We report on the formation of heteronuclear quantum droplets in an attractive bosonic mixture of 41K and 87Rb. We observe long-lived self-bound states, both in free space and in an optical waveguide. In the latter case, the dynamics under the effect of a species-dependent force confirms their bound nature. By tuning the interactions from the weakly to the strongly attractive regime, we study the transition from expanding to localized states, in both geometries. We compare the experimental results with beyond mean-field theory and we find a good agreement in the full range of explored interactions. Our findings open up the production of long-lived droplets with important implications for further research.
Formation Dynamics of Quantum Droplets for Homonuclear and Heteronuclear Mixtures
Instituto de Física, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学物理研究所）；Departamento de Psiquiatria, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学精神病学系）
We have theoretically investigated the structure of spinning self-bound droplets made of $^{41}$K-$^{87}$Rb Bose mixture by solving the Gross-Pitaevskii equation including beyond-mean-field correction in the Lee-Huang-Yang form. The structure and energetics of vortex formation in the self-bound mixture have been elucidated, showing that the formation of linear vortices in the heavier species is energetically favoured over other configurations. A fake (partially filled) core develops as a consequence in the other species, resulting in a hole which might be imaged in experiments. The interplay b…
Quantum droplets have intrigued much attention recently in view of their successful observations in the ultracold homonuclear atoms. In this work, we demonstrate a new mechanism for the formation of quantum droplet in heteronuclear atomic systems, i.e., by applying the synthetic spin-orbit coupling(SOC). Take the Bose-Fermi mixture for example, we show that by imposing a Rashba SOC between the spin states of fermions, the greatly suppressed Fermi pressure can enable the formation of Bose-Fermi droplets even for very weak boson-fermion attractions, which are insufficient to bound a droplet if w…
We study the three-body problem of two ultracold identical bosonic atoms (denoted by $B$) and one extra atom (denoted by $X$), where the scattering length $a_{BX}$ between each bosonic atom and atom $X$ is resonantly large and positive. We calculate the scattering length $a_{\rm ad}$ between one bosonic atom and the shallow dimer formed by the other bosonic atom and atom $X$, and investigate the effect induced by the interaction between the two bosonic atoms. We find that even if this interaction is weak (i.e., the corresponding scattering length $a_{BB}$ is of the same order of the van der Wa…
We exemplify the impact of beyond Lee-Huang-Yang (LHY) physics, especially due to intercomponent correlations, in the ground state and the quench dynamics of one-dimensional so-called quantum droplets using an ab-initio nonperturbative approach. It is found that the droplet Gaussian-shaped configuration arising for intercomponent attractive couplings becomes narrower for stronger intracomponent repulsion and transits towards a flat-top structure either for larger particle numbers or weaker intercomponent attraction. Additionally, a harmonic trap prevents the flat-top formation. At the balance …
Motivated by recent realizations of spin-1 NaRb mixtures in the experiments, here we investigate heteronuclear magnetism in the Mott-insulating regime. Different from the identical mixtures where the boson (fermion) statistics only admits even (odd) parity states from angular momentum composition, for heteronuclear atoms in principle all angular momentum states are allowed, which can give rise to new magnetic phases. Various magnetic phases can be developed over these degenerate spaces, however, the concrete symmetry breaking phases depend not only on the degree of degeneracy, but also the com…
We study the fate of an impurity in an ultracold heteronuclear Bose mixture, focusing on the experimentally relevant case of a $^{41}$K-$^{87}$Rb mixture, with the impurity in a $^{41}$K hyperfine state. Our work provides a comprehensive description of an impurity in a BEC mixture with contact interactions across its phase diagram. We present results for the miscible and immiscible regimes, as well as for the impurity in a self-bound quantum droplet. Here, varying the interactions, we find novel, exotic states where the impurity localizes either at the center or at the surface of the droplet.
