We present an experimental method for creating and verifying photon-number states created by non-degenerate, third-order nonlinear-optical photon-pair sources. By using spatially multiplexed, thresholding single-photon detectors and inverting a conditional probability matrix, we determine the photon-number probabilities created through heralded spontaneous four-wave-mixing. The deleterious effects of noise photons on reliable heralding are investigated and shown to degrade the conditional preparation of two-photon number states more than they degrade conditional single-photon states. We derive the equivalence between the presence of unwanted noise in the herald channel and loss in the signal channel of heralded experiments. A procedure for characterizing the noise-photon contributions, and a means of estimating the herald noise-free photon-number distribution is demonstrated.
We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral f…
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber desig…
A scheme for heralded generation of frequency-bin photonic qubits via spontaneous four-wave mixing in a system of coupled microring resonators (photonic molecule) is developed so that the qubit state is fully controlled by the frequency amplitude of the pump field. It is shown that coupling parameters of the photonic molecule can be optimized to provide generation of nearly pure heralded photons. The heralded qubit state does not depend on the microring resonator mode frequency, thereby allowing to take advantage of frequency multiplexing for improving efficiency of quantum information process…
A novel time-domain approach using the momentum operator is used to model spontaneous four-wave mixing in a lossless nonlinear waveguide. The effects of self- and cross-phase modulation on the photon-pair production rate and heralded photon purity are investigated. We show that in the special case where only one half of the photon-pair state is filtered that the generation rate and purity of the heralded photons are unmodified by the presence of self- and cross-phase modulation. The significance of this special case arises when we consider heralded single-photon sources, where future schemes a…
We study the generation of correlated photon pairs and heralded single photons via strongly non-degenerate spontaneous four-wave mixing (SFWM) in a series of identical micro-/nano fibers (MNF). Joint spectral intensity of the biphoton field generated at the wavelength of about 880 nm and 1310 nm has been measured under excitation by 100 ps laser pulses demonstrating good agreement with the theoretical prediction. The measured zero-time second-order autocorrelation function was about 0.2 when the emission rate of the heralded photons was of 4 Hz. The MNF-based source perfectly matches standard …
We interface a spontaneous parametric down conversion (SPDC) crystal and a cold atomic ensemble and demonstrate a highly efficient quantum memory through polarization-encoded single-photon qubits. Specifically, narrowband heralded single photons from a cavity-enhanced SPDC source is stored using cold atomic ensemble, with ~70% storage-and-retrieval efficiency and ~10$μ$s storage time at 50% efficiency. To prevent the degradation after storage, we also manipulate the single-photon wave profile so that the retrieved non-classical nature of single photon is preserved. On the other hand, the dual-…
A recent Brief Report [Phys. Rev. A 79, 035801 (2009)] investigates two figures of merit for heralded photon sources based on spontaneous parametric down-conversion with a continuous pump, namely the time-averaged temporal coherence between the signal and idler beams and the time-averaged conditioned second-order degree of coherence for photons in the heralded arm. However, contrary to what is claimed, no one-arm second-order effect is actually measured.
We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coi…
Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (sFWM), generate an entangled (so-called, continuous-variable) quantum state that contains contri…
We report on the experimental realization and characterization of an asynchronous heralded single photon source based on spontaneous parametric down conversion. Photons at 1550nm are heralded as being inside a single-mode fiber with more than 60% probability, and the multi-photon emission probability is reduced by up to a factor 600 compared to poissonian light sources. These figures of merit, together with the choice of telecom wavelength for the heralded photons are compatible with practical applications needing very efficient and robust single photon sources.
