Ting Yu, J. H. Eberly
We show that under the influence of pure vacuum noise two entangled qubits become completely disentangled in a finite time, and in a specific example we find the time to be given by $\ln \Big(\frac{2 +\sqrt 2}{2}\Big)$ times the usual spontaneous lifetime.
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We consider spontaneous emission of two two-level atoms interacting with vacuum fluctuations. We study the process of disentanglement in this system and show the possibility of changing disentanglement time by local operations.
Spontaneous disentanglement and thermalisation
通过在量子动力学中引入引发自发解纠缠与热化的非线性修正主方程，本文发现该非线性项能产生标准量子力学禁止的极限环稳态，其实验观测可为自发解纠缠假设提供重要证据。
Two recent experiments studying the potential effect of entanglement on the emission properties of excited atoms produced in molecular photodissociation have been interpreted in conflicting ways. We present a theoretical analysis of the problem, showing that the experimental results can be explained by a combination of three processes: entanglement, exchange effects associated with the identical nature of the atoms and disentanglement by spontaneous emission. According to our approach these experiments provide the first verification of the phenomenon of disentanglement by spontaneous emission.
The spontaneous disentanglement hypothesis and causality
本文提出基于最大熵原理的假说，通过拉格朗日乘数法确保与因果性一致，适用于有限维希尔伯特空间的量子系统。
Spontaneous disentanglement of indistinguishable particles
本研究提出适用于不可区分粒子的修正主方程，在玻色-哈伯德和费米-哈伯德模型中，发现退纠缠可引发量子相变。
The 'disentanglement eraser' or 'entanglement restorer' scheme allows retrieving entanglement by erasing the information about the formation of a classical (or separable) state. It suggests an analogy between the pairs of properties: entangled-separable and wave-particle, the latter as described in the 'quantum eraser'. The scheme illustrates the physical importance of information in quantum systems, and it is also useful as a building block for quantum computation. An optical setup for its simple implementation using three-photon decay in a centro-symmetrical crystal is proposed.
Disentanglement in the macroscopic limit
本研究针对宏观极限，采用具有已知精确解的多体模型，探究自发退纠缠假设，发现非局域纠缠在宏观极限下不稳定、局域纠缠未被排除稳定性，该假设可衔接微观量子性与宏观经典性。
We investigate the nature of quantum entanglement in long-range orders and spontaneous symmetry breaking. It is shown that diminishing of entanglement between the condensate mode and the rest of the system underlies off-diagonal long-range order, which is the hallmark of superconductivity and Bose-Einstein condensation. It is also revealed that disentanglement underlies various cases of long-range order and spontaneous symmetry breaking. In the course of the discussion, we also present some ideas on characterizing entanglement in many-body systems. Especially, it is shown how the connected cor…
The stability of entanglement of two atoms in a cavity is analyzed in this work. By studying the general Werner states we clarify the role of Bell-singlet state in the problem of suppression of disentanglement due to spontaneous emission. It is also shown explicitly that the final amount of entanglement depends on the initial ingredients of the Bell-singlet state.
We present a review of recent research on quantum entanglement, with special emphasis on entanglement between single atoms, processing of an encoded entanglement and its temporary evolution. Analysis based on the density matrix formalism are described. We give a simple description of the entangling procedure and explore the role of the environment in creation of entanglement and in disentanglement of atomic systems. A particular process we will focus on is spontaneous emission, usually recognized as an irreversible loss of information and entanglement encoded in the internal states of the syst…
The dynamics of entanglement between three - level atoms coupled to the common vacuum is investigated. We show that the collective effects such as collective damping, dipole - dipole interaction and the cross coupling between orthogonal dipoles, play a crucial role in the process of creation of entanglement. In particular, the additional cross coupling enhances the production of entanglement. For the specific initial states we find that the effect of delayed sudden birth of entanglement, recently invented by Ficek and Tanas [Phys. Rev. A 77, o54301(2008)] in the case of two - level atoms, can …
It is shown that the dissipation due to spontaneous emission can entangle two closely separated two-level atoms.
Spontaneous emission of graviton rates for the quantum bouncer states are evaluated.
