强电子关联既导致未掺杂La$_2$CuO$_4$的绝缘基态，也导致相邻自旋间的强反铁磁耦合$J$。我们考虑了有效低能$t - t' - t
英文摘要：
Strong electron correlations are responsible both for the insulator ground state of undoped La$_2$CuO$_4$ and strong antiferromagnetic coupling $J$ between neighbouring spins. We consider magnetic mechanism of superconducting pairing in the effective low energy $t - t' - t" - J^*$ model with all parameters calculated {\it ab initio}. Interaction of strongly correlated electrons with different phonon modes is also incorporated. In a BCS type theory the $d_{x^2 - y^2}$ gap is given by a sum of magnetic and phonon contributions. The phonon coupling parameter $λ= f(x)G$, where $G$ is a combination of bare electron-phonon couplings for all modes and the function $f$ depends on the hole concentration $x$ due to strong electron correlations. The main contribution to the only fitting parameter $G$ is determined by a competition of the breathing and buckling modes. Fitting the parameter $G$ from the isotope effect we obtain that magnetic and phonon contributions to the critical temperature $T_c $ work together and are of the same order of magnitude.
The oxygen isotope effect on the superconductivity, stripe phase and structure transition is systematically investigated in La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_4$ with static stripe phase. Substitution of $^{16}$O by $^{18}$O leads to a decrease in superconducting transition temperature T$_C$, while enhances the temperature of the structural transition from low-temperature-orthorhombic (LTO) phase to low-temperature-tetragonal (LTT) phase. Compared to the Nd free sample, a larger isotope effect on $T_C$ is observed in La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_4$. These results indicate that the distor…
We present a detailed analysis on the hopping between monolayer CuO$_2$ and bulk CuO$_2$ plane in the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ substrate. With a two-band model, we demonstrate that the nodeless gap can only exist when the hole concentration in monolayer CuO$_2$ plane is very large or very small. We argued that the possible phase separation may play important role in the recent experimental observation of nodeless gap.
The dispersion of the Cu-O bond-stretching vibrations in overdoped La$_{1.7}$Sr$_{0.3}$CuO$_4$ (not superconducting) has been studied by high resolution inelastic neutron scattering. It was found that the doping-induced renormalization of the so-called breathing and the half-breathing modes is larger than in optimally doped La$_{1.85}$Sr$_{0.15}$CuO$_4$. On the other hand, the phonon linewidths are generally smaller in the overdoped sample. Features observed in optimally doped La$_{1.85}$Sr$_{0.15}$CuO$_4$ which suggest a tendency towards charge stripe formation are absent in overdoped La$_{1.…
Superconductivity has recently been discovered in Pr$_{2}$Ba$_{4}$Cu$_{7}$O$_{15-δ}$ with a maximum $T_c$ of about 15K. Since the CuO planes in this material are believed to be insulating, it has been proposed that the superconductivity occurs in the double (or zigzag) CuO chain layer. On phenomenological grounds, we propose a theoretical interpretation of the experimental results in terms of a new phase for the zigzag chain, labelled by C$_1$S$_{3/2}$. This phase has a gap for some of the relative spin and charge modes but no total spin gap, and can have a divergent superconducting susceptibi…
To study the rare-earth doping effect on the phonon heat transport of La-based cuprates and shed light on the mechanism of phonon scattering, both $ab$-plane and c-axis thermal conductivities ($κ_{ab}$ and $κ_c$) are measured for La$_{2-y}$Eu$_y$CuO$_4$ ($y$ = 0, 0.02 and 0.2) and La$_{1.88-y}$Eu$_y$Sr$_{0.12}$CuO$_4$ ($y$ = 0 and 0.2) single crystals. It is found that the phonon peak (at 20 -- 25 K) in $κ_{ab}(T)$ of La$_{2-y}$Eu$_y$CuO$_4$ shows an anomalous Eu-doping dependence: it completely disappears for $y$ = 0.02, which is discussed to be due to the local lattice distortions around Eu …
The thermal conductivity of the antiferromagnet Nd$_2$CuO$_4$ was measured down to 50 mK. Using the spin-flop transition to switch on and off the acoustic Nd magnons, we can reliably separate the magnon and phonon contributions to heat transport. We find that magnons travel ballistically below 0.5 K, with a thermal conductivity growing as $T^3$, from which we extract their velocity. We show that the rate of scattering of acoustic magnons by phonons grows as $T^3$, and the scattering of phonons by magnons peaks at twice the average Nd magnon frequency.
