We present a study of the spectral properties of photon pairs generated through the process of spontaneous four wave mixing (SFWM) in single mode fiber. Our analysis assumes narrowband pumps, which are allowed to be frequency-degenerate or non-degenerate. Based on this analysis, we derive conditions on the pump frequencies and on the fiber dispersion parameters which guarantee the generation of ultra-broadband photon pairs. Such photon pairs are characterized by: i) a very large degree of entanglement, and ii) a very high degree of temporal synchronization between the signal and idler photons. Through a numerical exercise, we find that the use of photonic crystal fiber (PCF) facilitates the fulfilment of the conditions for ultra-broadband photon pair generation; in particular, the spectral region in which emission occurs can be adjusted to particular needs through an appropriate choice of the PCF parameters. In addition, we present a novel quantum interference effect, resulting from indistinguishable pathways to the same outcome, which can occur when pumping a SFWM source with multiple spectral lines.
We introduce the concept of a quantum pulse gate (QPG), a method for accessing the intrinsic broadband spectral mode structure of ultrafast quantum states of light. This mode structure can now be harnessed for applications in quantum information processing. We propose an implementation in a PPLN waveguide, based on spectrally engineered sum frequency generation (SFG). It allows us to pick well-defined spectral broadband modes from an ultrafast multi-mode state for interconversion to a broadband mode at another frequency. By pulse-shaping the bright SFG pump beam, different orthogonal broadband…
Engineered dissipation for faster adiabatic state preparation
International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料中心）；Wilczek Quantum Center, Shanghai Institute for Advanced Studies（上海高等研究院费曼量子中心）；University of Science and Technology of China（中国科学技术大学）；Hefei National Laboratory（合肥国家实验室）；Beijing Key Laboratory of Quantum Devices, Peking University（北京大学北京量子器件重点实验室）
We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled lithium niobate waveguide with a strongly-chirped poling period. The proposed non-standard asymmetric poling mitigates phase distortions associated with the process of chirping. Asymmetric poling significantly broadens the entangled source bandwidth while preserving high visibility quantum interferometric sensing.
The shift of energy levels owing to broadband electromagnetic vacuum fluctuations, the Lamb shift, has been pivotal in the development of quantum electrodynamics and in understanding atomic spectra. Currently, small energy shifts in engineered quantum systems are of paramount importance owing to the extreme precision requirements in applications such as quantum computing. However, without a tunable environment it is challenging to resolve the Lamb shift in its original broadband case. Consequently, the observations in other than atomic systems are limited to environments comprised of narrow-ba…
We present a scheme for the dissipative preparation of an entangled steady state of two superconducting qubits in a circuit QED setup. Combining resonator photon loss, a dissipative process already present in the setup, with an effective two-photon microwave drive, we engineer an effective decay mechanism which prepares a maximally entangled state of the two qubits. This state is then maintained as the steady state of the driven, dissipative evolution. The performance of the dissipative state preparation protocol is studied analytically and verified numerically. In view of the experimental imp…
We put forward schemes to prepare photons in multi-dimensional vector states of orbital angular momentum. We show realizable light distributions that yield prescribed states with finite or infinite normal modes. In particular, we show that suitable light vortex-pancakes allow the add-drop of specific vector projections. We suggest that such photons might allow the generation of it engineered quNits in multi-dimensional quantum information systems.
I demonstrate the potential of reinforcement learning (RL) to prepare quantum states of strongly periodically driven non-linear single-particle models. The ability of Q-Learning to control systems far away from equilibrium is exhibited by steering the quantum Kapitza oscillator to the Floquet-engineered stable inverted position in the presence of a strong periodic drive within several shaking cycles. The study reveals the potential of the intra-period (micromotion) dynamics, often neglected in Floquet engineering, to take advantage over pure stroboscopic control at moderate drive frequencies. …
We present a technique to control the spatial state of a small cloud of interacting particles at low temperatures with almost perfect fidelity using spatial adiabatic passage. To achieve this, the resonant trap energies of the system are engineered in such a way that a single, well-defined eigenstate connects the initial and desired states and is isolated from the rest of the spectrum. We apply this procedure to the task of separating a well-defined number of particles from an initial cloud and show that it can be implemented in radio-frequency traps using experimentally realistic parameters.
