The optimal superconductivity ($T_c \approx 30 $ K) in BaFe$_2$(As$_{1-x}$P$_x$)$_2$ can be reached when the coupled antiferromagnetic (AF) order ($T_N$) and orthorhombic lattice distortion ($T_s$) are suppressed to zero temperature with increasing of P concentration or hydrostatic pressure. Here we use transport and neutron scattering to study the $c$-axis pressure effects on electronic phases in underdoped BaFe$_2$(As$_{0.72}$P$_{0.28}$)$_2$, which has $T_N = T_s\approx 40$ K and $T_c \approx $ 28 K at zero pressure. With increasing $c$-axis pressure, $T_N$ and $T_s$ are slightly enhanced around $P_c \sim 20 $ MPa. Upon further increasing pressure, AF order is gradually suppressed to zero, while $T_c$ is enhanced to 30 K. Our results reveal the importance of magnetoelastic couplings in BaFe$_2$(As$_{1-x}$P$_x$)$_2$, suggesting that the $c$-axis pressure can be used as a tuning parameter to manipulate the electronic phases in iron pnictides.
Polarized inelastic neutron scattering experiments were performed to study magnetic excitations in the normal and superconducting phases of Co-underdoped BaFe$_2$As$_2$, which exhibits coexistence of antiferromagnetic order and superconductivity. In the normal state the antiferromagnetic order results in broadened spin gaps opening in all three spin directions that are reminiscent of the magnetic response in pure antiferromagnetic BaFe$_2$As$_2$. In particular longitudinal excitations exhibit a large gap. In the superconducting state we find two distinct resonance excitations, which both are a…
We report magnetic force microscopy (MFM) measurements on underdoped $BaFe_2(As_{1-x}P_x)_2$ ($x=0.26$) that show enhanced superconductivity along stripes parallel to twin boundaries. These stripes of enhanced diamagnetic response repel vortices when we cool in a finite magnetic field and act as barriers when we drag vortices with the magnetic MFM tip. The stripes disappear when we warm the sample towards the superconducting transition temperature. We show that stripes can move when we warm the sample and comment on the relationship between the stripes and similar stripes observed previously i…
We use neutron scattering to study the effect of uniaxial pressure on the tetragonal-to-orthorhombic structural ($T_s$) and paramagnetic-to-antiferromagnetic ($T_N$) phase transitions in NaFeAs and compare the outcome with similar measurements on as-grown and annealed BaFe$_2$As$_2$. In previous work on as-grown BaFe$_2$As$_2$, uniaxial pressure necessary to detwin the sample was found to induce a significant increase in zero pressure $T_N$ and $T_s$. However, we find that similar uniaxial pressure used to detwin NaFeAs and annealed BaFe$_2$As$_2$ has a very small effect on their $T_N$ and $T_…
We use neutron scattering to study magnetic order and spin excitations in BaFe$_{1.96}$Ni$_{0.04}$As$_{2}$. On cooling, the system first changes the lattice symmetry from tetragonal to orthoromhbic near $\sim$97 K, and then orders antiferromagnetically at $T_N=91$ K before developing weak superconductivity below $\sim$15 K. Although superconductivity appears to co-exist with static antiferromagnetic order from transport and neutron diffraction measurement, inelastic neutron scattering experiments reveal that magnetic excitations do not respond to superconductivity. Instead, the effect of elect…
We investigate the evolution of the electrical resistivity of BaFe2As2 single crystals with pressure. The samples used were from the same batch grown from self flux and showed properties that were highly reproducible. Samples were pressurised using three different pressure media: pentane-isopentane (in a piston cylinder cell), Daphne oil (in an alumina anvil cell) and steatite (in a Bridgman cell). Each pressure medium has its own intrinsic level of hydrostaticity, which dramatically affects the phase diagram. An increasing uniaxial pressure component in this system quickly reduces spin densit…