This paper has been withdrawn by the authors, because we had probably observed some spurious intensity with x=0.29 sample (Fig.3(b)). This came out after further studies of the detailed x-dependence of the highest energy LO phonon branch in LSCO.
In this Comment, we show that the experimental data reported by Li {\it et al.} (Phys. Rev. B {\bf 77}, 134501 (2008)) do not support the phonon specular reflection at low temperatures for high-T_c cuprates, because the phonon mean free path \ell calculated from their thermal conductivity data is much smaller than the averaged sample width above \sim 100 mK for both Nd_{2}CuO_{4} and YBa_{2}Cu_{3}O_{6.0} single crystals.
Superlattices of the repeated structure La(1.56)Sr(0.44)CuO(4)/La(2)CuO(4) (LSCO-LCO), where none of the constituents is superconducting, show a superconducting transition of T_c \simeq 25 K. In order to elucidate the nature of the superconducting state we have performed a low-energy muSR study. By applying a magnetic field parallel (Meissner state) and perpendicular (vortex state) to the film planes, we could show that superconductivity is sheet like, resulting in a very anisotropic superconducting state. This result is consistent with a simple charge-transfer model, which takes into account …
In their comment \cite{Sun} on our study of phonon heat transport in Nd$_2$CuO$_4$ \cite{Li}, Sun and Ando estimate that the phonon mean free path at low temperature is roughly half the width of the single crystal used in our study, from which they argue that phonon scattering cannot be dominated by sample boundaries. Here we show that their use of specific heat data on Nd$_2$CuO$_4$, which contains a large magnetic contribution at low temperature that is difficult to reliably extract, leads to an underestimate of the mean free path by a factor two compared to an estimate based on the specific…
The phonon dispersions of $\mathrm{Nd_{1.86}Ce_{0.14}CuO_{4+δ}}$ along the $[ξ,0,0]$ direction have been determined by inelastic x-ray scattering. Compared to the undoped parent compound, the two highest longitudinal phonon branches, associated with the Cu-O bond-stretching and out-of-plane oxygen vibration, are shifted to lower energies. Moreover, an anomalous softening of the bond-stretching band is observed around $\mathbf{q}=(0.2,0,0)$. These signatures provide evidence for strong electron-phonon coupling in this electron-doped high-temperature superconductor.
Meissner type superconductivity extending up to 13 - 18 degrees Celsius was confirmed in the composite material consisting of metallic particles Ag5Pb2O6 dispersed in an insulating CuO matrix, and superconductivity mechanism is based upon inter particle interaction acting in the quantum tunnelling regime.
We present a comparative experimental and theoretical investigation of the two--dimensional charge-transfer gap in the strongly correlated material Sr$_2$CuO$_2$Cl$_2$. We observe an Urbach behaviour in the absorption profile over a surprisingly wide range of energies and temperatures. We present a model that accounts for phonon scattering to infinite order and which allows us to explain the data accurately by assuming coupling of the charge transfer gap exciton to lower energy electronic excitations.
Phonons in nearly optimally doped HgBa$_2$CuO$_{4+δ}$ were studied by inelastic X-ray scattering. The dispersion of the low energy modes is well described by a shell model, while the Cu-O bond stretching mode at high energy shows strong softening towards the zone boundary, which deviates strongly from the model. This seems to be common in the hole-doped high-$T_\mathrm{c}$ superconducting cuprates, and, based on this work, not related to a lattice distortion specific to each material.