This work presents a feasible design of an integrated photonic circuit performing as a device for single-qubit preparation and rotations through the third-order nonlinear process of difference frequency generation (DFG) and defined in the temporal mode basis. The first stage of our circuit includes the generation of heralded single photons by spontaneous four-wave mixing in a micro-ring cavity engineered for delivering a single-photon state in a unique temporal mode. The second stage comprises the implementation of DFG in a spiral waveguide with controlled dispersion properties for reaching co…
This article reviews recent progress in quasi-phasematched $χ^{(2)}$ nonlinear nanophotonics, with a particular focus on dispersion-engineered nonlinear interactions. Throughout this article, we establish design rules for the bandwidth and interaction lengths of various nonlinear processes, and provide examples for how these processes can be engineered in nanophotonic devices. In particular, we apply these rules towards the design of sources of non-classical light and show that dispersion-engineered devices can outperform their conventional counterparts. Examples include ultra-broadband optica…
We propose various schemes for the dissipative preparation of a maximally entangled steady state of two atoms in an optical cavity. Harnessing the natural decay processes of cavity photon loss and spontaneous emission, we use an effective operator formalism to identify and engineer effective decay processes, which reach an entangled steady state of two atoms as the unique fixed point of the dissipative time evolution. We investigate various aspects that are crucial for the experimental implementation of our schemes in present-day and future cavity quantum electrodynamics systems and analytical…
We propose and demonstrate a frequency-multiplexed readout scheme in 3D cQED architecture. We use four transmon qubits coupled to individual rectangular cavities which are aperture-coupled to a common rectangular waveguide feedline. A coaxial to waveguide transformer at the other end of the feedline allows one to launch and collect the multiplexed signal. The reflected readout signal is amplified by an impedance engineered broadband parametric amplifier with 380 MHz of bandwidth. This provides us high fidelity single-shot readout of multiple qubits using compact microwave circuitry, an efficie…
We study theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fiber. We show that it is possible to engineer two-photon states with specific spectral correlation (``entanglement'') properties suitable for quantum information processing applications. We focus on the case exhibiting no spectral correlations in the two-photon component of the state, which we call factorability, and which allows heralding of single-photon pure-state wave packets without the need for spectral post filtering. We show that spontaneous four wave mixing exhibit…
We demonstrate theoretically that photon-photon attraction can be engineered in the continuum of scattering states for pairs of photons propagating in a hollow-core photonic crystal fiber filled with cold atoms. The atoms are regularly spaced in an optical lattice configuration and the photons are resonantly tuned to an internal atomic transition. We show that the hard-core repulsion resulting from saturation of the atomic transitions induces bunching in the photonic component of the collective atom-photon modes (polaritons). Bunching is obtained in a frequency range as large as tens of GHz, a…
Dissipative preparation and stabilization of d-mode multinomial cat states
Institute for Quantum Materials and Technology, Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院量子材料与技术研究所）；Institute for Theory of Condensed Matter, Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院凝聚态理论研究所）；Institut de Science et d’Ingénierie Supramoléculaires (ISIS, UMR7006), University of Strasbourg and CNRS（斯特拉斯堡大学及法国国家科学研究中心超分子科学与工程研究所）
A superconducting qubit coupled to an open transmission line represents an implementation of the spin-boson model with a broadband environment. We show that this environment can be engineered by introducing partial reflectors into the transmission line, allowing to shape the spectral function, J(ω), of the spin-boson model. The spectral function can be accessed by measuring the resonance fluorescence of the qubit, which provides information on both the engineered environment and the coupling between qubit and transmission line. The spectral function of a transmission line without partial refle…
We present an impedance engineered Josephson parametric amplifier capable of providing bandwidth beyond the traditional gain-bandwidth product. We achieve this by introducing a positive linear slope in the imaginary component of the input impedance seen by the Josephson oscillator using a $λ/2$ transformer. Our theoretical model predicts an extremely flat gain profile with a bandwidth enhancement proportional to the square root of amplitude gain. We experimentally demonstrate a nearly flat 20 dB gain over a 640 MHz band, along with a mean 1-dB compression point of -110 dBm and near quantum-lim…
We propose to use the integrated aluminum nitride waveguide with engineered width variation to achieve optical frequency conversion based on $χ^{(2)}$ nonlinear effect on a photonic chip. We show that in an adiabatically tapered waveguide, the frequency conversion has a much broader bandwidth and the efficiency within the bandwidth is almost constant, which is favorable for short pulses. We demonstrate both analytically and numerically an "area law" for the frequency conversion, i.e. the product of bandwidth and efficiency is conserved as long as peak conversion efficiency does not saturate. T…
