We demonstrate the existence of quantum droplets in two-component one-dimensional Bose-Hubbard chains. The droplets exist for any strength of repulsive intra-species interactions provided they are balanced by comparable attractive inter-species interactions. The ground-state phase diagram is presented and the different phases are characterized by examining the density profile and off-diagonal one- and two-body correlation functions. A rich variety of phases is found, including atomic superfluid gases, atomic superfluid droplets, pair superfluid droplets, pair superfluid gases and a Mott-insulator phase. A parameter region prone to be experimentally explored is identified, where the average population per site is lower than three atoms, thus avoiding three-body losses. Finally, the bipartite entanglement of the droplets is found to have a non-trivial dependence on the number of particles.
We analytically calculate the leading quantum corrections of the ground-state energy of two- and one-dimensional weakly interacting Rabi-coupled Bose-Bose mixtures in the frame of the Bogoliubov approximation. We show that to repulsive intraspecies and attractive interspecies interactions, the effect of quantum fluctuations favors the formation of self-bound droplets. These liquidlike states are crucially affected by the Rabi coupling, leading thus to the appearance of a quantum instability. We derive meaningful formulas to describe the droplet phase in the one-dimensional case.
We report on the formation of heteronuclear quantum droplets in an attractive bosonic mixture of 41K and 87Rb. We observe long-lived self-bound states, both in free space and in an optical waveguide. In the latter case, the dynamics under the effect of a species-dependent force confirms their bound nature. By tuning the interactions from the weakly to the strongly attractive regime, we study the transition from expanding to localized states, in both geometries. We compare the experimental results with beyond mean-field theory and we find a good agreement in the full range of explored interacti…
We explore the properties of weakly bound bosonic states in the strongly interacting regime. Combining a correlated-Gaussian (CG) basis set expansion with a complex scaling method, we extract the energies and structural properties of bosonic cluster states with $N\le6$ for different two-body potentials. The identification of five- and six-body resonances attached to an excited Efimov trimer provides strong support to the premise of Efimov universality in bosonic systems. Our study also reveals a rich structure of bosonic cluster states. Besides the lowest cluster states which behave as bosonic…
Ultradilute quantum droplets are intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in three-, one- and two-dimensional two-component Bose-Bose mixtures, by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the interspecies attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In three dimen…
We use exact Quantum Monte Carlo techniques to study the properties of quantum droplets in two-component bosonic mixtures with contact interactions in one spatial dimension. We systematically study the surface tension, the density profile and the breathing mode as a function of the number of particles in the droplet and of the ratio of coupling strengths between intra-species repulsion and inter-species attraction. We find that deviations from the predictions of the generalized Gross-Pitaevskii equation are small in most cases of interest.
Quantum droplets have intrigued much attention recently in view of their successful observations in the ultracold homonuclear atoms. In this work, we demonstrate a new mechanism for the formation of quantum droplet in heteronuclear atomic systems, i.e., by applying the synthetic spin-orbit coupling(SOC). Take the Bose-Fermi mixture for example, we show that by imposing a Rashba SOC between the spin states of fermions, the greatly suppressed Fermi pressure can enable the formation of Bose-Fermi droplets even for very weak boson-fermion attractions, which are insufficient to bound a droplet if w…
Collision and coalescence dynamics of bosonic quantum Hall droplets
State Key Laboratory of Information Photonics and Optical Communications, School of Physical Science and Technology, Beijing University of Posts and Telecommunications（北京邮电大学物理科学与技术学院信息光子学与光通信国家重点实验室）
Recently achieved two-component dipolar Bose-Einstein condensates open exciting possibilities for the study of mixtures of ultra-dilute quantum liquids. While non-dipolar self-bound mixtures are necessarily miscible with an approximately fixed ratio between the two densities, the density ratio for the dipolar case is free. As a result, self-bound dipolar mixtures present qualitatively novel and much richer physics, characterized by three possible ground-state phases: miscible, symmetric immiscible and asymmetric immiscible, which may in principle occur at any population imbalance. Self-bound i…
We study the formation of quantum droplets in the mixture of a single-component Bose-Einstein condensate (BEC), and a two-species Fermi superfluid across a wide Feshbach resonance. With repulsive boson-boson and attractive boson-fermion interactions, we show that quantum droplets can be stabilized by attractive fermion-fermion interactions in the Bardeen-Cooper-Schieffer (BCS) side of the resonance, and can also exist in deep BEC regime under weak boson-fermion interactions. We map out the phase diagram for stable droplets with respect to the boson-boson and boson-fermion interactions, and dis…