The recently discovered cuprate superconductor Ba$_2$CuO$_{3+δ}$ exhibits a high $T_c\simeq73$K at $δ\simeq0.2$. The polycrystal grown under high pressure has a structure similar to La$_2$CuO$_4$, but with dramatically different lattice parameters due to the CuO$_6$ octahedron compression. The crystal field in the compressed Ba$_2$CuO$_4$ leads to an inverted Cu $3d$ $e_g$ complex with the $d_{x^2-y^2}$ orbital sitting below the $d_{3z^2-r^2}$ and an electronic structure highly unusual compared to the conventional cuprates. We construct a two-orbital Hubbard model for the Cu $d^9$ state at hol…
The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La$_2$CuO$_4$ were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar thermal Hall conductivity in two cuprate Mott insulators with significantly different crystal structures and magnetic orders - Nd$_2$CuO$_4$ and Sr$_2$CuO$_2$Cl$_2$ - and show that two potential mechanisms can be excluded - the scattering of phonons by rare-earth impurities and by structural domains. Ou…
We report a doping dependant Electronic Raman Scattering (ERS) study of HgBa$_2$CuO$_{4+δ}$ (Hg-1201) single crystals. We investigate the dynamics of the antinodal and nodal quasiparticles. We show that the dynamical response of the antinodal quasiparticles is strongly reduced towards the underdoped regime in both the normal and superconducting states. When probing the nodal quasiparticles, we are able to distinguish between the energy scale of the pseudogap and that of the superconducting gap. A simple model relating the suppression of the dynamical response of the antinodal quasiparticles to…
We report an ultrahigh resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results s…
We report the local magnetic response of an electron-doped cuprate superconductor, Pr$_{0.89}$LaCe$_{0.11}$CuO$_{4}$ ($T_c\simeq26$ K), studied by muon spin rotation (\msr) over a field range from 200 Oe to 50 kOe. In the paramagnetic state, the muon Knight shift along the crystal c-axis ($K_μ^z$) is proportional to the in-plane susceptibility $χ_{ab}$. More surprisingly, $K_μ^z$ is strongly enhanced by the occurrence of superconductivity (below $\sim$40 kOe), changing its sign from positive to negative around $\sim1$ kOe with increasing field. This finding can be understood by considering the…
Recently, Matsukawa et al. have discovered a new superconductor Pr_2Ba_4Cu_7O_15-delta in which metallic CuO double chains are responsible for the superconductivity. To investigate the superconductivity, we employ the d-p double chain model where the tight-binding parameters are determined so as to fit the LDA band structure. On the basis of the Tomonaga-Luttinger liquid theory, we obtain the phase diagram including the superconducting phase in the weak coupling limit. We also calculate the Luttinger liquid parameter K_rho as a function of the electron density $n$ by using the Hartree-Fock app…
We use inelastic neutron scattering to study the evolution of the generalized phonon density of states (GDOS) of the $n$-type high-$T_c$ superconductor Nd$_{2-x}$Ce$_x$CuO$_{4+δ}$ (NCCO), from the half-filled Mott-insulator ($x=0$) to the $T_c=24$ K superconductor ($x=0.15$). Upon doping the CuO$_2$ planes in Nd$_2$CuO$_{4+δ}$ (NCO) with electrons by Ce substitution, the most significant change in the GDOS is the softening of the highest phonon branches associated with the Cu-O bond stretching and out-of-plane oxygen vibration modes. However, the softening occurs within the first few percent o…
We investigate the hole and lattice dynamics in a prototypical high temperature superconducting system La{2-x}Sr{x}CuO{4} using infrared spectroscopy. By exploring the anisotropy in the electronic response of CuO2 planes we show that our results support the notion of stripes. Nevertheless, charge ordering effects are not apparent in the phonon spectra. All crystals show only the expected infrared active modes for orthorhombic phases without evidence for additional peaks that may be indicative of static charge ordering. Strong electron-phonon interaction manifests itself through the Fano linesh…
Composite material was prepared from Byström-Evers metallic particles Ag5Pb2O6 dispersed in a semiconducting matrix CuO-Cu2O. Partial substitution of CuO by Cu2O increases electric conductivity at 673 K for 2-3 orders of magnitude above Landauer conductivity e2/ha indicated by pure CuO matrix. Onset of superconductivity at 86-375 K presented in this and previous works is discussed in the framework of the exciton-polariton mechanism occurring on the grain surfaces.
We have performed a series of elastic neutron scattering measurements on 1/8-hole doped La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ single crystals with {\it x} = 0.05, 0.06, 0.075 and 0.085. % Both charge-density-wave (CDW) and spin-density-wave (SDW) orders are found to develop simultaneously below the structural transition temperature between the low-temperature orthorhombic (LTO) and low-temperature tetragonal (LTT) or low-temperature less-orthorhombic (LTLO) phases. % In the ground state the CDW order is observed only in the LTT/LTLO phase and drastically degrades towards the LTO boundary…
This paper describes the first 63-Cu NMR study of an electron-doped infinitely-layered high Tc superconductor Sr$_0.9$La$_0.1$CuO$_2$ (Tc=42K). The spin dynamics in the normal state above Tc exhibits qualitatively the same behavior as some hole-doped materials with significantly enhanced spin fluctuations. Below Tc, we observed no signature of a Hebel-Slichter coherence peak, suggesting an unconventional nature of the symmetry of the superconducting order parameter.