The effect of uniaxial tensile stress and the resultant strain on the structural/magnetic transition in the parent compound of the iron arsenide superconductor, BaFe$_2$As$_2$, is characterized by temperature-dependent electrical resistivity, x-ray diffraction and quantitative polarized light imaging. We show that strain induces a measurable uniaxial structural distortion above the first-order magnetic transition and significantly smears the structural transition. This response is different from that found in another parent compound, SrFe$_2$As$_2$, where the coupled structural and magnetic tr…
We report neutron scattering measurements on single crystals of BaFe$_{1.92}$Co$_{0.08}$As$_2$. The magnetic Bragg peak intensity is reduced by 6 % upon cooling through T$_C$. The spin dynamics exhibit a gap of 8 meV with anisotropic three-dimensional (3d) interactions. Below T$_C$ additional intensity appears at an energy of $\sim$4.5(0.5) meV similar to previous observations of a spin resonance in other Fe-based superconductors. No further gapping of the spin excitations is observed below T$_C$ for energies down to 2 meV. These observations suggest the redistribution of spectral weight from …
We report neutron scattering experiments probing the influence of uniaxial strain on both the magnetic and structural order parameters in the parent iron pnictide compound, BaFe$_2$As$_2$. Our data show that modest strain fields along the in-plane orthorhombic b-axis can affect significant changes in phase behavior simultaneous to the removal of structural twinning effects. As a result, we demonstrate in BaFe$_2$As$_2$ samples detwinned via uniaxial strain that the in-plane C$_4$ symmetry is broken by \textit{both} the structural lattice distortion \textit{and} long-range spin ordering at temp…
We use transport and inelastic neutron scattering measurements to investigate single crystals of iron pnictide BaFe$_{2-x}$Ni$_{x}$As$_{2}$ ($x=0,0.03$), which exhibit a tetragonal-to-orthorhombic structural transition at $T_s$ and stripe antiferromagnetic order at $T_N$ ($T_s\geq T_N$). Using a tunable uniaxial pressure device, we detwin the crystals and study their transport and spin excitation properties at antiferromagnetic wave vector $S_1(1,0)$ and its 90$^\circ$ rotated wave vector $S_2(0,1)$ under different pressure conditions. We find that uniaxial pressure necessary to detwin and mai…
A small in-plane external uniaxial pressure has been widely used as an effective method to acquire single domain iron pnictide BaFe$_2$As$_2$, which exhibits twin-domains without uniaxial strain below the tetragonal-to-orthorhombic structural (nematic) transition temperature $T_s$. Although it is generally assumed that such a pressure will not affect the intrinsic electronic/magnetic properties of the system, it is known to enhance the antiferromagnetic (AF) ordering temperature $T_N$ ($<T_s$) and create in-plane resistivity anisotropy above $T_s$. Here we use neutron polarization analysis to …
Starting from the orthorhombic magnetically ordered phase, we investigate the effects of uniaxial tensile and compressive stresses along a, b, and the diagonal a+b directions in BaFe2As2 and CaFe2As2 in the framework of ab initio density functional theory (DFT) and a phenomonological Ginzburg-Landau model. While -contrary to the application of hydrostatic or c-axis uniaxial pressure- both systems remain in the orthorhombic phase with a pressure-dependent nonzero magnetic moment, we observe a sign-changing jump in the orthorhombicity at a critical uniaxial pressure, accompanied by a reversal of…
We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFe$_2$As$_2$ and its Co- and Ni-substituted members near optimal superconductivity. In the low temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11$\%$ increase under 40 MPa for BaFe$_{1.9}$Co$_{0.1}$As$_2$, and a 15$\%$ increase for BaFe$_{1.915}$Ni$_{0.085}$As$_2$. We also observe an increase of the AF ordering temperature ($T_N$) of about …
We have performed electrical resistivity measurements on single crystal BaFe2As2 under high pressure P up to 16 GPa with a cubic anvil apparatus, and up to 3 GPa with a modified Bridgman anvil cell. The samples were obtained from the same batch, which was grown with a self-flux method. A cubic anvil apparatus provides highly hydrostatic pressure, and a modified Bridgman anvil cell, which contains liquid pressure transmitting medium, provides quasi hydrostatic pressure. For highly hydrostatic pressure, the crystal phase and magnetic transition temperature decreases robustly with P and disappear…