We systematically investigate the properties of three-dimensional dipolar binary Bose mixture at low temperatures. A set of coupled self-consistent equations of motion are derived for the two condensates. In the homogeneous case, useful analytical formulas for the condensate depletion, the anomalous density, the ground-state energy, and the equation of state are obtained. The theory is extended to the inhomogeneous case and the importance of the inhomogeneity is highlighted. Our results open up a new avenue for studying dipolar mixture droplets. Impacts of the dipole-dipole interaction on the …
Quantum droplets have been realized in experiments on binary boson mixtures and dipolar Bose gases. In these systems, the mean-field energy of the Bose-Einstein condensation is attractive, and the repulsive Lee-Huang-Yang energy is crucial for stability. The Bogoliubov theory incorrectly predicts that the phonon mode is dynamically unstable in the long-wavelength limit. In this work, we go beyond the Bogoliubov theory to study how the phonon mode is stabilized in the quantum droplet of a binary boson mixture. Similar to Beliaev's approach to a single-component Bose gas, we compute higher-order…
We systematically study the effects of higher-order quantum and thermal fluctuations on the stabilization of self-bound droplets in Bose mixtures employing the time-dependent Hartree-Fock-Bogoliubov theory. We calculate the ground-state energy, the droplet equilibrium density, the depletion and anomalous density of the droplets as well as the critical temperature as a function of the relevant parameters. Our findings are compared with previous analytical predictions and diffusion Monte Carlo simulations. We employ our theory together with the local density approximation for quantum and thermal…
We study the equilibrium properties of self-bound droplets in two-dimensional Bose mixtures employing the time-dependent Hartree-Fock-Bogoliubov theory. This theory allows one to understand both the many-body and temperature effects beyond the Lee-Huang-Yang description. We calculate higher-order corrections to the excitations, the sound velocity, and the energy of the droplet. Our results for the ground-state energy are compared with the diffusion Monte Carlo data and good agreement is found. The behavior of the depletion and anomalous density of the droplet is also discussed. At finite tempe…
We have theoretically investigated the structure of spinning self-bound droplets made of $^{41}$K-$^{87}$Rb Bose mixture by solving the Gross-Pitaevskii equation including beyond-mean-field correction in the Lee-Huang-Yang form. The structure and energetics of vortex formation in the self-bound mixture have been elucidated, showing that the formation of linear vortices in the heavier species is energetically favoured over other configurations. A fake (partially filled) core develops as a consequence in the other species, resulting in a hole which might be imaged in experiments. The interplay b…
Breakdown of the single-mode description of ultradilute quantum droplets in binary Bose mixtures: A perspective from a microscopic bosonic pairing theory
Quantum droplets are small clusters of atoms self-bound by the balance of attractive and repulsive forces. Here we report on the observation of a novel type of droplets, solely stabilized by contact interactions in a mixture of two Bose-Einstein condensates. We demonstrate that they are several orders of magnitude more dilute than liquid helium by directly measuring their size and density via in situ imaging. Moreover, by comparison to a single-component condensate, we show that quantum many-body effects stabilize them against collapse. We observe that droplets require a minimum atom number to…
We study an impurity immersed in the mixture of Bose ultracold gases in the regime where a quantum droplet exists. The quasi-one-dimensional geometry is considered. We find an effective attractive potential that acts by the quantum droplet onto the impurity. The bound states of the impurity in this potential are investigated. These impurity bound states can provide potential probes for the presence of quantum fluctuations effects on the droplet properties. In the case of strong impurity-BEC coupling, we study the properties of the nonlinear local modes on the impurity induced by the quantum fl…
While quantum fluctuations in binary mixtures of bosonic atoms with short-range interactions can lead to the formation of a self-bound droplet, for equal intra-component interactions but an unequal number of atoms in the two components, there is an excess part that cannot bind to the droplet. Imposing confinement, as here through periodic boundary conditions in a one-dimensional setting, the droplet becomes amalgamated with a residual condensate. The rotational properties of this compound system reveal simultaneous rigid-body and superfluid behavior in the ground state and uncover that the res…
An ultradilute quantum droplet is a self-bound liquid-like state recently observed in ultracold Bose-Einstein condensates. In all previous theoretical studies, it is described by a phenomenological low-energy effective theory, termed as the extended Gross\textendash Pitaevskii equation. Here, we microscopically derive the Gross\textendash Pitaevskii equation for the condensate and also for a pairing field in an inhomogeneous quantum droplet realized by Bose-Bose mixtures with attractive inter-species interaction. We show that the inclusion of the pairing field is essential, in order to have a …