We derive the complete mixing-demixing phase-diagram relevant to a bosonic binary mixture confined in a ring trimer and modeled within the Bose-Hubbard picture. The mixing properties of the two quantum fluids, which are shown to be strongly affected by the fragmented character of the confining potential, are evaluated by means of a specific indicator imported from Statistical Thermodynamics and are shown to depend only on two effective parameters incorporating the asymmetry between the heteronuclear species. To closely match realistic experimental conditions, our study is extended also beyond …
We explore the phase diagram of two-component bosons with Feshbach resonant pairing interactions in an optical lattice. It has been shown in previous work to exhibit a rich variety of phases and phase transitions, including a paradigmatic Ising quantum phase transition within the second Mott lobe. We discuss the evolution of the phase diagram with system parameters and relate this to the predictions of Landau theory. We extend our exact diagonalization studies of the one-dimensional bosonic Hamiltonian and confirm additional Ising critical exponents for the longitudinal and transverse magnetic…
We demonstrate a generally applicable technique for mixing two-species quantum degenerate bosonic samples in the presence of an optical lattice, and we employ it to produce low-entropy samples of ultracold 87Rb133Cs Feshbach molecules with a lattice filling fraction exceeding 30%. Starting from two spatially separated Bose-Einstein condensates of Rb and Cs atoms, Rb-Cs atom pairs are efficiently produced by using the superfluid-to-Mott insulator quantum phase transition twice, first for the Cs sample, then for the Rb sample, after nulling the Rb-Cs interaction at a Feshbach resonance's zero cr…
We report the observation of a dimer-dimer inelastic collision resonance for ultracold Feshbach molecules made of bosonic sodium and rubidium atoms. This resonance, which we attribute to the crossing of the dimer-dimer threshold with a heteronuclear tetramer state, manifests itself as a pronounced inelastic loss peak of dimers when the interspecies scattering length between the constituent atoms is tuned. Near this resonance, a strong modification of the temperature dependence of the dimer-dimer scattering is observed. Our result provides insight into the heteronuclear four-body system consist…
We analytically calculate the leading quantum corrections of the ground-state energy of two- and one-dimensional weakly interacting Rabi-coupled Bose-Bose mixtures in the frame of the Bogoliubov approximation. We show that to repulsive intraspecies and attractive interspecies interactions, the effect of quantum fluctuations favors the formation of self-bound droplets. These liquidlike states are crucially affected by the Rabi coupling, leading thus to the appearance of a quantum instability. We derive meaningful formulas to describe the droplet phase in the one-dimensional case.
We demonstrate the existence of quantum droplets in two-component one-dimensional Bose-Hubbard chains. The droplets exist for any strength of repulsive intra-species interactions provided they are balanced by comparable attractive inter-species interactions. The ground-state phase diagram is presented and the different phases are characterized by examining the density profile and off-diagonal one- and two-body correlation functions. A rich variety of phases is found, including atomic superfluid gases, atomic superfluid droplets, pair superfluid droplets, pair superfluid gases and a Mott-insula…
We explore the properties of weakly bound bosonic states in the strongly interacting regime. Combining a correlated-Gaussian (CG) basis set expansion with a complex scaling method, we extract the energies and structural properties of bosonic cluster states with $N\le6$ for different two-body potentials. The identification of five- and six-body resonances attached to an excited Efimov trimer provides strong support to the premise of Efimov universality in bosonic systems. Our study also reveals a rich structure of bosonic cluster states. Besides the lowest cluster states which behave as bosonic…
Ultradilute quantum droplets are intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in three-, one- and two-dimensional two-component Bose-Bose mixtures, by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the interspecies attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In three dimen…
Collision and coalescence dynamics of bosonic quantum Hall droplets
State Key Laboratory of Information Photonics and Optical Communications, School of Physical Science and Technology, Beijing University of Posts and Telecommunications（北京邮电大学物理科学与技术学院信息光子学与光通信国家重点实验室）
We present a general discussion of the dipole modes of a heteronuclear bosonic mixture in a harmonic trap by comparing the prediction of the sum-rule approach with full Gross-Pitaevskii (GP) calculations. Yet in the range of interaction in which the mixture is miscible and stable at the mean field level, $g_{12}^2<g_{11}g_{22}$, we find that there are regimes where the sum rules displays significant deviations from the GP solution. We provide an interpretation for this behavior in terms of the Ehrenfest approach, which we show to be equivalent to the sum-rule approach for dipole excitations.
Breakdown of the single-mode description of ultradilute quantum droplets in binary Bose mixtures: A perspective from a microscopic bosonic pairing theory
We study an impurity immersed in the mixture of Bose ultracold gases in the regime where a quantum droplet exists. The quasi-one-dimensional geometry is considered. We find an effective attractive potential that acts by the quantum droplet onto the impurity. The bound states of the impurity in this potential are investigated. These impurity bound states can provide potential probes for the presence of quantum fluctuations effects on the droplet properties. In the case of strong impurity-BEC coupling, we study the properties of the nonlinear local modes on the impurity induced by the quantum fl…
While quantum fluctuations in binary mixtures of bosonic atoms with short-range interactions can lead to the formation of a self-bound droplet, for equal intra-component interactions but an unequal number of atoms in the two components, there is an excess part that cannot bind to the droplet. Imposing confinement, as here through periodic boundary conditions in a one-dimensional setting, the droplet becomes amalgamated with a residual condensate. The rotational properties of this compound system reveal simultaneous rigid-body and superfluid behavior in the ground state and uncover that the res…
In this paper we develop a theory for an infinitely long droplet state of a zero temperature dipolar bosonic gas. The infinite droplet theory yields simpler equations to solve for the droplet state and its collective excitations. We explore the behavior of infinite droplets using numerical and variational solutions, and demonstrate that it can provide a quantitative description of large finite droplets of the type produced in experiments. We also consider the axial speed of sound and the thermodynamic limit of a dipolar droplet.