We use neutron resonance spin echo and Larmor diffraction to study the effect of uniaxial pressure on the tetragonal-to-orthorhombic structural ($T_s$) and antiferromagnetic (AF) phase transitions in iron pnictides BaFe$_{2-x}$Ni$_{x}$As$_{2}$ ($x=0,0.03,0.12$), SrFe$_{1.97}$Ni$_{0.03}$As$_2$, and BaFe$_2$(As$_{0.7}$P$_{0.3}$)$_2$. In antiferromagnetically ordered BaFe$_{2-x}$Ni$_{x}$As$_{2}$ and SrFe$_{1.97}$Ni$_{0.03}$As$_2$ with $T_N$ and $T_s$ ($T_N\leq T_s$), a uniaxial pressure necessary to detwin the sample also increases $T_N$, smears out the structural transition, and induces an ortho…
Raman scattering can detect spontaneous point-group symmetry breaking without resorting to single-domain samples. Here we use this technique to study $\mathrm{BaFe_2As_2}$, the parent compound of the "122" Fe-based superconductors. We show that an applied compression along the Fe-Fe direction, which is commonly used to produce untwinned orthorhombic samples, changes the structural phase transition at temperature $T_{\mathrm{s}}$ into a crossover that spans a considerable temperature range above $T_{\mathrm{s}}$. Even in crystals that are not subject to any applied force, a distribution of subs…
We present the ultra-low-temperature heat transport study of iron-based superconductors Ba(Fe$_{1-x}$Ru$_x$)$_2$As$_2$ and BaFe$_2$(As$_{1-x}$P$_x$)$_2$. For optimally doped Ba(Fe$_{0.64}$Ru$_{0.36}$)$_2$As$_2$, a large residual linear term $κ_0/T$ at zero field and a $\sqrt{H}$ dependence of $κ_0(H)/T$ are observed, which provide strong evidences for nodes in the superconducting gap. This result demonstrates that the isovalent Ru doping can also induce nodal superconductivity, as P does in BaFe$_2$(As$_{0.67}$P$_{0.33}$)$_2$. Furthermore, in underdoped Ba(Fe$_{0.77}$Ru$_{0.23}$)$_2$As$_2$ and…
Strange Metal Hall Effect in Underdoped BaFe$_2$(As$_{1-x}$P$_x$)$_2$
University of California, Berkeley(加州大学伯克利分校);Lawrence Berkeley National Laboratory(劳伦斯伯克利国家实验室);Max Planck Institute for the Structure and Dynamics of Matter(马克斯·普朗克物质与结构动态研究所);National High Magnetic Field Laboratory(国家强磁场实验室);Los Alamos National Laboratory(洛斯阿拉莫斯国家实验室);Boston University(波士顿大学)
We report a systematic investigation on c-axis point-contact Andreev reflection (PCAR) in BaFe$_{2-x}$Ni$_x$As$_2$ superconducting single crystals from underdoped to overdoped regions (0.075 $\leq x\leq 0.15$). At optimal doping ($x=0.1$) the PCAR spectrum feature the structures of two superconducting gap and electron-boson coupling mode. In the $s\pm$ scenario, quantitative analysis using a generalized Blonder-Tinkham-Klapwijk (BTK) formalism with two gaps: one isotropic and another angle dependent, suggest a nodeless state in strong-coupling limit with gap minima on the Fermi surfaces. Upon …
TThe parent compounds of iron-arsenide superconductors, $A$Fe$_{2}$As$_{2}$ ($A$=Ca, Sr, Ba), undergo a tetragonal to orthorhombic structural transition at a temperature $T_{\mathrm{TO}}$ in the range 135 to 205K depending on the alkaline earth element. Below $T_{\mathrm{TO}}$ the free standing crystals split into equally populated structural domains, which mask intrinsic, in-plane, anisotropic properties of the materials. Here we demonstrate a way of mechanically detwinning CaFe$_{2}$As$_{2}$ and BaFe$_{2}$As$_{2}$. The detwinning is nearly complete, as demonstrated by polarized light imaging…
We investigate the in-plane anisotropy of Fe 3d orbitals occurring in a wide temperature and composition range of BaFe2(As1-xPx)2 system. By employing the angle-resolved photoemission spectroscopy, the lifting of degeneracy in dxz and dyz orbitals at the Brillouin zone corners can be obtained as a measure of the orbital anisotropy. In the underdoped regime, it starts to evolve on cooling from high temperatures above both antiferromagnetic and orthorhombic transitions. With increasing x, it well survives into the superconducting regime, but gradually gets suppressed and finally disappears aroun…