We demonstrate a monolithically integrable heralded photon source in a femtosecond laser direct written glass waveguide. The generation of photon pairs with a wide wavelength separation requires a concomitant large birefringence in the normal dispersion regime. Here, by incorporation of side-stress tracks, we produce a waveguide with a birefringence of $1.64\times~10^{-4}$ and propagation loss as low as 0.21 dB/cm near 980~nm. We measure photon pairs with 300~nm wavelength separation at an internal generation rate exceeding $5.05\times10^6$/s. The second order correlations indicate that the ge…
We describe an experimental demonstration of a novel three-photon NOON state generator using a single source of photons based on spontaneous parametric down-conversion (SPDC). The three-photon number-entangled state is deterministically generated by the detection of a heralding photon. Interference fringes measured with an emulated three-photon absorber reveal the three-photon de Broglie wavelength and exhibit visibility > 70% without background subtraction.
We demonstrate a method for time gating the standard heralded continuous- wave (cw) spontaneous parametric down-converted (SPDC) single photon source by using pulsed pumping of the optical parametric oscillator (OPO) below threshold. The narrow bandwidth, high purity, high spectral brightness and the pseudo-deterministic character make the source highly suitable for light-atom interfaces with atomic memories.
We describe a new scheme to fully control the joint spectrum of paired photons generated in spontaneous parametric down-conversion. We show the capability of this method to generate frequency-uncorrelated photon pairs that are pure and indistinguishable, and whose bandwidth can be readily tuned. Importantly, the scheme we propose here can be implemented in any nonlinear crystal and frequency band of interest.
Heralding of single photon at 1550 nm from pump pulsed non degenerate spontaneous parametric downconversion is demonstrated. P(1) and P(2) of our source are 0.1871 and 2.4 x 10 ^-3 respectively. Triggering of our source is 2.16 x 10^5 trigger.s^-1. This source may be used in QKD system.
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
We present the optimal design for an on-chip single-photon source based on spontaneous four-wave mixing in a system of coupled ring microresonators, which provides frequency uncorrelated joint spectral amplitude of the biphoton field and thereby generation of pure single-photon heralded states. A simple method is proposed for suppressing negative dispersion effects by optimizing the controlled spectroscopic parameters of the system. It shown that the optimal coupling parameters, in combination with the optimal spectral width of the pump pulse, give rise to the highest purity of the heralded ph…
We analyze theoretically performance of four-state quantum key distribution protocols implemented with a realistic heralded single-photon source. The analysis assumes a noisy model for the detector heralding generation of individual photons via spontaneous parametric down-conversion, including dark counts and imperfect photon number resolution. We identify characteristics of the heralding detector that defines the attainable cryptographic key rate and the maximum secure distance. Approximate analytical formulas are applied to multiplexed detection and compared with results of numerical calcula…
The heralded generation of entangled states is a long-standing goal in quantum information processing, because it is indispensable for a number of quantum protocols. Polarization entangled photon pairs are usually generated through spontaneous parametric down-conversion, but the emission is probabilistic. Their applications are generally accompanied by post-selection and destructive photon detection. Here, we report a source of entanglement generated in an event-ready manner by conditioned detection of auxiliary photons. This scheme benefits from the stable and robust properties of spontaneous…
A simple, room-temperature, cavity- and vacuum-free interface for a photon-matter interaction is implemented. In the experiment, a heralded single photon generated by the process of spontaneous parametric down-conversion is absorbed by an ensemble of nitrogen-vacancy color centers. The broad absorption spectrum associated with the phonon sideband solves the mismatch problem of a narrow absorption bandwidth in a typical atomic medium and broadband spectrum of quantum light. The heralded single photon source is tunable in the spectral range 452-575 nm, which overlaps well with the absorption spe…
We present a multiplexed single photon source that re-synchronises heralded single photons generated by four-wave mixing in photonic crystal fibre using a fibre delay loop controlled by a single switch. By combining the probabilities of generating heralded single photons on four consecutive pump pulses we obtain an enhancement of the per-bin single-photon delivery probability. Our source demonstrates a way in which single-photon source multiplexing may be carried out with minimised resource overhead while retaining the benefits of a robust and alignment-free platform.