We study the electronic structure and superconductivity in CuO$_2$ monolayer grown recently on $d$-wave cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. Density functional theory calculations indicate significant charge transfer across the interface such that the CuO$_2$ monolayer is heavily overdoped into the hole-rich regime yet inaccessible in bulk cuprates. We show that both the Cu $d_{x^2-y^2}$ and $d_{3z^2-r^2}$ orbitals become important and the Fermi surface contains one electron and one hole pocket associated with the two orbitals respectively. Constructing a minimal correlated tw…
We identify a distinct superconducting phase at the interface of a La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ (LNSCO)/La$_{1.84}$Sr$_{0.16}$CuO$_4$ (LSCO) epitaxial bilayer system using ac screening measurements. A model based on inter-diffusion of quasiparticles and condensate at the interface yields a thickness of $\sim$ 25 nm for the interfacial layer. Two-dimensional superconductivity of the interface layer appears to be governed by Kosterlitz-Thouless-Berezinskii transition. A parallel magnetic field suppresses the superconducting transition temperature of this layer with a pair breaking par…
Superconductivity in high temperature superconductors is achieved by introducing charge carriers into cuprate insulators containing CuO$_2$ planes. Perturbation in these CuO$_2$ planes suppresses superconductivity by strongly affecting the electronic environment. Here we have use photoinduced electronic modification of Cu ion in CuO$_2$ plane to investigate the effect of local perturbation in Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$. This method has been used to suppress superconducting transition temperature T$_c$. We show that our results on photoinduced suppression of superconductivity are consis…
We reinterpret neutron scattering and Raman spectroscopy experiments in La(2-x)Sr(x)CuO(4), showing modulation of spin and lattice degrees of freedom both in the low-temperature orthorhombic and tetragonal phases, in terms of a magneto-elastic coupling between noncollinear configurations for the copper spins and the oxygen octahedra. The magneto-elastic coupling furthermore explains the recently discovered magnetic-field induced untwinning in La(2-x)Sr(x)CuO(4), for x<2%, and allows us to understand why in La(2-x-y)Sr(x)Nd(y)CuO(4) with y=0.4 and x=1/8, for example, when (1,0) and/or (0,1) sta…
The possible inhomogeneity of superconductivity has been investigated by means of bulk-sensitive probes, using La_2-x_Sr_x_CuO_4_ (LSCO) single crystals from the underdoped to optimally doped regime. Measurements of the magnetic susceptibility, chi, on field cooling and specific heat have revealed that both the absolute value of chi at 2 K, regarded as corresponding to the superconducting (SC) volume fraction in a sample, and the Sommerfeld constant, reflecting the density of states of quasiparticles at the Fermi level, exhibit significant dependence on x, namely, on the hole concentration. Th…
The interplay between superconductivity and the pseudogap is an important aspect of cuprate physics. However, the nature of the pseudogap remains controversial, in part because different experiments have suggested different gap functions. Here we present a photon-energy-dependence angle-resolved photoemission spectroscopy (ARPES) study on Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$. We find that antinodal ARPES spectra at low photon energies are dominated by background signals which can lead to a misevaluation of the spectral gap size. Once background is properly accounted for, indepe…
Electron-doped and hole-doped superconducting cuprates exhibit a symmetric phase diagram as a function of doping. This symmetry is however only approximate. Indeed, electron-doped cuprates become superconductors only after a specific annealing process: This annealing affects the oxygen content by only a tiny amount, but has a dramatic impact on the electronic properties of the sample. Here we report the occurrence of superconductivity in oxygen-deficient Nd$_{2-x}$Ce$_x$CuO$_4$ thin films grown in an oxygen-free environment, after annealing in pure argon flow. As verified by x-ray diffraction,…
Strong correlation between field-induced antiferromagnetic (AF) order and superconductivity is demonstrated for an electron-doped cuprate superconductor, Pr$_{1-x}$LaCe$_{x}$CuO$_{4-δ}$ (PLCCO). In addition to the specimen with $x=0.11$ (which is close to the AF phase boundary, $x\simeq0.10$), we show that the one with $x=0.15$ ($T_c\simeq16$ K at zero field) also exhibits the field-induced AF order with a reduced magnitude of the induced moment. The uniform muon Knight shift at a low magnetic field ($\sim10^2$ Oe) indicates that the AF order is not localized within the cores of flux lines, wh…