We theoretically investigate the finite-temperature structure and collective excitations of a self-bound ultradilute Bose droplet in a flat space realized in a binary Bose mixture with attractive inter-species interactions on the verge of mean-field collapse. As the droplet formation relies critically on the repulsive force provided by Lee-Huang-Yang quantum fluctuations, which can be easily compensated by thermal fluctuations, we find a significant temperature effect in the density distribution and collective excitation spectrum of the Bose droplet. A finite-temperature phase diagram as a fun…
We study the properties of self-bound liquid droplets of three-dimensional Bose mixtures in a weak random potential with Gaussian correlation function at both zero and finite temperatures. Using the Bogoliubov theory, we derive useful formulas for the ground-state energy, the equilibrium density, the depletion, and the anomalous density of the droplet. The quantum fluctuation induced by the disorder known as the glassy fraction is also systematically computed. At finite temperature, we calculate the free energy, the thermal equilibrium density, and the critical temperature in terms of the diso…
Self-bound quantum droplets form when the mean-field tendency of the gas to collapse is stabilized by the effectively repulsive beyond mean-field fluctuations. The beyond mean-field effects depend on Rabi-frequency $ω_R$ and quadratic Zeeman effect $q$ for the Rabi-coupled Bose mixtures and the spinor gases, respectively. The effects of varying $ω_R$ and $q$ on the quantum droplet have recently been examined for unpolarized Rabi-coupled Bose mixture with zero detuning $δ= 0$ and unpolarized spinor gas with $\langle F_z \rangle=0$. In this paper, we theoretically explore the stability of the dr…
Laser induced transitions between internal states of atoms have been playing a fundamental role to manipulate atomic clouds for many decades. In absence of interactions each atom behaves independently and their coherent quantum dynamics is described by the Rabi model. Since the experimental observation of Bose condensation in dilute gases, static and dynamical properties of multicomponent quantum gases have been extensively investigated. Moreover, at very low temperatures quantum fluctuations crucially affect the equation of state of many-body systems. Here we study the effects of quantum fluc…
Formation Dynamics of Quantum Droplets for Homonuclear and Heteronuclear Mixtures
Instituto de Física, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学物理研究所）；Departamento de Psiquiatria, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学精神病学系）
In a binary quantum droplet, the interspecies attraction dominates over the intraspecies repulsions and the mean-field energy is unstable. The mechanical stability is restored by the repulsive Lee-Huang-Yang (LHY) energy [1]. In the Bogoliubov theory of the binary quantum droplet, there are two branches of gapless excitations. The lower branch describes the phonon excitation and its energy is imaginary in the long-wavelength limit, implying dynamical instability. Recently it is found that the phonon energy is renormalized by higher-order quantum fluctuations and the dynamical instability is re…
We revisit the Bogoliubov theory of quantum droplets proposed by Petrov {[}Phys. Rev. Lett. \textbf{115}, 155302 (2015){]} for an ultracold Bose-Bose mixture, where the mean-field collapse is stabilized by the Lee-Huang-Yang quantum fluctuations. We show that a loophole in Petrov's theory, i.e., the ignorance of the softening complex Bogoliubov spectrum, can be naturally removed by the introduction of bosonic pairing. The pairing leads to weaker mean-field attractions, and also stronger Lee-Huang-Yang term in the case of unequal intraspecies interactions. As a result, the equilibrium density f…
We study the collective modes of a binary Bose mixture across the soliton to droplet crossover in a quasi one dimensional waveguide with a beyond-mean-field equation of state and a variational Gaussian ansatz for the scalar bosonic field of the corresponding effective action. We observe a sharp difference in the collective modes in the two regimes. Within the soliton regime modes vary smoothly upon the variation of particle number or interaction strength. On the droplet side collective modes are inhibited by the emission of particles. This mechanism turns out to be dominant for a wide range of…
According to the mean-field theory a condensed Bose-Bose mixture collapses when the interspecies attraction becomes stronger than the geometrical average of the intraspecies repulsions, $g_{12}^2>g_{11} g_{22}$. We show that instead of collapsing such a mixture gets into a dilute liquid-like droplet state stabilized by quantum fluctuations thus providing a direct manifestation of beyond mean-field effects. We study various properties of the droplet and find, in particular, that in a wide range of parameters its excitation spectrum lies entirely above the particle emission threshold. The drople…
We consider a mixture of two bosonic species with tunable interspecies interaction in a periodic potential and discuss the advantages of low filling factors on the detection of the pair-superfluid phase. We show how the emergence of such a phase can be put dramatically into evidence by looking at the interference pictures and density correlations after expansion and by changing the interspecies interaction from attractive to repulsive.
