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arXiv 2601.01643cond-mat.supr-concond-mat.str-el
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在La$_{2-x}$Sr$_{x}$CuO$_4$中分离电荷有序与超导性

Orbital Separation of Charge Order and Superconductivity in La$_{2-x}$Sr$_{x}$CuO$_4$

Universität Zürich(苏黎世大学);PSI Center for Neutron and Muon Sciences CNM(瑞士保罗谢勒研究所中子与μ子科学中心);European Synchrotron Radiation Facility(欧洲同步辐射装置);Diamond Light Source(钻石光源);Korea Advanced Institute of Science & Technology (KAIST)(韩国科学技术院);Helmholtz-Zentrum Berlin für Materialien und Energie(柏林亥姆霍兹材料与能源中心);Hokkaido University(北海道大学);Muroran Institute of Technology(室兰工业技术学院)

I. Biało, O. Gerguri, L. Martinelli, J. Küspert, J. Choi, M. Garcia-Fernandez, S. Agrestini, K. J. Zhou, E. Weschke, T. Kurosawa, N. Momono, M. Oda, C. Lin, Q. Wang, J. Chang

AI总结:

通过c轴压力研究La$_{2-x}$Sr$_{x}$CuO$_4$中电荷有序与超导性的轨道分离,揭示其共存机制及多序相图的复杂性。

摘要:

我们报告了对欠掺杂La$_{2-x}$Sr$_{x}$CuO$_4$(x=0.125)在单轴c轴压力下的联合X射线吸收(XAS)和氧K边共振非弹性X射线散射(RIXS)研究。我们发现压缩的c轴应变仅在超导态内修改电荷有序,具有显著的极化依赖性:在d$_{x^2-y^2}$通道中抑制,在d$_{z^2}$通道中增强。X射线吸收光谱揭示了应变诱导的氧预边和上Hubbard带的修改,一致于增加d$_{z^2}$轨道混合物。我们的结果表明,c轴压力驱动了超导性(根植于d$_{x^2-y^2}$态)和电荷有序之间的轨道分离,后者逐渐转移到d$_{z^2}$通道。这种轨道分离揭示了在铜基超导体中超导性和电荷有序共存的途径,最小化竞争。此外,它表明La$_{2-x}$Sr$_{x}$CuO$_4$的多序相图不能在通常用于描述铜基超导体物理的单带模型中合理描述。

英文摘要:

We report a combined x-ray absorption (XAS) and oxygen $K$-edge resonant inelastic x-ray scattering (RIXS) study of charge order in underdoped La$_{2-x}$Sr$_x$CuO$_4$ ($x=0.125$) under uniaxial $c$-axis pressure. We find that compressive $c$-axis strain modifies the charge order only within the superconducting state, with a striking polarization dependence: suppression in the $d_{x^2-y^2}$ channel and enhancement in the $d_{z^2}$ channel. X-ray absorption spectra reveal concomitant strain-induced modifications of the oxygen pre-edge and upper Hubbard band, consistent with increased $d_{z^2}$ orbital admixture. Our results suggest that $c$-axis pressure drives an orbital separation between superconductivity, rooted in $d_{x^2-y^2}$ states, and charge order, which gradually shifts to the $d_{z^2}$ channel. This orbital separation reveals a way for superconductivity and charge order to coexist in the cuprates with minimal competition. Furthermore, it suggests that the multi-order phase diagram of La$_{2-x}$Sr$_{x}$CuO$_4$ cannot be realistically described within single band models usually used to describe cuprate physics.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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