Comment on "Light-induced melting of competing stripe orders without introducing superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_4$" (arXiv:2306.07869v1)
Optical excitation of stripe-ordered La$_{2-x}$Ba$_x$CuO$_4$ has been shown to transiently enhance superconducting tunneling between the CuO$_2$ planes. This effect was revealed by a blue-shift, or by the appearance of a Josephson Plasma Resonance in the terahertz-frequency optical properties. Here, we show that this photo-induced state can be strengthened by the application of high external magnetic fields oriented along the c-axis. For a 7-Tesla field, we observe up to a ten-fold enhancement in the transient interlayer phase correlation length, accompanied by a two-fold increase in the relax…
Recent experiments on Pr$_{0.89}$LaCe$_{0.11}$CuO$_4$ observe an anisotropic spin-correlation gap and a nonmonotonic superconducting (SC) gap, which we analyze within the framework of a $t-t^{\prime}-t^{\prime\prime}-t^{\prime\prime\prime}-t^{iv}-U$ model with a $d_{x^2-y^2}$ pairing interaction including a third harmonic contribution. By introducing a realistic broadening of the quasiparticle spectrum to reflect small-angle scattering, our computations explain the experimental observations, especially the presence of a maximum in the leading edge gap in the vicinity of the hot-spots. Our anal…
The phonon densities-of-states of La(1.475)Nd(0.4)Sr(0.125)CuO(4) and La(1.9)Sr(0.1)CuO(4) were measured using inelastic neutron scattering. The ~70 meV phonon band which appears due to hole doping in La(1.9)Sr(0.1)CuO(4) is known to arise from strong electron-lattice coupling. This phonon band is strongly suppressed in the Nd-doped compound for which T_c is also suppressed, establishing a link between in-plane oxygen optical phonons and superconductivity. This suppression is attributed to hole localization which becomes strong near the stripe ordering condition of certain cuprates near x=1/8 …
We report enhanced superconductivity in bilayer thin films consisting of superconducting La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_{4}$ with 0.06 $\leq x<$ 0.20 and metallic but non-superconducting La$_{1.55}$Sr$_{0.45}$CuO$_{4}$. These bilayers show a maximum increase in superconducting transition temperature ($T_c$) of more than 200% for $x$ = 0.06 while no change in $T_c$ is observed for the bilayers with $x\geq$ 0.20. The analysis of the critical current and kinetic inductance data suggests 2-3 unit cells thick interfacial layer electronically perturbed to have a higher $T_c$. A simple charge tra…
Two critical points have been revealed in the normal-state phase diagram of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$ by exploring the Fermi surface properties of high quality single crystals by high-field magnetotransport. First, the quantitative analysis of the Shubnikov-de Haas effect shows that the weak superlattice potential responsible for the Fermi surface reconstruction in the overdoped regime extrapolates to zero at the doping level $x_c = 0.175$ corresponding to the onset of superconductivity. Second, the high-field Hall coefficient exhibits a sharp drop right…
Using resonant X-ray diffraction and Raman spectroscopy, we study charge correlations and lattice dynamics in two model cuprates, HgBa$_{2}$CuO$_{4+δ}$ and HgBa$_{2}$CaCu$_{2}$O$_{6+δ}$. We observe a maximum of the characteristic charge order temperature around the same hole concentration ($p \approx 0.09$) in both compounds, and concomitant pronounced anomalies in the lattice dynamics that involve the motion of atoms in and/or adjacent to the CuO$_2$ layers. These anomalies are already present at room temperature, and therefore precede the formation of the static charge correlations, and we a…
We present a comprehensive study of the phonon dispersion in an underdoped, superconducting Ca$_{2-x}$CuO$_2$Cl$_2$ crystal. We interpret the results using lattice dynamical calculations based on a shell model, and we compare the results, to other hole-doped cuprates, in particular to the ones isomorphic to La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). We found that an anomalous dip in the Cu-O bond stretching dispersion develops in oxychlorides with a simultaneous marked broadening of the mode. The broadening is maximum at $\approx (π/ (2a) ~ 0 ~ 0)$ that corresponds to the charge-modulations propagation v…