The local-field renormalization of the spontaneous emission rate in a dielectric is explicitly obtained from a fully microscopic quantum-electrodynamical, many-body derivation of Langevin-Bloch operator equations for two-level atoms embedded in an absorptive and dispersive, linear dielectric host. We find that the dielectric local-field enhancement of the spontaneous emission rate is smaller than indicated by previous studies.
Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a π-pulse, resulting in amplified spontaneous emission. The application of a second π-pulse leads to a coherent echo of the amplified spontaneous emission that is correlated in both amplitude and phase. For small optical thicknesses, we see evidence that the amplified spontaneous emission and its echo are entangled.
The detrimental effect of spontaneous emission on the performance of control schemes designed to achieve population inversion between the ground state and a highly excited atomic state are studied using computer simulations.
We demonstrate how spontaneous emission in a cavity can be controlled by the application of a dc field. The method is specially suitable for Rydberg atoms. We present a simple argument for the control of emission.
Amplified spontaneous emission is usually treated as an incoherent noise process. Recent theoretical and experimental work using rephasing optical pulses has shown that rephased amplified spontaneous emission (RASE) is a potential source of wide bandwidth time-delayed entanglement. Due to poor echo efficiency the plain RASE protocol doesn't in theory achieve perfect entanglement. Experiments done to date show a very small amount of entanglement at best. Here we show that rephased amplified spontaneous emission can, in principle, produce perfect multimode time-delayed two mode squeezing when th…
The production of single photons using rephased amplified spontaneous emission is examined. This process produces single photons on demand with high efficiency by detecting the spontaneous emission from an atomic ensemble, then applying a population-inverting pulse to rephase the ensemble and produce a photon echo of the spontaneous emission events. The theoretical limits on the efficiency of the production are determined for several variants of the scheme. For an ensemble of uniform optical density, generating the initial spontaneous emission and its echo using transitions of different streng…
Unexpected Robustness of Multipartite Entanglement against Sudden Death from Spontaneous Emission
本研究挑战多体纠缠更易受自发辐射导致的纠缠突然死亡影响的假设，发现多体纠缠反而表现出更强的鲁棒性。
We investigate the quantum dynamics of a driven two-level system under spontaneous emission and its application in clock frequency estimation. By using a Lindblad equation to describe the system, we analytically obtain its exact solutions, which show three different regimes: Rabi oscillation, damped oscillation and overdamped decay. From the analytical solutions, we explore how the spontaneous emission affects the clock frequency estimation. We find that, under a modest spontaneous emission rate, the transition frequency can still be inferred from the Rabi oscillation. Our results provide pote…
Recent work has shown that collective single photon emission from an ensemble of resonate two-level atoms, i.e. single photon superradiance, is a rich field of study. The present paper addresses the flip side of superradiance, i.e. subradiance. Single photon subradiant states are potentially stable against collective spontaneous emission and can have ultrafast readout. In particular it is shown how many atom collective effects provide a new way to control spontaneous emission by preparing and switching between subradiant and superradiant states.
We present a dissipative protocol to engineer two $^{87}Rb$ atoms into a form of three-dimensional entangled state via spontaneous emission. The combination of coupling between ground states via microwave fields and dissipation induced by spontaneous emission make the current scheme deterministic and a stationary entangled state can always be achieved without state initialization. Moreover, this scheme can be straightforwardly generalized to preparation of an $N$-dimensional entangled state in principle.
An electronically excited atom or molecule located outside but near a planar optical waveguide can decay by spontaneous emission of a photon into a guided mode of the waveguide. We outline a QED theory for calculating the probability for this process and describe general physical insights from that theory. A couple of representative examples are discussed in detail.
We study evolution of entanglement of two two-level atoms in the presence of dissipation caused by spontaneous emission. We find explicit fromulas for the amount of entanglement as a function of time, in the case of destruction of the initial entanglement and possible creation of a transient entanglement between atoms. We also discuss how spontaneous emission influences nonlocality of states expressed by violation of Bell - CHSH inequality. It is shown that evolving system very quickly becomes local, even if entanglement is still present or produced.
It has been shown that strong Stark interaction of a quantum particle with a vacuum electromagnetic field reduces the speed of the one-quantum spontaneous radiation and leads to additional shift of frequency of radiation transition.