A series of high quality BaFe$_{2-x}$Ni$_x$As$_2$ pnictide superconductors were studied using magnetic relaxation and isothermal magnetic measurements in order to study the second magnetization peak (SMP) and critical current behaviour in Ni-doped 122 family. The temperature dependence of the magnetic relaxation rate suggests a pinning crossover, whereas, it's magnetic field dependence hints a vortex-lattice structural phase-transition. The activation energy ($U$) estimated using the magnetic relaxation data was analyzed in detail for slightly-underdoped, slightly-overdoped and an overdoped sa…
High-temperature superconductivity in iron pnictides occurs when electrons are doped into their antiferromagnetic (AF) parent compounds. In addition to inducing superconductivity, electron-doping also changes the static commensurate AF order in the undoped parent compounds into short-range incommensurate AF order near optimal superconductivity. Here we use neutron scattering to demonstrate that the incommensurate AF order in BaFe$_{2-x}$Ni$_{x}$As$_{2}$ is not a spin-density-wave arising from the itinerant electrons in nested Fermi surfaces, but consistent with a cluster spin glass in the matr…
Neutron and x-ray diffraction studies show that the simultaneous first-order transition to an orthorhombic and antiferromagnetic (AFM) ordered state in BaFe2As2 splits into two transitions with Co doping. For Ba(Fe0.953Co0.047)2As2, a tetragonal-orthorhombic transition occurs at TS = 60 K, followed by a second-order transition to AFM order at TN = 47 K. Superconductivity (SC) occurs in the orthorhombic state below TC = 15 K and coexists with AFM. Below TC, the static Fe moment is reduced and a 4 meV spin gap develops indicating competition between coexisting SC and AFM order.
We report specific-heat experiments under the influence of high pressure on a strongly underdoped Co-substituted BaFe2As2 single crystal. This allows us to study the phase diagram of this iron pnictide superconductor with a bulk thermodynamic method and pressure as a clean control parameter. The data show large specific-heat anomalies at the superconducting transition temperature, which proves the bulk nature of pressure-induced superconductivity. The transitions in the specific heat are sharper than in resistivity, which demonstrates the necessity of employing bulk thermodynamic methods to ex…
Temperature-dependent inter-plane resistivity, $ρ_c(T)$, was measured in hole-doped iron-arsenide superconductor (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ over a doping range from parent compound to optimal doping $T_c\approx 38~K$, $0\leq x \leq 0.34$. Measurements were undertaken on high-quality single crystals grown from FeAs flux. The coupled magnetic/structural transition at $T_{SM}$ leads to clear accelerated decrease of $ρ_c(T)$ on cooling in samples with $T_c <$26~K ($x <0.25$). This decrease in hole-doped material is in notable contrast to an increase in $ρ_c(T)$ in the electron-doped Ba(Fe$_{1-x…
Superconductivity in BaFe2(As1-xPx)2 iron pnictides emerges when its in-plane two-dimensional (2D) orthorhombic lattice distortion associated with nematic phase at Ts and three-dimensional (3D) collinear antiferromagnetic (AF) order at TN (Ts = TN) are gradually suppressed with increasing x, reaching optimal superconductivity around x = 0.30 with Tc $\approx$ 30 K. Here we show that a moderate uniaxial pressure along the c-axis in BaFe2(As0.70P0.30)2 spontaneously induces a 3D collinear AF order with TN = Ts > 30 K, while only slightly suppresses Tc. Although a ~ 400 MPa pressure compresses th…
High-resolution thermal-expansion and specific-heat measurements were performed on single crystalline BaFe2(As1-xPx)2 (0 < x < 0.33, x = 1). The observation of clear anomalies allows to establish the thermodynamic phase diagram which features a small coexistence region of SDW and superconductivity with a steep rise of Tc on the underdoped side. Samples that undergo the tetragonal-orthorhombic structural transition are detwinned in situ, and the response of the sample length to the magneto-structural and superconducting transitions is studied for all three crystallographic directions. It is sho…