We propose and experimentally demonstrate a novel approach to a heralded single photon source based on spectral multiplexing (SMUX) and feed-forward-based spectral manipulation of photons created by means of spontaneous parametric down-conversion in a periodically-poled LiNbO3 crystal. As a proof-of-principle, we show that our 3-mode SMUX increases the heralded single-photon rate compared to that of the individual modes without compromising the quality of the emitted single-photons. We project that by adding further modes, our approach can lead to a deterministic SPS.
Heralded single photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal and signal-signal-idler coincidences of photons generated by continuous wave pumped cavity-enhanced spontaneous pa…
We present an all-fibre source of high-purity heralded single photons with an integrated conditional optical gate that reduces uncorrelated noise by almost an order of magnitude. Generating photon pairs by four-wave mixing in photonic crystal fibre, we observe with the noise gate active a factor of 7 reduction in the rate of single counts in the heralded channel with no measurable drop in coincidence count rate. In contrast to electronic post-selection of coincidence events, the real reduction in the flux of unwanted photons is beneficial for example to avoid bleaching light-sensitive samples …
Efficient heralded generation of entanglement together with its manipulation is of great importance for quantum communications. In addition, states generated with bandwidths naturally compatible with atomic transitions allow a more efficient mapping of light into matter which is an essential requirement for long distance quantum communications. Here we propose a scheme where the indistinguishability between two spontaneous four-wave mixing processes is engineered to herald generation of single-photon frequency-bin entangled states, i.e., single-photons shared by two distinct frequency modes. W…
Heralded single photon sources are often implemented using spontaneous parametric downconversion, but their quality can be restricted by optical loss, double pair emission and detector dark counts. Here, we show that the performance of such sources can be improved using cascaded downconversion, by providing a second trigger signal to herald the presence of a single photon, thereby reducing the effects of detector dark counts. We find that for a setup with fixed detectors, an improved heralded second-order correlation function $g^{(2)}$ can always be achieved with cascaded downconversion given …
Photons have proven to be excellent carriers of quantum information, and play essential roles in numerous quantum information processing (QIP) applications. In particular, heralded single- photon sources via spontaneous parametric-down conversion (SPDC) have been a key technology for demonstrating small-scale QIP, yet their low generation efficiency is a critical limitation for further scaling up optical QIP technology. In order to efficiently overcome the probabilistic nature of SPDC, here we demonstrate time multiplexing for up to 30 time slots of a periodically pumped heralded single-photon…
We report the experimental realization of heralded distribution of single-photon path entanglement at telecommunication wavelengths in a repeater-like architecture. The entanglement is established upon detection of a single photon, originating from one of two spontaneous parametric down conversion photon pair sources, after erasing the photon's which-path information. In order to certify the entanglement, we use an entanglement witness which does not rely on post-selection. We herald entanglement between two locations, separated by a total distance of 2 km of optical fiber, at a rate of 1.6 kH…
Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order tem…
We demonstrate a way to prepare single photons with a temporal envelope that resembles the time reversal of photons from the spontaneous decay process. We use the photon pairs generated from a time-ordered atomic cascade decay: the detection of the first photon of the cascade is used as a herald for the ground-state transition resonant second photon. We show how the interaction of the heralding photon with an asymmetric Fabry-Perot cavity reverses the temporal shape of its twin photon from a decaying to a rising exponential envelope. This single photon is expected to be ideal for interacting w…
We report on quantum frequency conversion of near-infrared photons from a wavelength of 854nm to the telecommunication O-band at 1310nm with 8% overall conversion efficiency. Entangled photon pairs at 854nm are generated via type-II spontaneous parametric down conversion. One photon is mixed with a strong pump field in a nonlinear ridge waveguide for its conversion to 1310nm. We demonstrate preservation of first and second order coherence of the photons in the conversion process. Based on this we infer the coherence function of the two-photon state and compare it with the actual measured one. …
We present Hong-Ou-Mandel interference of single photons generated via two different physical processes by two independent atomic systems: scattering by a single atom, and parametric generation via four-wave mixing in a cloud of cold atoms. Without any spectral filtering, we observe a visibility of V=62$\pm$4%. After correcting for accidental coincidences, we obtain V=93$\pm$6%. The observed interference demonstrates the compatibility of the two sources, forming the basis for an efficient quantum interface between different physical systems.
Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multi-photon events. We propose a scheme to overcome this purity-yield trade-off by suppressing multi-photon events in a cavity-enhanced SPDC via the photon blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon …
We report on the quantum storage of a heralded frequency-multiplexed single photon in an integrated laser-written rare-earth doped waveguide. The single photon contains 15 discrete frequency modes separated by 261 MHz and spaning across 4 GHz. It is obtained from a non-degenerate photon pair created via cavity-enhanced spontaneous down conversion, where the heralding photon is at telecom wavelength and the heralded photon is at 606 nm. The frequency-multimode photon is stored in a praseodymium-doped waveguide using the atomic frequency comb (AFC) scheme, by creating multiple combs within the i…
Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous p…
Single photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum optics. However, their non-determinism presents a bottleneck to scaling up photonic and hybrid quantum-enhanced technologies. Furthermore, photon pairs are typically emitted into many correlated frequency modes, producing an undesirable mixed state on heralding. Here we present a complete fibre-integrated heralded single photon source that addresses both these difficulties simultaneously. We use active switching to provide a path to deterministic operation by multiplexing separate s…
The generation of heralded pure Fock states via spontaneous parametric down conversion (PDC) relies on perfect photon-number correlations in the output modes. Correlations in any other degree of freedom, however, degrade the purity of the heralded state. In this paper, we investigate spectral entanglement between the two output modes of a periodically poled waveguide. With the intent of generating heralded 1- and 2-photon Fock states, we expand the output state of the PDC to second order in photon number. We explore the effects of spectral filtering and inefficient detection, of the heralding …
We demonstrate heralded single photon generation in a CMOS-compatible silicon nanophotonic device. The strong modal confinement and slow group velocity provided by a coupled resonator optical waveguide (CROW) produced a large four-wave-mixing nonlinearity coefficient gamma_eff ~4100 W^-1 m^-1 at telecommunications wavelengths. Spontaneous four-wave-mixing using a degenerate pump beam at 1549.6 nm created photon pairs at 1529.5 nm and 1570.5 nm with a coincidence-to-accidental ratio exceeding 20. A photon correlation measurement of the signal (1529.5 nm) photons heralded by the detection of the…
We investigate different strategies suitable to generate pure heralded single photons through spontaneous parametric down-conversion, comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. Our analysis is based on the correlation of twin photons in the temporal domain,a non-standard approach that provides a physical view of the mechanisms that permit to eliminate the temporal entanglement of the state and to generate high-purity heralde…
We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely non-degenerate narrow-band ($\approx 2\,\mathrm{MHz}$) photon-pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr$^{3+}$ transition. The signal photons are stored and retrieved using the atomic frequency comb pr…
Photonics is a promising platform for quantum technologies. However, photon sources and two-photon gates currently only operate probabilistically. Large-scale photonic processing will therefore be impossible without a multiplexing strategy to actively select successful events. High time-bandwidth-product quantum memories - devices that store and retrieve single photons on-demand - provide an efficient remedy via active synchronisation. Here we interface a GHz-bandwidth heralded single-photon source and a room-temperature Raman memory with a time-bandwidth product exceeding 1000. We store heral…
We present a detailed study on the properties of single photons generated by spontaneous parametric down conversion (SPDC) when both the spectral and spatial degrees of freedom are controlled by means of filters. Our results show that it is possible to obtain pure heralded single photons with high heralding efficiency despite the use of filters. Moreover, we report an asymmetry on the single photon properties exhibited in type-II SPDC sources that depends on choosing the signal or the idler photon as the heralding one.