We investigate the formation of weakly bound, electronically excited, heteronuclear 6Li40K* molecules by single-photon photoassociation in a magneto-optical trap. We performed trap loss spectroscopy within a range of 325 GHz below the Li(2S_(1/2))+K(4P_(3/2)) and Li(2S_(1/2))+K(4P_(1/2)) asymptotic states and observed more than 60 resonances, which we identify as rovibrational levels of 7 of 8 attractive long-range molecular potentials. The long-range dispersion coefficients and rotational constants are derived. We find large molecule formation rates of up to ~3.5x10^7s^(-1), which are shown t…
We revisit the Bogoliubov theory of quantum droplets proposed by Petrov {[}Phys. Rev. Lett. \textbf{115}, 155302 (2015){]} for an ultracold Bose-Bose mixture, where the mean-field collapse is stabilized by the Lee-Huang-Yang quantum fluctuations. We show that a loophole in Petrov's theory, i.e., the ignorance of the softening complex Bogoliubov spectrum, can be naturally removed by the introduction of bosonic pairing. The pairing leads to weaker mean-field attractions, and also stronger Lee-Huang-Yang term in the case of unequal intraspecies interactions. As a result, the equilibrium density f…
We have created a triply quantum degenerate mixture of bosonic $^{41}$K and two fermionic species $^{40}$K and $^6$Li. The boson is shown to be an efficient coolant for the two fermions, spurring hopes for the observation of fermionic superfluids with imbalanced masses. We observe multiple heteronuclear Feshbach resonances, in particular a wide s-wave resonance for the combination $^{41}$K-$^{40}$K, opening up studies of strongly interacting {\it isotopic} Bose-Fermi mixtures. For large imbalance, we enter the polaronic regime of dressed impurities immersed in a bosonic or fermionic bath.
Quantum droplets can emerge in bosonic binary magnetic gases (BMGs) from the interplay of short- and long-ranged interactions, and quantum fluctuations. We develop an extended meanfield theory for this system and use it to predict equilibrium and dynamical properties of BMG droplets. We present a phase diagram and characterize miscible and immiscible droplet states. We also show that a single component self-bound droplet can be used to bind another magnetic component which is not in the droplet regime. Our results should be realizable in experiments with mixtures of highly-magnetic lanthanide …
In this article, we illustrate the scaling properties of a family of solutions for N attractive bosonic atoms in the limit of large $N$. These solutions represent the quantized dynamics of solitonic degrees of freedom in atomic droplets. In dimensions lower than two, or $d=2-ε$, we demonstrate that the number of isotropic droplet states scales as $N^{3/2}/ε^{1/2}$, and for $ε=0$, or $d=2$, scales as ${N^2}$. The ground state energies scale as $N^{2 / ε+ 1}$ in $d=2-ε$, and when $d=2$, scale as an exponential function of N. We obtain the universal energy spectra and the generalized Tjon relatio…
We use exact Quantum Monte Carlo techniques to study the properties of quantum droplets in two-component bosonic mixtures with contact interactions in one spatial dimension. We systematically study the surface tension, the density profile and the breathing mode as a function of the number of particles in the droplet and of the ratio of coupling strengths between intra-species repulsion and inter-species attraction. We find that deviations from the predictions of the generalized Gross-Pitaevskii equation are small in most cases of interest.