We report a Raman scattering study of nematic degrees of freedom in the iron-based superconductor parent compound BaFe$_2$As$_2$ under tunable uniaxial strain. We demonstrate that the polarization resolved arsenic (As) phonon intensity can be used to monitor the nematic order parameter as a function of both temperature and strain. At low temperature in the nematic ordered phase we use it to track the continuous and reversible orientation of nematic domains under variable strain. At higher temperature, the evolution of the As phonon intensity under strain reflects an enhanced nematic susceptibi…
The origin of nematic order remains one of the major debates in iron-based superconductors. In theories based on spin nematicity, one major prediction is that the spin-spin correlation length at (0,$π$) should decrease with decreasing temperature below the structural transition temperature $T_s$. Here we report inelastic neutron scattering studies on the low-energy spin fluctuations in BaFe$_{1.935}$Ni$_{0.065}$As$_2$ under uniaxial pressure. Both intensity and spin-spin correlation start to show anisotropic behavior at high temperature, while the reduction of the spin-spin correlation length …
Application of pressures or electron-doping through Co substitution into Fe sites transforms the itinerant antiferromagnet BaFe(2)As(2) into a superconductor with the Tc exceeding 20K. We carried out systematic transport measurements of BaFe(2-x)Co(x)As(2) superconductors in pressures up to 2.5GPa, and elucidate the interplay between the effects of electron-doping and pressures. For the underdoped sample with nominal composition x = 0.08, application of pressure strongly suppresses a magnetic instability while enhancing Tc by nearly a factor of two from 11K to 21K. In contrast, the optimally d…
For applying tensile or compressive uniaxial strain to functional thin films, we propose a novel approach in combining a piezoelectric-based device and a technical metallic substrate used widely in the 2nd generation coated conductors (i.e. superconducting tapes). A strain-induced shift of the superconducting transition temperature of 0.1 K for Co-doped BaFe2As2 was observed along [100] direction, corresponding to a uniaxial pressure derivative dTc/dp100=-4 K/GPa. For Mn3CuN, a uniaxial strain derivative along [100] direction of the Curie temperature dTC/de100=13 K/% was observed. The current …
We investigated the anisotropy in the in-plane optical spectra of detwinned Ba(Fe1-xCox)2As2. The optical conductivity spectrum of BaFe2As2 shows appreciable anisotropy in the magnetostructural ordered phase, whereas the dc resistivity is almost isotropic at low temperatures. Upon Co doping, the resistivity becomes highly anisotropic, while the finite-energy intrinsic anisotropy is suppressed. It is found that anisotropy in resistivity arises from anisotropic impurity scattering from doped Co atoms, extrinsic in origin. Intensity of a specific optical phonon mode is also found to show striking…
Sizable single crystals of $BaFe_2As_2$ have been grown with self-flux method. The crystals are plate-like with c-axis perpendicular to the plane. The size can be as large as 3 x 5 x 0.2 $mm^3$. The resistivity anisotropy ($ρ_c/ρ_{ab}$) is as large as about 150, and independent of temperature. The transport in ab plane and along c-axis direction shares the same scattering mechanism. In contrast to the magnetic behavior of polycrystalline samples, no Curie-Weiss behavior are observed, a temperature linear dependent susceptibility occurs above spin-density-wave (SDW) transition. The susceptibili…
We report that the pressure-temperature phase diagram of single-crystalline SrFe$_2$As$_2$ is easily affected by the hydrostaticity of a pressure-transmitting medium. For all of the three mediums we used, superconductivity with zero resistance appears, accompanied by the suppression of an antiferromagnetic (orthorhombic) phase, but the critical pressure $P_c$ was found to depend on the type of medium. $P_c$ was estimated to be 4.4 GPa under almost hydrostatic condition, but it decreased to $3.4-3.7$ GPa with the use of the medium already solidified at room temperature. The uniaxial stress alon…