Interference between independent single photons is perhaps the most fundamental interaction in quantum optics. It has become increasingly important as a tool for optical quantum information science, as one of the rudimentary quantum operations, together with photon detection, for generating entanglement between non-interacting particles. Despite this, demonstrations of large-scale photonic networks involving more than two independent sources of quantum light have been limited due to the difficulty in constructing large arrays of high-quality single photon sources. Here, we solve the key challe…
We present a Heralded Photon Source based only on linear optics and weak coherent states. By time-tuning a Hong-Ou-Mandel interferometer fed with frequency-displaced coherent states, the output photons can be synchronously heralded following sub-Poisson statistics, which is indicated by the second-order correlation function ($g^2\left(0\right)=0.556$). The absence of phase-matching restrictions makes the source widely tunable, with 100-nm spectral tunability on the telecom bands. The technique presents yield comparable to state-of-the-art spontaneous parametric down-conversion-based sources, w…
We make a thorough analysis of heralded single photon sources regarding how factors such as the detector gate-period, the photon rates, the fiber coupling efficiencies, and the system losses affect the performance of the source. In the course of this we give a detailed description of how to determine fiber coupling efficiencies from experimentally measurable quantities. We show that asynchronous sources perform, under most conditions, better than synchronous sources with respect to multiphoton events, but only for nearly perfect coupling efficiencies. We apply the theory to an asynchronous sou…
Scalable generation of heralded single photons via active feed-forward switching of a fiber delay line
Institute of Space Research, German Aerospace Center（德国航空航天中心空间研究所）；Institut für Physik, Humboldt-Universität zu Berlin（柏林洪堡大学物理研究所）；Institut für Optik und Atomare Physik, Technische Universität Berlin（柏林工业大学光学与原子物理研究所）；AQLS GmbH（AQLS有限公司）
Photonic time-frequency entanglement is a promising resource for quantum information processing technologies. We investigate swapping of continuous-variable entanglement in the time-frequency degree of freedom using three-wave mixing in the low-gain regime with the aim of producing heralded biphoton states with high purity and low multi-pair probability. Heralding is achieved by combining one photon from each of two biphoton sources via sum-frequency generation to create a herald photon. We present a realistic model with pulsed pumps, investigate the effects of resolving the frequency of the h…
We report on the observation of a high visibility Hong-Ou-Mandel interference of two heralded photons emitted from a spontaneous parametric down conversion~(SPDC) pumped by continuous-wave~(cw) light. A non-degenerate photon pair at 1541~nm and 1580~nm is generated by cw-pumped SPDC through a periodically poled lithium niobate waveguide. The heralded single photon at 1541~nm is prepared by the detection of the photon at 1580~nm. We performed the experiment of the Hong-Ou-Mandel interference between heralded single photons in separated time bins and observed a high visibility interference. All …
Quantum phase transitions are usually studied in terms of Hermitian Hamiltonians. However, cold-atom experiments are intrinsically non-Hermitian due to spontaneous decay. Here, we show that non-Hermitian systems exhibit quantum phase transitions that are beyond the paradigm of Hermitian physics. We consider the non-Hermitian XY model, which can be implemented using three-level atoms with spontaneous decay. We exactly solve the model in one dimension and show that there is a quantum phase transition from short-range order to quasi-long-range order despite the absence of a continuous symmetry in…
Harnessing nonlinearities strong enough to allow two single photons to interact with one another is not only a fascinating challenge but is central to numerous advanced applications in quantum information science. Currently, all known approaches are extremely challenging although a few have led to experimental realisations with attenuated classical laser light. This has included cross-phase modulation with weak classical light in atomic ensembles and optical fibres, converting incident laser light into a non-classical stream of photon or Rydberg blockades as well as all-optical switches with a…
