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arXiv 1608.06260cond-mat.mes-hall
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含磁性离子量子点的磁场诱导自旋态突变

Magnetic-field-induced abrupt spin state transition in a quantum dot containing magnetic ions

Maciej Koperski, Tomasz Smoleński, Mateusz Goryca, Piotr Wojnar, Marek Potemski, Piotr Kossacki

摘要:

我们提出了一个全面的磁光特性的单一的CdTe量子点含有几个Mn 2+离子的结果。我们发现一些量子点的激子光致发光谱随磁场的变化呈现出意想不到的演化。在特定的磁场值下,对于每个量子点,与限制在量子点内的各种激子复合物的复合有关的宽谱线中的每一条都转变为一对窄线,分裂为几个meV。我们解释这种激子发射光谱的字符的突变的结果从一个非极化状态的Mn 2+自旋在低场制度的高度(几乎完全)极化状态以上的临界磁场的过渡。各种光学实验,包括偏振分辨研究,不同的激发制度和时间分辨测量的调查证实了这一点。然而,这些测量也表明,所观察到的效果是不相关的或受光产生的载流子的影响,但它是源于不寻常的自旋配置在集群的Mn 2+离子。

英文摘要:

We present the results of a comprehensive magneto-optical characterization of single CdTe quantum dots containing a few Mn2+ ions. We find that some quantum dots exhibit an unexpected evolution of excitonic photoluminescence spectrum with the magnetic field. At a certain value of the magnetic field, specific for every quantum dot, each of the broad spectral lines related to the recombination of various excitonic complexes confined inside the dot transforms into a pair of narrow lines split by several meV. We interpret this abrupt change in the character of excitonic emission spectrum as a consequence of a transition from a non-polarized state of the Mn2+ spins in a low field regime to a highly (almost fully) polarized state above the critical magnetic field. Various optical experiments, including polarization-resolved studies, investigation of different excitation regimes and time-resolved measurements corroborate this scenario. However, these measurements indicate also that the observed effect is not related or influenced by the photo-created charge carriers, but it is rather originating from unusual spin configuration in the cluster of Mn2+ ions.

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