In this work, we report on the preparation of an ultra-broadband continuously-tunable, highly polarization-entangled photon-pair source covering the C+L telecom bands using a single type-II phase-matched bulk PPKTP crystal. Over 60 nm turning band of the down-converted photons is achieved experimentally. The broad tuning ability is due to operating near an extended phase match point in this crystal. The S parameter value of CHSH inequality is in the range between 2.60+/-0.04 (minimum) and 2.72+/-0.07 (maximum), which clearly demonstrates the high entanglement of the source over the whole tunab…
Strong amplification in integrated photonics is one of the most desired optical functionalities for computing, communications, sensing, and quantum information processing. Semiconductor gain and cubic nonlinearities, such as four-wave mixing and stimulated Raman and Brillouin scattering, have been among the most studied amplification mechanisms on chip. Alternatively, material platforms with strong quadratic nonlinearities promise numerous advantages with respect to gain and bandwidth, among which nanophotonic lithium niobate is one of the most promising candidates. Here, we combine quasi-phas…
We study the dissipative preparation of pure non-Gaussian states of a target mode which is coupled both linearly and quadratically to an auxiliary damped mode. We show that any pure state achieved independently of the initial condition is either (i) a cubic phase state, namely a state given by the action of a non-Gaussian (cubic) unitary on a squeezed vacuum or (ii) a (squeezed and displaced) finite superposition of Fock states. Which of the two states is realized depends on whether the transformation induced by the engineered reservoir on the target mode is canonical (i) or not (ii). We discu…
Non-Gaussian quantum states have been deterministically prepared and autonomously stabilized in single- and two-mode circuit quantum electrodynamics architectures via engineered dissipation. However, it is currently unknown how to scale up this technique to multi-mode non-Gaussian systems. Here, we upgrade dissipation engineering to collective (normal) modes of nonlinear resonator arrays and show how to stabilize multi-mode Schrodinger cat states. These states are multi-photon and multi-mode quantum superpositions of coherent states in a single normal mode delocalized over an arbitrary number …
We experimentally study a broadband implementation of the atomic frequency comb (AFC) rephasing protocol with a cryogenically cooled Pr$^{3+}$:Y$_2$SiO$_5$ crystal. To allow for storage of broadband pulses, we explore a novel regime where the input photonic bandwidth closely matches the inhomogeneous broadening of the material $(\sim5\,\textrm{GHz})$, thereby significantly exceeding the hyperfine ground and excited state splitting $(\sim10\,\textrm{MHz})$. Through an investigation of different AFC preparation parameters, we measure a maximum efficiency of $10\%$ after a rephasing time of $12.5…
The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse operation. Obtaining a full understanding of photon dynamics in such broadband devices, however, poses major challenges in the modeling and simulation of multimode non-Gaussian quantum physics, highlighting the need for sophisticated reduced models that facilitate efficient numerical study while providing useful physical insight. In this manuscript, we revie…
We present an effective operator formalism for open quantum systems. Employing perturbation theory and adiabatic elimination of excited states for a weakly driven system, we derive an effective master equation which reduces the evolution to the ground-state dynamics. The effective evolution involves a single effective Hamiltonian and one effective Lindblad operator for each naturally occurring decay process. Simple expressions are derived for the effective operators which can be directly applied to reach effective equations of motion for the ground states. We compare our method with the hither…
Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission measurement of frequency-entangled broadband photon pairs generated via parametric down-conversion with a monochromatic laser. It is observed that state-to-state dynamics in the system under study are temporally resolved by adjusting the path difference between the entangled twin beams when the entanglement time is sufficiently short. The non-classical photon corr…
Spontaneous parametric down-conversion (SPDC) is a widely used source for photonic entanglement. Years of focused research have led to a solid understanding of the process, but a cohesive analytical description of the paraxial biphoton state has yet to be achieved. We derive a general expression for the spatio-temporal biphoton state that applies universally across common experimental settings and correctly describes the non-separability of spatial and spectral modes. We formulate a criterion on how to decrease the coupling of the spatial from the spectral degree of freedom by taking into acco…
Suppression of wave scattering and the realization of transparency effects in engineered optical media and surfaces have attracted great attention in the past recent years. In this work the problem of transparency is considered for optical wave propagation in a nonlinear dielectric medium with second-order $χ^{(2)}$ susceptibility. Because of nonlinear interaction, a reference signal wave at carrier frequency $ω_1$ can exchange power, thus being amplified or attenuated,when phase matching conditions are satisfied and frequency conversion takes place. Therefore, rather generally the medium is n…