In contrast to the simultaneous structural and magnetic first order phase transition $T_{0}$ previously reported, our detailed investigation on an underdoped Ba$_{0.84}$K$_{0.16}$Fe$_{2}$As$_{2}$ single crystal unambiguously revealed that the transitions are not concomitant. The tetragonal ($τ$: I4/mmm) - orthorhombic ($\vartheta$: Fmmm) structural transition occurs at $T_{S}\simeq$ 110 K, followed by an adjacent antiferromagnetic (AFM) transition at $T_{N}\simeq$ 102 K. Hysteresis and coexistence of the $τ$ and $\vartheta$ phases over a finite temperature range observed in our NMR experiments…
Uniaxial stress, as well as hydrostatic pressure are often used to tune material properties in condensed matter physics. Here, we present a setup which allows for the study of the combined effects of quasi-uniaxial stress and hydrostatic pressure. Following earlier designs for measurements under finite stress at ambient pressure (e.g., Chu et al., Science 337, 710 (2012)), the present setup utilizes a piezoelectric actuator to change stress in situ inside the piston-cylinder pressure cell. We show that the actuator can be operated over the full temperature (from 30K up to 260 K) and pressure r…
Overshadowing the superconducting dome in hole-doped cuprates, the pseudogap state is still one of the mysteries that no consensus can be achieved. It has been suggested that the rotational symmetry is broken in this state and may result in a nematic phase transition, whose temperature seems to coincide with the onset temperature of the pseudogap state $T^*$ around optimal doping level, raising the question whether the pseudogap results from the establishment of the nematic order. Here we report results of resistivity measurements under uniaxial pressure on several hole-doped cuprates, where t…
We use neutron scattering to study the electron-doped superconducting NaFe$_{0.985}$Co$_{0.015}$As ($T_c=14$ K), which has co-existing static antiferromagnetic (AF) order ($T_N=31$ K) and exhibits two neutron spin resonances ($E_{r1}\approx 3.5$ meV and $E_{r2}\approx 6$ meV) at the in-plane AF ordering wave vector ${\bf Q}_{\rm AF}={\bf Q}_{1}=(1,0)$ in reciprocal space. In the twinned state below the tetragonal-to-orthorhombic structural transition $T_s$, both resonance modes appear at ${\bf Q}_{1}$ but cannot be distinguished from ${\bf Q}_{2}=(0,1)$. By detwinning the single crystal with u…
We have carried out in-plane resistivity measurements under a uniaxial pressure in NaFe$_{1-x}$Co$_x$As single crystals. A clear distinction of the in-plane resistivity $ρ_a$ and $ρ_b$ with the uniaxial pressure along $b$-axis was discovered in the parent and underdoped regime with the doping level up to about x=0.025$\pm$0.002. From the deviating point of $ρ_a$ and $ρ_b$, and the unique kinky structure of resistivity together with the published data we determined the temperatures for the nematic, structural and antiferromagnetic transitions. It is clearly shown that the nematic electronic sta…
The characteristic features of Ca$_{10}$(Pt$_3$As$_8$)[(Fe$_{1-x}$Pt$_x$)$_2$As$_2$]$_5$ ("10-3-8") superconductor are relatively high anisotropy and a clear separation of superconductivity and structural/magnetic transitions, which allows studying the superconducting gap without complications due to the coexisting order parameters. The London penetration depth, measured in underdoped single crystals of 10-3-8 ($x =$ 0.028, 0.041, 0.042, and 0.097), shows behavior remarkably similar to other Fe-based superconductors, exhibiting robust power-law, $Δλ(T) = A T^n$. The exponent $n$ decreases from…
We have systematically studied the nematic susceptibility in non-superconducting Ba(Fe$_{1-x}$TM$_{x}$)$_2$As$_2$ (TM = Cr, Mn, V and Cu) by measuring the uniaxial pressure dependence of the resistivity along the Fe-As-Fe direction. The nematic susceptibilities in all samples show the Curie-Weiss-like behavior at high temperatures, where the nematic Curie constant $A_n$ can be derived, similar to the Curie constant in a paramagnetism. While all these dopants do not introduce superconductivity in BaFe$_2$As$_2$, their effects on nematic fluctuations are different. In Mn, Cr and V doped samples,…