We investigate the spontaneous emission from an inverted Y-type atomic system coupled by three coherent fields. We use the Schrödinger equation to calculate the probability amplitudes of the wave function of the system and derive an analytical expression of the spontaneous emission spectrum to trace the origin of the spectral features. Quantum interference effects, such as the spectral line narrowing, spectrum splitting and dark resonance are observed. The number of spectral components, the spectral linewidth, and relative heights can be very different depending on the physical parameters. A v…
We study two distinct multi-level atomic models in which one transition is coupled to a Markovian reservoir, while another linked transition is coupled to a non-Markovian reservoir. We show that by choosing appropriately the density of modes of the non-Markovian reservoir the spontaneous emission to the Markovian reservoir is greatly altered. The existence of `dark lines' in the spontaneous emission spectrum in the Markovian reservoir due to the coupling to specific density of modes of the non-Markovian reservoir is also predicted.
Quasi-stationary states of the quantum system in the driving resonant field are considered without rotating wave approximation. Conditions under which the spontaneous emission could be suppressed in this system are investigated in the special case when the frequency of the driving field is essentially less than the frequency of spontaneous emission. It is shown that the characteristic parameters of the effect are substantially changed in comparison with the results corresponding to RWA. The real physical system for which the considered effects could be observed is described.
We report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse. The ensembles are Erbium ions doped into two LiNbO3 crystals with channel waveguides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emissi…
We study theoretically the effects of dissipation on the performances of a variational quantum algorithm used to approximately solve a combinatorial optimization problem, the Maximum Independent Set, on a platform of neutral atoms. We take a realistic model of dissipation with spontaneous emission, and show numerically that the detrimental effects of these incoherent processes are spontaneously attenuated by the variational nature of the procedure. We furthermore implement an alternative optimization scheme recently proposed, where one uses the expected shortfall of the mean energy as the obje…
We present a quantum error correcting code that is invariant under the conditional time evolution between spontaneous emissions and which can correct for one general error. The code presented here generalizes previous error correction codes in that not all errors lead to different error syndromes. This idea may lead to shorter codes than previously expected.
We consider local time evolution given by spontaneous emission in the system of independent two-level atoms. It is shown that all classically correlated initial states are driven into the states with transient non-zero quantum discord. Thus local creation of genuine quantum correlations can be observed in a simple physical system of non-interacting atoms which are not completely isolated from the environment.
We propose two quantum error correction schemes which increase the maximum storage time for qubits in a system of cold trapped ions, using a minimal number of ancillary qubits. Both schemes consider only the errors introduced by the decoherence due to spontaneous emission from the upper levels of the ions. Continuous monitoring of the ion fluorescence is used in conjunction with selective coherent feedback to eliminate these errors immediately following spontaneous emission events, and the conditional time evolution between quantum jumps is removed by symmetrizing the quantum codewords.
Here we discuss an effect of dephasing induced by a weak gravitational field on the collective radiation dynamics of an atomic system in timed single-photon Dicke states. We show that a photon absorbed by the stationary system of randomly placed stationary atoms is no longer spontaneously emitted in the direction of the impinging photon. Gravity leads to broadening of the angular distribution of emission.
We derive spontaneous emission rate and line shift for two-level atoms coupled to the radiation field using causal perturbation theory. In this approach, employing the theory of distribution splitting prevents the occurrence of divergent integrals. Our method confirms the result for atomic decay rate but suggests that the cutoff frequency for the atomic line shift is determined by the atomic mass, rather than Bohr radius or electron mass.
We discuss a simple example demonstrating that spontaneous emission from "space-time-superposed" atomic center-of-mass wave packets is nontrivially and time-dependent modified with respect to the standard dipole-pattern typical of "space-superposed" wave packets. Our approach provides an approximate description of a nonsimultaneous interaction of electromagnetic field with different parts of a wave packet.
We compute the modification in the spontaneous emission rate for a two-level atom when it is located between two parallel plates of different nature: a perfectly conducting plate $(ε\to \infty)$ and an infinitely permeable one $(μ\to \infty)$. We also discuss the case of two infinitely permeable plates. We compare our results with those found in the literature for the case of two perfectly conducting plates.