We develop two approximate theories to describe the miscible and immiscible droplets that can occur in a binary mixture of highly magnetic bosonic atoms. In addition to allowing simpler calculations, the approximate theories provide insight into the role of quantum fluctuations in the two regimes. Results are validated by comparison to those from the extended Gross-Pitaevskii equation. As an application we solve for the ground state droplets crossing the miscible-immiscible transition as function of the short-ranged interspecies interaction parameter. We consider regimes where the transition o…
We theoretically investigate the droplets formation in a tightly trapped one-dimensional dipolar gas of bosonic atoms. When the strength of the dipolar interaction becomes sufficiently attractive compared to the contact one, we show how a solitonic-like density profile evolves into a liquid-like droplet on increasing the number of particles in the trap. The incipient gas-liquid transition is also signalled by a steep increase of the breathing mode and a change in sign of the chemical potential. Upon a sudden release of the trap, varying the number of trapped atoms and the scattering length, th…
In a joint experimental and theoretical effort, we report on the formation of a macro-droplet state in an ultracold bosonic gas of erbium atoms with strong dipolar interactions. By precise tuning of the s-wave scattering length below the so-called dipolar length, we observe a smooth crossover of the ground state from a dilute Bose-Einstein condensate (BEC) to a dense macro-droplet state of more than $10^4$ atoms. Based on the study of collective excitations and loss features, we quantitative prove that quantum fluctuations stabilize the ultracold gas far beyond the instability threshold impose…
We calculate the excitation spectrum of a one-dimensional self-bound quantum droplet in a two-component bosonic mixture described by the Gross-Pitaevskii equation (GPE) with cubic and quadratic nonlinearities. The cubic term originates from the mean-field energy of the mixture proportional to the effective coupling constant $δg$, whereas the quadratic nonlinearity corresponds to the attractive beyond-mean-field contribution. The droplet properties are governed by a control parameter $γ\propto δg N^{2/3}$, where $N$ is the particle number. For large $γ>0$ the droplet features the flat-top shape…
In this article we develop the framework to describe Bose-Fermi mixtures of magnetic atoms, focusing on the interaction of bosonic self-bound dipolar quantum droplets with a small number of fermions. We find an attractive interaction potential due to the dipolar interaction with several bound states, which can be occupied by one fermion each, resulting in a very weak back-action on the bosons. We conclude, that these impurities might act as unique probes giving access to inherent properties of dipolar quantum droplets.
We study the quantum fluctuations in the condensates of a mixture of bosonic atoms and molecules with interspecies p-wave interaction. Our analysis shows that the quantum phase of coexisting atomic and molecular condensates is unstable at the mean-field level. Unlike the mixture of s-wave interaction, the Lee-Huang-Yang correction of p-wave interaction is unexpectedly found here to exhibit an opposite sign with respect to its mean-field term above a critical particle density. This quantum correction to the mean-field energy provides a remarkable mechanism to self-stabilize the phase. The order…
We study the collective modes of a binary Bose mixture across the soliton to droplet crossover in a quasi one dimensional waveguide with a beyond-mean-field equation of state and a variational Gaussian ansatz for the scalar bosonic field of the corresponding effective action. We observe a sharp difference in the collective modes in the two regimes. Within the soliton regime modes vary smoothly upon the variation of particle number or interaction strength. On the droplet side collective modes are inhibited by the emission of particles. This mechanism turns out to be dominant for a wide range of…
We consider two-dimensional weakly-bound heterospecies molecules formed in a Fermi-Bose mixture with attractive Fermi-Bose and repulsive Bose-Bose interactions. Bosonic exchanges lead to an intermolecular attraction, which can be controlled and tuned to a p-wave resonance. Such attractive fermionic molecules can be realized in quasi-two-dimensional ultracold isotopic or heteronuclear mixtures. We show that they are stable with respect to the recombination to deeply-bound molecular states and with respect to the formation of higher-order clusters (trimers, tetramers, etc.)
We have investigated self-bound binary ultra dilute bosonic mixtures at zero temperature within Density Functional Theory using a Local Density Approximation. We provide the explicit expression of the Lee-Huang-Yang correction in the general case of heteronuclear mixtures, and investigate the general thermodynamic conditions which lead to the formation of self-bound systems. We have determined the conditions for stability against the evaporation of one component, as well as the mechanical and diffusive spinodal lines. We have also calculated the surface tension of the self-bound state as a fun…
We make use of numerical exact diagonalization calculations to explore the physics of $ν= 1/2$ bosonic fractional quantum Hall (FQH) droplets in the presence of experimentally realistic cylindrically symmetric hard-wall potentials. This kind of confinement is found to produce very different many-body spectra compared to a harmonic trap or the so-called extremely steep limit. For a relatively weak confinement, the degeneracies are lifted and the low-lying excited states organize themselves in energy branches that can be explained in terms of their Jack polynomial representation. For a strong co…
Multimode optical cavities can be used to implement interatomic interactions which are highly tunable in strength and range. For bosonic atoms trapped in an optical lattice, cavity-mediated interactions compete with the short-range interatomic repulsion, which we study using an extended Bose-Hubbard model. Already in a single-mode cavity, where the corresponding interaction has an infinite range, a rich phase diagram has been experimentally observed, featuring density-wave and supersolid self-organized phases in addition to the usual superfluid and Mott insulator. Here we show that, for any fi…
The main theme of this review is the many-body physics of vortices in quantum droplets of bosons or fermions, in the limit of small particle numbers. Systems of interest include cold atoms in traps as well as electrons confined in quantum dots. When set to rotate, these in principle very different quantum systems show remarkable analogies. The topics reviewed include the structure of the finite rotating many-body state, universality of vortex formation and localization of vortices in both bosonic and fermionic systems, and the emergence of particle-vortex composites in the quantum Hall regime.…
