal fiber for the generation of photon pairs at telecommunication wavelength through spontaneous four-wave-mixing. We show that the optimization procedure in view of this application links the choice of the nonlinear liquid to the design parameters of the fiber, and we give an example of such an optimization at telecom wavelengths. Combining the modeling of the fiber and classical characterization techniques at these wavelengths, we identify, for the chosen fiber and liquid combination, s…
The coupling between single-photon emitters and phonons opens many possibilities to store and transmit quantum properties. In this paper we apply the independent boson model to describe the coupling between an optically driven two-level system and a discrete phonon mode. Tailored optical driving allows not only to generate coherent phonon states, but also to generate coherent superpositions in the form of Schrödinger cat states in the phonon system. We analyze the influence of decay and dephasing of the two-level system on these phonon preparation protocols. We find that the decay transforms t…
Boson-sampling has emerged as a promising avenue towards post-classical optical quantum computation, and numerous elementary demonstrations have recently been performed. Spontaneous parametric down-conversion (SPDC) is the mainstay for single-photon state preparation, the technique employed in most optical quantum information processing implementations to-date. Here we present a simple architecture for boson-sampling based on multiplexed SPDC sources and demonstrate that the architecture is limited only by the post-selection detection efficiency assuming that other errors, such as spectral imp…
Understanding how correlations can be used for quantum communication protocols is a central goal of quantum information science. While many authors have linked global measures of correlations such as entanglement or discord to the performance of specific protocols, in general the latter may require only correlations between specific observables. In this work, we first introduce a general measure of correlations for two-qubit states based on the classical mutual information between local observables. We then discuss the role of the symmetry in the state's correlations distribution and according…
The study of phases is useful for understanding novel states of matter. One such state of matter are time crystals which constitute periodically driven interacting many-body systems that spontaneously break time translation symmetry. Time crystals with arbitrary periods (and dimensions) can be realized using the model of Bose-Einstein condensates bouncing on periodically-driven mirror(s). In this work, we identify the different phases that characterize the two-dimensional time crystal. By determining the optimal initial conditions and value of system parameters, we provide a practical route to…
We demonstrate sub-shot-noise photon-number correlations in a (temporal) multimode mesoscopic ($\sim 10^3$ detected photons) twin-beam produced by ps-pulsed spontaneous non-degenerate parametric downconversion. We have separately detected the signal and idler distributions of photons collected in twin coherence areas and found that the variance of the photon-count difference goes below the shot-noise limit by 3.25 dB. The number of temporal modes contained in the twin-beam, as well as the size of the twin coherence areas, depends on the pump intensity. Our scheme is based on spontaneous downco…
We propose a scheme for preparation of large-scale entangled $W$ states based on the fusion mechanism via quantum Zeno dynamics. By sending two atoms belonging to an $n$-atom $W$ state and an $m$-atom $W$ state, respectively, into a vacuum cavity (or two separate cavities), we may obtain a ($n+m-2$)-atom $W$ state via detecting the two-atom state after interaction. The present scheme is robust against both spontaneous emission of atoms and decay of cavity, and the feasibility analysis indicates that it can also be realized in experiment.
Tripartite entangled states, such as GHZ and W states, are typically generated by manipulating two pairs of polarization-entangled photons in bulk optics. Here we propose a scheme to generate W states that are entangled in the energy degree of freedom in an integrated optical circuit. Our approach employs photon pairs generated by spontaneous four-wave mixing (SFWM) in a micro- ring resonator. We also present a feasible procedure for demonstrating the generation of such a state, and we compare polarization-entangled and energy-entangled schemes for the preparation of W states.