We present a fully quantum mechanical treatment of optically rephased photon echoes. These echoes exhibit noise due to amplified spontaneous emission, however this noise can be seen as a consequence of the entanglement between the atoms and the output light. With a rephasing pulse one can get an "echo" of the amplified spontaneous emission, leading to light with nonclassical correlations at points separated in time, which is of interest in the context of building wide bandwidth quantum repeaters. We also suggest a wideband version of DLCZ protocol based on the same ideas.
The problem of spontaneous emission is studied by a direct computer simulation of the dynamics of a combined system: atom + radiation field. The parameters of the discrete finite model, including up to 20k field oscillators, have been optimized by a comparison with the exact solution for the case when the oscillators have equidistant frequencies and equal coupling constants. Simulation of the effect of multi-pulse sequence of phase kicks and emission by a pair of atoms shows that both the frequency and the linewidth of the emitted spectrum could be controlled.
We demonstrate strong confinement of the optical field by depositing a micron sized metallic disk on a planar interferential mirror. Zero dimensional Tamm plasmon modes are evidenced both experimentally and theoretically, with a lateral confinement limited to the disk area and strong coupling to TE polarized fields. Single quantum dots deterministically coupled to these modes are shown to experience acceleration of their spontaneous emission when spectrally resonant with the mode. For quantum dots spectrally detuned from the confined Tamm Plasmon mode, an inhibition of spontaneous emission by …
Non dispersive electronic Rydberg wave packets may be created in atoms illuminated by a microwave field of circular polarization. We discuss the spontaneous emission from such states and show that the elastic incoherent component (occuring at the frequency of the driving field) dominates the spectrum in the semiclassical limit, contrary to earlier predictions. We calculate the frequencies of single photon emissions and the associated rates in the "harmonic approximation", i.e. when the wave packet has approximately a Gaussian shape. The results agree well with exact quantum mechanical calculat…
Controlling the spontaneous emission of trapped ions
提出基于空间光调制器的囚禁离子自发辐射操控装置，可实现单光子探测多离子纠缠及发射体可见度控制，适用于现有离子阱。
We have measured the variation of the spontaneous emission rate with polarization for self-assembled single quantum dots in two-dimensional photonic crystal membranes. We observe a maximum anisotropy factor of 6 between the decay rates of the two bright exciton states. This large anisotropy is attributed to the substantially different projected local density of optical states for differently oriented dipoles in the photonic crystal.
We study the probe spectrum of light generated by spontaneous emission into the mode of a cavity QED system. The probe spectrum has a maximum on-resonance when the number of inverted atoms for an input drive is maximal. For a larger number of atoms N, the maximum splits and develops into a doublet, but its frequencies are different from those of the so-called vacuum Rabi splitting.
We study the collective spontaneous emission of three identical two-level atoms initially prepared in the excited states by measuring Glauber's third-order photon correlation function. Assuming two atoms at sub-wavelength distance from each other such that they are subject to the dipole-dipole interaction while the third one is located several wavelengths away, we observe super- and subradiant decay alike, depending on the direction of observation. Unlike the case where no remote atom is introduced or no conditional measurements are performed, the spontaneous emission behavior of the condition…
We revisit the back-action of emitted photons on the motion of the relative position of two cold atoms. We show that photon recoil resulting from the spontaneous emission can induce the localization of the relative position of the two atoms through the entanglement between the spatial motion of individual atoms and their emitted photons. The result provides a more realistic model for the analysis of the environment-induced localization of a macroscopic object.
We present a very simple model of a spontaneous emission from a two-level atom, interacting with a field of a finite number of states. Such a process is often said to occur because of the large number of equally-probable states of environment. We show that in our model increasing the number of field states may and may not cause a practically permanent emission, depending on the details of the model. We also describe how irreversibility emerges with growing number of states. Mathematical tools are reduced to a necessary minimum and hopefully can be well understood by undergraduate students.