We systematically investigate the ground-state properties of self-bound droplets of quasi-two-dimensional binary Bose gases by using the Gaussian state theory. We find that quantum droplets consists two macroscopic squeezed phases and a macroscopic coherent phase. We map out the phase diagram and determine all phase boundaries via both numerical and nearly analytical methods. In particular, we find three easily accessible signatures for the quantum phases and the stablization mechanism of the self-bound droplets by precisely measuring their radial size. Our studies indicate that binary droplet…
The existence of quantum droplets in binary Bose-Einstein condensate mixtures rely on beyondmean field effects, competing with mean-field effects. Interestingly, the beyond-mean field effect is changing from repulsive in 3D to attractive in 1D leading to drastically different behaviors. We study in detail the crossover between these two regimes in a quasi-1D regime where the radial wavefunction is frozen. Quantum droplets exist for all values and sign of the mean-field interaction. We find that approaching the crossover is experimentally appealing as it reduces the relative importance of three…
We report on the dynamical formation of self-bound quantum droplets in attractive mixtures of $^{39}$K atoms. Considering the experimental observations of Semeghini et al., Phys. Rev. Lett. 120, 235301 (2018), we perform numerical simulations to understand the relevant processes involved in the formation of a metastable droplet from an out-of-equilibrium mixture. We first analyze the so-called self-evaporation mechanism, where the droplet dissipates energy by releasing atoms, and then we consider the effects of losses due to three-body recombinations and to the balancing of populations in the …
Attractive Bose-Einstein condensates can host two types of macroscopic self-bound states of different nature: bright solitons and quantum liquid droplets. Here, we investigate the connection between them with a Bose-Bose mixture confined in an optical waveguide. We develop a simple theoretical model to show that, depending on atom number and interaction strength, solitons and droplets can be smoothly connected or remain distinct states coexisting only in a bi-stable region. We experimentally measure their spin composition, extract their density for a broad range of parameters and map out the b…
The droplet crystal phase of a symmetric binary mixture of Rydberg-blockaded dipolar Bose gases is studied by computer simulation. At high temperature each droplet comprises on average equal numbers of particles of either component, but the two components demix below the supersolid transition temperature, i.e., droplets mostly consist of particles of one component. Droplets consisting of the same component will also favor clustering. Demixing is driven by quantum tunnelling of particles across droplets over the system, and does not take place in a non-superfluid crystal. This effect should be …
Quantum droplets can emerge in bosonic binary magnetic gases (BMGs) from the interplay of short- and long-ranged interactions, and quantum fluctuations. We develop an extended meanfield theory for this system and use it to predict equilibrium and dynamical properties of BMG droplets. We present a phase diagram and characterize miscible and immiscible droplet states. We also show that a single component self-bound droplet can be used to bind another magnetic component which is not in the droplet regime. Our results should be realizable in experiments with mixtures of highly-magnetic lanthanide …
We present a general discussion of the dipole modes of a heteronuclear bosonic mixture in a harmonic trap by comparing the prediction of the sum-rule approach with full Gross-Pitaevskii (GP) calculations. Yet in the range of interaction in which the mixture is miscible and stable at the mean field level, $g_{12}^2<g_{11}g_{22}$, we find that there are regimes where the sum rules displays significant deviations from the GP solution. We provide an interpretation for this behavior in terms of the Ehrenfest approach, which we show to be equivalent to the sum-rule approach for dipole excitations.
In this article, we illustrate the scaling properties of a family of solutions for N attractive bosonic atoms in the limit of large $N$. These solutions represent the quantized dynamics of solitonic degrees of freedom in atomic droplets. In dimensions lower than two, or $d=2-ε$, we demonstrate that the number of isotropic droplet states scales as $N^{3/2}/ε^{1/2}$, and for $ε=0$, or $d=2$, scales as ${N^2}$. The ground state energies scale as $N^{2 / ε+ 1}$ in $d=2-ε$, and when $d=2$, scale as an exponential function of N. We obtain the universal energy spectra and the generalized Tjon relatio…
We report the observation of many-body interaction effects for a homonuclear bosonic mixture in a three-dimensional optical lattice with variable state dependence along one axis. Near the superfluid-to-Mott insulator transition for one component, we find that the presence of a second component can reduce the apparent superfluid coherence, most significantly when it either experiences a strongly localizing lattice potential or none at all. We examine this effect by varying the relative populations and lattice depths, and discuss the observed behavior in view of recent proposals for scattering f…