We propose and experimentally verify a scheme to engineer arbitrary states of traveling light field up to the two-photon level. The desired state is remotely prepared in the signal channel of spontaneous parametric down-conversion by means of conditional measurements on the idler channel. The measurement consists of bringing the idler field into interference with two ancilla coherent states, followed by two single-photon detectors, which, in coincidence, herald the preparation event. By varying the amplitudes and phases of the ancillae, we can prepare any arbitrary superposition of zero- one- …
We analyze the statistics of photons originating from amplified spontaneous emission generated by a quantum dot superluminescent diode. Experimentally detectable emission properties are taken into account by parametrizing the corresponding quantum state as a multi-mode phase-randomized Gaussian density operator. The validity of this model is proven in two subsequent experiments using fast two-photon-absorption detection observing second order equal-time- as well as second order fully time-resolved intensity correlations on femtosecond timescales. In the first experiment, we study the photon st…
Cavity-assisted spontaneous parametric down-conversion (SPDC) and spontaneous four-wave mixing (SFWM) in nonlinear optical materials are practical and versatile methods to generate narrowband time-energy entangled photon pairs. Time-energy entangled photons with tailored spectro-temporal properties are particularly useful for efficient quantum optical interfaces. In this work we study the generation of photon pairs in cavity-assisted SPDC and SFWM for the general case of off-resonant conversion, namely, when the frequencies of the generated photons do not match the cavity resonances. Such a fr…
We investigate optimal discrimination between two projective quantum measurements on a single qubit. We consider scenario where the measurement that should be identified can be performed twice and we show that adaptive discrimination strategy, entangled probe states, and feed-forward all help to increase the probability of correct identification of the measurement. We also experimentally demonstrate the studied discrimination strategies and test their performance. The employed experimental setup involves projective measurements on polarization states of single photons and preparation of requir…
We analyse the influence of entanglement on the emission properties of atoms. To this end, first, we propose a scheme for the preparation of a pair of entangled Helium atoms, one in the ortho and the other in the para spin configuration. We discuss a realistic scenario for this process, based in the double ionization of He by intense laser fields. These states are used to analyse disentanglement and the role of entanglement in the spontaneous emission from the pair. In particular, we show that the decaying rate of an entangled atom is different from that in a product state, modifying the tempo…
We report measurements of two-photon interference using a cw-pumped type-II spontaneous parametric down-conversion source based on a multimode perodically poled potassium titanyl phosphate waveguide. We have used the recently demonstrated technique of controlling the spatial characteristics of the down-conversion process via intermodal dispersion to generate photon pairs in fundamental transverse modes, thus ensuring their spatial indistinguishability. Good spatial overlap of photon modes within pairs has been verified using the Hong-Ou-Mandel interferometer and the preparation of polarization…
It has been a longstanding goal in quantum optics to realize controllable sources generating joint multiphoton states, particularly, photon triplet with arbitrary spectral characteristics. We demonstrate that such sources can be realized via cascaded parametric down-conversion (PDC) in superlattice structures of nonlinear and linear segments. We consider scheme that involves two parametric processes: $ω_{0}\rightarrowω_{1}+ω_{2}$, $ω_{2}\rightarrowω_{1}+ω_{1}$ under pulsed pump and investigate spontaneous creation of photon triplet as well as generation of high-intensity mode in intracavity th…
The ability to harness light-matter interactions at the few-photon level plays a pivotal role in quantum technologies. Single photons - the most elementary states of light - can be generated on-demand in atomic and solid state emitters. Two-photon states are also key quantum assets, but achieving them in individual emitters is challenging because their generation rate is much slower than competing one-photon processes. We demonstrate that atomically thin plasmonic nanostructures can harness two-photon spontaneous emission, resulting in giant far-field two-photon production, a wealth of resonan…
Different attempts to solve the measurement problem of the quantum mechanics (QM) by denying the collapse principle, and replacing it with changes in the quantum formalism, failed because the changes in the formalism lead to contradictions with QM predictions. To the difference, Ghirardi, Rimini and Weber took the collapse as a real phenomenon, and proposed a calculus by which the wave-function should undergo a sudden localization. Later on, Ghirardi, Pearle and Rimini came with a change of this calculus into the CSL (continuous spontaneous localization) model of collapse. Both these proposals…
We propose a scheme for perfect excitation of a single two-level atom by a single photon in free space. The photon state has to match the time reversed photon state originating from spontaneous decay of a two-level system. We discuss its experimental preparation. The state is characterized by a particular asymmetric exponentially-shaped temporal profile. Any deviations from this ideal state limit the maximum absorption. Although perfect excitation requires an infinite amount of time we demonstrate that there is a class of initial one-photon quantum states which can achieve almost perfect absor…