We investigate decoherence of quantum superpositions induced by gravitational time dilation and spontaneous emission between two atomic levels. It has been shown that gravitational time dilation can be an universal decoherence source. Here, we consider decoherence induced by gravitational time dilation only in the situation of spontaneous emission. Then, we obtain that the coherence of particle's position state depends on reference frame due to the time dilation changing the distinguishability of emission photon from two positions of particle. Changing the direction of light field can also res…
In a previous paper [B. Deb and G. S. Agarwal, Phys. Rev. A 90, 063417 (2014)], it was theoretically shown that, magneto-optical manipulation of low energy scattering resonances and atom-molecule transitions could lead to the formation of a bound state in continuum (BIC), provided there is no spontaneous emission. We find that even an exceedingly small spontaneous decay from exited molecular states can spoil the BIC. In this paper, we show how to circumvent the detrimental effect of spontaneous emission by making use of vacuum-induced coherence (VIC) which results in the cancellation or suppre…
Quantum-Referenced Spontaneous Emission Tomography
提出量子参考自发发射断层扫描（Q-SpET），利用目标源与参考源的量子干涉，通过四次光谱分辨测量提取自发发射光子对的联合光谱相位，并在微环谐振器源上验证其与受激发射的差异。
The q-deformation of a single quantized radiation mode interacting with a collection of two level atoms is introduced, analysing its effects on the cooperative behavior of the system.
Hilbert - Schmidt and trace norm geometric quantum discord are compared with regard to their behavior during local time evolution. We consider the system of independent two - level atoms with time evolution given by the dissipative process of spontaneous emission. It is explicitly shown that the Hilbert - Schmidt norm discord has nonphysical properties with respect to such local evolution and cannot serve as a reasonable measure of quantum correlations and the better choice is to use trace norm discord as such a measure.
A universal and fault tolerant scheme for quantum computation is proposed which utilizes a class of error correcting codes that is based on the detection of spontaneous emission (of, e.g., photons, phonons, and ripplons). The scheme is compatible with a number of promising solid-state and quantum-optical proposals for quantum computer implementations, such as quantum dots in cavities, electrons on helium, and trapped ions.
The spontaneous emission is investigated for an effective atomic two-level system in an intense coherent field with frequency lower than the vacuum-induced decay width. As this additional low-frequency field is assumed to be intense, multiphoton processes may be induced, which can be seen as alternative transition pathways in addition to the simple spontaneous decay. The interplay of the various interfering transition pathways influences the decay dynamics of the two-level system and may be used to slow down the spontaneous decay considerably. We derive from first principles an expression for …
In this work, we consider atomic spontaneous emission in a system consisting of two identical two-level atoms interacting dispersively with the quantized electromagnetic field in a high-Q cavity. We investigate the destructive effect of the atomic decay on the generation of maximally entangled states, following the proposal by Zheng S B and Guo G C (2000 Phys. Rev. Lett. 85 2392). In particular, we analyze the fidelity of teleportation performed using such a noisy channel and calculatethe maximum spontaneous decay rate we may have in order to realize teleportation.
We study the possibility to enhance the phase space density of non-interacting particles submitted to a classical laser field without spontaneous emission. We clearly state that, when no spontaneous emission is present, a quantum description of the atomic motion is more reliable than semi-classical description which can lead to large errors especially if no care is taken to smooth structures smaller than the Heisenberg uncertainty principle. Whatever the definition of position - momentum phase space density, its gain is severely bounded especially when started from a thermal sample. More preci…
Spontaneous Emission from Electronic Metastable Resonance States
本文提出利用复标度变换和激发束缚态方法计算亚稳态共振态的自发辐射衰减率，并通过双势垒势示例验证了该方法的快速收敛性，为多电子系统等复杂体系中的亚稳态自发辐射研究提供了新途径。
We have theoretically studied the effect of deterministic temporal control of spontaneous emission in a dynamic optical microcavity. We propose a new paradigm in light emission: we envision an ensemble of two-level emitters in an environment where the local density of optical states is modified on a time scale shorter than the decay time. A rate equation model is developed for the excited state population of two-level emitters in a time-dependent environment in the weak coupling regime in quantum electrodynamics. As a realistic experimental system, we consider emitters in a semiconductor micro…
We study the light generated by spontaneous emission into a mode of a cavity QED system under weak excitation of the orthogonally polarized mode. Operating in the intermediate regime of cavity QED with comparable coherent and decoherent coupling constants, we find an enhancement of the emission into the undriven cavity mode by more than a factor of 18.5 over that expected by the solid angle subtended by the mode. A model that incorporates three atomic levels and two polarization modes quantitatively explains the observations.
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