The fluctuation exchange, or FLEX, approximation for interacting electrons is applied to study instabilities in the standard three-band model for CuO2 layers in the high-temperature superconductors. Both intra-orbital and near-neigbor Coulomb interactions are retained. The filling dependence of the d(x2-y2) transition temperature is studied in both the "hole-doped" and "electron-doped" regimes using parameters derived from constrained-occupancy density-functional theory for La2CuO4. The agreement with experiment on the overdoped hole side of the phase diagram is remarkably good, i.e., transiti…
Using the numerical diagonalization method, we examine the one-dimensional t_1-t_2-J_1-J_2 model (zigzag chain t-J model) which represents an effective model for metallic CuO double chain in the superconductor Pr_2Ba_4Cu_7O_15-δ. Based on the Tomonaga-Luttinger liquid theory, we calculate the Luttinger-liquid parameter K_ρas a function of electron density n. It is found that superconductivity is realized in parameter region corresponding to the experimental result. We show phase diagram of spin gap on the t_2/|t_1|-n plane by analyzing the expectation value of twist-operator Z_σin the spin sec…
The strength of the electron-phonon coupling parameter and its evolution throughout a solid's phase diagram often determines phenomena such as superconductivity, charge- and spin-density waves. Its experimental determination relies on the ability to distinguish thermally activated phonons from those emitted by conduction band electrons, which can be achieved in an elegant way by ultrafast techniques. Separating the electronic from the out-of-equilibrium lattice subsystems, we probed their re-equilibration by monitoring the transient lattice temperature through femtosecond X-ray diffraction in …
The evolution of the electronic state through the reduction annealing has been investigated in electron-doped Pr_1.3-x_La_0.7_Ce_x_CuO_4+delta_ (x=0.10) single crystals with the so-called T' structure. From the ab plane and c axis electrical resistivity measurements in magnetic fields, it has been found that, through the reduction annealing, the strongly localized state of carriers accompanied by the antiferromagnetic (AF) pseudogap in the as-grown crystal changes to a metallic state bringing about the Kondo effect without AF pseudogap and to a superconducting state. These results are able to …
To understand the recently observed high temperature superconductivity in the monolayer CuO$_2$ grown on the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ substrates, we propose a two band model of the hybridized oxygen $p_x$ and $p_y$ orbitals with the proximity effect of the substrate. We demonstrate that both the nodal and nodeless d-wave superconducting states can be induced by the proximity effect, depending on the strengths of the pairing parameters.
Bulk crystals of electron-doped cuprates with the T'-type structure require both Ce substitutions and reduction annealing for the emergence of superconductivity while the reduction annealing alone can induce superconductivity in thin films of the T'-type cuprates. In order to reveal low-energy electronic states which are responsible for the superconductivity, we have conducted angle-resolved photoemission spectroscopy measurements on thin films of the superconducting Ce-free T'-type cuprate Pr$_2$CuO$_4$. The results indicate that the overall band structure and the Fermi surface area of the su…
The reflectivity $R (ω)$ of both the $ab$ plane and the c axis of two single crystals of La$_{1.875}$Ba$_{0.125-y}$Sr$_{y}$CuO$_4$ has been measured down to 5 cm$^{-1}$, using coherent synchrotron radiation below 30 cm$^{-1}$. For $y$ = 0.085, a Josephson Plasma Resonance is detected at $T \ll T_c$ = 31 K in $R_{c} (ω)$, and a far-infrared peak (FIP) appears in the optical conductivity below 50 K, where non-static charge ordering (CO) is reported by X-ray scattering. For $y$ = 0.05 ($T_c$ = 10 K), a FIP is observed in the low-temperature tetragonal phase below the ordering temperature $T_{CO}$…
We show that hole-doped cuprates can harbor {\it Fermi-surface-free superconductivity} similar to the case of the pnictides. This occurs near the doping at which a new Fermi surface pocket appears in the antinodal region. The change in Fermi surface topology is accompanied by a characteristic rise in spectral weight. Our results support the presence of a trisected superconducting dome, and suggest that superconductivity is responsible for stabilizing the $(π,π)$ magnetic order.