Understanding the nature of the electronic nematic phase in iron pnictide superconductors is important for elucidating its impact on high-temperature superconductivity. Here we use transport and inelastic neutron scattering to study spin excitations and in-plane resistivity anisotropy in uniaxial pressure detwinned BaFe$_2$As$_2$ and SrFe$_2$As$_2$, the parent compounds of iron pnictide superconductors. While BaFe$_2$As$_2$ exhibits weakly first order tetragonal-to-orthorhombic structural and antiferromagnetic (AF) phase transitions below $T_s > T_N\approx 138$ K, SrFe$_2$As$_2$ has strongly c…
We report a comprehensive Cu L$_3$-edge resonant x-ray scattering study of two- and three-dimensional (2D and 3D) incommensurate charge correlations in single crystals of the underdoped high-temperature superconductor YBa$_2$Cu$_3$O$_{6.67}$ under uniaxial compression up to 1% along the two inequivalent Cu-O-Cu bond directions (a and b) in the CuO$_2$ planes. The pressure response of the 2D charge correlations is symmetric: pressure along a enhances correlations along b, and vice versa. Our results imply that the underlying order parameter is uniaxial. In contrast, 3D long-range charge order i…
We report comprehensive resistivity measurements of single crystalline samples of the Ba(Fe(1-x)Co(x))2As2 high Tc superconductor under hydrostatic pressure up to 2.75 GPa and over a broad concentration range, 0 < x < 0.099. We show that application of pressure progressively suppresses the SDW transition temperature, T_SDW, in the underdoped regime. There is no sign of pressure-induced superconductivity in the undoped BaFe2As2 down to 1.8 K, but applied pressure dramatically enhances Tc in the underdoped regime. The effect of pressure on Tc is very small in the optimally and overdoped regimes.…
In a magnetically driven electronic nematic state, an externally applied uniaxial strain rounds the nematic transition and increases the magnetic transition temperature. We study both effects in a simple classical model of the iron-pnictides expressed in terms of local SO(N) spins (with N = 3) which we solve to leading order in 1=N. The magnetic transition temperature is shown to increase linearly in response to an external strain while a sharp crossover, which is a remnant of the nematic transition, can only be identified for extremely small strain. We show that these results can reasonably a…
The momentum dependence of the nematic order parameter is an important ingredient in the microscopic description of iron-based high-temperature superconductors. While recent reports on FeSe indicate that the nematic order parameter changes sign between electron and hole bands, detailed knowledge is still missing for other compounds. Combining angle-resolved photoemission spectroscopy (ARPES) with uniaxial strain tuning, we measure the nematic band splitting in both FeSe and BaFe$_2$As$_2$ without interference from either twinning or magnetic order. We find that the nematic order parameter exhi…
In two recent articles (cond-mat/0606177 and arXiv:0804.1615), we have suggested a unified theory of superconductivity based on the real-space spin-parallel electron pairing and superconducting mechanism and have shown that the stable hexagonal and tetragonal vortex lattices (the optimal doping phases) can be expected in the newly discovered LaO{1-x}F{x}FeAs (x0=1/7=0.1428) and SmO{1-x}F{x}FeAs (x0=1/6=0.1667), respectively. In this paper, we present a theoretical study of the effects of hydrostatic and anisotropic pressure on the superconducting transition temperature Tc of the Fe-based layer…
Orbital Separation of Charge Order and Superconductivity in La$_{2-x}$Sr$_{x}$CuO$_4$
Universität Zürich(苏黎世大学);PSI Center for Neutron and Muon Sciences CNM(瑞士保罗谢勒研究所中子与μ子科学中心);European Synchrotron Radiation Facility(欧洲同步辐射装置);Diamond Light Source(钻石光源);Korea Advanced Institute of Science & Technology (KAIST)(韩国科学技术院);Helmholtz-Zentrum Berlin für Materialien und Energie(柏林亥姆霍兹材料与能源中心);Hokkaido University(北海道大学);Muroran Institute of Technology(室兰工业技术学院)