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arXiv 1707.06256cond-mat.mes-hall
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光子晶体阻带对$a$ $_{1-x}$ C $_x$:H光致发光的影响

Effect of photonic crystal stop-band on photoluminescence of $a$-Si$_{1-x}$C$_x$:H

Mikhail V. Rybin, Alexander V. Zherzdev, Nikolay A. Feoktistov, Alexander B. Pevtsov

摘要:

分析了由\textit{a} C $_x$:H和\textit{a}非晶层交替构成的一维(1D)光子晶体的周期结构中光子态局域密度变化的影响.使用\textit{a} -Si $_{1-x}$ C $_x$:H作为发射材料使得可以检查光致发光光谱轮廓的变换,其在宽度上与光子阻带相当。实验表明,在阻带附近,发光被增强和抑制。在阻带不同边缘的发光峰的相对强度随单个\textit{a} -Si $_{1-x}$ C $_x$:H薄膜的阻带位置和光致发光峰的失谐而变化。在所考虑的系统中的Purcell效应的理论描述的方法,其中的局域光子态密度的计算方面的一维模型。%实验测量和计算光谱之间获得了良好的一致性。结果表明,局域态密度的特定部分在1D光子晶体的阻带的长波长(低频)边缘处显著增加,这是由于光波的电场在\textit{a} -Si $_{1-x}$ C $_x$:H的空间区域中的主要局域化,该空间区域与\textit{a} -SiO $_2$相比具有更高的相对介电常数。

英文摘要:

Effects associated with the change in the local density of photonic states in a periodic structure based on alternating \textit{a}-Si$_{1-x}$C$_x$:H and \textit{a}-SiO$_2$ amorphous layers forming a one-dimensional (1D) photonic crystal have been analyzed. The use of \textit{a}-Si$_{1-x}$C$_x$:H as the emitting material made it possible to examine the transformation of the photoluminescence spectrum contour that is comparable in width with the photonic stop-band. It was experimentally demonstrated that the emission is enhanced and suppressed in the vicinity of the stop-band. The relative intensities of the luminescence peaks at different edges of the stop-band vary with the detuning of the stop-band position and photoluminescence peak of a single \textit{a}-Si$_{1-x}$C$_x$:H film. The Purcell effect in the system under consideration was theoretically described by the method in which the local density of photonic states is calculated in terms of a 1D model. %A good agreement was obtained between the experimentally measured and calculated spectra. It was shown that the specific part of local density of states substantially increases at the long-wavelength (low-frequency) edge of the stop-band of a 1D photonic crystal as a result of the predominant localization of the electric field of the light wave in the spatial regions of \textit{a}-Si$_{1-x}$C$_x$:H which have a higher relative permittivity as compared with \textit{a}-SiO$_2$.

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