We study electronic states of multilayer cuprates in the normal phases as functions of the number of CuO_2 planes and the doping rate. The resonating valence bond wave function and the Gutzwiller approximation are used for a two-dimensional multilayer t-t'-t''-J model. We calculate the electron-removal spectral functions at (π,0) in the CuO_2 plane next to the surface to understand the angle-resolved photoemission spectroscopy (ARPES) spectra. We find that the trilayer spectrum is narrower than the bilayer spectrum but is wider than the monolayer spectrum. In the tri- and tetralayer systems, t…
The cuprates exhibit a prominent charge-density-wave (CDW) instability with wavevector along [100], i.e., the Cu-O bond direction. Whereas CDW order is most prominent at moderate doping and low temperature, there exists increasing evidence for dynamic charge correlations throughout a large portion of the temperature-doping phase diagram. In particular, signatures of incipient charge order have been observed as phonon softening and/or broadening near the CDW wavevector approximately half-way through the Brillouin zone. Most of this work has focused on moderately-doped cuprates, for which the CD…
We examine the effect of CuO intergrowths on the superconductivity in epitaxial La_{2/3}Ca_{1/3}MnO_3/YBa_2Cu_3O_{7-δ} (LCMO/YBCO) thin-film heterostructures. Scanning transmission electron microscopy on bilayer LCMO/YBCO thin films revealed double CuO-chain intergrowths which form regions with the 247 lattice structure in the YBCO layer. These nanoscale 247 regions do not appear in x-ray diffraction, but can physically account for the reduced critical temperature Tc of bilayer thin films relative to unilayer films with the same YBCO thickness, at least down to ~25 nm. We attribute the CuO int…
A mixture of powdered Cu and CuO has been subjected to a shock-wave pressure of 350 kbar with following quenching of the vacuum-encapsulated product to 77 K. The ac magnetic susceptibility measurements of the samples have revealed metastable superconductivity with Tc = 19.5 K, characterized by glassy dynamics of the shielding currents below Tc . Comparison of the ac susceptibility and the dc magnetization measurements infers that the superconductivity arises within the granular interfacial layer formed between metallic Cu and its oxides due to the shock-wave treatment.
Electron-doped infinite-layer Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ films over a wide doping range have been prepared epitaxially on SrTiO$_3$(001) using reactive molecular beam epitaxy. In-plane transport measurements of the single crystalline samples reveal a dome-shaped nodeless superconducting phase centered at $x$ $\sim$ 0.15, a Fermi-liquid behavior and pronounced upturn in low temperature resistivity. We show that the resistivity upturn follows square-root temperature dependence, suggesting the emergence of superconductivity via a three-dimensional percolation process. The percolative supercond…
In superconducting copper oxides some Cu-O bond-stretching phonons around 70meV show anomalous giant softening and broadening of electronic origin and electronic dispersions have large renormalization kinks near the same energy. These observations suggest that phonon broadening originates from quasiparticle excitations across the Fermi surface and the electronic dispersion kinks originate from coupling to anomalous phonons. We measured the phonon anomaly in underdoped (x=0.05) and overdoped (x=0.20,0.25) La$_{2-x}$Sr$_x$CuO$_4$ by inelastic neutron and x-ray scattering with high resolution. Co…
We address the kinetic competition between charge striped order and superconductivity in La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_{4}$. Ultrafast optical excitation is tuned to a mid-infrared vibrational resonance that destroys charge order and promptly establishes transient coherent interlayer coupling in this material. This effect is evidenced by the appearance of a longitudinal plasma mode reminiscent of a Josephson plasma resonance. We find that coherent interlayer coupling can be generated up to the charge order transition $T_{CO} \approx$ 80 K, far above the equilibrium superconducting tra…
A nodeless superconducting (SC) gap was reported in a recent scanning tunneling spectroscopy experiment of a copper-oxide monolayer grown on the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi2212) substrate [Y. Zhong {\it et al.}, Sci. Bull. {\bf 61}, 1239 (2016)], which is in stark contrast to the nodal d-wave pairing gap in the bulk cuprates. Motivated by this experiment, we first show with first-principles calculations that the tetragonal CuO (T-CuO) monolayer on the Bi2212 substrate is more stable than the commonly postulated CuO$_{2}$ structure. The T-CuO monolayer is composed of two CuO$_2$ layers sh…
